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RESEARCH PAPER · Inorganic Chemistry · 2015

Series of SHG Materials Based on Lanthanide Borate–Acetate Mixed Anion Compounds

Hui Yang, Chun‐Li Hu, Xiang Xu, Jiang‐Gao Mao

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Series of SHG Materials Based on Lanthanide Borate–Acetate Mixed Anion CompoundsOriginalAlkali metal–alkaline earth metal borate crystal LiBa 3 (OH)(B 9 O 16 )[B(OH) 4 ] as a new deep-UV nonlinear optical material34Two novel pillared-layer lanthanide borates built by Ln@B 12 O 28/29 ring clusters and dicarboxylate linkers (Ln = Pr, Nd)26Evaluation of f-element borate chemistry76Structural and physical systematization of the nonlinear-optical borate crystals1Ln2Ga[B3O6(OH)]2[B7O9(OH)2](CH3CO2)2 (Ln = Y, Sm, Eu, Gd, Dy): A Series of Lanthanide Galloborates Decorated by Acetate Anions26K3B3O4(OH)4·2H2O: A UV Nonlinear Optical Crystal with Isolated [B3O4(OH)4]3– Anion Groups21Interrelationship of the structural and nonlinear-optical properties of the carbonate crystals2Ba 1.31 Sr 3.69 (BO 3 ) 3 Cl: A new structure type in the M 5 (BO 3 ) 3 Cl (M = bivalent cation) system12Na7[Ga2B13O24(OH)4]: A Luminescent Sodium Gallium Borate Containing Two Different Types of Oxoboron Framework Building Blocks4Solvent-controlled syntheses of mixed-alkali-metal borates exhibiting UV nonlinear optical properties23Two tartratoborates with hybrid anionic groups from unusual condensation reactions9(H 3 O)Ca 2 Zn 3.5 (PO 4 ) 4 and Ba 2 Cd 3 (PO 4 ) 2 (HPO 4 ) 2 : Syntheses, crystal structures and characterizations of two mixed metal phosphates12Comparative Interrelationship of the Structural, Nonlinear-Optical and Other Acentric Properties for Oxide, Borate and Carbonate Crystals16Lanthanide Inorganic Solids Based on Main Group Borates and Oxyanions of Lone Pair Cations12Recent advances in ultraviolet and deep-ultraviolet second-order nonlinear optical crystals257Syntheses, Crystal Structures and Properties of Two Novel Mixed Anion Hybrids with Formulas of Pb 6 O 2 (BO 3 ) 2 (C 2 O 4 ) and Pb 4 (CO 3 ) 2 (C 2 O 4 )(OH) 21From LiB3O5 to NaRbB6O9F2: Fluorine‐Directed Evolution of Structural Chemistry33Ferroelectric Property, Switchable Dielectric, and Excellent Second Harmonic Generation Response in a Homochiral Organic Salt: l -Prolinammonium 1-Adamantane Carboxylate13Ba 4 Bi 2 (Si 8−x B 4+x O 29 ) ( x = 0.09): a new acentric metal borosilicate as a promising nonlinear optical material53Three Cadmium Tartratoborates with Good Second Harmonic Generation (SHG) or Luminescence Performances10Competing Crystallization between Lanthanide and Actinide in Acidic Solution Leading to Their Efficient Separation27β‐CsB9O14: A Triple‐Layered Borate with Edge‐Sharing BO4 Tetrahedra Exhibiting a Short Cutoff Edge and a Large Birefringence30Prediction of Fluorooxoborates with Colossal Second Harmonic Generation (SHG) Coefficients and Extremely Wide Band Gaps: Towards Modulating Properties by Tuning the BO 3 /BO 3 F Ratio in Layers99Prediction of Fluorooxoborates with Colossal Second Harmonic Generation (SHG) Coefficients and Extremely Wide Band Gaps: Towards Modulating Properties by Tuning the BO3/BO3F Ratio in Layers24Experiment and First-Principles Calculations of A2Mg2TeB2O10 (A = Pb, Ba): Influences of the Cosubstitution on the Structure Transformation and Optical Properties21The tunable luminescent property and wide band gap in three 1D hybrid templated borates containing different metallic ions and oxoboron clusters7Synthesis, structure, and characterization of RbNdGe2O6 as a novel visible-light-driven catalyst for photodegradation methylene blue5High-Performance Second-Harmonic-Generation (SHG) Materials: New Developments and New Strategies323Recent advances in nonlinear optical rare earth structures63Magnetic Properties and Second Harmonic Generation of Noncentrosymmetric Cyanido-Bridged Ln(III)–W(V) Assemblies16Detection of Sub‐Terahertz Raman Response and Nonlinear Optical Effects for Luminescent Yb(III) Complexes31A 2 B 6 O 9 F 2 (A = NH 4 , K): new members of A 2 B 6 O 9 F 2 family with deep-UV cutoff edges and moderate birefringence17Noncentrosymmetric (C3H7N6)6(H2PO4)4(HPO4)·4H2O and Centrosymmetric (C3H7N6)2SO4·2H2O: Exploration of Acentric Structure by Combining Planar and Tetrahedral Motifs via Hydrogen Bonds37La2B3O4(OH)3(SO4)2: A new rare-earth borate-sulfate with second-harmonic generation response5KREP2Se6 (RE = Sm, Gd, Tb): The First Rare‐Earth Selenophosphates with Remarkable Nonlinear Optical Activities Realized by Synergistic Effect of RE‐ and P‐Based Motifs39Recent advances and future perspectives on rare-earth-based nonlinear optical materials with π-conjugated [XO3] (X = B, C, N) units66Ce-centered polyhedral arrangement pattern and optical performance in Ce-based nonlinear optical materials3Ternary Anion‐Engineered Rare Earth Crystals for Broadband UV Transparency and Enhanced Second‐Harmonic Generation1A Polar Cerium Iodate Ce 2 (IO 3 ) 6 (H 2 O) with a Strong Second-Harmonic Generation Response in Trivalent Ce-Based Materials1

