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RESEARCH PAPER · Coordination Chemistry Reviews · 2022

Ag-based chalcogenides and derivatives as promising infrared nonlinear optical materials

Wenfeng Zhou, Jiajing Wu, Wenlong Liu, Sheng‐Ping Guo

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Ag-based chalcogenides and derivatives as promising infrared nonlinear optical materialsOriginalAn overview of Mg-based IR nonlinear optical materials22Recent progress on sulfide infrared nonlinear optical materials with large SHG response and wide band gap26Solvent-free synthesis of magnesium phosphite-oxalates that show second-harmonic generation responses5Growth and Optical Properties of Large-Sized NaVO2(IO3)2(H2O) Crystals for Second-Harmonic Generation Applications12Recent advances in non-π-conjugated nonlinear optical sulfates with deep-UV absorption edge53[K2PbX][Ga7S12] (X = Cl, Br, I): The First Lead‐Containing Cationic Moieties with Ultrahigh Second‐Harmonic Generation and Band Gaps Exceeding the Criterion of 2.33 eV46Host–Guest Symmetry Matching in Two Crystalline Magnesium Sulfate Oxalates Obtained Via a Solvent-Free Route8Structure and Optical Properties of LixAg1–xGaSe2 and LixAg1–xInSe27Nonlinear Optical Sulfides LiMGa8S14 (M = Rb/Ba, Cs/Ba) Created by Li+ Driven 2D Centrosymmetric to 3D Noncentrosymmetric Transformation20Theoretical Prediction‐Assisted Synthesis and Characterization of Infrared Nonlinear Optical Material NaSrBS324Recent progress of newly developed functional building units and corresponding nonlinear optical materials14Host–Guest Symmetry and Charge Matching in Glycine-Templated Metal Sulfate–Oxalates Obtained by a Solvent-Free Method9Recent advances in IR nonlinear optical chalcogenides with well-balanced comprehensive performance56AgSbTe2 semi-nanocrystalline thin films as a multifunctional platform for optoelectronic and diode applications29Wide band gaps in nonlinear optical materials AMgAgGa6S11 (A = K, Rb) achieved by the incorporation of dual s-block elements in Ag-based sulfide11Three-in-One Tetrahedral Functional Units Constructing Diamondlike Ag2In2SiS3.06Se2.94 with High-Performance Nonlinear-Optical Activity4Mixed Anionic Tetrahedra Guided Design of New Infrared Nonlinear Optical Material Cs 3 Ga 8 S 13 Cl with High Laser‐Induced Damage Threshold26Evolution of Structures and Optical Properties in a Series of Infrared Nonlinear Optical Crystals LixAg1–xInSe2 (0 ≤ x ≤ 1)12A new nonlinear optical crystal Li0.81Ag0.19InSe2 with balanced properties for efficient nonlinear conversion in the mid-IR region10Enhancing second harmonic generation response in infrared nonlinear optical material through Pb substitution: A study of LiPbSiS compound2Nonlinear Optical Phosphide CuInSi2P4: The Inaugural Member of Diamond-Like Family I–III–IV2–V4 Inspired by ZnGeP216Computer-aided screening of bismuth molybdates nonlinear optical crystals γ -Bi 2 MoO 63Exploration of silver borates with diverse low-dimensional anion frameworks by introducing monovalent heteroanions6Multi-step cation substitution facilitating the exploration of potential infrared nonlinear optical materials6Solvent-free synthesis and optical properties of two open-framework metal oxalates with zeolitic ABW and diamondoid topologies3Structural strategy for advancing nonlinear optical effects in 1D-[MX 2 ] ∞ chains: internal distortion and atomic types2Exploring the nonlinear optical properties of gold nanoparticle colloids capped with Gum Arabic: A study utilizing continuous wave laser and Z-scan technique18Solvent-assisted investigation of NLO responses of 3,5-dihydroxybenzoic acid and pyrazine-2-carboxamide cocrystal14Phase Equilibria and Thermodynamic Properties of Selected Compounds in the Ag-Ga-Te-AgBr System4Phosphosulfide semiconductors for optoelectronics and solar energy conversion9Design of Pentanary Mixed-Chalcogenides Ag2In2SiS6–xSex (x = 1, 2) Based on the Bucket Effect: Local Structural Difference and High-Performance Nonlinear-Optical