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RESEARCH PAPER · Chemistry of Materials · 2016

Two New Non-centrosymmetric n = 3 Layered Dion–Jacobson Perovskites: Polar RbBi2Ti2NbO10 and Nonpolar CsBi2Ti2TaO10

Hyung Gu Kim, T. Thao Tran, Woongjin Choi, Tae‐Soo You, P. Shiv Halasyamani, Kang Min Ok

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Two New Non-centrosymmetric n = 3 Layered Dion–Jacobson Perovskites: Polar RbBi2Ti2NbO10 and Nonpolar CsBi2Ti2TaO10OriginalPolar Noncentrosymmetric ZnMoSb2O7 and Nonpolar Centrosymmetric CdMoSb4O10: d10 Transition Metal Size Effect Influencing the Stoichiometry and the Centricity38ChemInform Abstract: Two New Non‐Centrosymmetric n = 3 Layered Dion—Jacobson Perovskites: Polar RbBi2Ti2NbO10 and Nonpolar CsBi2Ti2TaO10.0Pb2BO3Cl: A Tailor‐Made Polar Lead Borate Chloride with Very Strong Second Harmonic Generation381Pb2BO3Cl: A Tailor‐Made Polar Lead Borate Chloride with Very Strong Second Harmonic Generation129A High Laser Damage Threshold and a Good Second-Harmonic Generation Response in a New Infrared NLO Material: LiSm3SiS725Na 6 Si 3 S 8 O: the first example of a sulfide silicate exhibiting unusual tri-polymerized [Si 3 S 8 O] 6− units without S–O bonds8Li2HgMS4 (M = Si, Ge, Sn): New Quaternary Diamond-Like Semiconductors for Infrared Laser Frequency Conversion64Synthesis, second-harmonic generations (SHG), and photoluminescence (PL) properties of Ca 4 Bi 6-x Ln x O 13 (Ln=La and Eu) solid solutions3New Compressed Chalcopyrite-like Li2BaMIVQ4 (MIV = Ge, Sn; Q = S, Se): Promising Infrared Nonlinear Optical Materials245Nanoarchitectonics in dielectric/ferroelectric layered perovskites: from bulk 3D systems to 2D nanosheets62NaBaM III Q 3 (M III = Al, Ga; Q = S, Se): first quaternary chalcogenides with isolated edge-sharing (MIII2Q 6 ) 6− dimers8Remarkable multimember-ring configurations in a new family of Na 7 M II Sb 5 S 12 (M II = Zn, Cd, Hg) exhibiting various three-dimensional tunnel structures25Effect of Element Substitution on Structural Transformation and Optical Performances in I2BaMIVQ4 (I = Li, Na, Cu, and Ag; MIV = Si, Ge, and Sn; Q = S and Se)63Ferroelectric Sr 3 Zr 2 O 7 : Competition between Hybrid Improper Ferroelectric and Antiferroelectric Mechanisms132Syntheses, Structures, and Properties of Non-Centrosymmetric Quaternary Tellurates BiMTeO6 (M = Al, Ga)21Two-Dimensional-Layered Perovskite ALaTa2O7:Bi3+ (A = K and Na) Phosphors with Versatile Structures and Tunable Photoluminescence115Functional layered materials with heavy metal lone pair cations, Pb 2+ , Bi 3+ , and Te 4+90Investigation on two new antimony-based quaternary chalcogenides: Na 6 CdSb 4 S 10 and Na 3 CdSbSe 41Bi2Te2O6(NO3)2(OH)2(H2O): A layered bismuth tellurium nitrate hydroxide with multiple noncentrosymmetric chromophores14β‐CsB9O14: A Triple‐Layered Borate with Edge‐Sharing BO4 Tetrahedra Exhibiting a Short Cutoff Edge and a Large Birefringence30Infrared Nonlinear Optical Polymorphs α- and β-SrCu 2 SnS 4 Exhibiting Large Second Harmonic Generation Responses with Requisite Phase-Matching Behavior442D organic‐inorganic hybrid perovskite materials for nonlinear optics131PbB5O7F3: A High-Performing Short-Wavelength Nonlinear Optical Material120Design of Lead-Free and Stable Two-Dimensional Dion–Jacobson-Type Chalcogenide Perovskite A′La2B3S10 (A′ = Ba/Sr/Ca; B = Hf/Zr) with Optimal Band Gap, Strong Optical Absorption, and High Efficiency for