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RESEARCH PAPER · Crystal Growth & Design · 2022

Explorations of Second-Order Nonlinear Optical Materials in the Monovalent Trithiocyanurate System

Xia Hao, Chensheng Lin, Ning Ye, Donghong Lin, Dan Zhao, Yuqiao Zhou, Enbo Shangguan, Min Luo

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Explorations of Second-Order Nonlinear Optical Materials in the Monovalent Trithiocyanurate SystemOriginalCs 2 Mg(H 2 C 3 N 3 S 3 ) 4 ·8H 2 O: An Excellent Birefringent Material with Giant Optical Anisotropy in π-Conjugated Trithiocyanurate19Recent progress of newly developed functional building units and corresponding nonlinear optical materials14Large second harmonic generation and birefringence from extended octupolar π-conjugated structures35Amino substitution strategy achieves significant blue shift while preserving high optical anisotropy: A2(H3C3N4S2)2•H2O (A =NH4, K, Rb, Cs)6Assisting the Effective Design of an SBBO-Like Vanadium-Iodate Crystal with Mixed Metal Cations2Decoupling the SHG‐Birefringence Trade‐off in UV NLO Materials via Triple‐Control Coordination Engineering: Achieving Synergistic Performance Optimization88Decoupling the SHG‐Birefringence Trade‐off in UV NLO Materials via Triple‐Control Coordination Engineering: Achieving Synergistic Performance Optimization13Giant Birefringence and Solar‐Blind Ultraviolet Transmission by Coordination‐Induced Assembly of π‐Conjugated Pyridine–Carboxylate8Giant Birefringence and Solar‐Blind Ultraviolet Transmission by Coordination‐Induced Assembly of π‐Conjugated Pyridine–Carboxylate24(CN4H7)H2C3N3S3: Trithiocyanurate Exhibiting Giant Optical Anisotropy via Weak Interaction-Mediated Functional Module Alignment3Regulating the coplanarity of π-conjugated units through hydrogen bonding in FAHC2O4 and FAH2C3N3S3 crystals5Achieving Ultra‐High Optical Anisotropy via Structural Regulation and Coplanar Engineering of Extended π‐Conjugated [H 2–x C 3 N 3 S 3 ] (x = 1, 2) Groups3Na2(C6H4NO3)2·H2O: A promising ultraviolet nonlinear optical crystal with strong second-harmonic generation effect and large birefringence1Confinement-assembled ultraviolet nonlinear optical crystal from pyridine-expanded π-systems with exhibiting strong SHG and birefringence18Unveiling the Superior Birefringence Property of a Record‐Birefringent Crystal with Unique Building Block12Unveiling the Superior Birefringence Property of a Record‐Birefringent Crystal with Unique Building Block4Ultrawide Bandgap and Record-High Birefringence in a Covalent Beryllium-Organic Framework7Decoupling Contributions of Distinct Strategies for Enhancing Polarizability Anisotropy in Crystals Containing π-Conjugated Groups0

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  1. Cs 2 Mg(H 2 C 3 N 3 S 3 ) 4 ·8H 2 O: An Excellent Birefringent Material with Giant Optical Anisotropy in π-Conjugated Trithiocyanurate

    Inorganic Chemistry · 2023-05-11

    Xia Hao, Chensheng Lin, Min Luo, Yuqiao Zhou, Ning Ye, Enbo Shangguan

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  2. Recent progress of newly developed functional building units and corresponding nonlinear optical materials

    Chinese Journal of Structural Chemistry · 2023-05-11

    Wenjing Tan, Chenyang Zhang, Chenyang Zhang, Tingting Huang, Bingbing Zhang

    Read original paper ↗ ·

  3. Large second harmonic generation and birefringence from extended octupolar π-conjugated structures

    Chemical Science · 2024-01-01

    Danyang Dou, Bingbing Zhang, Daqing Yang, Ying Wang

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  4. Amino substitution strategy achieves significant blue shift while preserving high optical anisotropy: A2(H3C3N4S2)2•H2O (A =NH4, K, Rb, Cs)

    Chinese Chemical Letters · 2024-11-10

    Shuang Zhao, Fei Jia, Kaibei Zhan, Rui‐Xi Wang, Pengfei Tan, Lin Shen, Li‐Ming Wu, Ling Chen

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  5. Assisting the Effective Design of an SBBO-Like Vanadium-Iodate Crystal with Mixed Metal Cations

    Crystal Growth & Design · 2025-05-22

    Xia Hao, Xuan Liu, Ruijie Wang, Chensheng Lin, Min Luo, Guang Peng, Tao Yan, Ning Ye

    Read original paper ↗ ·

  6. Decoupling the SHG‐Birefringence Trade‐off in UV NLO Materials via Triple‐Control Coordination Engineering: Achieving Synergistic Performance Optimization