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  1. Alkali metal–alkaline earth metal borate crystal LiBa 3 (OH)(B 9 O 16 )[B(OH) 4 ] as a new deep-UV nonlinear optical material

    Journal of Materials Chemistry C · 2016-01-01

    Chao Wu, Jun‐Ling Song, Longhua Li, Mark Graeme Humphrey, Chi Zhang

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  2. Two novel pillared-layer lanthanide borates built by Ln@B 12 O 28/29 ring clusters and dicarboxylate linkers (Ln = Pr, Nd)

    Dalton Transactions · 2016-01-01

    Lei-Lei Li, Rui Pan, Junwei Zhao, Bai‐Feng Yang, Guo‐Yu Yang

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  3. Evaluation of f-element borate chemistry

    Coordination Chemistry Reviews · 2016-03-19

    Mark A. Silver, Thomas E. Albrecht‐Schmitt

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  4. Structural and physical systematization of the nonlinear-optical borate crystals

    International Forum on Strategic Technology · 2016-06-01

    Vladimir K. Makukha, Boris I. Kidyarov

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  5. Ln2Ga[B3O6(OH)]2[B7O9(OH)2](CH3CO2)2 (Ln = Y, Sm, Eu, Gd, Dy): A Series of Lanthanide Galloborates Decorated by Acetate Anions

    Inorganic Chemistry · 2016-06-06

    Hui Yang, Chun‐Li Hu, Jiang‐Gao Mao

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  6. K3B3O4(OH)4·2H2O: A UV Nonlinear Optical Crystal with Isolated [B3O4(OH)4]3– Anion Groups

    Inorganic Chemistry · 2016-08-09

    Qiong Liu, Xiangyu Zhang, Zhihua Yang, Fangfang Zhang, Lili Liu, Jian Wei Han, Zhi Li, Shilie Pan

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  7. Interrelationship of the structural and nonlinear-optical properties of the carbonate crystals

    International Scientific-Technical Conference on Actual Problems of Electronics Instrument Engineering (APEIE) · 2016-10-01

    Boris I. Kidyarov, Vladimir K. Makukha

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  8. Ba 1.31 Sr 3.69 (BO 3 ) 3 Cl: A new structure type in the M 5 (BO 3 ) 3 Cl (M = bivalent cation) system

    Journal of Alloys and Compounds · 2016-12-26

    Jing Zhao, Lei Kang, Zheshuai Lin, Rukang K. Li

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  9. Na7[Ga2B13O24(OH)4]: A Luminescent Sodium Gallium Borate Containing Two Different Types of Oxoboron Framework Building Blocks

    Journal of Cluster Science · 2016-12-29

    Pei-Li Xu, Congcong Jin, Tingting Deng, Er-Rong Wang, Jian‐Wen Cheng

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  10. Solvent-controlled syntheses of mixed-alkali-metal borates exhibiting UV nonlinear optical properties

    Inorganic Chemistry Frontiers · 2017-01-01

    Chao Wu, Longhua Li, Jun‐Ling Song, Gang Yang, Mark Graeme Humphrey, Chi Zhang

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  11. Two tartratoborates with hybrid anionic groups from unusual condensation reactions

