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RESEARCH PAPER · Coordination Chemistry Reviews · 2023

A review of the relationship between the structure and nonlinear optical properties of organic-inorganic hybrid materials

Yuwei Kang, Qi Wu

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A review of the relationship between the structure and nonlinear optical properties of organic-inorganic hybrid materialsOriginal[(C 5 H 6 N 2 ) 2 H](Sb 4 F 13 ): a polyfluoroantimonite with a strong second harmonic generation effect60Advancing nonlinear optics: discovery and characterization of new non-centrosymmetric phenazine-based halides6An organic–inorganic hybrid perovskite material [Me 3 NCMe 3 ]GaCl 4 exhibits a two-step off–on–off SHG response with a large temperature interval6Ba 2 Ga 2 F 6 (IO 3 )(PO 4 ): the first fluoride-containing iodate-phosphate with a 1D [Ga 2 F 6 (IO 3 )(PO 4 )] 4− helix chain2Chemical modulation of A I RE III C IV QVI4 family compounds for band gap and optical anisotropy enhancement16Halide-driven polarity tuning and optimized SHG-bandgap balance in (C 4 H 11 N 2 )ZnX 3 (X = Cl, Br, I)34Noncentrosymmetric tellurite halides created by a depolymerization strategy: toward strong SHG intensity and wide bandgap16Wide band gap selenide infrared nonlinear optical materials A II Mg 6 Ga 6 Se 16 with strong SHG responses and high laser-induced damage thresholds31From C4H7N2Ge0.4Sn0.6Br3 to C6H11N2Ge0.4Sn0.6Br3: Effective Modulation of the Second Harmonic Generation Effect and Optical Band Gap by Planar π-Conjugated Organic Cation Size11Designing Optical Anisotropy: Silver-Aminoalkylpyridine Nitrate Complexes with Tunable Structures3Centrosymmetric CaBaMF8 and Noncentrosymmetric Li2CaMF8 (M = Zr, Hf): Dimension Variation and Nonlinear Optical Activity Resulting from an Isovalent Cation Substitution-Oriented Design17Magneto‐chiral Nonlinear Optical Effect with Large Anisotropic Response in Two‐Dimensional Halide Perovskite52Magneto‐chiral Nonlinear Optical Effect with Large Anisotropic Response in Two‐Dimensional Halide Perovskite3A Noncentrosymmetric Metal‐Free Borophosphate: Achieving a Large Birefringence and Excellent Stability by Covalent‐Linkage27Room-Temperature Phase Transition Material with Switchable Second-Order Nonlinear Optical Properties9Two Mixed Alkali Metal Isocyanurates with Wide Band Gap and Giant Birefringence2Photocatalysis toward Microplastics Conversion: A Critical Review150Nonlinear Optical Effects of Hybrid Antimony(III) Halides Induced by Stereoactive 5s 2 Lone Pairs and Trimethylammonium Cations23An Anisotropic Noncombustible Nanocomposite Based on a Fiberglass–Chitosan 3D Network for Building Insulation7Chiral Organic Cations and Distorted Inorganic Polyhedra Composing Metal Halide Nonlinear Optical Materials22Giant Anisotropic Thermal Expansion Phase Transition of Silver Iodide Anionic Organic–Inorganic Hybrid7All-Optical 3-Input XOR Gate Design Using 4:1 Optical Multiplexer with the Proper Application of Nonlinear Kerr Switches0Halogen Bond Unlocks Ultra‐High Birefringence74Halogen Bond Unlocks Ultra‐High Birefringence14Effects of ZnPc substrates on the electro-optical properties of MgSe thin films and the applications of Al/ZnPc/MgSe/(Ag, C, Au) hybrid devices as resonant negative capacitance sources0(C3N2H5)B3O3F2(OH)2: Realizing Large Birefringence via a Synergistic Effect between Anion F/OH‐Ratio Optimization and Cation Activation25Second-Order Nonlinear Switching and Photoluminescence Properties of Cd-Based Hybrid Perovskite with High-Temperature Phase Transition8A 9R-Type Hexagonal Perovskite Polytype Structure, Me3HyPbBr3, Exhibits Reversible Phase Transition and Fluorescent Semiconductor Properties4A zero-dimensional 1-butylpiperazine-cadmium(II) hybrid material: Synthesis, structural analysis, and DFT studies3Polar Thiazole Derivative-Induced Second Harmonic Response in Hybrid Bismuth Chlorate with Reversible Photochromism9Li2NaB3S2O12: A Deep-UV Transparent Borosulfate with Moderate Birefringence Derived from the [B3S2O12]∞ Infinite Chain Designed by the High Boron-to-Sulfur Ratio Strategy6The synthesis, structures and characterizations of (C5H12NO)4Cd3Cl10·2H2O and (C5H12NO)2BiCl6·H5O2 