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RESEARCH PAPER · Journal of the American Chemical Society · 2025

Conversion of Compositionally Diverse Plastic Waste over Earth-Abundant Sulfides

Esun Selvam, Zoé O. G. Schyns, Jessie A. Sun, Pavel A. Kots, Yeonsu Kwak, LaShanda T. J. Korley, Raúl F. Lobo, Dionisios G. Vlachos

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Conversion of Compositionally Diverse Plastic Waste over Earth-Abundant SulfidesOriginalBase-Metal Heterogeneous Catalysts for Upgrading Plastics to Light Olefins3Selective hydrocracking of polyolefin waste into branched liquid fuels over a non-noble metal bifunctional Ni–W/ZrO 2 catalyst4Tandem Catalysis to Mitigate Coke Formation in the Upcycling of Mixed Polyolefin Wastes11Speciation of Nitrogen‐Containing Molecules in the Distilled Fractions of Plastic Pyrolysis Oils Using Comprehensive Two‐Dimensional Gas Chromatography Coupled With High‐Resolution Mass Spectrometry and a Nitrogen Chemiluminescence Detector2Plasma catalytic hydrogenolysis of polyethylene to gasoline-range fuels over Sm/USY catalysts10Toward Sustainable Plastic Waste Valorization: Green Synergistic Catalytic Strategies for Plastic Upcycling12Development of highly efficient and sulfur-tolerant metal catalysts via carbon layer encapsulation for nitro-compound hydrogenation2Solvent swelling-induced microstructural modulation of polypropylene for targeted pyrolysis: Product distribution and pyrolysis mechanisms explored through experimental and DFT investigations2Identification of organochlorides in distilled fractions of plastic pyrolysis oil using GC × GC coupled with high-resolution time-of-flight mass spectrometry (GC × GC-HR-TOFMS) and GC coupled with a halogen selective detector (GC-XSD)1Intrinsically Bifunctional and Tunable Tungsten Carbide Catalysts Enable Efficient PVC-Compatible Polyolefin Hydrocracking8Recent developments in recycling technologies for polymeric plastics8Biodegradability and sustainability of biopolymers and composites0Contaminant-Tolerant Conversion of Polyethylene Waste to α-Olefins6Direct upcycling of mixed plastic waste into liquid alkanes3Hydrogen bond regulation to enhance catalytic C–C bond cleavage of polylactic acid wastes in H 2 O to produce H 20Current perspective on heterogeneous thermal catalytic approaches for closed-loop polyolefin plastic recycling1Rational design of bifunctional catalysts for hydrocracking of polyethylene waste plastics to narrow-distributed liquid fuels4Structure–performance relationships in heterogeneous catalysts for polyolefin plastic hydroconversion1iPDA-Assisted Design of Hierarchical Beta Zeolites for the Sustainable Upcycling of Polyethylene to Naphtha with Ultra-Low Pt Loading1Hydrotreatment of Nylon 66 and Amide Model Compounds Over Sulfided NiMo Catalysts0A Panoramic View on Plastic Waste Recycling and Upcycling: Heterogeneous Catalytic Strategies for Diverse Plastics and Multiple Pathways6Co 1 /Ru Single‐Atom Alloy Catalyst for Sustainable Polypropylene Hydrogenolysis to Long‐Chain Liquid Products1Bifunctional nanocatalyst design for polyolefin hydrocracking2Catalyst-free, microdroplet-mediated waste plastic conversion to diacids4Comprehensive quantitative analysis of polyolefin hydrogenolysis toward plastic waste management0Challenges in polyolefin re/upcycling catalysis specific to polymer feedstock0

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  1. Base-Metal Heterogeneous Catalysts for Upgrading Plastics to Light Olefins

    Research · 2025-01-01

    Zhen Yu, Yafei Fan, Fawei Lin

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  2. Selective hydrocracking of polyolefin waste into branched liquid fuels over a non-noble metal bifunctional Ni–W/ZrO 2 catalyst

    Journal of Materials Chemistry A · 2025-01-01

    Changhu Leng, Hui Li, Qifeng Zhou, Chenyang Ma, Yongchao Wang, Shengdong Zhang, Chuanya Li, Wanglei Wang, Zhi-Jun Li