    Dalton Transactions · 2017-01-01

    Dong Yan, Fei‐Fei Mao, Tingting Ruan, Jiang‐Gao Mao

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  12. (H 3 O)Ca 2 Zn 3.5 (PO 4 ) 4 and Ba 2 Cd 3 (PO 4 ) 2 (HPO 4 ) 2 : Syntheses, crystal structures and characterizations of two mixed metal phosphates

    Journal of Solid State Chemistry · 2017-04-08

    Tong-Ying Chang, Chun‐Li Hu, Dong Yan, Jiang‐Gao Mao

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  13. Comparative Interrelationship of the Structural, Nonlinear-Optical and Other Acentric Properties for Oxide, Borate and Carbonate Crystals

    Crystals · 2017-04-12

    Boris I. Kidyarov

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  14. Lanthanide Inorganic Solids Based on Main Group Borates and Oxyanions of Lone Pair Cations

    Chinese Journal of Chemistry · 2017-11-17

    Fang Kong, Yun‐Xiang Ma, Jiang‐Gao Mao

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  15. Recent advances in ultraviolet and deep-ultraviolet second-order nonlinear optical crystals

    Coordination Chemistry Reviews · 2018-03-15

    Chao Wu, Gang Yang, Mark Graeme Humphrey, Chi Zhang

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  16. Syntheses, Crystal Structures and Properties of Two Novel Mixed Anion Hybrids with Formulas of Pb 6 O 2 (BO 3 ) 2 (C 2 O 4 ) and Pb 4 (CO 3 ) 2 (C 2 O 4 )(OH) 2

    ChemistrySelect · 2018-05-22

    Hui Yang, Fei‐Fei Mao, Cuixia Xu

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  17. From LiB3O5 to NaRbB6O9F2: Fluorine‐Directed Evolution of Structural Chemistry

    Chemistry - A European Journal · 2018-06-04

    Shujuan Han, Bingbing Zhang, Zhihua Yang, Shilie Pan

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  18. Ferroelectric Property, Switchable Dielectric, and Excellent Second Harmonic Generation Response in a Homochiral Organic Salt: l -Prolinammonium 1-Adamantane Carboxylate

    Crystal Growth & Design · 2018-09-14

    Shaopeng Chen, Changfeng Wang, Haitao Zhou, Yu‐Hui Tan, He‐Rui Wen, Yun‐Zhi Tang

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  19. Ba 4 Bi 2 (Si 8−x B 4+x O 29 ) ( x = 0.09): a new acentric metal borosilicate as a promising nonlinear optical material

    Chemical Science · 2018-10-31

    Ru‐Ling Tang, Chun‐Li Hu, Fei‐Fei Mao, Jiang-He Feng, Jiang‐Gao Mao

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  20. Three Cadmium Tartratoborates with Good Second Harmonic Generation (SHG) or Luminescence Performances

    Inorganic Chemistry · 2018-12-10

    Tingting Ruan, Chun‐Li Hu, Jiang-He Feng, Fei‐Fei Mao, Jiang‐Gao Mao

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  21. Competing Crystallization between Lanthanide and Actinide in Acidic Solution Leading to Their Efficient Separation

    Chinese Journal of Chemistry · 2018-12-14

    Xuemiao Yin, Yaxing Wang, Xiaoyan Li, Jian Xie, Mark A. Silver, Lanhua Chen, Daopeng Sheng, Guoxun Ji, Zhifang Chai, Shuao Wang

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  22. β‐CsB9O14: A Triple‐Layered Borate with Edge‐Sharing BO4 Tetrahedra Exhibiting a Short Cutoff Edge and a Large Birefringence

    Chemistry - A European Journal · 2019-06-18

    Shujuan Han, Chunmei Huang, Abudukadi Tudi, Shuaishuai Hu, Zhihua Yang, Shilie Pan

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  23. Prediction of Fluorooxoborates with Colossal Second Harmonic Generation (SHG) Coefficients and Extremely Wide Band Gaps: Towards Modulating Properties by Tuning the BO 3 /BO 3 F Ratio in Layers

    Angewandte Chemie International Edition · 2019-06-30

    Bingbing Zhang, Evgenii Tikhonov, Congwei Xie, Zhihua Yang, Shilie Pan

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  24. Prediction of Fluorooxoborates with Colossal Second Harmonic Generation (SHG) Coefficients and Extremely Wide Band Gaps: Towards Modulating Properties by Tuning the BO3/BO3F Ratio in Layers

