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RESEARCH PAPER · Angewandte Chemie International Edition · 2008

Capitalizing on Differing Coordination Environments and Redox Potentials to Prepare an Ordered Heterobimetallic UVI/NpIV Diphosphonate

Anna‐Gay D. Nelson, Travis H. Bray, Thomas E. Albrecht‐Schmitt

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Capitalizing on Differing Coordination Environments and Redox Potentials to Prepare an Ordered Heterobimetallic UVI/NpIV DiphosphonateOriginalThe actinides1Periodic Trends in Actinide Phosphonates: Divergence and Convergence between Thorium, Uranium, Neptunium, and Plutonium Systems471D and 3D arrays of isomeric cadmium(II) diphosphonates constructed from N,N-dimethylaminomethane-1,1-diphosphonate ligand5Homometallic UO22+ diphosphonates assembled under ambient and hydrothermal conditions29Hydrothermal Synthesis and Crystal Structures of Actinide Compounds2Novel double-chained or double-layered metal diphosphonates: synergic coordination effect of two closely linked phosphonate moieties promoted by large metal ionic radius10Neptunium Diverges Sharply from Uranium and Plutonium in Crystalline Borate Matrixes: Insights into the Complex Behavior of the Early Actinides Relevant to Nuclear Waste Storage74Neptunium Diverges Sharply from Uranium and Plutonium in Crystalline Borate Matrixes: Insights into the Complex Behavior of the Early Actinides Relevant to Nuclear Waste Storage8Synthesis and Characterization of 1‐, 2‐, and 3‐Dimensional Bimetallic UO22+/Zn2+ Phosphonoacetates66USING PHOSPHONATES TO PROBE STRUCTURAL DIFFERENCES BETWEEN TRANSURANIUM ELEMENTS AND THEIR PROPOSED SURROGATES24Cerium(IV), Neptunium(IV), and Plutonium(IV) 1,2-Phenylenediphosphonates: Correlations and Differences between Early Transuranium Elements and Their Proposed Surrogates54Advances in actinide solid-state and coordination chemistry37Two new layer structures of zinc(II) or strontium(II) diphosphonates based on N,N-dimethylaminomethane-1,1-diphosphonate ligand4Deviation Between the Chemistry of Ce(IV) and Pu(IV) and Routes to Ordered and Disordered Heterobimetallic 4f/5f and 5f/5f Phosphonates50Mixed-Valent Uranium(IV,VI) Diphosphonate: Synthesis, Structure, and Spectroscopy26Barium uranyl diphosphonates16Systematic Evolution from Uranyl(VI) Phosphites to Uranium(IV) Phosphates43Uranium diphosphonates templated by interlayer organic amines22From Order to Disorder and Back Again: In Situ Hydrothermal Redox Reactions of Uranium Phosphites and Phosphates28Regulation of Platelet Activity in a Changing Redox Environment13Ionothermal and Hydrothermal Flux Syntheses of Five New Uranyl Phosphonates43Three New Silver Uranyl Diphosphonates: Structures and Properties23Incorporation of Cu2+ Ions into Nanotubular Uranyl Diphosphonates28Use of 2,2-Bipyrimidine for the Preparation of UO22+-3d Diphosphonates18Structural chemistry of uranium phosphonates143Structural and spectroscopic characterization of two new layered uranyl(VI) p-xylenediphosphonate compounds synthesized via ionothermal method13Surprising coordination for low-valent actinides resembling uranyl( vi ) in thorium( iv ) organic hybrid layered and framework structures based on a graphene-like (6,3) sheet topology34Subtle Interactions and Electron Transfer between UIII, NpIII, or PuIII and Uranyl Mediated by the Oxo Group46Subtle Interactions and Electron Transfer between UIII, NpIII, or PuIII and Uranyl Mediated by the Oxo Group16Systematic Investigation of the in Situ Reduction Process from U(VI) to U(IV) in a Phosphonate System under Mild Solvothermal Conditions23New Uranyl Open Framework and Sheet Compounds Formed via In-Situ Protonation of Piperazine by Phosphorous Acid1Actinides12Synthesis of a heterobimetallic actinide nitride and an analysis of its bonding18The Structures of Metal–Organic Frameworks1The Structures of Metal–Organic Frameworks1The Structures of Metal–Organic Frameworks3The crystal and coordination chemistry of neptunium in all its oxidation states: An expanded structural hierarchy of neptunium compounds41An updated status and trends in actinide metal-organic frameworks (An-MOFs): From synthesis to application145f‐block MOFs: A Pathway to Heterometallic Transuranics29f‐block MOFs: A Pathway to Heterometallic Transuranics1