Properties Realized by Partial Congener Substitution5Influence of Cation-Size Effects of Alkaline Earth (Ae) Metals on Dimensionality and Optical Anisotropy Regulation in K4AeP2S8 Thiophosphates5Homoatomic Polychalcogenide Nonlinear Optical Anionic Groups with Ultra-Large Optical Anisotropy31A Rare Earth Chalcogenide Nonlinear Optical Crystal KLaGeS4: Achieving Good Balance among Band Gap, Second Harmonic Generation Effect, and Birefringence12Ag 2 GeS 3 : A Diamond‐Like Chalcogenide as an IR Nonlinear Optical Material with Outstanding Second‐Harmonic Generation Response28AAg2MS4 (A = Na, K, Rb; M = P, As) Nonlinear Optical Series with Unique Cation‐Regulated Highly Anisotropic [AgS4] Hypertetrahedral Layered Framework10Structure and optical properties of LixAg1–xAlSe23Native Defects Hybridization and Electronic Transport in Cu2Se‐CuGaSe2 Hierarchical Composites3Structure and disorder resulting in ultralow thermal conductivity in the defect chalcopyrite AgInSnSe44Revealing the Effects of Defect States on the Nonlinear Absorption Properties of the TlInsse and Tl 2 In 2 S 3 Se Crystals in Near-Infrared Optical Limiting Applications46Impressive nonlinear optical response of π-conjugated, photoluminescent soft nanoparticles in polymer matrix6A review of chalcogenide-based perovskites as the next novel materials: Solar cell and optoelectronic applications, catalysis and future perspectives111LaAgSiS4: Increasing Optical Birefringence in Rare Earth Chalcogenide by Addition of Planar [AgS3] Groups5Crystal Growth and Property Characterization of a Novel Long-Wave Infrared Nonlinear Optical Crystal BaHgGeSe 49Achieving Phase‐Matching in Nonlinear Optical Materials CsM 2 In 2 S 6 (M = Cd/In, Hg/In) by the Incorporation of Unprecedented Trigonal Planar MS 3 Motifs6Computer‐Aided Development of New Nonlinear Optical Materials38Computer‐Aided Development of New Nonlinear Optical Materials14Tin chalcohalide Sn 11 (PS 4 ) 4 I 10 obtained from structural-template-oriented synthesis: exhibiting balanced infrared nonlinear optical performance6Emergent Mid‐Infrared Nonlinear Optical Candidates With Targeted Balance Performances17A wide band gap selenohalide Cs 9 Si 8 Se 20 Cl with unprecedented [CsSe 7 Cl] mixed anionic units2Aliovalent Al 3+ substituted ultra-wide bandgap CuAlX 4 (X = Cl, Br) for infrared nonlinear optics6Enhancement in the nonlinear optical properties of silver nanoprisms through graphene oxide anchoring7Exploring new horizons in mid-to-far infrared nonlinear optical crystals: the significant potential of trigonal pyramidal [TeS 3 ] 2− functional units18Correlations in Cu-based chalcogenides for optical and transport performance in sustainable technologies: First-principles calculation9AgGaS2 and Derivatives: Design, Synthesis, and Optical Properties8Assembly between diverse polycations and diamond-like anionic frameworks in salt-inclusion phosphides enables excellent nonlinear optical properties4Synergically Assembling Advantageous Groups toward High‐Performance Infrared Nonlinear Optical Materials A II CdSiSe 4 (A II = Sr, Ba)40SrZnGeSe 4 : a promising infrared nonlinear optical material with strong second harmonic generation and high laser-induced damage threshold4Non-centrosymmetric Y3FeGaSe7 and Y3Mn0·5SiSe7 with extremely low thermal conductivities2Synthesis and third-order nonlinear optical properties of PEGylated platinum nanoparticles0Pressure optimized 2D-IV monochalcogenide for enhanced photovoltaic performance in skyscraper-integrated solar cell: A computational insight2Icosahedral carboranes-based metal nanoclusters: From fascinating structures to polychrome properties and applications12First report on electrochemical sensing of antimalarial drug lumefantrine in blood using Ag2BaS4 nanostructures anchored on Ni foam2Nonlinear Optical Series A(VO2)3(SeO3)2 (A = NH4+, K+, and H3O+) with Large Birefringence Derived from High-Anisotropic VO6 Octahedra and SeO3 Pyramids8Achieving excellent nonlinear optical performance via “dimensionality elevation”-driven transformation from centrosymmetric to non-centrosymmetric structures1SrZnGeSe4: An Infrared Nonlinear Optical Crystal Material with Wide Transmission Range and Large SHG Response6NaAg3Ga8S14: A new diamond-like framework infrared nonlinear optical material derived from AgGaS26BaAl2MS6 (M = Si and Ge): the rational construction of diamond-like structures with ultrawide band gap by group-optimization approach6A high-performance IR nonlinear optical material Sr 3 MnGe 2 S 8 achieved via partial cation substitution-induced structural transformation2Maximizing the second-harmonic generation response via coordination-induced localization of nonbonding electrons12ABCQ4型硫属化物红外非线性光学材料的构效关系（特邀）0Diamond-like Ag x Cu 3− x PS 4 ( x = 1 and 2) synthesized by the metal oxide–boron–chalcogen (MOBQ) routine: local high-entropy engineering for balanced infrared nonlinear optical performance1Polyhedral replacement-guided design of Ce3MnGaSe7 featuring strong second-harmonic genera-tion and high laser-induced damage threshold0Selenium-Based Molecular Cage Crystal β-P 4 Se 3 Br 2 : A Promising Candidate for Infrared Nonlinear Optical Applications1Rare-earth doping of AgGaGe3Se8: A pathway to multifunctional materials for tunable optoelectronics1Comparative study of functionalized silver nanoparticles for solar-driven photocatalytic degradation of atrazine and organic contaminants1The Power of Pnictogen Bond: As─As Linkages Drive Wide Bandgap, Strong NLO Response and Large Birefringence in SrGa 3 Si 4 As 115The Power of Pnictogen Bond: As─As Linkages Drive Wide Bandgap, Strong NLO Response and Large Birefringence in SrGa 3 Si 4 As 110Cd/V Ratio-Driven Centrosymmetric Transition of Crystal Structures in Cesium Cadmium Vanadate Oxychlorides Cs 3 CdV 4 O 12 Cl and CsCdV 2 O 6 Cl0Heterovalent Coexistence‐Driven Symmetry Breaking and Dimensional Evolution: Designing Polar Heart‐Shaped Channels for Exceptional MFIR Nonlinear Optics5A Rigid‐Flexible Cooperative Bond‐Engineering Strategy for the Rational Design of Advanced Infrared Nonlinear Optical Crystals2Quaternary rare-earth sulfides RE2Ag2SnS6 (RE = Nd, Sm, Gd, Tb) with two- and three-coordinate silver0From KBa 4 Ge 3 S 10 Cl to ABa 3 EuGe 3 S 11 (A = Na, K) Synthesized by Reactive Flux Assisted Metal Oxide-Boron-Chalcogen (MOBQ) Method: Effect of Cation/Anion Cosubstitution on Crystal Structure and Nonlinear Optical Properties0A 3 Zr 2 (PS 4 )(P 2 S 7 ) 2 (A = K, Rb, Cs) Synthesized by the Metal Oxide-Boron-Chalcogen Routine: A Series of Zirconium-Based Thiophosphate Nonlinear Optical Crystals Featuring PS 4 Tetrahedron and P 2 S 7 Dimer0Solution-Grown Cs2HgI4 Bulk Crystals: Achieving Strong SHG and High Damage Threshold Synergistically for IR Nonlinear Optics1Cation-substitution-driven electronic, nonlinear optical, elastic, and thermal transport properties of layered AeHgGeSe4 (Ae = Ba, Sr): A first-principles study0AgEuPS4: Unlocking the Centrosymmetric Shackle of Rare-Earth Thiophosphates via Microscopic Distortion Cascading for Enhanced Second-Harmonic Generation Response0Entropy‐Driven Precursor Symmetry Breaking for Phase‐Selective Synthesis of Noncentrosymmetric Rb 2 CdCl 2 I 20AlGaS3: a wide band gap ternary diamond-like infrared nonlinear optical material with high laser-induced damage threshold1Beyond the bandgap bottleneck: structure–property design principles for infrared nonlinear optical phosphides0

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  48. Tin chalcohalide Sn 11 (PS 4 ) 4 I 10 obtained from structural-template-oriented synthesis: exhibiting balanced infrared nonlinear optical performance

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  49. Emergent Mid‐Infrared Nonlinear Optical Candidates With Targeted Balance Performances

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  50. A wide band gap selenohalide Cs 9 Si 8 Se 20 Cl with unprecedented [CsSe 7 Cl] mixed anionic units

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