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RESEARCH PAPER · Crystal Growth & Design · 2020

Chalcophosphates: A Treasure House of Infrared Nonlinear Optical Materials

Zhuang Li, Jiyong Yao, Yicheng Wu

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Chalcophosphates: A Treasure House of Infrared Nonlinear Optical MaterialsOriginalA 3 Mn 2 Sb 3 S 8 (A = K and Rb): a new type of multifunctional infrared nonlinear optical material based on unique three-dimensional open frameworks53A series of M 3 PS 4 (M = Ag, Cu and Ag/Cu) thiophosphates with diamond-like structures exhibiting large second harmonic generation responses and moderate ion conductivities28M 6 PS 5 X (M = Ag, Cu; X = Cl, Br) chalcohalides exhibiting strong nonlinear optical responses and high laser damage resistances9Na 4 SnS 4 and Na 4 SnSe 4 exhibiting multifunctional physicochemical performances as potential infrared nonlinear optical crystals and sodium ion conductors27Recent progress in oxychalcogenides as IR nonlinear optical materials79Revisiting thiophosphate Pb 3 P 2 S 8 : a multifunctional material combining a nonlinear optical response and photocurrent response23Structural Modulation from Cu 3 PS 4 to Cu 5 Zn 0.5 P 2 S 8 : Single-Site Aliovalent-Substitution-Driven Second-Harmonic-Generation Enhancement28A review of the structural diversity of [P x S y ] n − motifs and their potential application prospects in metal thiophosphates21Transition-metal-based chalcogenides: A rich source of infrared nonlinear optical materials184The Rise of Infrared Nonlinear Optical Pnictides: Advances and Outlooks36Hg-based chalcogenides: An intriguing class of infrared nonlinear optical materials129Pnictides: An emerging class of infrared nonlinear optical material candidates47A 2 Zn 3 P 4 S 13 (A = Rb and Cs): First Infrared Nonlinear Optical Materials with Mixed Thiophosphate Functional Motifs PS 4 and P 2 S 621AAg 2 PS 4 (A = K, Na/K): the first-type of noncentrosymmetric alkali metal Ag-based thiophosphates exhibiting excellent second-order nonlinear optical performances21Ba 6 In 2 Ge 2 Te 15 : a THz birefringent material with an intriguing quasi-[Te 5 ] 4− chain possessing large optical anisotropy and an ultrawide transmission range7Unprecedented mid-infrared nonlinear optical materials achieved by crystal structure engineering, a case study of (KX)P 2 S 6 (X = Sb, Bi, Ba)59Quaternary Noncentrosymmetric Rare-Earth Sulfides Ba4RE2Cd3S10 (RE = Sm, Gd, or Tb): A Joint Experimental and Theoretical Investigation17From Cc to P 6 3 mc : Structural Variation in La 3 S 2 Cl 2 [SbS 3 ] and La 3 OSCl 2 [SbS 3 ] Induced by the Isovalent Anion Substitution22Synthesis, Crystal and Electronic Structures, and Nonlinear Optical Properties of Y4Si3S1212The Combination of Structure Prediction and Experiment for the Exploration of Alkali‐Earth Metal‐Contained Chalcopyrite‐Like IR Nonlinear Optical Material105Ba2MAsQ5 (Q = S and Se) Family of Polar Structures with Large Second Harmonic Generation and Phase Matchability23RbBiP2S6: A Promising IR Nonlinear Optical Material with a Giant Second-Harmonic Generation Response Designed by Aliovalent Substitution80Eu 2 P 2 S 6 : The First Rare‐Earth Chalcogenophosphate Exhibiting Large Second‐Harmonic