Photovoltaics30Synergistic Influence of d0 (Nb5+) and d10 (Cd2+) Cations in Stabilizing Noncentrosymmetric Dion–Jacobson Layered Perovskites, A′Cd2Nb3O10 (A′ = Rb, Cs)12Two Pyrophosphates with Large Birefringences and Second‐Harmonic Responses as Ultraviolet Nonlinear Optical Materials137Two Pyrophosphates with Large Birefringences and Second‐Harmonic Responses as Ultraviolet Nonlinear Optical Materials29Second harmonic generation in 2D layered materials120Phase transitions in RbPrNb2O7, a layer structured ferroelectric with a high Curie point26Tuning between Proper and Hybrid-Improper Mechanisms for Polar Behavior in Cs Ln 2Ti2NbO10 Dion-Jacobson Phases22Structural and thermal properties of La-containing Dion – Jacobson homologous series12Facile one-step synthesis and enhanced photocatalytic activity of a WC/ferroelectric nanocomposite8Pb 2 TiFO(SeO 3 ) 2 Br: a new polar compound with the strongest second harmonic generation in the selenite bromide family29Layered Double Perovskites75Solid-State NMR of Spin-9/2 Nuclei 115In and 209Bi in Functional Inorganic Complex Oxides0Solid‐state nuclear magnetic resonance of spin‐9/2 nuclei 115 In and 209 Bi in functional inorganic complex oxides8Structural Origin of Very Large Second-Harmonic Generation of a Layered Perovskite, Na0.5Bi2.5Nb2O921Synthesis and properties of layered perovskite-like compounds PbBi2Nb2O9 and PbBi3Ti2NbO122Review of experimental progress of hybrid improper ferroelectricity in layered perovskite oxides36Visible-light excited polar Dion–Jacobson Rb(Bi 1− x Eu x ) 2 Ti 2 NbO 10 perovskites: photoluminescence properties and in vitro bioimaging20Dion–Jacobson A′M iii NaNb 3 O 10 (A′ = Rb, Cs; M( iii ) = Sm, Bi) and RbSmNa 2 Nb 4 O 13 layered perovskites and their luminescent function8Wide bandgaps and strong SHG responses of hetero-oxyfluorides by dual-fluorination-directed bandgap engineering28Designing new polar materials1Harmonic Generation in Low‐Dimensional Materials44Uncovering the Structural Diversity and Excellent Performance of a Deep Ultraviolet Nonlinear Optical System Li(B2O3)nF (n= 1, 1.5, 2, and 3) by Multicomponent Prediction26Local atomic structure distortions in the Dion-Jacobson ferroelectric CsBiNb2O71Novel self-assembled two-dimensional layered oxide structure incorporated with Au nanoinclusions towards multifunctionalities11Synthesis, crystal structure and photocatalytic activity of new Dion-Jacobson type titanoniobates18Syntheses, structures, and optical properties of n = 3 layered Dion–Jacobson perovskites, RbEu2-Bi Ti2NbO10 (0 ≤ x ≤ 2)1Toward Large Second-Harmonic Generation and Deep-UV Transparency in Strongly Electropositive Transition Metal Sulfates112Second Harmonic Generation in the Polar A′SmNb2O7 (A′ = Rb, Cs) Dion–Jacobson Layered Perovskites11A Polar Tetragonal Tungsten Bronze with Colossal Second‐Harmonic Generation18Yb Substitution and Ultralow Thermal Conductivity of the Ca3–xYbxAlSb3 (0 ≤ x ≤ 0.81(1)) System5Dion–Jacobson (n = 2) Layered Perovskites (A′SmTa2O7; A′ = Rb, Cs) As Potential Ferroelectric Materials6Structural distortions leading to potential polar materials in n $=$ 3 and 4 Dion–Jacobson-layered perovskite series1Structural Phase Transitions in Layered Perovskite CsFeF4${\rm CsFeF}_{4}$ and Weak Polar Response in CsFeF4${\rm CsFeF}_{4}$/RbFeF4${\rm RbFeF}_{4}$ Superlattice0Synthesis, crystal structure and high-temperature investigation of new Dion-Jacobson type titanoniobates0

