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RESEARCH PAPER · Small · 2023

Designing a Hybrid Perovskite with Enlarged Birefringence and Bandgap for Modulation of Light Polarization

Weiqi Huang, Xianyu Song, Yanqiang Li, Zhou Yang, Qian-Ting Xu, Yipeng Song, Han Wang, Minjuan Li, Sangen Zhao, Junhua Luo

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Designing a Hybrid Perovskite with Enlarged Birefringence and Bandgap for Modulation of Light PolarizationOriginalExceptional Optical Anisotropy Enhancement Achieved Through Dual‐Ions Cosubstitution Strategy in Novel Hybrid Bismuth Halides23A Highly Optical Anisotropic Hybrid Perovskite for Efficient Manipulation of Light Polarization64Halogen Bond Unlocks Ultra‐High Birefringence73Halogen Bond Unlocks Ultra‐High Birefringence14A Rare-Earth-Based Borate Optical Crystal with Enlarged Dihedral Angles of Distinct [BO3] Groups Exhibiting a Wide UV Transparent Range8Multiwavelength Temperature-Controlled Phase Modulator Based on Cs 4 PbBr 6 /CsPbBr 3 Perovskite Crystals1A Highly Optical Anisotropic Hybrid Metal Halide for Modulation and Generation of Polarized Light44Strategically designed anisotropic organic–inorganic metal halides (OIMHs) with superior balance between bandgap and birefringence12(C 6 H 5 N 2 )HgCl 3 : Discovery of a Polar Hg‐Based Hybrid Halide as Preeminent Nonlinear Optical and Birefringent Material Activated by π‐Conjugated Organic Cation Substitution38Highly stable and reversible birefringence switching triggered by thermally stimulated phase transition1Realizing large birefringence via S-substitution and anisotropic arrangement optimization4Designing Polar Covalent Hybrid Cadmium‐Based Chalcohalides Ultraviolet Nonlinear Optical Crystal with Strong Optical Anisotropy via Double‐Site Dual FBUs Tailoring25Giant Birefringence Enabled by the Highly Anisotropic Linear IX 2 − (X = Cl, Br) Building Blocks6Giant Birefringence Enabled by the Highly Anisotropic Linear IX 2 − (X = Cl, Br) Building Blocks32Achieving high symmetry and significant optical anisotropy in a hybrid metal halide25Light‐Programmable Positive‐Negative Photoconductivity Dual‐Mode Photodetection based on Up‐Conversion Nanoparticles/Perovskite Heterostructures5Controlling d10 Metal in Phenylthiourea‐Based Hybrid Metal Halides to Actualize Dimensional Transformation and Significantly Improve the Birefringence11Low‐Dimensional Organic–Inorganic Hybrid Metal Halide with Large Optical Anisotropy9Giant Birefringence Induced by Intermolecular Aromatic Interactions in Hydrogen‐Bonded Organic Frameworks37Five-Membered [C 5 O 5 ] 2 – Rings as Birefringence-Active Genes for Ultrabirefringent Crystals27CsGaGe₃Se₈: Enhanced optical anisotropy and bandgap via cation-substitution-driven dimensionality reduction0Covalent hybrid cadmium halides with heteroleptic tetrahedral units exhibiting a wideband nonlinear optical response0Rational design of large birefringence infrared oxychalcogenides via heteroanionic octahedron engineering0Unveiling the Superior Birefringence Property of a Record‐Birefringent Crystal with Unique Building Block12Unveiling the Superior Birefringence Property of a Record‐Birefringent Crystal with Unique Building Block4H/F Substitution Strategy in 0D Organic–Inorganic Hybrid Metal Cyanides Designing Ferroelastic Phase-Transition Materials3Significant Birefringence Enhancement via Cs + Alloying in Layered Perovskites: Synergistic Alignment of Organic Cations and Inorganic Framework1Linear Cyano Substitution Unlocks Highly Birefringent Tricyanomethanide1One-dimensional halide perovskite single crystals for optoelectronic applications1Heavy‐Halide Coordination and Lattice‐Confined Molecular Alignment Enable Giant Birefringence in Hybrid Metal Halides0Lateral‐Site Unblocking Enables Bilateral π ‐Chromophore Organization for Giant Birefringence in One‐Dimensional Lead Hybrids0Lateral‐Site Unblocking Enables Bilateral π ‐Chromophore Organization for Giant Birefringence in One‐Dimensional Lead Hybrids0