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  3. Tandem Catalysis to Mitigate Coke Formation in the Upcycling of Mixed Polyolefin Wastes

    Journal of the American Chemical Society · 2025-08-14

    Jiayang Zhao, Qikun Hu, Yuqi Wang, Yizhen Che, Zhiqiang Niu

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  4. Speciation of Nitrogen‐Containing Molecules in the Distilled Fractions of Plastic Pyrolysis Oils Using Comprehensive Two‐Dimensional Gas Chromatography Coupled With High‐Resolution Mass Spectrometry and a Nitrogen Chemiluminescence Detector

    Journal of Separation Science · 2025-09-01

    Bruno da Costa Magalhães, Pascal Pijcke, Niels Verhoosel, Ron Bassie, Philip Janssen, Cesare Benedetti, Matthijs Ruitenbeek, Georgios Bellos, Melissa N. Dunkle

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  5. Plasma catalytic hydrogenolysis of polyethylene to gasoline-range fuels over Sm/USY catalysts

    Applied Catalysis B: Environmental · 2025-09-08

    Chengxin Hou, Yanan Diao, Tianqi Yun, Jianhui Han, Tianhao Shi, Bingbing Chen, Chuan Shi

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  6. Toward Sustainable Plastic Waste Valorization: Green Synergistic Catalytic Strategies for Plastic Upcycling

    Advanced Sustainable Systems · 2025-10-10

    Luyao Zhang, Junliang Chen, Jinzhou Li, Jing Wu, Pin Gao, Jianping Yang

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  7. Development of highly efficient and sulfur-tolerant metal catalysts via carbon layer encapsulation for nitro-compound hydrogenation

    Carbon · 2025-11-17

    Wei He, Yanni Li, Liang Wu, Shuhan Dong, Hao Su, Haodong Tang, Xiao‐Nian Li, Chunshan Lu

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  8. Solvent swelling-induced microstructural modulation of polypropylene for targeted pyrolysis: Product distribution and pyrolysis mechanisms explored through experimental and DFT investigations

    Fuel · 2025-11-20

    Shanglong Zhang, Qiuxiang Yao, Yongliang Wang, Wei Wang, Lei He, Linyang Wang, Ming Sun

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  9. Identification of organochlorides in distilled fractions of plastic pyrolysis oil using GC × GC coupled with high-resolution time-of-flight mass spectrometry (GC × GC-HR-TOFMS) and GC coupled with a halogen selective detector (GC-XSD)

    The Analyst · 2025-12-05

    Bruno da Costa Magalhães, Pascal Pijcke, Niels Verhoosel, Philip Janssen, Cesare Benedetti, Matthijs Ruitenbeek, Georgios Bellos, Melissa N. Dunkle

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  10. Intrinsically Bifunctional and Tunable Tungsten Carbide Catalysts Enable Efficient PVC-Compatible Polyolefin Hydrocracking

    Journal of the American Chemical Society · 2025-12-17

    Uchenna C. Nwachukwu, Matthew J. Moegling, Sinhara M. H. D. Perera, Arsalaan Nisar Pathan, Jun Chen, Fereshteh Rezvani, Aswathi Rajeevan Vannante Valappil, Cong Zhou, Lamisa Rahman, Jian Liu, Sung Min Kim, James M. Eagan, Siddharth Deshpande, Marc D. Porosoff, Linxiao Chen

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  11. Recent developments in recycling technologies for polymeric plastics

    Polymer Chemistry · 2025-12-29

    Zhihao Wang, En Fang, Liangyu Chen, Zhiqiang Fan, Shaofei Song

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  12. Biodegradability and sustainability of biopolymers and composites

    Elsevier eBooks · 2026-01-01

    Aissata Ousmane Kane, Ibrahima Gueye Faye, B.D. Ngom, Alain Dufresne

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  13. Contaminant-Tolerant Conversion of Polyethylene Waste to α-Olefins

    ACS Sustainable Chemistry & Engineering · 2026-01-01

    Carlos Posada, Hongwei Sun, Adrian DiMarco, Nuwayo Eric Munyaneza, Oscar Valenzuela, Candace E. Wall, Guoliang Liu

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  14. Direct upcycling of mixed plastic waste into liquid alkanes

