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RESEARCH PAPER · Chemical Science · 2024

Large second harmonic generation and birefringence from extended octupolar π-conjugated structures

Danyang Dou, Bingbing Zhang, Daqing Yang, Ying Wang

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Large second harmonic generation and birefringence from extended octupolar π-conjugated structuresOriginal“Three functions in one”: multifunctional rare-earth cyamelurates with magnetism, luminescence, and giant optical nonlinearity6Exploring ultra-high optical anisotropy in polyiodides7Hydrogen bonding regulation-oriented design of pyridine sulfonate as a promising UV birefringent crystal characterized by enhanced structural anisotropy11Double Sb‐N Coordination Enables Record‐High Birefringence in UV‐Transparent Crystals71Double Sb‐N Coordination Enables Record‐High Birefringence in UV‐Transparent Crystals8Ultra‐High Optical Anisotropy with UV Transmission Achieved by Rational Arrangement of Extended π‐Conjugated Groups5Ultra‐High Optical Anisotropy with UV Transmission Achieved by Rational Arrangement of Extended π‐Conjugated Groups46Hydrogen‐Bonded Assembly of Functional Units for Constructing Linear and Nonlinear Optical Crystals10Polar Lithium l -Aspartate Monohydrate: A Semiorganic Ultraviolet Transparent Nonlinear Optical Crystal1Designing an all-organic wide bandgap ultraviolet nonlinear optical crystal3A novel metal-free crystal demonstrating superior birefringence attributed to the synergistic interaction of dual π-conjugated units8Designing Hybrid Sb-Based Nonlinear Optical Crystals with Large Birefringence by Combining the Lone Pair and π-Conjugated Genes10Achieving the birefringence-bandgap trade-off: Hydrogen-bond engineered biuret-cyanurate14Low‐Dimensional Organic–Inorganic Hybrid Metal Halide with Large Optical Anisotropy9Enhancing Birefringence via a Planar‐Conformation‐Locking Strategy3Five-Membered [C 5 O 5 ] 2 – Rings as Birefringence-Active Genes for Ultrabirefringent Crystals27Sulfonated Module Aggregation for Ultrahigh Birefringence in Aqueous-Processable Crystals26Enhanced Second Harmonic Generation Response via Rational Design of Iodinated π-Conjugated Pyridine Group5Insights into the Strong Nonlinear Optical Ability of Functionalized Pyridinium-Benzimidazole Derivatives0K 2 ZnMoP 2 O 10 : crystal growth, optical characterization, and structure–property insights into phase matching0The condensation of π-conjugated units: a new paradigm for designing high-performance optical crystals4Confinement-assembled ultraviolet nonlinear optical crystal from pyridine-expanded π-systems with exhibiting strong SHG and birefringence18The modulation of structural polarity facilitating the gradient enhancement of second harmonic generation effects in hybrid metal halides5Halogen‐Bond Coupled Halogenated‐π‐Conjugation Enables Giant Birefringence in Hydrogen‐Bonded Organic Frameworks13Unveiling the Superior Birefringence Property of a Record‐Birefringent Crystal with Unique Building Block12Unveiling the Superior Birefringence Property of a Record‐Birefringent Crystal with Unique Building Block4Ultrawide Bandgap and Record-High Birefringence in a Covalent Beryllium-Organic Framework7Noncovalent Assembly Engineering Achieves Excellent Birefringence in Crystals0Synthesis, structural characterization, and hyperpolarizability studies of novel barbituric acid and coumarin derivatives2Redox‐Driven Strategy Enabling Leapfrog Enhancement of Birefringence in Layered Tin‐Based Optical Crystals1Interlayer Electronic Decoupling Unlocks Giant Birefringence in π‐Conjugated Metal‐Organic Frameworks0Steric‐Guided Coordination Engineering Enables Significantly Optimized Optical Anisotropy via Sulfur‐Driven [C 5 H 5 NS] Birefringence‐Active Groups0Reversible Symmetry Switching, Giant Birefringence, and UV Second‐Harmonic Generation in Hybrid Niobium Oxyfluorides0Reversible Symmetry Switching, Giant Birefringence, and UV Second‐Harmonic Generation in Hybrid Niobium Oxyfluorides0A novel tetrafluoroborate with giant birefringence assembled from biocompatible adenine0