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  1. Polar Noncentrosymmetric ZnMoSb2O7 and Nonpolar Centrosymmetric CdMoSb4O10: d10 Transition Metal Size Effect Influencing the Stoichiometry and the Centricity

    Inorganic Chemistry · 2016-05-26

    Hongil Jo, Kang Min Ok

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  2. ChemInform Abstract: Two New Non‐Centrosymmetric n = 3 Layered Dion—Jacobson Perovskites: Polar RbBi2Ti2NbO10 and Nonpolar CsBi2Ti2TaO10.

    ChemInform · 2016-06-01

    Hyung Gu Kim, T. Thao Tran, Woongjin Choi, Tae‐Soo You, P. Shiv Halasyamani, Kang Min Ok

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  3. Pb2BO3Cl: A Tailor‐Made Polar Lead Borate Chloride with Very Strong Second Harmonic Generation

    Angewandte Chemie International Edition · 2016-08-24

    Guohong Zou, Chensheng Lin, Hongil Jo, Gnu Nam, Tae‐Soo You, Kang Min Ok

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  4. Pb2BO3Cl: A Tailor‐Made Polar Lead Borate Chloride with Very Strong Second Harmonic Generation

    Angewandte Chemie · 2016-08-24

    Guohong Zou, Chensheng Lin, Hongil Jo, Gnu Nam, Tae‐Soo You, Kang Min Ok

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  5. A High Laser Damage Threshold and a Good Second-Harmonic Generation Response in a New Infrared NLO Material: LiSm3SiS7

    Crystals · 2016-09-23

    Ni Zhen, Leyan Nian, Guangmao Li, Kui Wu, Shilie Pan

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  6. Na 6 Si 3 S 8 O: the first example of a sulfide silicate exhibiting unusual tri-polymerized [Si 3 S 8 O] 6− units without S–O bonds

    Dalton Transactions · 2017-01-01

    Kui Wu, Zhihua Yang, Shilie Pan

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  7. Li2HgMS4 (M = Si, Ge, Sn): New Quaternary Diamond-Like Semiconductors for Infrared Laser Frequency Conversion

    Crystals · 2017-04-12

    Kui Wu, Shilie Pan

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  8. Synthesis, second-harmonic generations (SHG), and photoluminescence (PL) properties of Ca 4 Bi 6-x Ln x O 13 (Ln=La and Eu) solid solutions

    Journal of Solid State Chemistry · 2017-05-04

    Hoyong Jung, Hongil Jo, Seung‐Jin Oh, Kang Min Ok

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  9. New Compressed Chalcopyrite-like Li2BaMIVQ4 (MIV = Ge, Sn; Q = S, Se): Promising Infrared Nonlinear Optical Materials

    Journal of the American Chemical Society · 2017-09-25

    Kui Wu, Bingbing Zhang, Zhihua Yang, Shilie Pan

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  10. Nanoarchitectonics in dielectric/ferroelectric layered perovskites: from bulk 3D systems to 2D nanosheets

    Dalton Transactions · 2017-11-22

    Minoru Osada, Takayoshi Sasaki

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  11. NaBaM III Q 3 (M III = Al, Ga; Q = S, Se): first quaternary chalcogenides with isolated edge-sharing (MIII2Q 6 ) 6− dimers

    Dalton Transactions · 2018-01-01

    Ailijiang Abudurusuli, Kui Wu, Yilimiranmu Rouzhahong, Zhihua Yang, Shilie Pan

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  12. Remarkable multimember-ring configurations in a new family of Na 7 M II Sb 5 S 12 (M II = Zn, Cd, Hg) exhibiting various three-dimensional tunnel structures

    Chemical Communications · 2018-01-01

    Kui Wu, Bingbing Zhang, Zhihua Yang, Shilie Pan

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  13. Effect of Element Substitution on Structural Transformation and Optical Performances in I2BaMIVQ4 (I = Li, Na, Cu, and Ag; MIV = Si, Ge, and Sn; Q = S and Se)