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  1. The actinides

    Annual Reports Section A (Inorganic Chemistry) · 2009-01-01

    S. A. Cotton

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  2. Periodic Trends in Actinide Phosphonates: Divergence and Convergence between Thorium, Uranium, Neptunium, and Plutonium Systems

    Inorganic Chemistry · 2009-04-06

    Anna‐Gay D. Nelson, Travis H. Bray, Forrest A. Stanley, Thomas E. Albrecht‐Schmitt

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  3. 1D and 3D arrays of isomeric cadmium(II) diphosphonates constructed from N,N-dimethylaminomethane-1,1-diphosphonate ligand

    Inorganic Chemistry Communications · 2009-10-31

    Zi‐Yi Du, Yu-Hui Sun, Yong‐Rong Xie, Jing Lin, He‐Rui Wen

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  4. Homometallic UO22+ diphosphonates assembled under ambient and hydrothermal conditions

    Dalton Transactions · 2010-01-01

    Karah E. Knope, Christopher L. Cahill

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  5. Hydrothermal Synthesis and Crystal Structures of Actinide Compounds

    Springer eBooks · 2010-01-01

    Wolfgang Runde, Mary P. Neu

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  6. Novel double-chained or double-layered metal diphosphonates: synergic coordination effect of two closely linked phosphonate moieties promoted by large metal ionic radius

    CrystEngComm · 2010-01-01

    Zi‐Yi Du, Yu-Hui Sun, Xiuzhi Zhang, Shu-Fen Luo, Yong‐Rong Xie, Dong‐Bei Wan

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  7. Neptunium Diverges Sharply from Uranium and Plutonium in Crystalline Borate Matrixes: Insights into the Complex Behavior of the Early Actinides Relevant to Nuclear Waste Storage

    Angewandte Chemie International Edition · 2010-01-18

    Shuao Wang, Evgeny V. Alekseev, Jie Ling, S. Skanthakumar, L. Soderholm, Wulf Depmeier, Thomas E. Albrecht‐Schmitt

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  8. Neptunium Diverges Sharply from Uranium and Plutonium in Crystalline Borate Matrixes: Insights into the Complex Behavior of the Early Actinides Relevant to Nuclear Waste Storage

    Angewandte Chemie · 2010-01-18

    Shuao Wang, Evgeny V. Alekseev, Jie Ling, S. Skanthakumar, L. Soderholm, Wulf Depmeier, Thomas E. Albrecht‐Schmitt

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  9. Synthesis and Characterization of 1‐, 2‐, and 3‐Dimensional Bimetallic UO22+/Zn2+ Phosphonoacetates

    European Journal of Inorganic Chemistry · 2010-01-29

    Karah E. Knope, Christopher L. Cahill

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  10. USING PHOSPHONATES TO PROBE STRUCTURAL DIFFERENCES BETWEEN TRANSURANIUM ELEMENTS AND THEIR PROPOSED SURROGATES

    Comments on Inorganic Chemistry · 2010-03-30

    Juan Diwu, Anna‐Gay D. Nelson, Thomas E. Albrecht‐Schmitt

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  11. Cerium(IV), Neptunium(IV), and Plutonium(IV) 1,2-Phenylenediphosphonates: Correlations and Differences between Early Transuranium Elements and Their Proposed Surrogates

    Inorganic Chemistry · 2010-10-04

    Juan Diwu, Shuao Wang, Zuolei Liao, Peter Carman Burns, Thomas E. Albrecht‐Schmitt

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  12. Advances in actinide solid-state and coordination chemistry

    MRS Bulletin · 2010-11-01

    Peter Carman Burns, Yasuhisa Ikeda, Ken Czerwinski

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  13. Two new layer structures of zinc(II) or strontium(II) diphosphonates based on N,N-dimethylaminomethane-1,1-diphosphonate ligand

    Journal of Molecular Structure · 2011-03-13

    Yu-Hui Sun, Zi‐Yi Du, Zhonggao Zhou, Shi‐Yong Zhang, Guohai Xu, Yong‐Rong Xie

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  14. Deviation Between the Chemistry of Ce(IV) and Pu(IV) and Routes to Ordered and Disordered Heterobimetallic 4f/5f and 5f/5f Phosphonates