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  1. Exceptional Optical Anisotropy Enhancement Achieved Through Dual‐Ions Cosubstitution Strategy in Novel Hybrid Bismuth Halides

    Small · 2024-01-17

    Zhiyong Bai, Kang Min Ok

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  2. A Highly Optical Anisotropic Hybrid Perovskite for Efficient Manipulation of Light Polarization

    Advanced Functional Materials · 2024-05-08

    Jieyu Zheng, Xianyu Song, Yiran Wu, Yulong Lian, Yanqiang Li, Qian-Ting Xu, Yang Zhou, Ziyi Wang, Lei Wang, Junhua Luo, Sangen Zhao

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  3. Halogen Bond Unlocks Ultra‐High Birefringence

    Angewandte Chemie International Edition · 2024-07-10

    Jin Chen, Mingsheng Xu, Huai‐Yu Wu, Jun‐Yan Wu, Ke‐Zhao Du

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  4. Halogen Bond Unlocks Ultra‐High Birefringence

    Angewandte Chemie · 2024-07-10

    Jin Chen, Miao‐Bin Xu, Huai‐Yu Wu, Jun‐Yan Wu, Ke‐Zhao Du

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  5. A Rare-Earth-Based Borate Optical Crystal with Enlarged Dihedral Angles of Distinct [BO3] Groups Exhibiting a Wide UV Transparent Range

    Inorganic Chemistry · 2024-07-26

    Jie Song, Xianghao Kong, Conggang Li, Jinmiao Jiao, Yuheng She, Ning Ye, Zhanggui Hu, Yicheng Wu

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  6. Multiwavelength Temperature-Controlled Phase Modulator Based on Cs 4 PbBr 6 /CsPbBr 3 Perovskite Crystals

    ACS Photonics · 2024-09-04

    Xiaoting Wang, Qianxi Yin, Rongrong Xu, Yu Gu, Xianliang Huang, Mulin Li, Teng Ma, Ziyi Chen, Jun Chen, Haibo Zeng

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  7. A Highly Optical Anisotropic Hybrid Metal Halide for Modulation and Generation of Polarized Light

    Advanced Functional Materials · 2024-10-10

    Qian-Ting Xu, Ziyi Wang, Zhou Yang, Weiqi Huang, Yipeng Song, Jieyu Zheng, Yanqiang Li, Linxi Hou, Junhua Luo, Sangen Zhao

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  8. Strategically designed anisotropic organic–inorganic metal halides (OIMHs) with superior balance between bandgap and birefringence

    Inorganic Chemistry Frontiers · 2024-12-16

    Mingchang Wang, Huaiyu Wu, Miao‐Bin Xu, Jiajia Li, Ke‐Zhao Du, Jin Chen

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  9. (C 6 H 5 N 2 )HgCl 3 : Discovery of a Polar Hg‐Based Hybrid Halide as Preeminent Nonlinear Optical and Birefringent Material Activated by π‐Conjugated Organic Cation Substitution

    Advanced Optical Materials · 2024-12-30

    Ru‐Ling Tang, Die‐Xue Yang, Liang Ma, Yi‐Lei Lv, Wenlong Liu, Sheng‐Ping Guo

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  10. Highly stable and reversible birefringence switching triggered by thermally stimulated phase transition

    Inorganic Chemistry Frontiers · 2025-01-01

    Cheng Chen, Yunjie Bai, Qi Wu Shi, Mingye Han, Bingbing Zhang, Ying Wang

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  11. Realizing large birefringence via S-substitution and anisotropic arrangement optimization