    Inorganic Chemistry · 2018-03-06

    Leyan Nian, Kui Wu, Guijie He, Zhihua Yang, Shilie Pan

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  14. Ferroelectric Sr 3 Zr 2 O 7 : Competition between Hybrid Improper Ferroelectric and Antiferroelectric Mechanisms

    Advanced Functional Materials · 2018-05-28

    Suguru Yoshida, Koji Fujita, Hirofumi Akamatsu, Olivier Hernandez, Arnab Sen Gupta, Forrest G. Brown, Haricharan Padmanabhan, Alexandra S. Gibbs, Toshihiro Kuge, Ryosuke Tsuji, Shunsuke Murai, James M. Rondinelli, Venkatraman Gopalan, Katsuhisa Tanaka

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  15. Syntheses, Structures, and Properties of Non-Centrosymmetric Quaternary Tellurates BiMTeO6 (M = Al, Ga)

    Inorganic Chemistry · 2018-06-15

    Fenghua Ding, Matthew Lander Nisbet, Hongwei Yu, Weiguo Zhang, Liyuan Chai, P. Shiv Halasyamani, Kenneth Reinhard Poeppelmeier

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  16. Two-Dimensional-Layered Perovskite ALaTa2O7:Bi3+ (A = K and Na) Phosphors with Versatile Structures and Tunable Photoluminescence

    ACS Applied Materials & Interfaces · 2018-07-03

    Guojun Zhou, Xingxing Jiang, Jing Zhao, Мaxim S. Моlokeev, Zheshuai Lin, Quanlin Liu, Zhiguo Xia

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  17. Functional layered materials with heavy metal lone pair cations, Pb 2+ , Bi 3+ , and Te 4+

    Chemical Communications · 2019-01-01

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  18. Investigation on two new antimony-based quaternary chalcogenides: Na 6 CdSb 4 S 10 and Na 3 CdSbSe 4

    New Journal of Chemistry · 2019-01-01

    Yi Huang, Xiaowen Wu, Sadeh Beysen

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  19. Bi2Te2O6(NO3)2(OH)2(H2O): A layered bismuth tellurium nitrate hydroxide with multiple noncentrosymmetric chromophores

    Journal of Solid State Chemistry · 2019-01-11

    Soyon Lee, Hongil Jo, Kang Min Ok

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  20. β‐CsB9O14: A Triple‐Layered Borate with Edge‐Sharing BO4 Tetrahedra Exhibiting a Short Cutoff Edge and a Large Birefringence

    Chemistry - A European Journal · 2019-06-18

    Shujuan Han, Chunmei Huang, Abudukadi Tudi, Shuaishuai Hu, Zhihua Yang, Shilie Pan

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  21. Infrared Nonlinear Optical Polymorphs α- and β-SrCu 2 SnS 4 Exhibiting Large Second Harmonic Generation Responses with Requisite Phase-Matching Behavior

    Chemistry of Materials · 2020-01-21

    Ya Feng Yang, Kui Wu, Bingbing Zhang, Xiaowen Wu, Ming‐Hsien Lee

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  22. 2D organic‐inorganic hybrid perovskite materials for nonlinear optics

    Nanophotonics · 2020-02-01

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  23. PbB5O7F3: A High-Performing Short-Wavelength Nonlinear Optical Material

    Chemistry of Materials · 2020-02-11

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  24. Design of Lead-Free and Stable Two-Dimensional Dion–Jacobson-Type Chalcogenide Perovskite A′La2B3S10 (A′ = Ba/Sr/Ca; B = Hf/Zr) with Optimal Band Gap, Strong Optical Absorption, and High Efficiency for Photovoltaics

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  25. Synergistic Influence of d0 (Nb5+) and d10 (Cd2+) Cations in Stabilizing Noncentrosymmetric Dion–Jacobson Layered Perovskites, A′Cd2Nb3O10 (A′ = Rb, Cs)

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  26. Two Pyrophosphates with Large Birefringences and Second‐Harmonic Responses as Ultraviolet Nonlinear Optical Materials

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  27. Two Pyrophosphates with Large Birefringences and Second‐Harmonic Responses as Ultraviolet Nonlinear Optical Materials