    Angewandte Chemie International Edition · 2025-05-22

    Yaolong Zhu, Jie Gou, Can Yang, Qingwen Zhu, Yi Xiong, Qi Wu

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  7. Decoupling the SHG‐Birefringence Trade‐off in UV NLO Materials via Triple‐Control Coordination Engineering: Achieving Synergistic Performance Optimization

    Angewandte Chemie · 2025-05-22

    Yaolong Zhu, Jie Gou, Can Yang, Qingwen Zhu, Yi Xiong, Qi Wu

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  8. Giant Birefringence and Solar‐Blind Ultraviolet Transmission by Coordination‐Induced Assembly of π‐Conjugated Pyridine–Carboxylate

    Angewandte Chemie · 2025-06-02

    Peng-Hui Guo, Xia Zhang, Yao Guo, Nan Zhang, Yi-Gang Chen, Xingxing Jiang, Zheshuai Lin, Xian‐Ming Zhang

    Read original paper ↗ ·

  9. Giant Birefringence and Solar‐Blind Ultraviolet Transmission by Coordination‐Induced Assembly of π‐Conjugated Pyridine–Carboxylate

    Angewandte Chemie International Edition · 2025-06-02

    Peng‐Hui Guo, Xia Zhang, Xia Zhang, Yao Guo, Nan Zhang, Yi‐Gang Chen, Xingxing Jiang, Zheshuai Lin, Xian‐Ming Zhang, Xian‐Ming Zhang

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  10. (CN4H7)H2C3N3S3: Trithiocyanurate Exhibiting Giant Optical Anisotropy via Weak Interaction-Mediated Functional Module Alignment

    Inorganic Chemistry · 2025-08-19

    Xia Hao, Y.K. Su, Chensheng Lin, Min Luo, Lingli Wu, Ruijie Wang, Xin Wen, Ning Ye

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  11. Regulating the coplanarity of π-conjugated units through hydrogen bonding in FAHC2O4 and FAH2C3N3S3 crystals

    Chinese Journal of Structural Chemistry · 2025-09-06

    Yi‐Chang Yang, Rui‐Xi Wang, Li‐Ming Wu, Ling Chen

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  12. Achieving Ultra‐High Optical Anisotropy via Structural Regulation and Coplanar Engineering of Extended π‐Conjugated [H 2–x C 3 N 3 S 3 ] (x = 1, 2) Groups

    Advanced Functional Materials · 2025-12-12

    Muhammad Arif, Xu Liu, Hangwei Jia, Zhihua Yang, Xueling Hou, Shilie Pan

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  13. Na2(C6H4NO3)2·H2O: A promising ultraviolet nonlinear optical crystal with strong second-harmonic generation effect and large birefringence

    Chinese Journal of Structural Chemistry · 2025-12-23

    Xuan Pang, Leyan Nian, Yongzhang Wang, Chunmei Huang

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  14. Confinement-assembled ultraviolet nonlinear optical crystal from pyridine-expanded π-systems with exhibiting strong SHG and birefringence

    Science China Chemistry · 2026-01-04

    Chunmei Huang, Xuan Pang, Fuming M. Li, Shumei Cao, Shilie Pan, Miriding Mutailipu

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  15. Unveiling the Superior Birefringence Property of a Record‐Birefringent Crystal with Unique Building Block

    Angewandte Chemie International Edition · 2026-01-27

    Kaijie Xie, Zhiyong Bai, Weiqi Huang, Ji Qi, Tingjuan Lin, Muhammad Zeeshan, Yanqiang Li, Yang Zhou, Junhua Luo, Sangen Zhao

    Read original paper ↗ ·

  16. Unveiling the Superior Birefringence Property of a Record‐Birefringent Crystal with Unique Building Block

    Angewandte Chemie · 2026-01-27

    Kaijie Xie, Zhiyong Bai, Weiqi Huang, Ji Qi, Tingjuan Lin, Muhammad Zeeshan, Yanqiang Li, Yang Zhou, Junhua Luo, Sangen Zhao

    Read original paper ↗ ·

  17. Ultrawide Bandgap and Record-High Birefringence in a Covalent Beryllium-Organic Framework

    Journal of the American Chemical Society · 2026-04-21

    Peng-Hui Guo, Xia Zhang, Xia Zhang, Miriding Mutailipu, Sangen Zhao, Nan Zhang, Yao Guo, Lei Huai, Yi-Gang Chen, Xian-Ming Zhang, Xian-Ming Zhang

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  18. Decoupling Contributions of Distinct Strategies for Enhancing Polarizability Anisotropy in Crystals Containing π-Conjugated Groups

    Inorganic Chemistry · 2026-08-23

    Haoran Liu, Chenhui Hu, Xueli Du, Qingyu Liu, Xiaona Li, Zhihua Yang, Min Zhang

    Read original paper ↗ ·
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