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RESEARCH PAPER · Journal of the American Chemical Society · 2018

Autoluminescent Metal–Organic Frameworks (MOFs): Self-Photoemission of a Highly Stable Thorium MOF

Jacopo Andreo, Emanuele Priola, Gabriele Alberto, Paola Benzi, Domenica Marabello, Davide Maria Proserpio, Carlo Lamberti, Eliano Diana

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Autoluminescent Metal–Organic Frameworks (MOFs): Self-Photoemission of a Highly Stable Thorium MOFOriginalStabilization of an Unprecedented Hexanuclear Secondary Building Unit in a Thorium-Based Metal–Organic Framework44A Thorium Metal‐Organic Framework with Outstanding Thermal and Chemical Stability50A Flexible Two‐Fold Interpenetrated Indium MOF Exhibiting Dynamic Response to Gas Adsorption and High‐Sensitivity Detection of Nitroaromatic Explosives35Four alkaline earth metal (Mg, Ca, Sr, Ba)-based MOFs as multiresponsive fluorescent sensors for Fe3+, Pb2+ and Cu2+ ions in aqueous solution43Metal–Organic Frameworks in Modern Physics: Highlights and Perspectives104A Double-Walled Thorium-Based Metal–Organic Framework as a Promising Dual-Function Absorbent for Efficiently Capturing Iodine and Dyes54Unexpected structural complexity of thorium coordination polymers and polyoxo cluster built from simple formate ligands34Noncomplexed Cucurbituril-Mediated Structural Evolution of Layered Uranyl Terephthalate Compounds13A mixed-ligand strategy regulates thorium-based MOFs55Heat-resistant Pb( ii )-based X-ray scintillating metal–organic frameworks for sensitive dosage detection via an aggregation-induced luminescent chromophore42In Situ Fluorescence Imaging of the Levels of Glycosylation and Phosphorylation by a MOF-Based Nanoprobe in Depressed Mice36Ultrastable Thorium Metal–Organic Frameworks for Efficient Iodine Adsorption162Advancement of Actinide Metal–Organic Framework Chemistry via Synthesis of Pu-UiO-6660From Isolated Molecular Complexes to Extended Networks: Synthesis and Characterization of Thorium Furanmono‐ and Dicarboxylates2Rational Design of a Uranyl Metal–Organic Framework for the Capture and Colorimetric Detection of Organic Dyes22Luminescent Cd(Ⅱ) metal-organic frameworks with anthracene nitrogen-containing organic ligands as novel multifunctional chemosensors for the detection of picric acid, pesticides, and ferric ions51Metal-organic frameworks as a versatile platform for radionuclide management163Boosting the Iodine Adsorption and Radioresistance of Th‐UiO‐66 MOFs via Aromatic Substitution118Beyond structural motifs: the frontier of actinide-containing metal–organic frameworks65Emergence of a thorium–organic framework as a radiation attenuator for selective X-ray dosimetry20Synthesis of luminescent thorium-based metal–organic frameworks with 1,2,4,5-tetrakis(4-carboxyphenyl)benzene10Structural Evolution from Noninterpenetrated to Interpenetrated Thorium–Organic Frameworks Exhibiting High Propyne Storage19An Azobenzene-Modified Photoresponsive Thorium–Organic Framework: Monitoring and Quantitative Analysis of Reversible trans–cis Photoisomerization30An updated status and trends in actinide metal-organic frameworks (An-MOFs): From synthesis to application145An fcu Th-MOF Constructed from In Situ Coupling of Monovalent Ligands7Multifunctional Two-Dimensional Metal–Organic Frameworks for Radionuclide Sequestration and Detection19Stepwise Assembly of a Multicomponent Heterometallic Metal–Organic Framework via Th6-Based Metalloligands15Isotypic lanthanide–organic frameworks and scintillating films with colour-tunable X-ray radioluminescence for imaging applications13State-of-the-art progress for the selective crystallization of actinides, synthesis of actinide compounds and their functionalization20Recent advances in the applications of thorium-based metal–organic frameworks and molecular clusters50Synthesis and structural characterization of a novel lead dinuclear complex: [Pb(L)(I)(sba) 0.5 ] 20MOFs with 12-Coordinate 5f-Block Metal Centers41Leveraging Nitrogen Linkages in the Formation of a Porous Thorium–Organic Nanotube Suitable for Iodine Capture24Modular Assembly of Isostructural Mixed-Ligand Uranyl Coordination Polymers Based on a Patterning Strategy9Efficient Separation of Trace SO2 from SO2/CO2/N2 Mixtures in a Th-Based MOF23Th-MOF showing six-fold imide-sealed pockets for middle-size-separation of propane from natural gas34Role of Metal Selection in the Radiation Stability of Isostructural M-UiO-66 Metal–Organic Frameworks58Achieving High Photo/Thermocatalytic Product Selectivity and Conversion via Thorium Clusters with Switchable Functional Ligands87Synthesis of Thorium Dioxide Nanocrystals by Pyrolysis of a Thorium‐based Metal‐organic Framework4Cu2+@NMOFs-to-bimetallic CuFe PBA transformation: An instant catalyst with oxidase-mimicking activity for highly sensitive impedimetric biosensor19A robust thorium–organic