    Inorganic Chemistry · 2011-04-25

    Juan Diwu, Shuao Wang, Justin J. Good, V.H. DiStefano, Thomas E. Albrecht‐Schmitt

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  15. Mixed-Valent Uranium(IV,VI) Diphosphonate: Synthesis, Structure, and Spectroscopy

    Inorganic Chemistry · 2012-03-29

    Juan Diwu, Thomas E. Albrecht‐Schmitt

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  16. Barium uranyl diphosphonates

    Journal of Solid State Chemistry · 2012-04-06

    Anna‐Gay D. Nelson, Evgeny V. Alekseev, Rodney Charles Ewing, Thomas E. Albrecht‐Schmitt

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  17. Systematic Evolution from Uranyl(VI) Phosphites to Uranium(IV) Phosphates

    Inorganic Chemistry · 2012-05-30

    Eric M. Villa, Connor J. Marr, Laurent J. Jouffret, Evgeny V. Alekseev, Wulf Depmeier, Thomas E. Albrecht‐Schmitt

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  18. Uranium diphosphonates templated by interlayer organic amines

    Journal of Solid State Chemistry · 2012-10-24

    Anna‐Gay D. Nelson, Evgeny V. Alekseev, Thomas E. Albrecht‐Schmitt, Rodney Charles Ewing

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  19. From Order to Disorder and Back Again: In Situ Hydrothermal Redox Reactions of Uranium Phosphites and Phosphates

    Inorganic Chemistry · 2013-01-09

    Eric M. Villa, Connor J. Marr, Juan Diwu, Evgeny V. Alekseev, Wulf Depmeier, Thomas E. Albrecht‐Schmitt

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  20. Regulation of Platelet Activity in a Changing Redox Environment

    Antioxidants and Redox Signaling · 2013-11-10

    Desmond D. Murphy, Emily C. Reddy, Niamh M. Moran, Sarah O'Neill

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  21. Ionothermal and Hydrothermal Flux Syntheses of Five New Uranyl Phosphonates

    Crystal Growth & Design · 2013-12-11

    T. Gannon Parker, Justin N. Cross, Matthew J. Polinski, Jian Hung Lin, Thomas E. Albrecht‐Schmitt

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  22. Three New Silver Uranyl Diphosphonates: Structures and Properties

    Inorganic Chemistry · 2014-02-13

    Anna‐Gay D. Nelson, Zsolt Rak, Thomas E. Albrecht‐Schmitt, Udo Becker, Rodney Charles Ewing

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  23. Incorporation of Cu2+ Ions into Nanotubular Uranyl Diphosphonates

    Inorganic Chemistry · 2014-04-04

    Pius O. Adelani, Nathaniel D. Cook, Jean‐Marie Babo, Peter Carman Burns

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  24. Use of 2,2-Bipyrimidine for the Preparation of UO22+-3d Diphosphonates

    Crystal Growth & Design · 2014-10-12

    Pius O. Adelani, Nathaniel D. Cook, Peter Carman Burns

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  25. Structural chemistry of uranium phosphonates

    Coordination Chemistry Reviews · 2015-05-30

    Weiting Yang, T. Gannon Parker, Zhong‐Ming Sun

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  26. Structural and spectroscopic characterization of two new layered uranyl(VI) p-xylenediphosphonate compounds synthesized via ionothermal method

    Inorganica Chimica Acta · 2015-07-04

    Tao Zheng, Yang Gao, Lanhua Chen, Juan Diwu, Zhifang Chai, Thomas E. Albrecht‐Schmitt, Shuao Wang

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  27. Surprising coordination for low-valent actinides resembling uranyl( vi ) in thorium( iv ) organic hybrid layered and framework structures based on a graphene-like (6,3) sheet topology

    Dalton Transactions · 2015-12-08

    Yuxiang Li, Zhehui Weng, Yanlong Wang, Lanhua Chen, Daopeng Sheng, Juan Diwu, Zhifang Chai, Thomas E. Albrecht‐Schmitt, Shuao Wang

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  28. Subtle Interactions and Electron Transfer between UIII, NpIII, or PuIII and Uranyl Mediated by the Oxo Group