Generation Response and High Laser‐Induced Damage Threshold144Eu2P2S6: The First Rare‐Earth Chalcogenophosphate Exhibiting Large Second‐Harmonic Generation Response and High Laser‐Induced Damage Threshold7A comprehensive review on metal chalcogenides with three-dimensional frameworks for infrared nonlinear optical applications115Ag4SnGe2S7: A Noncentrosymmetric Chalcogenide in I4–II–IV2–VI7 System with Non-Diamond-Like Structure Featuring 1D ∞[SnGe2S8]6– Infinite Chain2Chalcohalides: A Rising Type of Second‐Order Nonlinear Optical Materials28A review of structures and physical properties of rare earth chalcophosphates78Ag-based chalcogenides and derivatives as promising infrared nonlinear optical materials90KREP2Se6 (RE = Sm, Gd, Tb): The First Rare‐Earth Selenophosphates with Remarkable Nonlinear Optical Activities Realized by Synergistic Effect of RE‐ and P‐Based Motifs39Enhanced Second-Harmonic Generation of van der Waals CuInP 2 S 6 via Pressure-Regulated Cationic Displacement61Stabilization of the Polar Structure and Giant Second‐Order Nonlinear Response of Single Crystal γ‐NaAs0.95Sb0.05Se219γ-P 4 S 3 I 2 : a new metal-free infrared second-order nonlinear optical crystal designed by polymorphism strategy17Quaternary alkaline-earth metal thiophosphate SrAgPS 4 : syntheses, structures, and optical properties9Recent advances in F-containing iodate nonlinear optical materials6Revisiting two thiophosphate compounds constituting d 0 transition metal HfP 2 S 6 and d 10 transition metal α-Ag 4 P 2 S 6 as multifunctional materials for combining second harmonic generation response and photocurrent response12The Kurtz–Perry Powder Technique Revisited: A Study of the Effect of Reference Selection on Powder Second-Harmonic Generation Response20Machine Learning Regression Model for Predicting the Formation Energy of Nonlinear Optical Crystals5Recent progress in the design of IR nonlinear optical materials by partial chemical substitution: Structural evolution and performance optimization133Nonlinear optical properties of gold nanoparticles containing borate glasses at spectral region of surface plasmon resonance10Recent advances in IR nonlinear optical chalcogenides with well-balanced comprehensive performance57Defect diamond-like tellurides as infrared nonlinear optical materials with giant second-harmonic generation tensor14ACd 4 Ga 5 Te 12 (A = K, Rb, Cs): Tellurides with a Strong Nonlinear Optical Response and Purple Emission24NaREP 2 Se 6 (RE = Y, Sm, Gd–Dy): Quaternary Rare-Earth Selenophosphates with Unique 3D {[REP 2 Se 6 ] − } ∞ Framework Built by RESe 8 and P 2 Se 6 Motifs and Multiple Properties4Noncentrosymmetric Na6Pb3P4S16 and Centrosymmetric K2MIIP2S6 (MII = Mg and Zn) Displaying Multiple Membered-Ring Configurations and Strong Optical Anisotropy10Synthesis, crystal and electronic structures, linear and nonlinear optical properties, and photocurrent response of oxyhalides CeHaVIO 4 (Ha = Cl, Br; VI = Mo, W)10Ga-based IR nonlinear optical materials: Synthesis, structures, and properties65Chalcophosphate metasurfaces with multipolar resonances and electro-optic tuning7Novel cesium cerium( iv ) iodate Cs 2 Ce(IO 3 ) 6 : hydrothermal synthesis, crystal structures and thermal