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  28. Second harmonic generation in 2D layered materials

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  29. Phase transitions in RbPrNb2O7, a layer structured ferroelectric with a high Curie point

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  30. Tuning between Proper and Hybrid-Improper Mechanisms for Polar Behavior in Cs Ln 2Ti2NbO10 Dion-Jacobson Phases

    Chemistry of Materials · 2020-09-22

    Vanessa A. Cascos, Jennifer Roberts-Watts, Chloe Skingle, Igor Levin, Weiguo Zhang, P. Shiv Halasyamani, Martin Christopher. Stennett, Neil Christian Hyatt, Éric Bousquet, Emma E. McCabe

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  31. Structural and thermal properties of La-containing Dion – Jacobson homologous series

    Journal of Solid State Chemistry · 2020-10-26

    Alexander Vladimirovich Knyazev, E.V. Syrov, О. В. Крашенинникова, Vladimir M. Kyashkin, Dmitry N. Titaev, Diana Georgievna Fukina

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  32. Facile one-step synthesis and enhanced photocatalytic activity of a WC/ferroelectric nanocomposite

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  33. Pb 2 TiFO(SeO 3 ) 2 Br: a new polar compound with the strongest second harmonic generation in the selenite bromide family

    Journal of Materials Chemistry C · 2021-01-01

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  34. Layered Double Perovskites

    Annual Review of Materials Research · 2021-05-05

    Hayden A. Evans, Lingling Mao, Ram Seshadri, Anthony Kevin Cheetham

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  35. Solid-State NMR of Spin-9/2 Nuclei 115In and 209Bi in Functional Inorganic Complex Oxides

    ChemRxiv · 2021-05-25

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  36. Solid‐state nuclear magnetic resonance of spin‐9/2 nuclei 115 In and 209 Bi in functional inorganic complex oxides

    Magnetic Resonance in Chemistry · 2021-06-03

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  37. Structural Origin of Very Large Second-Harmonic Generation of a Layered Perovskite, Na0.5Bi2.5Nb2O9

    Chemistry of Materials · 2021-08-04

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  38. Synthesis and properties of layered perovskite-like compounds PbBi2Nb2O9 and PbBi3Ti2NbO12

    Solid State Sciences · 2021-09-14

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  39. Review of experimental progress of hybrid improper ferroelectricity in layered perovskite oxides

    Journal of Physics D Applied Physics · 2021-10-22

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  40. Visible-light excited polar Dion–Jacobson Rb(Bi 1− x Eu x ) 2 Ti 2 NbO 10 perovskites: photoluminescence properties and in vitro bioimaging

    Journal of Materials Chemistry B · 2021-12-31

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  41. Dion–Jacobson A′M iii NaNb 3 O 10 (A′ = Rb, Cs; M( iii ) = Sm, Bi) and RbSmNa 2 Nb 4 O 13 layered perovskites and their luminescent function

    Journal of Materials Chemistry C · 2022-01-01

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  42. Wide bandgaps and strong SHG responses of hetero-oxyfluorides by dual-fluorination-directed bandgap engineering

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  43. Designing new polar materials

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  44. Harmonic Generation in Low‐Dimensional Materials

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  45. Uncovering the Structural Diversity and Excellent Performance of a Deep Ultraviolet Nonlinear Optical System Li(B2O3)nF (n= 1, 1.5, 2, and 3) by Multicomponent Prediction

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  46. Local atomic structure distortions in the Dion-Jacobson ferroelectric CsBiNb2O7

    Physical review. B./Physical review. B · 2022-07-06

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  47. Novel self-assembled two-dimensional layered oxide structure incorporated with Au nanoinclusions towards multifunctionalities

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  48. Synthesis, crystal structure and photocatalytic activity of new Dion-Jacobson type titanoniobates

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  49. Syntheses, structures, and optical properties of n = 3 layered Dion–Jacobson perovskites, RbEu2-Bi Ti2NbO10 (0 ≤ x ≤ 2)

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  50. Toward Large Second-Harmonic Generation and Deep-UV Transparency in Strongly Electropositive Transition Metal Sulfates

    Journal of the American Chemical Society · 2023-01-12

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