    Angewandte Chemie International Edition · 2016-09-15

    Polly Louise Arnold, Michał S. Dutkiewicz, Markus Zegke, Olaf Walter, Christos Apostolidis, Emmalina Hollis, Anne‐Frédérique Pécharman, Nicola Magnani, Jean‐Christophe Griveau, Éric Colineau, R. Caciuffo, Xiaobin Zhang, Georg Schreckenbach, Jason B. Love

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  29. Subtle Interactions and Electron Transfer between UIII, NpIII, or PuIII and Uranyl Mediated by the Oxo Group

    Angewandte Chemie · 2016-09-15

    Polly Louise Arnold, Michał S. Dutkiewicz, Markus Zegke, Olaf Walter, Christos Apostolidis, Emmalina Hollis, Anne‐Frédérique Pécharman, Nicola Magnani, Jean‐Christophe Griveau, Éric Colineau, R. Caciuffo, Xiaobin Zhang, Georg Schreckenbach, Jason B. Love

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  30. Systematic Investigation of the in Situ Reduction Process from U(VI) to U(IV) in a Phosphonate System under Mild Solvothermal Conditions

    Inorganic Chemistry · 2017-05-26

    Lanhua Chen, Juan Diwu, Daxiang Gui, Yaxing Wang, Zhehui Weng, Zhifang Chai, Thomas E. Albrecht‐Schmitt, Shuao Wang

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  31. New Uranyl Open Framework and Sheet Compounds Formed via In-Situ Protonation of Piperazine by Phosphorous Acid

    Minerals · 2018-11-01

    Eric M. Villa, Justin N. Cross, Thomas E. Albrecht‐Schmitt

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  32. Actinides

    Elsevier eBooks · 2019-12-02

    Sascha T. Löffler, Karsten Meyer

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  33. Synthesis of a heterobimetallic actinide nitride and an analysis of its bonding

    Chemical Science · 2021-01-01

    Selena L. Staun, Guang Xin Wu, Wayne W. Lukens, Trevor W. Hayton

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  34. The Structures of Metal–Organic Frameworks

    Unknown journal · 2021-04-19

    Yuehong Wen, Xin‐Tao Wu, Qi‐Long Zhu

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  35. The Structures of Metal–Organic Frameworks

    Unknown journal · 2021-04-19

    Yuehong Wen, Xin‐Tao Wu, Qi‐Long Zhu

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  36. The Structures of Metal–Organic Frameworks

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    Yuehong Wen, Xin‐Tao Wu, Qi‐Long Zhu

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  37. The crystal and coordination chemistry of neptunium in all its oxidation states: An expanded structural hierarchy of neptunium compounds

    Coordination Chemistry Reviews · 2021-06-05

    Sara E. Gilson, Peter Carman Burns

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  38. An updated status and trends in actinide metal-organic frameworks (An-MOFs): From synthesis to application

    Coordination Chemistry Reviews · 2021-07-07

    Kai Lv, Sebastian Fichter, Mei Gu, Juliane März, Moritz Schmidt

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  39. f‐block MOFs: A Pathway to Heterometallic Transuranics

    Angewandte Chemie International Edition · 2022-11-30

    Kyoung Chul Park, Preecha Kittikhunnatham, Jaewoong Lim, Grace C. Thaggard, Yuan Liu, Corey R. Martin, Gabrielle A. Leith, Donald J. Toler, An T. Ta, Nancy R. Birkner, Ingrid Lehman‐Andino, Alejandra Hernandez-Jimenez, Gregory W. Morrison, Jake Amoroso, Hans‐Conrad zur Loye, D. P. DiPrete, Mark D. Smith, Kyle S. Brinkman, Simon Robert Phillpot, Natalia B. Shustova

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  40. f‐block MOFs: A Pathway to Heterometallic Transuranics

    Angewandte Chemie · 2022-11-30

    Kyoung Chul Park, Preecha Kittikhunnatham, Jaewoong Lim, Grace C. Thaggard, Yuan Liu, Corey R. Martin, Gabrielle A. Leith, Donald J. Toler, An T. Ta, Nancy R. Birkner, Ingrid Lehman‐Andino, Alejandra Hernandez-Jimenez, Gregory W. Morrison, Jake Amoroso, Hans‐Conrad zur Loye, D. P. DiPrete, Mark D. Smith, Kyle S. Brinkman, Simon Robert Phillpot, Natalia B. Shustova

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