crystals0Design of hybrid Bi-Zr Perovskite polymer nanocomposites for multifunctional high-performance electrochemical and photonic applications3Halogen substitution effects in Chlorostannate(II) hybrid material: Insights from DFT study on 2(C4H4FN3O)·SnX6·2(H2O), (X = F, Cl, Br, I)0Nonlinear optical properties and structural characterization of a series of carboxyanilinium hydrogen selenite hybrids: Synthesis, first-principles calculations and correlation analysis for advanced photonic applications14Chiral-driven formation of hybrid cyanurates with large birefringence2Unconventional Heterobidentate Coordination of 4‐Hydroxypyridine Leading to Remarkably Strong Second‐Harmonic Generation in Zn(C 5 H 4 NO) 267Unconventional Heterobidentate Coordination of 4‐Hydroxypyridine Leading to Remarkably Strong Second‐Harmonic Generation in Zn(C 5 H 4 NO) 222Two l -Proline Cadmium Thiocyanates with Moderate Second-Harmonic-Generation Responses and Large Birefringences13Design and synthesis of PDSPTCF as an influential Brønsted-Lewis acidic catalyst for the producing benzo[a]benzo[6,7]chromeno[2,3-c]phenazines1Computer‐Aided Development of New Nonlinear Optical Materials38Computer‐Aided Development of New Nonlinear Optical Materials14Strategically designed anisotropic organic–inorganic metal halides (OIMHs) with superior balance between bandgap and birefringence13Supramolecular Assembly Enhanced Linear and Nonlinear Chiroptical Properties of Chiral Manganese Halides9Supramolecular Assembly Enhanced Linear and Nonlinear Chiroptical Properties of Chiral Manganese Halides48“All-four-in-one”: a novel mercury tellurite–nitrate Hg 3 (TeO 3 )(Te 3 O 7 )(NO 3 ) 2 exhibiting exceptional optical anisotropy29A chloride-doped Cu 18 nanocluster: synthesis, bonding and nonlinear optical properties7Dynamic control of halide perovskite structures for tailored ferroelectric and second-order nonlinear optical functionalities39Hg[CS(NH 2 ) 2 ] 4 (SiF 6 ): a fluorosilicate crystal with large birefringence achieved via multi-functional group modification6Ligand substitution in organic–inorganic hybrid zinc iodides for second-harmonic generation8One-dimensional silver iodide homo-helical chains induced by achiral ammonium featuring second-order optical nonlinearity1Structural chemistry of antimony( iii ) oxalates with lone pairs: polyhedral distortion [SbO 4 F 2 ], π-conjugation [C 2 O 4 ], and birefringence tuning1Unveiling the Effects of Conjugated Gradient Bridges: Inducing Intramolecular Charge Transfer Significantly Enhances Nonlinear Response0X-ray luminescent metal–organic frameworks: design strategies and functional applications22Cationic Modification in Hybrid Iodates: A Pathway to Superior Performance13Electron density distribution in bis(guanidinium) disodium hypodiphosphate heptahydrate, (CH 6 N 3 ) 2 Na 2 (P 2 O 6 )·7H 2 O1Chemical Substitution‐Driven Design of a High‐Performance Noncentrosymmetric Bismuth Molybdenum Selenite10Guest-Molecule-Induced Glass-Crystal Transition in Organic–Inorganic Hybrid Antimony 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Fluoride10Chemisorption of Emerging Contaminants (F−, AsIII/V, Pb2+) Using MOF for Sustainable Water Treatment: A Critical Review13Rational design of a high-efficiency lead halide organic-inorganic hybrid nonlinear optical switch via molecular engineering5Properties of blown composite films of polypropylene/calcium carbonate and polypropylene/calcium oxide1A novel Zero-Dimensional trimer framework with dielectric switching Characteristic in Organic-Inorganic hybrid materials2Advances in Nanoelectronics: Carbon Nanotubes, Graphene, and Smart Polymers: A review10Multifunctional Cd‐based Hybrid with Large Birefringence Achieving Excellent Second Harmonic Generation and Reversible Temperature‐Activated Fluorescence for Anti‐counterfeiting16[C(NH2)3]Y(HCOO)4: Constructing 3D Framework for Guanidine-Based UV Nonlinear Optical Crystals with Good Performance8Planar [HgCl 3 ] and V‑Shaped [HgCl 2 ] Units Synergistically Creating a Prominent Halide Birefringent Crystal β ‐CsHg 2 Cl 5 with 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Transmission Range and Large SHG Response7Investigation of the electronic structural and