stability2Reconstructing nearly isotropic microstructures to construct a one-dimensional framework causing record birefringence in thiophosphates13Studies on the physical properties of solution-grown pure and impurity-added triglycine formate single crystals1Molecular Crystals Constructed by Polar Molecular Cages: A Promising System for Exploring High‐performance Infrared Nonlinear Optical Crystals6Molecular Crystals Constructed by Polar Molecular Cages: A Promising System for Exploring High‐performance Infrared Nonlinear Optical Crystals34Cs 3 In(In 4 Se 7 )(P 2 Se 6 ): A Multi‐Chromophore Chalcogenide with Excellent Nonlinear Optical Property Designed by Group Grafting55Cs3In(In4Se7)(P2Se6): A Multi‐Chromophore Chalcogenide with Excellent Nonlinear Optical Property Designed by Group Grafting2KREP 2 S 6 (RE = Sm, Gd, Tb, Dy): A Series of Polar Rare-Earth Thiophosphates with High Laser-Induced Damage Thresholds and Moderate Nonlinear-Optical Responses Synergistically Contributed by Isolated P 2 S 6 Units and {[RE 2 S 15 ] 24– } ∞ Layers8Influence of Cation-Size Effects of Alkaline Earth (Ae) Metals on Dimensionality and Optical Anisotropy Regulation in K4AeP2S8 Thiophosphates5NLOphoric Anthraquinone Dyes – A Review11Recent advances and future perspectives on rare-earth-based nonlinear optical materials with π-conjugated [XO3] (X = B, C, N) units66β-Pb3P2S8: A new optical crystal with exceptional birefringence effect12Phase-Matching Second-Harmonic Generation and Enhanced Laser-Induced Damage Threshold Induced by Cs Substitution: Cu 3 PSe 4 vs Cs 2 CuP 3 S 94Cd 5 Te 4 O 12 X 2 (X = Cl, Br, I): a new oxyhalide family with [CdO 4 X] mixed anionic units and adjustable optical properties4Design of a high-performance infrared birefringent crystal Ba 4 HgP 2 Se 10 via a low-dimensional motif intercalation strategy2Chalcophosphates: A plentiful source of infrared nonlinear optical materials42Symmetry over Chemistry: Harmonic Generation of Low-Dimensional Alkali Chalcopnictates RbMP2S6 (M = Sb, Bi)6Metal- and Solvent-Free Synthesis of Phosphinothioates, Phosphonothioates, Phosphorothioates, and Related Selenium Derivatives: An Efficient Green Protocol5Methyl substitution induced noncentrosymmetric alignment: a new thiazolium-based nonlinear optical crystal of HDT-N1S2Alkali Metal Substitution-Induced Structural Transformation for RbREP2Se6 (RE = Gd, Tb, Dy) with Second-Harmonic Generation Responses6Vacancy-driven tetrahedral distortion leading to exceptional second harmonic generation3Maximizing the second-harmonic generation response via coordination-induced localization of nonbonding electrons12ABCQ4型硫属化物红外非线性光学材料的构效关系（特邀）0From KBa 4 Ge 3 S 10 Cl to ABa 3 EuGe 3 S 11 (A = Na, K) Synthesized by Reactive Flux Assisted Metal Oxide-Boron-Chalcogen (MOBQ) Method: Effect of Cation/Anion Cosubstitution on Crystal Structure and Nonlinear Optical Properties0Chiral (Stereoselective) Drugs, Asymmetric Synthesis, and Racemic Resolution Methods1First‐Principles Investigation of the Structural, Electronic, Optical, Elastic, and Thermal Properties of Defect Diamond‐Like Hg 3 P 2 S 80From AgGaSe2 to MIIGa2Se4 (MII = Zn, Cd): Heterovalent Substitution Creates Ordered Vacancies for Balanced IR-NLO Performance0