    Inorganic Chemistry Frontiers · 2025-01-01

    Zhiwei Sun, Bingbing Wu, Zihao Yu, Qingran Ding, Yu‐Ling Wang, Ming Zhong, Sangen Zhao, Junhua Luo

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  12. Designing Polar Covalent Hybrid Cadmium‐Based Chalcohalides Ultraviolet Nonlinear Optical Crystal with Strong Optical Anisotropy via Double‐Site Dual FBUs Tailoring

    Small · 2025-01-26

    Yi‐Fan Fu, Wen‐Dong Yao, Jiajing Wu, Qiao‐Feng Huang, Yumei Zhang, Wenfeng Zhou, Wenlong Liu, Sheng‐Ping Guo

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  13. Giant Birefringence Enabled by the Highly Anisotropic Linear IX 2 − (X = Cl, Br) Building Blocks

    Angewandte Chemie · 2025-04-16

    Chong‐An Chen, Yang Li, Hongbo Huang, Congcong Jin, Bingbing Zhang, Kang Min Ok

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  14. Giant Birefringence Enabled by the Highly Anisotropic Linear IX 2 − (X = Cl, Br) Building Blocks

    Angewandte Chemie International Edition · 2025-04-16

    Chong‐An Chen, Yang Li, Hongbo Huang, Congcong Jin, Bingbing Zhang, Kang Min Ok

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  15. Achieving high symmetry and significant optical anisotropy in a hybrid metal halide

    Newton · 2025-05-01

    Weiqi Huang, Belal Ahmed, Yipeng Song, Xu Chen, Zhou Yang, Qian-Ting Xu, Kunpeng Wang, Yanqiang Li, Junhua Luo, Sangen Zhao

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  16. Light‐Programmable Positive‐Negative Photoconductivity Dual‐Mode Photodetection based on Up‐Conversion Nanoparticles/Perovskite Heterostructures

    Advanced Functional Materials · 2025-06-01

    Liangyu Wang, Zhenpeng Cheng, Tianle Wang, Bo Sun, Mingyu Li, Haifei Lu, Xiaoyan Wen, Jihoon H. Lee, Xin Tong, Sisi Liu

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  17. Controlling d10 Metal in Phenylthiourea‐Based Hybrid Metal Halides to Actualize Dimensional Transformation and Significantly Improve the Birefringence

    Advanced Optical Materials · 2025-07-20

    Yi‐Lei Lv, Ru‐Ling Tang, Liang Ma, Cheng Chen, Wenlong Liu, Sheng‐Ping Guo

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  18. Low‐Dimensional Organic–Inorganic Hybrid Metal Halide with Large Optical Anisotropy

    Advanced Optical Materials · 2025-08-05

    Siyu Li, Yakun Zhang, Dongxue Sun, Baoli Gao, Bingbing Zhang, Daqing Yang, Ying Wang

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  19. Giant Birefringence Induced by Intermolecular Aromatic Interactions in Hydrogen‐Bonded Organic Frameworks

    Advanced Materials · 2025-08-29

    Yayong Sun, Hongyuan Sha, Yanqiang Li, Yayu Yan, Weiqi Huang, Tao Ouyang, Liyang Qin, Siwen Zhang, Hao Huang, Qiaohong Li, Sangen Zhao, Chao He, Rongjian Sa, Jianguo Zhang, Tianhua Zhou

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  20. Five-Membered [C 5 O 5 ] 2 – Rings as Birefringence-Active Genes for Ultrabirefringent Crystals

    Journal of the American Chemical Society · 2025-09-16

    Jiachen Lu, Yang Li, Kang Min Ok

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  21. CsGaGe₃Se₈: Enhanced optical anisotropy and bandgap via cation-substitution-driven dimensionality reduction

    Inorganic Chemistry Communications · 2025-10-01

    Yue Wang, Rongfang Jiang, Zihao Lou, Yong‐Fang Shi

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  22. Covalent hybrid cadmium halides with heteroleptic tetrahedral units exhibiting a wideband nonlinear optical response