    Energy & Environmental Science · 2026-01-01

    Hongshun Ran, Shen Run-jie, Wenyi Ni, Mengying Zheng, Xinyang Sun, Shuo Zhang, Zhiqiang Wang, Shourong Zheng, Xiaolei Qu, Yaxuan Jing

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  15. Hydrogen bond regulation to enhance catalytic C–C bond cleavage of polylactic acid wastes in H 2 O to produce H 2

    Green Chemistry · 2026-01-01

    Jianfeng Wang, Zirui Peng, Ziyue Hou, Shuaijun Huang, Tianliang Lu, Yuxuan Liu, Xin Liu, Xiaoqin Si

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  16. Current perspective on heterogeneous thermal catalytic approaches for closed-loop polyolefin plastic recycling

    Discover Chemistry. · 2026-01-20

    Haokun Wang, Dermot O’Hare

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  17. Rational design of bifunctional catalysts for hydrocracking of polyethylene waste plastics to narrow-distributed liquid fuels

    CHINESE JOURNAL OF CATALYSIS (CHINESE VERSION) · 2026-02-11

    Zhe Ma, Chenzhao Wang, Peng Xu, Xin Zhou, Xiang Feng, De Chen

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  18. Structure–performance relationships in heterogeneous catalysts for polyolefin plastic hydroconversion

    Applied Catalysis A General · 2026-03-09

    Haokun Wang, Frederick Z.T. Yang, Supatpong Juntarawatt, Yiyang Li, Roland C. Turnell‐Ritson

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  19. iPDA-Assisted Design of Hierarchical Beta Zeolites for the Sustainable Upcycling of Polyethylene to Naphtha with Ultra-Low Pt Loading

    ACS Sustainable Chemistry & Engineering · 2026-04-27

    Guojing Shi, Zhenlei Zhang, Yuliang Li, Xiaochun Zhu, Zhenchen Tang, Zhentao Chen, Y Chen, Jiaqi Feng, bingyu li, Xiangping Zhang

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  20. Hydrotreatment of Nylon 66 and Amide Model Compounds Over Sulfided NiMo Catalysts

    ChemCatChem · 2026-05-01

    Boda Yang, Cheng Zhu, Oliver Y. Gutiérrez, Sungmin Kim, Huamin Wang

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  21. A Panoramic View on Plastic Waste Recycling and Upcycling: Heterogeneous Catalytic Strategies for Diverse Plastics and Multiple Pathways

    Advanced Materials · 2026-05-12

    Chang‐Jie Yang, Xin-Yu Wang, Mei‐Qi Zhu, Tianyou Zhao, Yong-Zhou Pan, Yuhai Dou, Jie Yang, Zechao C. Zhuang, Zhenglong Li, Zhijun Wu, Wen‐Gang Cui, Hongge Pan, Weiwei Li, Dingsheng S. Wang

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  22. Co 1 /Ru Single‐Atom Alloy Catalyst for Sustainable Polypropylene Hydrogenolysis to Long‐Chain Liquid Products

    Advanced Materials · 2026-06-10

    Yuzhen Ge, Yimeng Jin, Alexandra Krestnikova, Sibei Zou, Antonio José Martín, Gonzalo Guillén‐Gosálbez, Javier Pérez‐Ramírez

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  23. Bifunctional nanocatalyst design for polyolefin hydrocracking

    Nature Nanotechnology · 2026-07-01

    Shuheng Tian, Mufan Li, Weimin Yang, Jihong Yu, Ding Ma

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  24. Catalyst-free, microdroplet-mediated waste plastic conversion to diacids

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    Ruiliang Gao, Liwei Zhang, Richard J. Lewis, Hao Wang, Zhiyan Pan, Yage Zhang, Zekai Yu, Zhiqiang Liu, Xiaolin Guo, Xiangbowen Du, Wencong Liu, Minghang Li, Shipan Liang, Bing Lu, Ichiro Daigo, Shanjun Mao, Graham John Hutchings, Yong Wang

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  25. Comprehensive quantitative analysis of polyolefin hydrogenolysis toward plastic waste management

    Nature Protocols · 2026-07-24

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  26. Challenges in polyolefin re/upcycling catalysis specific to polymer feedstock

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