optical properties of CN2H5HgI3 single crystal0Tunable optical properties and enhanced nonlinear performance of Cr@Cr₂O₃ films via laser power modulation1Structural, spectral, dielectric, and nonlinear optical properties of 2,4,6-Trinitrophenol with optical limiting behavior3Theoretical investigation of noncentrosymmetric Ruddlesden-Popper germanium perovskites Cs 2 Ge X 4 ( X = Cl , Br, and I) for second harmonic generation0Synthesis, characterization, nonlinear optical properties, and DFT analysis of a new azo-Schiff base dye2Achieving Ultra‐High Optical Anisotropy via Structural Regulation and Coplanar Engineering of Extended π‐Conjugated [H 2–x C 3 N 3 S 3 ] (x = 1, 2) Groups3Coordination Polyhedron‐Selective Luminescence and Efficient X‐Ray Scintillation of Zn 2+ ‐Doped Cesium Cadmium Chloride Perovskites2Unveiling nonlinear absorption properties of 2,4-dihydroxybenzoic acid and nicotine amide metal complexes for optical limiting applications2(C 4 H 8 N 5 )(PhPHO 2 )·H 2 O: a polar ionic cocrystal with strong second-harmonic generation and high birefringence0[Rb 4 Cl][Cd 11 In 9 Se 26 ]: a salt inclusion chalcogenide with a diamond-like framework for infrared nonlinear optics0A[N(SO 2 NH 2 ) 2 ] (A = Na, K, Rb, and Cs): enhancing birefringence of non π-conjugated deep-ultraviolet crystals via novel dimeric disulfonamide [N(SO 2 NH 2 ) 2 ] − groups0Achieving an optimal performance balance in UV nonlinear optical crystals via hydrogen-bond regulation1Cation-dominated second-harmonic generation in chiral tetrahydro-1-naphthylammonium halides0Chiral Eu–K Metal–organic Framework Based on Lactate Derivative and Its Second-Order Nonlinear Optical Properties0Crystal structure, phase transitions, and Hirshfeld surface analysis of the organic–inorganic hybrid [N(CH 3 ) 2 (C 2 H 5 )(i-Pr)] 2 ZnBr 4 compound0Halide anion-mediated crystal structure engineering in guanidinoacetic acid halides for tunable birefringence0Halogen-ion-driven polymorphs for high-performance nonlinear optical crystalline materials3In-plane optical anisotropy and nonlinear optical effects in 2D InTeO 3 Cl0Isoniazid nitrate: synergistic dual π-conjugation triggering prominent second-harmonic generation0KGdSiSe 4 and KGdGeSe 4 : two rare earth-based selenides with wide bandgaps and large nonlinear optical responses0Polyhedral replacement-guided design of Ce3MnGaSe7 featuring strong second-harmonic genera-tion and high laser-induced damage threshold0Stable lead succinate-iodides with strong second-harmonic generation response and large birefringence0Suppressing antiparallel dipole alignment: A molecular engineering strategy toward sem-organic UV NLO crystals0Synergism of [C 2 N 4 H 7 S] cations and anionic modulators: tailoring second-order nonlinear optics and birefringence in organic–inorganic crystals6Unit Symmetry‐Breaking and Layered Linear Ordering Enabling Superior Short‐Wave Ultraviolet Birefringent Crystal9Unit Symmetry‐Breaking and Layered Linear Ordering Enabling Superior Short‐Wave Ultraviolet Birefringent Crystal2Zn 4 (BO 3 ) 2 (CO 2 CH 2 NH 2 ) 2 ·H 2 O: An Organic–Inorganic Hybridized KBe 2 BO 3 F 2 -like Ultraviolet Nonlinear Optical Crystal3The Metal Coordination Effects on the Optoelectronic Properties of Perylene Diimide and Nucleotide Supramolecular Complex (GMP:PDI: Ag(I)/Co(II)/Zn(II)): Computational and Experimental Studies3Nonlinear Optical Responses in One-Dimensional Zinc Thiocyanates Functionalized with Natural Amino Acids81D Cobalt‐Cytidine Monophosphate Coordination Polymer Exhibiting Efficient Ultraviolet Second‐Harmonic Generation8Coordination Geometry-Directed Optical Anisotropy and Phase-Matched Nonlinear Optics in Chiral Metal–Organic Frameworks2Enhanced tripling-performance in [C(NH2)3]4P2O7·H2O as UV nonlinear optical material due to π-conjugated cation and hydrogen bonding intervention1Controllable Photoluminescence Modulation of 2D Hybrid Materials Based on (DFCBA) 2 PbX 4 (X = I, Br) via Halogen Regulation2Hydrogen-Bond-Directed Assembly of an Intramolecular Charge-Transfer Compound for Second-Order Nonlinear Optics1Polar Antiperovskite Oxides: Promising Mid-Infrared Nonlinear Optical Materials with Strong Second-Harmonic Generation3KNa2(Hf,Zr)F7 and