    Inorganic Chemistry Frontiers · 2026-01-01

    Yi-Fan Fu, Wen‐Dong Yao, Ruo‐Nan Li, Qiuwei Huang, Qiu-Xia Tang, Jiajing Wu, Sheng‐Ping Guo

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  23. Rational design of large birefringence infrared oxychalcogenides via heteroanionic octahedron engineering

    Chemical Communications · 2026-01-01

    Xinyao Qi, Haonan Liu, Yu-Jie Zhang, Shihui Ma, Hongping Wu, Zhanggui Hu, Hongwei Yu

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  24. Unveiling the Superior Birefringence Property of a Record‐Birefringent Crystal with Unique Building Block

    Angewandte Chemie International Edition · 2026-01-27

    Kaijie Xie, Zhiyong Bai, Weiqi Huang, Ji Qi, Tingjuan Lin, Muhammad Zeeshan, Yanqiang Li, Yang Zhou, Junhua Luo, Sangen Zhao

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  25. Unveiling the Superior Birefringence Property of a Record‐Birefringent Crystal with Unique Building Block

    Angewandte Chemie · 2026-01-27

    Kaijie Xie, Zhiyong Bai, Weiqi Huang, Ji Qi, Tingjuan Lin, Muhammad Zeeshan, Yanqiang Li, Yang Zhou, Junhua Luo, Sangen Zhao

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  26. H/F Substitution Strategy in 0D Organic–Inorganic Hybrid Metal Cyanides Designing Ferroelastic Phase-Transition Materials

    Inorganic Chemistry · 2026-02-09

    Luan-Ying Ji, Shuyi Liu, Jun-si Zhou, Zhilin Liao, Siqi Yu, Di Gao, H J Wang, Jian-Chun Liu, Kai-Wen Jiang, Xiao‐Gang Chen

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  27. Significant Birefringence Enhancement via Cs + Alloying in Layered Perovskites: Synergistic Alignment of Organic Cations and Inorganic Framework

    Advanced Optical Materials · 2026-02-25

    Weiqi Huang, Jin Zhou, Yipeng Song, Liangmeng Zhu, Ji Qi, Kaijie Xie, Yanqiang Li, Yang Zhou, Zhiyong Bai, Junhua Luo, Sangen Zhao

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  28. Linear Cyano Substitution Unlocks Highly Birefringent Tricyanomethanide

    ACS Materials Letters · 2026-03-24

    Bin Chen, Yanqiang Li, Weiqi Huang, Ji Qi, Xianyu Song, Yipeng Song, Zhenchao Bai, Yang Zhou, Junhua Luo, Sangen Zhao

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  29. One-dimensional halide perovskite single crystals for optoelectronic applications

    Journal of Applied Physics · 2026-04-13

    Zhenhua Chen, Yujie Yang, Zhiqiang Liu, Pengcheng Cai, Xiangfeng Wei, Jiehua Liu

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  30. Heavy‐Halide Coordination and Lattice‐Confined Molecular Alignment Enable Giant Birefringence in Hybrid Metal Halides

    Advanced Functional Materials · 2026-08-07

    Mingshu Zhang, Shuya Zhao, Zhen‐Cheng Wu, Zheyu Zhang, Sheng‐Ping Guo, Yan Zhou

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  31. Lateral‐Site Unblocking Enables Bilateral π ‐Chromophore Organization for Giant Birefringence in One‐Dimensional Lead Hybrids

    Angewandte Chemie International Edition · 2026-08-07

    Yu Yan, Yingzi Zhang, Liyi Zhang, Ling Huang, Yuqiao Zhou, Xuehua Dong, Guohong Zou

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  32. Lateral‐Site Unblocking Enables Bilateral π ‐Chromophore Organization for Giant Birefringence in One‐Dimensional Lead Hybrids

    Angewandte Chemie · 2026-08-07

    Yu Yan, Yingzi Zhang, Liyi Zhang, Ling Huang, Yuqiao Zhou, Xuehua Dong, Guohong Zou

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