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  1. A 3 Mn 2 Sb 3 S 8 (A = K and Rb): a new type of multifunctional infrared nonlinear optical material based on unique three-dimensional open frameworks

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  2. A series of M 3 PS 4 (M = Ag, Cu and Ag/Cu) thiophosphates with diamond-like structures exhibiting large second harmonic generation responses and moderate ion conductivities

    Dalton Transactions · 2021-01-01

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  3. M 6 PS 5 X (M = Ag, Cu; X = Cl, Br) chalcohalides exhibiting strong nonlinear optical responses and high laser damage resistances

    Dalton Transactions · 2021-01-01

    Lihua Gao, Xiaowen Wu, Daqing Yang, Xinyu Tian, Jingjing Xu, Bingbing Zhang, Kui Wu

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  4. Na 4 SnS 4 and Na 4 SnSe 4 exhibiting multifunctional physicochemical performances as potential infrared nonlinear optical crystals and sodium ion conductors

    New Journal of Chemistry · 2021-01-01

    Lihua Gao, Gang Bian, Ya Feng Yang, Bingbing Zhang, Xiaowen Wu, Kui Wu

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  5. Recent progress in oxychalcogenides as IR nonlinear optical materials

    Dalton Transactions · 2021-01-01

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  6. Revisiting thiophosphate Pb 3 P 2 S 8 : a multifunctional material combining a nonlinear optical response and photocurrent response

    Physical Chemistry Chemical Physics · 2021-01-01

    Bingheng Ji, Elizabeth Guderjahn, Kui Wu, Tajamul Hussain Syed, Wei Wei, Bingbing Zhang, Jian Wang

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  7. Structural Modulation from Cu 3 PS 4 to Cu 5 Zn 0.5 P 2 S 8 : Single-Site Aliovalent-Substitution-Driven Second-Harmonic-Generation Enhancement

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    Bang-Jun Song, Zuju Ma, Bingxuan Li, Xintao Wu, Hua Lin, Qi‐Long Zhu

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  8. A review of the structural diversity of [P x S y ] n − motifs and their potential application prospects in metal thiophosphates

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  9. Transition-metal-based chalcogenides: A rich source of infrared nonlinear optical materials

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  10. The Rise of Infrared Nonlinear Optical Pnictides: Advances and Outlooks

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  11. Hg-based chalcogenides: An intriguing class of infrared nonlinear optical materials

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  12. Pnictides: An emerging class of infrared nonlinear optical material candidates

    Journal of Alloys and Compounds · 2021-12-22

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  13. A 2 Zn 3 P 4 S 13 (A = Rb and Cs): First Infrared Nonlinear Optical Materials with Mixed Thiophosphate Functional Motifs PS 4 and P 2 S 6

    Journal of Materials Chemistry C · 2022-01-01

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  14. AAg 2 PS 4 (A = K, Na/K): the first-type of noncentrosymmetric alkali metal Ag-based thiophosphates exhibiting excellent second-order nonlinear optical performances

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  15. Ba 6 In 2 Ge 2 Te 15 : a THz birefringent material with an intriguing quasi-[Te 5 ] 4− chain possessing large optical anisotropy and an ultrawide transmission range

    Inorganic Chemistry Frontiers · 2022-01-01

    Mengran Sun, Xingyu Zhang, Wenhao Xing, Ece Uykur, Wenlong Yin, Zheshuai Lin, Jiyong Yao

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  16. Unprecedented mid-infrared nonlinear optical materials achieved by crystal structure engineering, a case study of (KX)P 2 S 6 (X = Sb, Bi, Ba)

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    Vivian Nguyen, Bingheng Ji, Kui Wu, Bingbing Zhang, Jian Wang

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  17. Quaternary Noncentrosymmetric Rare-Earth Sulfides Ba4RE2Cd3S10 (RE = Sm, Gd, or Tb): A Joint Experimental and Theoretical Investigation

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  18. From Cc to P 6 3 mc : Structural Variation in La 3 S 2 Cl 2 [SbS 3 ] and La 3 OSCl 2 [SbS 3 ] Induced by the Isovalent Anion Substitution

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  19. Synthesis, Crystal and Electronic Structures, and Nonlinear Optical Properties of Y4Si3S12

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  20. The Combination of Structure Prediction and Experiment for the Exploration of Alkali‐Earth Metal‐Contained Chalcopyrite‐Like IR Nonlinear Optical Material

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  21. Ba2MAsQ5 (Q = S and Se) Family of Polar Structures with Large Second Harmonic Generation and Phase Matchability

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  22. RbBiP2S6: A Promising IR Nonlinear Optical Material with a Giant Second-Harmonic Generation Response Designed by Aliovalent Substitution

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  23. Eu 2 P 2 S 6 : The First Rare‐Earth Chalcogenophosphate Exhibiting Large Second‐Harmonic Generation Response and High Laser‐Induced Damage Threshold

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  24. Eu2P2S6: The First Rare‐Earth Chalcogenophosphate Exhibiting Large Second‐Harmonic Generation Response and High Laser‐Induced Damage Threshold

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  25. A comprehensive review on metal chalcogenides with three-dimensional frameworks for infrared nonlinear optical applications