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  1. “Three functions in one”: multifunctional rare-earth cyamelurates with magnetism, luminescence, and giant optical nonlinearity

    Chemical Science · 2025-01-01

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  2. Exploring ultra-high optical anisotropy in polyiodides

    Inorganic Chemistry Frontiers · 2025-01-01

    Mingye Han, Hongbo Huang, Siyu Li, Xiao Yan, Bingbing Zhang, Ying Wang

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  3. Hydrogen bonding regulation-oriented design of pyridine sulfonate as a promising UV birefringent crystal characterized by enhanced structural anisotropy

    Chemical Science · 2025-01-01

    Longyun Xu, Conggang Li, Shuaifeng Li, Huijian Zhao, Xianghao Kong, Zaixin Qu, Wen-Jie Feng, Ke Xu, Ning Ye, Zhanggui Hu

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  4. Double Sb‐N Coordination Enables Record‐High Birefringence in UV‐Transparent Crystals

    Angewandte Chemie International Edition · 2025-03-11

    Pu Zhang, Xuehua Dong, Ling Huang, Zhien Lin, Yuqiao Zhou, Guohong Zou

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  5. Double Sb‐N Coordination Enables Record‐High Birefringence in UV‐Transparent Crystals

    Angewandte Chemie · 2025-03-11

    Pu Zhang, Xuehua Dong, Ling Huang, Zhien Lin, Yuqiao Zhou, Guohong Zou

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  6. Ultra‐High Optical Anisotropy with UV Transmission Achieved by Rational Arrangement of Extended π‐Conjugated Groups

    Angewandte Chemie · 2025-03-25

    Danyang Dou, Chao Wei, Bingbing Zhang, Daqing Yang, Ying Wang

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  7. Ultra‐High Optical Anisotropy with UV Transmission Achieved by Rational Arrangement of Extended π‐Conjugated Groups

    Angewandte Chemie International Edition · 2025-03-25

    Danyang Dou, Chao Wei, Bingbing Zhang, Daqing Yang, Ying Wang

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  8. Hydrogen‐Bonded Assembly of Functional Units for Constructing Linear and Nonlinear Optical Crystals

    Advanced Optical Materials · 2025-04-29

    Ziqi Chen, Changyou Liu, Chenxu Li, Juanjuan Lu, Zhihua Yang, Shilie Pan, Miriding Mutailipu

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  9. Polar Lithium l -Aspartate Monohydrate: A Semiorganic Ultraviolet Transparent Nonlinear Optical Crystal

    Inorganic Chemistry · 2025-06-20

    Yong Wang, Zhiyong Bai, Shanshan Chen, Chen Xu, Liangmeng Zhu, Tao Ouyang, Yanqiang Li, Weiqi Huang, Yipeng Song, Sangen Zhao, Junhua Luo

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  10. Designing an all-organic wide bandgap ultraviolet nonlinear optical crystal

    Science China Chemistry · 2025-06-30

    Shanshan Chen, Zhiyong Bai, Liangmeng Zhu, Tao Ouyang, Chen Xu, Shoufeng Wang, Yanqiang Li, Weiqi Huang, Sangen Zhao, Junhua Luo

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  11. A novel metal-free crystal demonstrating superior birefringence attributed to the synergistic interaction of dual π-conjugated units

    Science China Materials · 2025-07-07

    Die-Xue Yang, Ru‐Ling Tang, Yi‐Lei Lv, Bing-Wei Miao, Wenlong Liu, Sheng‐Ping Guo

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  12. Designing Hybrid Sb-Based Nonlinear Optical Crystals with Large Birefringence by Combining the Lone Pair and π-Conjugated Genes

    Inorganic Chemistry · 2025-07-28

    Kang Yang, Duanliang Wang, Fangcong Liu, Chuanrui Zhu, Qiyao Wang, Kui Wu, Jiyang Wang, Chuanying Shen

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  13. Achieving the birefringence-bandgap trade-off: Hydrogen-bond engineered biuret-cyanurate

    Chinese Journal of Structural Chemistry · 2025-07-29

    Ziqi Chen, Miriding Mutailipu

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  14. Low‐Dimensional Organic–Inorganic Hybrid Metal Halide with Large Optical Anisotropy

    Advanced Optical Materials · 2025-08-05

    Siyu Li, Yakun Zhang, Dongxue Sun, Baoli Gao, Bingbing Zhang, Daqing Yang, Ying Wang

