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RESEARCH ARTICLE · Dalton Transactions · 2017

Two excellent phase-matchable infrared nonlinear optical materials based on 3D diamond-like frameworks: RbGaSn 2 Se 6 and RbInSn 2 Se 6

Hua Lin, Hong Chen, Yujun Zheng, Ju‐Song Yu, Xin‐Tao Wu, Li‐Ming Wu

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Two excellent phase-matchable infrared nonlinear optical materials based on 3D diamond-like frameworks: RbGaSn 2 Se 6 and RbInSn 2 Se 6OriginalSyntheses and characterization of three new sulfides with large band gaps: acentric Ba 4 Ga 4 SnS 12 , centric Ba 12 Sn 4 S 23 and Ba 7 Sn 3 S 1327Synthesis and characterization of two lead-containing metal chalcogenides: Ba5Pb2Sn3S13 and Ba6PbSn3Se137Na 6 Zn 3 MIII2Q 9 (M III = Ga, In; Q = S, Se): four new supertetrahedron-layered chalcogenides with unprecedented vertex-sharing T 3 -clusters and desirable photoluminescence performances31NaBaM III Q 3 (M III = Al, Ga; Q = S, Se): first quaternary chalcogenides with isolated edge-sharing (MIII2Q 6 ) 6− dimers8Effect of Element Substitution on Structural Transformation and Optical Performances in I2BaMIVQ4 (I = Li, Na, Cu, and Ag; MIV = Si, Ge, and Sn; Q = S and Se)63Modifying Disordered Sites with Rational Cations to Regulate Band-Gaps and Second Harmonic Generation Responses Markedly: Ba6Li2ZnSn4S16 vs Ba6Ag2ZnSn4S16 vs Ba6Li2.67Sn4.33S1625ABaSbQ 3 (A = Li, Na; Q = S, Se): diverse arrangement modes of isolated SbQ 3 ligands regulating the magnitudes of birefringences50Nonlinear Optical Crystals for Second Harmonic Generation19Rational design of infrared nonlinear optical chalcogenides by chemical substitution287A new type of novel salt-inclusion chalcogenide with ultralow thermal conductivity14Coordinated regulation on critical physiochemical performances activated from mixed tetrahedral anionic ligands in new series of Sr 6 A 4 M 4 S 16 (A = Ag, Cu; M = Ge, Sn) nonlinear optical materials28KInSi1.32Sn0.68Se6: An Infrared Nonlinear Optical Material Containing Three Types of Tetrahedral Units19Inherent laws between tetrahedral arrangement pattern and optical performance in tetrahedron-based mid-infrared nonlinear optical materials131Phase Matching, Strong Frequency Doubling, and Outstanding Laser-Induced Damage Threshold in the Biaxial, Quaternary Diamond-like Semiconductor Li 4 CdSn 2 S 779Ultralow thermal conductivity in the quaternary semiconducting chalcogenide Cs 4 [Ho 26 Cd 7 Se 48 ] with an unprecedented closed cavity architecture7A 3 Mn 2 Sb 3 S 8 (A = K and Rb): a new type of multifunctional infrared nonlinear optical material based on unique three-dimensional open frameworks53Aliovalent-cation-substitution-induced structure transformation: a new path toward high-performance IR nonlinear optical materials47Cu 4 MnGe 2 S 7 and Cu 2 MnGeS 4 : two polar thiogermanates exhibiting second harmonic generation in the infrared and structures derived from hexagonal diamond22Design and synthesis of Ba 3 SiSe 5 with suitable birefringence modulated via M IV atoms in the Ba–M IV –Q (M IV = Si, Ge; Q = S, Se) system3Noncentrosymmetric Tetrel Pnictides RuSi4P4 and IrSi3P3: Nonlinear Optical Materials with Outstanding Laser Damage Threshold47Introduction of Li into Ag-Based Noncentrosymmetric Sulfides for High-Performance Infrared Nonlinear Optical Materials40Inorganic Chalcogenides: From Zero‐Dimensional Clusters to Three‐Dimensional Frameworks5Transition-metal-based chalcogenides: A rich source of infrared nonlinear optical materials184AAg 3 Ga 8 Se 14 (A = Rb, Cs): second-harmonic generation responses realized through the parallel arrangement of AgSe 4 and GaSe 4 tetrahedrons5Two Nonlinear Optical Thiophosphates Cu 5 Hg 0.5 P 2 S 8 and AgHg 3 PS 6 Activated by Their Tetrahedra-Stacking Architecture12A comprehensive review on metal chalcogenides with three-dimensional frameworks for infrared nonlinear optical applications115d6versus d10, Which Is Better for Second Harmonic Generation Susceptibility? A Case Study of K2TGe3Ch8 (T = Fe, Cd; Ch = S, Se)18Stereochemically active lone-pair-driven giant enhancement of birefringence from three-dimensional CsZn 4 Ga 5 Se 12 to two-dimensional CsZnAsSe 319Recent progress in the design of IR nonlinear optical materials by partial chemical substitution: Structural evolution and performance optimization133Ga-based IR nonlinear optical materials: Synthesis, structures, and properties65Recent advances in rational structure design for nonlinear optical crystals: leveraging advantageous templates153Infrared nonlinear optical materials with multiple strongly ionic cations5Recent advances and future perspectives on rare-earth-based nonlinear optical materials with π-conjugated [XO3] (X = B, C, N) units66Cationic substitution engineering induces a new quaternary chalcogenide in the A–M IIIA –M IVA –Q system for optical crystal applications1Exploring new horizons in mid-to-far infrared nonlinear optical crystals: the significant potential of trigonal pyramidal [TeS 3 ] 2− functional units18Structure-property relationships in IR nonlinear optical chalcogenides with stereochemically active lone pairs29Ba 10 Zn 7 Ga 6 S 26 : Promising Infrared Nonlinear Optical Crystal Exhibiting a High Laser Damage Threshold0Physicochemical and computational studies of diamond-like quaternary chalcogenide CsCd₄In₅Te₁₂0Mid‐ to Far‐Infrared Nonlinear Optical Crystals: Design Strategies, Structure–Property Relationships and Engineering Prospects0