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  26. Ag4SnGe2S7: A Noncentrosymmetric Chalcogenide in I4–II–IV2–VI7 System with Non-Diamond-Like Structure Featuring 1D ∞[SnGe2S8]6– Infinite Chain

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  27. Chalcohalides: A Rising Type of Second‐Order Nonlinear Optical Materials

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  28. A review of structures and physical properties of rare earth chalcophosphates

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  29. Ag-based chalcogenides and derivatives as promising infrared nonlinear optical materials

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  30. KREP2Se6 (RE = Sm, Gd, Tb): The First Rare‐Earth Selenophosphates with Remarkable Nonlinear Optical Activities Realized by Synergistic Effect of RE‐ and P‐Based Motifs

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  31. Enhanced Second-Harmonic Generation of van der Waals CuInP 2 S 6 via Pressure-Regulated Cationic Displacement

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  32. Stabilization of the Polar Structure and Giant Second‐Order Nonlinear Response of Single Crystal γ‐NaAs0.95Sb0.05Se2

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  33. γ-P 4 S 3 I 2 : a new metal-free infrared second-order nonlinear optical crystal designed by polymorphism strategy

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  34. Quaternary alkaline-earth metal thiophosphate SrAgPS 4 : syntheses, structures, and optical properties

    Dalton Transactions · 2023-01-01

    Wenhao Xing, Jian Tang, Fei Liang, Chunlan Tang, Jieyun Wu, Wenlong Yin, Bin Kang, Jianguo Deng

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  35. Recent advances in F-containing iodate nonlinear optical materials

    Chinese Journal of Structural Chemistry · 2023-01-01

    Dong Gao, Hongping Wu, Zhanggui Hu, Jiyang Wang, Yicheng Wu, Hongwei Yu

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  36. Revisiting two thiophosphate compounds constituting d 0 transition metal HfP 2 S 6 and d 10 transition metal α-Ag 4 P 2 S 6 as multifunctional materials for combining second harmonic generation response and photocurrent response

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  37. The Kurtz–Perry Powder Technique Revisited: A Study of the Effect of Reference Selection on Powder Second-Harmonic Generation Response

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  38. Machine Learning Regression Model for Predicting the Formation Energy of Nonlinear Optical Crystals

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  39. Recent progress in the design of IR nonlinear optical materials by partial chemical substitution: Structural evolution and performance optimization

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  40. Nonlinear optical properties of gold nanoparticles containing borate glasses at spectral region of surface plasmon resonance

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  41. Recent advances in IR nonlinear optical chalcogenides with well-balanced comprehensive performance

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  42. Defect diamond-like tellurides as infrared nonlinear optical materials with giant second-harmonic generation tensor

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  43. ACd 4 Ga 5 Te 12 (A = K, Rb, Cs): Tellurides with a Strong Nonlinear Optical Response and Purple Emission

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  44. NaREP 2 Se 6 (RE = Y, Sm, Gd–Dy): Quaternary Rare-Earth Selenophosphates with Unique 3D {[REP 2 Se 6 ] − } ∞ Framework Built by RESe 8 and P 2 Se 6 Motifs and Multiple Properties

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  45. Noncentrosymmetric Na6Pb3P4S16 and Centrosymmetric K2MIIP2S6 (MII = Mg and Zn) Displaying Multiple Membered-Ring Configurations and Strong Optical Anisotropy

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  46. Synthesis, crystal and electronic structures, linear and nonlinear optical properties, and photocurrent response of oxyhalides CeHaVIO 4 (Ha = Cl, Br; VI = Mo, W)

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  47. Ga-based IR nonlinear optical materials: Synthesis, structures, and properties

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  48. Chalcophosphate metasurfaces with multipolar resonances and electro-optic tuning

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  49. Novel cesium cerium( iv ) iodate Cs 2 Ce(IO 3 ) 6 : hydrothermal synthesis, crystal structures and thermal stability

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  50. Reconstructing nearly isotropic microstructures to construct a one-dimensional framework causing record birefringence in thiophosphates

    Chemical Science · 2024-01-01

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