framework as a bifunctional platform for iodine adsorption and Cr( vi ) sensitization9Fabrication of a Cd( ii ) metal–organic framework as a dual functional material: efficient iodine capture and selective adsorption of a cationic dye24Improved quantum yield in geometrically constrained tetraphenylethylene-based metal–organic frameworks4Recent advances in metal–organic framework-based photoelectrochemical and electrochemiluminescence biosensors64Unveiling Structural Diversity of Uranyl Compounds of Aprotic 4,4′-Bipyridine N,N′-Dioxide Bearing O-Donors8Metal-organic frameworks: Synthetic methods for industrial production92Fabrication of a Large-Area Flexible Scintillating Membrane for High-Resolution X-ray Imaging Using an AIEgen-Functionalized Metal–Organic Framework30Assembling a Heterobimetallic Actinide Metal‐Organic Framework by a Reaction‐Induced Preorganization Strategy21Assembling a Heterobimetallic Actinide Metal‐Organic Framework by a Reaction‐Induced Preorganization Strategy0Luminescence intensity-tunable X-ray scintillation based on zirconium-based metal-organic frameworks9Self-adjusting coordination of carboxylate for constructing stable 4-connected tetrazolate porous frameworks with luminescence2Radiation‐Responsive Metal–Organic Frameworks: Fundamentals and Applications36Scintillating Metal Organic Frameworks (MOFs) for radioactive gas detection0Surfactant‐Mediated Crystalline Structure Evolution Enabling the Ultrafast Green Synthesis of Bismuth‐MOF in Aqueous Condition38From structure to function: MOF-based and COF-based catalysts for efficient electrocatalytic H 2 O 2 production via 2e − ORR39Designed assembly of heterometallic cluster organic frameworks based on Th6 cluster14Cellulose nanocrystals as bridges to construct CNCs@ZIF-8 3D network with topological chirality for realizing efficient photocatalytic reduction of CO219Metal-organic frameworks (MOFs) and covalent organic frameworks (COFs)-based prototyping of integrated sensing devices for robust analysis43Friends or Foes: Fundamental Principles of Th-Organic Scaffold Chemistry Using Zr-Analogs as a Guide22Ultrafast Removal of Thorium and Uranium from Radioactive Waste and Groundwater Using Highly Efficient and Radiation-Resistant Functionalized Triptycene-Based Porous Organic Polymers44Ratiometric temperature sensing with non-thermally coupled levels from Pr–Al co-doped MgGa2O47Emergence of a bismuth-based metal–organic framework as an X-ray scintillator3Insights into the role of the phosphate group in vastly improved adsorption of thorium and uranium using a triptycene-based knitted aryl polymer network3Lanthanide metal–organic frameworks as multifunctional sensors for chemicals and temperature6The inorganic chemist's guide to actinide radiation chemistry: a review10Self‐Induced Radioluminescence in Supramolecular Metal Halide Doped with Radioactive Isotope Strontium‐903Pioneering radiation dosimetry and photothermal conversion in a photochromic and radiochromic thorium cluster13Cadmium MOF-Based Varied {Cd 2 } Clusters as Multifunctional Fluorescence Sensors to Detect Fe 3+ , Cr 2 O 7 2– , TNP, and NFT13Applications and advantages of MOFs-based triboelectric nanogenerators for self-powered system13Nickel Ion Induced Multistage Assembly of Th13 Cluster4Integrating High- Z Thorium Nodes with AIEgens in a Metal–Organic Framework for Superior X-ray Scintillation5State of the art challenges and prospects of advanced materials in radiation detection for nuclear energy: a review13A Zn-based MOF with honeycomb topology for highly efficient iodine uptake from vapor and liquid phases: synthesis, crystal structure, topology and dual-phase sorption performance4The first bimetallic Np( v ) MOF with a Np 4 Cs 2 O 8 structural unit: sorption properties and thermal and radiation stability0The dynamic adaptability of mixed-ligand zinc MOFs: from fundaments to applications18Metal-organic frameworks and covalent-organic frameworks in thermal transport0Conformationally Adaptive Exfoliation of Porphyrin MOFs Liberates Interlayer Confinement for Enhanced Photocatalytic CO 2 Reduction0Lanthanide-based metal-organic gels for flexible X-ray imaging0Photoinduced Electronic Modulation in a Thorium Cluster: Enabling Dual Radiation Sensing and Photothermal Conversion0Metal-organic framework scintillators: mechanisms, design strategies and perspectives0

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  5. Metal–Organic Frameworks in Modern Physics: Highlights and Perspectives

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  6. A Double-Walled Thorium-Based Metal–Organic Framework as a Promising Dual-Function Absorbent for Efficiently Capturing Iodine and Dyes

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  18. Boosting the Iodine Adsorption and Radioresistance of Th‐UiO‐66 MOFs via Aromatic Substitution

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