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  1. Syntheses and characterization of three new sulfides with large band gaps: acentric Ba 4 Ga 4 SnS 12 , centric Ba 12 Sn 4 S 23 and Ba 7 Sn 3 S 13

    Dalton Transactions · 2017

    Ruihuan Duan, Pengfei Liu, Hua Lin, Shangxiong Huangfu, Li‐Ming Wu

    Read original paper ↗ ·

  2. Synthesis and characterization of two lead-containing metal chalcogenides: Ba5Pb2Sn3S13 and Ba6PbSn3Se13

    Journal of Solid State Chemistry · 2017

    Ailijiang Abudurusuli, Hanqin Ding, Kui Wu

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  3. Na 6 Zn 3 MIII2Q 9 (M III = Ga, In; Q = S, Se): four new supertetrahedron-layered chalcogenides with unprecedented vertex-sharing T 3 -clusters and desirable photoluminescence performances

    Inorganic Chemistry Frontiers · 2018

    Ailijiang Abudurusuli, Kui Wu, Yilimiranmu Rouzhahong, Zhihua Yang, Shilie Pan

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  4. NaBaM III Q 3 (M III = Al, Ga; Q = S, Se): first quaternary chalcogenides with isolated edge-sharing (MIII2Q 6 ) 6− dimers

    Dalton Transactions · 2018

    Ailijiang Abudurusuli, Kui Wu, Yilimiranmu Rouzhahong, Zhihua Yang, Shilie Pan

    Read original paper ↗ ·

  5. Effect of Element Substitution on Structural Transformation and Optical Performances in I2BaMIVQ4 (I = Li, Na, Cu, and Ag; MIV = Si, Ge, and Sn; Q = S and Se)

    Inorganic Chemistry · 2018

    Leyan Nian, Kui Wu, Guijie He, Zhihua Yang, Shilie Pan

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  6. Modifying Disordered Sites with Rational Cations to Regulate Band-Gaps and Second Harmonic Generation Responses Markedly: Ba6Li2ZnSn4S16 vs Ba6Ag2ZnSn4S16 vs Ba6Li2.67Sn4.33S16

    Crystal Growth & Design · 2018

    Ruihuan Duan, Rui‐An Li, Pengfei Liu, Hua Lin, Yue Wang, Li‐Ming Wu

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  7. ABaSbQ 3 (A = Li, Na; Q = S, Se): diverse arrangement modes of isolated SbQ 3 ligands regulating the magnitudes of birefringences

    Chemical Communications · 2019

    Ailijiang Abudurusuli, Kui Wu, Abudukadi Tudi, Zhihua Yang, Shilie Pan

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  8. Nonlinear Optical Crystals for Second Harmonic Generation

    Crystallography Reports · 2019

    Somayeh Solgi, Majid Jafar Tafreshi, Morteza Sasani Ghamsari

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  9. Rational design of infrared nonlinear optical chalcogenides by chemical substitution

    Coordination Chemistry Reviews · 2019

    Hua Lin, Wenbo Wei, Hong Chen, Xintao Wu, Qi‐Long Zhu

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  10. A new type of novel salt-inclusion chalcogenide with ultralow thermal conductivity