    Angewandte Chemie · 2019-07-01

    Bingbing Zhang, Evgenii Tikhonov, Congwei Xie, Zhihua Yang, Shilie Pan

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  25. Experiment and First-Principles Calculations of A2Mg2TeB2O10 (A = Pb, Ba): Influences of the Cosubstitution on the Structure Transformation and Optical Properties

    Inorganic Chemistry · 2019-07-29

    Ming Wen, Hongping Wu, Cong Hu, Zhihua Yang, Shilie Pan

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  26. The tunable luminescent property and wide band gap in three 1D hybrid templated borates containing different metallic ions and oxoboron clusters

    Journal of Solid State Chemistry · 2019-11-05

    Jun-Xia Deng, Kang Zhou, Chun‐Yang Pan

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  27. Synthesis, structure, and characterization of RbNdGe2O6 as a novel visible-light-driven catalyst for photodegradation methylene blue

    Journal of Solid State Chemistry · 2020-02-08

    Jian‐Han Zhang, Xian-Dong Hao, Xin Wang, Zhizhong Su, Ju-Xiang Luo, Hongyan Wu, Fuxing Lin

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  28. High-Performance Second-Harmonic-Generation (SHG) Materials: New Developments and New Strategies

    Accounts of Chemical Research · 2021-05-27

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  29. Recent advances in nonlinear optical rare earth structures

    Journal of Rare Earths · 2021-07-15

    Jun Zhao, Dajiang Mei, Weikang Wang, Yuandong Wu, Dongfeng Xue

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  30. Magnetic Properties and Second Harmonic Generation of Noncentrosymmetric Cyanido-Bridged Ln(III)–W(V) Assemblies

    Inorganic Chemistry · 2021-07-28

    Kunal Kumar, Olaf Stefańczyk, Nicholas F. Chilton, Koji Nakabayashi, Kenta Imoto, Richard E. P. Winpenny, Shin‐ichi Ohkoshi

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  31. Detection of Sub‐Terahertz Raman Response and Nonlinear Optical Effects for Luminescent Yb(III) Complexes

    Advanced Optical Materials · 2021-11-01

    Kunal Kumar, Olaf Stefańczyk, Koji Nakabayashi, Kenta Imoto, Yurie Oki, Shin‐ichi Ohkoshi

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  32. A 2 B 6 O 9 F 2 (A = NH 4 , K): new members of A 2 B 6 O 9 F 2 family with deep-UV cutoff edges and moderate birefringence

    Chemical Communications · 2022-01-01

    Zilong Chen, Zi‐Jian Li, Dongdong Chu, Fangfang Zhang, Xiaojing Li, Zhihua Yang, Xifa Long, Shilie Pan

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  33. Noncentrosymmetric (C3H7N6)6(H2PO4)4(HPO4)·4H2O and Centrosymmetric (C3H7N6)2SO4·2H2O: Exploration of Acentric Structure by Combining Planar and Tetrahedral Motifs via Hydrogen Bonds

    Inorganic Chemistry · 2022-06-16

    Shu‐Fang Li, Liang Hu, Yao Ma, Fei‐Fei Mao, Jie Zheng, Xiu‐Du Zhang, Dong Yan

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  34. La2B3O4(OH)3(SO4)2: A new rare-earth borate-sulfate with second-harmonic generation response

    Journal of Solid State Chemistry · 2022-11-11

    Hui Yang, Ziyu Wang, Cuixia Xu, Yuan Hua Lin, Guoliang Liu

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  35. KREP2Se6 (RE = Sm, Gd, Tb): The First Rare‐Earth Selenophosphates with Remarkable Nonlinear Optical Activities Realized by Synergistic Effect of RE‐ and P‐Based Motifs

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    Zi‐Xia Chen, Chen‐Yi Zhao, Xiaohui Li, Wen‐Dong Yao, Wenlong Liu, Sheng‐Ping Guo

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  36. Recent advances and future perspectives on rare-earth-based nonlinear optical materials with π-conjugated [XO3] (X = B, C, N) units

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  37. Ce-centered polyhedral arrangement pattern and optical performance in Ce-based nonlinear optical materials

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  38. Ternary Anion‐Engineered Rare Earth Crystals for Broadband UV Transparency and Enhanced Second‐Harmonic Generation

    Chinese Journal of Chemistry · 2026-03-12

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  39. A Polar Cerium Iodate Ce 2 (IO 3 ) 6 (H 2 O) with a Strong Second-Harmonic Generation Response in Trivalent Ce-Based Materials

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