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  15. Enhancing Birefringence via a Planar‐Conformation‐Locking Strategy

    Laser & Photonics Review · 2025-09-04

    Yaoguo Shen, Jiajia Xiong, Mengqing Wu, M.-R. Li, Yingwu Zhou, Yanjie Zhang

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  16. Five-Membered [C 5 O 5 ] 2 – Rings as Birefringence-Active Genes for Ultrabirefringent Crystals

    Journal of the American Chemical Society · 2025-09-16

    Jiachen Lu, Yang Li, Kang Min Ok

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  17. Sulfonated Module Aggregation for Ultrahigh Birefringence in Aqueous-Processable Crystals

    Journal of the American Chemical Society · 2025-10-14

    Congcong Jin, Yang Li, Chong‐An Chen, Jihyun Lee, Chanhee Ko, Soo‐Yeon Lee, Kang Min Ok

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  18. Enhanced Second Harmonic Generation Response via Rational Design of Iodinated π-Conjugated Pyridine Group

    Inorganic Chemistry · 2025-10-29

    Deshuai Xiao, Xinyuan Zhang, Pifu Gong, Zheshuai Lin, Zhanggui Hu, Ning Ye

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  19. Insights into the Strong Nonlinear Optical Ability of Functionalized Pyridinium-Benzimidazole Derivatives

    The Journal of Physical Chemistry C · 2025-12-10

    S. Taboukhat, Chengjun Wu, Dylan Amelot, Duong Tuan Pham, Salwa Simona Jamil, Abdelkrim El‐Ghayoury, Jamal Moussa, Andriy V. Kityk, B. Sahraoui

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  20. K 2 ZnMoP 2 O 10 : crystal growth, optical characterization, and structure–property insights into phase matching

    CrystEngComm · 2026-01-01

    Youbin Wang, Haonan Liu, Yujie Zhang, Hongping Wu, Hongping Wu, Zhanggui Hu

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  21. The condensation of π-conjugated units: a new paradigm for designing high-performance optical crystals

    Chemical Society Reviews · 2026-01-01

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  22. Confinement-assembled ultraviolet nonlinear optical crystal from pyridine-expanded π-systems with exhibiting strong SHG and birefringence

    Science China Chemistry · 2026-01-04

    Chunmei Huang, Xuan Pang, Fuming M. Li, Shumei Cao, Shilie Pan, Miriding Mutailipu

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  23. The modulation of structural polarity facilitating the gradient enhancement of second harmonic generation effects in hybrid metal halides

    Science China Chemistry · 2026-01-04

    Ru‐Ling Tang, Die-Xue Yang, Jian-Dong Guo, C. Z. Chen, Wenlong Liu, Sheng‐Ping Guo

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  24. Halogen‐Bond Coupled Halogenated‐π‐Conjugation Enables Giant Birefringence in Hydrogen‐Bonded Organic Frameworks

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  25. Unveiling the Superior Birefringence Property of a Record‐Birefringent Crystal with Unique Building Block

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  26. Unveiling the Superior Birefringence Property of a Record‐Birefringent Crystal with Unique Building Block

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  27. Ultrawide Bandgap and Record-High Birefringence in a Covalent Beryllium-Organic Framework

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  28. Noncovalent Assembly Engineering Achieves Excellent Birefringence in Crystals

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  29. Synthesis, structural characterization, and hyperpolarizability studies of novel barbituric acid and coumarin derivatives

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  30. Redox‐Driven Strategy Enabling Leapfrog Enhancement of Birefringence in Layered Tin‐Based Optical Crystals

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  31. Interlayer Electronic Decoupling Unlocks Giant Birefringence in π‐Conjugated Metal‐Organic Frameworks

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  32. Steric‐Guided Coordination Engineering Enables Significantly Optimized Optical Anisotropy via Sulfur‐Driven [C 5 H 5 NS] Birefringence‐Active Groups

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  33. Reversible Symmetry Switching, Giant Birefringence, and UV Second‐Harmonic Generation in Hybrid Niobium Oxyfluorides

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  34. Reversible Symmetry Switching, Giant Birefringence, and UV Second‐Harmonic Generation in Hybrid Niobium Oxyfluorides

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  35. A novel tetrafluoroborate with giant birefringence assembled from biocompatible adenine

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