    Chemical Communications · 2020

    Hong Chen, Pengfei Liu, Hua Lin, Xin‐Tao Wu

    Read original paper ↗ ·

  11. Coordinated regulation on critical physiochemical performances activated from mixed tetrahedral anionic ligands in new series of Sr 6 A 4 M 4 S 16 (A = Ag, Cu; M = Ge, Sn) nonlinear optical materials

    Dalton Transactions · 2020

    Ya Feng Yang, Miao Song, Jie Zhang, Lihua Gao, Xiaowen Wu, Kui Wu

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  12. KInSi1.32Sn0.68Se6: An Infrared Nonlinear Optical Material Containing Three Types of Tetrahedral Units

    Inorganic Chemistry · 2020

    Xiaohui Li, Yi-Ting Chen, Huaiguo Xue, Sheng‐Ping Guo

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  13. Inherent laws between tetrahedral arrangement pattern and optical performance in tetrahedron-based mid-infrared nonlinear optical materials

    Coordination Chemistry Reviews · 2020

    Weikang Wang, Dajiang Mei, Fei Liang, Jun Zhao, Yuandong Wu, Zheshuai Lin

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  14. Phase Matching, Strong Frequency Doubling, and Outstanding Laser-Induced Damage Threshold in the Biaxial, Quaternary Diamond-like Semiconductor Li 4 CdSn 2 S 7

    Chemistry of Materials · 2020

    Jian‐Han Zhang, Stanislav S. Stoyko, Andrew J. Craig, P. Grima, Joshua W. Kotchey, Joon Ik Jang, Jennifer A. Aitken

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  15. Ultralow thermal conductivity in the quaternary semiconducting chalcogenide Cs 4 [Ho 26 Cd 7 Se 48 ] with an unprecedented closed cavity architecture

    Inorganic Chemistry Frontiers · 2020

    Hong Chen, Pengfei Liu, Hua Lin, Xin‐Tao Wu

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  16. A 3 Mn 2 Sb 3 S 8 (A = K and Rb): a new type of multifunctional infrared nonlinear optical material based on unique three-dimensional open frameworks

    Inorganic Chemistry Frontiers · 2021

    Yu Xiao, Man-Man Chen, Yaying Shen, Pengfei Liu, Hua Lin, Yi Liu

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  17. Aliovalent-cation-substitution-induced structure transformation: a new path toward high-performance IR nonlinear optical materials

    Journal of Materials Chemistry C · 2021

    Chang Liu, Shenghua Zhou, Yu Xiao, Chao Zhang, Hua Lin, Yi Liu

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  18. Cu 4 MnGe 2 S 7 and Cu 2 MnGeS 4 : two polar thiogermanates exhibiting second harmonic generation in the infrared and structures derived from hexagonal diamond

    Dalton Transactions · 2021

    Jennifer R. Glenn, Jeong Bin Cho, Yiqun Wang, Andrew J. Craig, Jian‐Han Zhang, Marvene Cribbs, Stanislav S. Stoyko, Kate E. Rosello, Christopher Barton, Allyson Bonnoni, P. Grima, Joseph H. MacNeil, James M. Rondinelli, Joon Ik Jang, Jennifer A. Aitken

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  19. Design and synthesis of Ba 3 SiSe 5 with suitable birefringence modulated via M IV atoms in the Ba–M IV –Q (M IV = Si, Ge; Q = S, Se) system

    Dalton Transactions · 2021

    Huanhuan Cheng, Abudukadi Tudi, Peng Wang, Kewang Zhang, Zhihua Yang, Shilie Pan

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  20. Noncentrosymmetric Tetrel Pnictides RuSi4P4 and IrSi3P3: Nonlinear Optical Materials with Outstanding Laser Damage Threshold

    Advanced Functional Materials · 2021

    Shannon Lee, Scott L. Carnahan, Georgiy Akopov, Philip Yox, Linlin Wang, Aaron J. Rossini, Kui Wu, Kirill A. Kovnir

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  21. Introduction of Li into Ag-Based Noncentrosymmetric Sulfides for High-Performance Infrared Nonlinear Optical Materials

    Inorganic Chemistry · 2021

    Wenfeng Zhou, Wen‐Dong Yao, Qing Zhang, Huaiguo Xue, Sheng‐Ping Guo

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  22. Inorganic Chalcogenides: From Zero‐Dimensional Clusters to Three‐Dimensional Frameworks

    Venue not supplied by source · 2021

    Hua Lin, Xin‐Tao Wu, Qi‐Long Zhu

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  23. Transition-metal-based chalcogenides: A rich source of infrared nonlinear optical materials

    Coordination Chemistry Reviews · 2021

    Hong Chen, Wenbo Wei, Hua Lin, Xintao Wu

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  24. AAg 3 Ga 8 Se 14 (A = Rb, Cs): second-harmonic generation responses realized through the parallel arrangement of AgSe 4 and GaSe 4 tetrahedrons