KNa2HfF7: isostructural fluorides with phase-matchable second-harmonic generation0Chirality-driven polar lattice engineering for high-performance organic nonlinear optical crystals3Optical, Thermal and Mechanical Properties of Creatininium 5-Sulphosalicylate Organic Crystal for Optical Limiting Applications3Structural analysis of Pb-based organic–inorganic metal halide perovskites modified with Cetyltrimethylammonium bromide and 2-Aminopyrazine: Effects on stability and band gap0Recent Progress in Hg-Based Oxysalt Crystals for Nonlinear Optics and Birefringence Applications5Eco-sustainable cellulose/polyaniline/GO@TiO2 bio-nanocomposites for efficient dye removal from wastewater1Strong Optical Nonlinearity in Polar Hypophosphites via Chiral Cation Assembly1K 3 Mg 2 [K 6 MgCl 3 ][Ga 20 S 36 ]: A Diamond-like Framework Based on Mixed-Type Supertetrahedra for Excellent Nonlinear Optical Property1Enhancement of nonlinear optical properties in germanium clusters via copper doping and charge modulation: a density functional theory study0Unlocking Nonlinear Optics and Photoluminescence with Simultaneous Enhancement of Bandgap and Birefringence in Hybrid Sb-Based Halides2Single Crystal Growth and Characterization of Semi-Organic L-Phenylalanine Barium Chloride via Slow Evaporation Method0Second-order nonlinear optical organic crystals exhibit reversible photoisomerization0Potassium-Stabilized 2H-Type Indium Sulfide in the Noncentrosymmetric Crystal K0.33[Zn0.33In1.67S3] Probed by Azimuthal SHG0Research advances in rare-earth nonlinear optical crystalline materials in 20251Growth and Investigation of the Nonlinear Optical Electrical and Antibacterial Properties of Organic Single Crystal: P‐Toluidinium p‐Toluenesulfonate0Machine Learning for Second‐ and Third‐Harmonic Generation: Benchmarks, Challenges, and a Roadmap for Data‐Driven Photonic Materials0Designing Novel Solar‐Blind Ultraviolet Nonlinear Optical Crystals Based on Local Proton Distribution Complementary Effect0Designing Novel Solar‐Blind Ultraviolet Nonlinear Optical Crystals Based on Local Proton Distribution Complementary Effect0Local Aromatic Overlap Microregulation Enables Birefringence Enhancement in Isocompositional Hybrid Antimony Halides1Optical limiting properties of MAPbBr 3 PQD/TPU composite films0Reversible Symmetry Switching, Giant Birefringence, and UV Second‐Harmonic Generation in Hybrid Niobium Oxyfluorides0Reversible Symmetry Switching, Giant Birefringence, and UV Second‐Harmonic Generation in Hybrid Niobium Oxyfluorides0Linear vs bent carbazole isomers: Molecular-shape-dependent assessment of their linear and nonlinear optical properties across gaseous and solvated phases0pH-controlled fabrication of halloysite/Congo red hybrid pigments with tunable color and enhanced chemical stability0The static nonlinear optical properties of imidazole-based π-Conjugated Scaffolds in Organic Electronics: Experimental synthesis and theoretical investigation0Coordination chemistry of Sb(III)-based optical crystals: from lone-pair-induced distortion to birefringence and second-harmonic generation0A Composition-Matched Intermediate Reveals Site-Specific Symmetry Evolution with Retained Second-Harmonic Generation in Supertetrahedral Sulfides0

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  1. [(C 5 H 6 N 2 ) 2 H](Sb 4 F 13 ): a polyfluoroantimonite with a strong second harmonic generation effect

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  3. An organic–inorganic hybrid perovskite material [Me 3 NCMe 3 ]GaCl 4 exhibits a two-step off–on–off SHG response with a large temperature interval

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  4. Ba 2 Ga 2 F 6 (IO 3 )(PO 4 ): the first fluoride-containing iodate-phosphate with a 1D [Ga 2 F 6 (IO 3 )(PO 4 )] 4− helix chain

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  5. Chemical modulation of A I RE III C IV QVI4 family compounds for band gap and optical anisotropy enhancement

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  34. Halogen substitution effects in Chlorostannate(II) hybrid material: Insights from DFT study on 2(C4H4FN3O)·SnX6·2(H2O), (X = F, Cl, Br, I)

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