    Dalton Transactions · 2022

    Zhi-Xin Qiu, Shao‐Min Pei, Wen‐Fa Chen, Xiao‐Ming Jiang, Bin‐Wen Liu, Guo‐Cong Guo

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  25. Two Nonlinear Optical Thiophosphates Cu 5 Hg 0.5 P 2 S 8 and AgHg 3 PS 6 Activated by Their Tetrahedra-Stacking Architecture

    Inorganic Chemistry · 2022

    Yang Wang, Yuqiang Fang, Yunzhen Cao, Fuqiang Huang

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  26. A comprehensive review on metal chalcogenides with three-dimensional frameworks for infrared nonlinear optical applications

    Coordination Chemistry Reviews · 2022

    Hong Chen, Mao‐Yin Ran, Wenbo Wei, Xintao Wu, Hua Lin, Qi‐Long Zhu

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  27. d6versus d10, Which Is Better for Second Harmonic Generation Susceptibility? A Case Study of K2TGe3Ch8 (T = Fe, Cd; Ch = S, Se)

    Inorganic Chemistry · 2022

    Bingheng Ji, Fei Wang, Kui Wu, Bingbing Zhang, Jian Wang

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  28. Stereochemically active lone-pair-driven giant enhancement of birefringence from three-dimensional CsZn 4 Ga 5 Se 12 to two-dimensional CsZnAsSe 3

    Inorganic Chemistry Frontiers · 2023

    Chao Zhang, Mao‐Yin Ran, Xin Chen, Shenghua Zhou, Hua Lin, Yi Liu

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  29. Recent progress in the design of IR nonlinear optical materials by partial chemical substitution: Structural evolution and performance optimization

    Coordination Chemistry Reviews · 2023

    Mao‐Yin Ran, A-Yang Wang, Wenbo Wei, Xintao Wu, Hua Lin, Qi‐Long Zhu

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  30. Ga-based IR nonlinear optical materials: Synthesis, structures, and properties

    Coordination Chemistry Reviews · 2023

    Jiaxiang Zhang, Ping Feng, Mao‐Yin Ran, Xintao Wu, Hua Lin, Qi‐Long Zhu

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  31. Recent advances in rational structure design for nonlinear optical crystals: leveraging advantageous templates

    Chemical Society Reviews · 2024

    Ziting Yan, Jinbin Fan, Shilie Pan, Min Zhang

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  32. Infrared nonlinear optical materials with multiple strongly ionic cations

    Progress in Solid State Chemistry · 2024

    Yang Wang, Yuqiang Fang, Ruiqi Wang, Fuqiang Huang

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  33. Recent advances and future perspectives on rare-earth-based nonlinear optical materials with π-conjugated [XO3] (X = B, C, N) units

    Coordination Chemistry Reviews · 2024

    Bo Zhang, Mao‐Yin Ran, Xin‐Tao Wu, Hua Lin, Qi‐Long Zhu

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  34. Cationic substitution engineering induces a new quaternary chalcogenide in the A–M IIIA –M IVA –Q system for optical crystal applications

    CrystEngComm · 2025

    Yue Wang, Xuezhong Li, Zihao Lou, Yong‐Fang Shi

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  35. Exploring new horizons in mid-to-far infrared nonlinear optical crystals: the significant potential of trigonal pyramidal [TeS 3 ] 2− functional units

    Chemical Science · 2025

    Bo Zhang, Sheng-Hua Zhou, Bingxuan Li, Xin‐Tao Wu, Hua Lin, Qi‐Long Zhu

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  36. Structure-property relationships in IR nonlinear optical chalcogenides with stereochemically active lone pairs

    Coordination Chemistry Reviews · 2025

    Hong Chen, Xin‐Tao Wu, Hua Lin

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  37. Ba 10 Zn 7 Ga 6 S 26 : Promising Infrared Nonlinear Optical Crystal Exhibiting a High Laser Damage Threshold

    Zeitschrift für anorganische und allgemeine Chemie · 2025

    Li‐Wen Fan, Rui‐Xi Wang, Mengyue Li, Ling Chen, Li‐Ming Wu

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  38. Physicochemical and computational studies of diamond-like quaternary chalcogenide CsCd₄In₅Te₁₂

    Journal of Alloys and Compounds · 2026

    Karuppannan Aravinth, S. Raja, Manikandan Kandasamy, P. Balaji Bhargav

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  39. Mid‐ to Far‐Infrared Nonlinear Optical Crystals: Design Strategies, Structure–Property Relationships and Engineering Prospects

    Advanced Optical Materials · 2026

    Xiangran Kong, Jingdong Yan, Zi Wang, Hongwei Leng, Shichao Cheng, Sue Hao, Xiaoran Niu, Zuotao Lei, Chunhui Yang

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