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RESEARCH PAPER · Inorganic Chemistry · 2021

Structural Modulation from Cu 3 PS 4 to Cu 5 Zn 0.5 P 2 S 8 : Single-Site Aliovalent-Substitution-Driven Second-Harmonic-Generation Enhancement

Bang-Jun Song, Zuju Ma, Bingxuan Li, Xintao Wu, Hua Lin, Qi‐Long Zhu

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Structural Modulation from Cu 3 PS 4 to Cu 5 Zn 0.5 P 2 S 8 : Single-Site Aliovalent-Substitution-Driven Second-Harmonic-Generation EnhancementOriginalAliovalent-cation-substitution-induced structure transformation: a new path toward high-performance IR nonlinear optical materials47Transition-metal-based chalcogenides: A rich source of infrared nonlinear optical materials184AAg 2 PS 4 (A = K, Na/K): the first-type of noncentrosymmetric alkali metal Ag-based thiophosphates exhibiting excellent second-order nonlinear optical performances21Rational design via dual-site aliovalent substitution leads to an outstanding IR nonlinear optical material with well-balanced comprehensive properties69Two Nonlinear Optical Thiophosphates Cu 5 Hg 0.5 P 2 S 8 and AgHg 3 PS 6 Activated by Their Tetrahedra-Stacking Architecture12The Kurtz-Perry powder technique revisited: A case study on the importance of reference quality and broadband nonlinear optical measurements using LiInSe232First Investigation of Nonlinear Optical Oxychalcogenide with Three‐Dimensional Anionic Framework and Special Windmill‐Like Functional Motifs †28Recent progress in the design of IR nonlinear optical materials by partial chemical substitution: Structural evolution and performance optimization133Recent advances in IR nonlinear optical chalcogenides with well-balanced comprehensive performance57Modulation of the Band Gap and Redox Properties by Mixed Addenda in Sandwich Polyoxometalates2ACu4AsS4 (A = K, Rb): Two infrared nonlinear optical crystals with strong second-harmonic generation responses originating from multiple chromophores12Phosphosulfide semiconductors for optoelectronics and solar energy conversion9Vacancy‐Induced Extraordinary Second Harmonic Generation Response for Diamond‐Like Cu3PS49Ag 2 GeS 3 : A Diamond‐Like Chalcogenide as an IR Nonlinear Optical Material with Outstanding Second‐Harmonic Generation Response28Phase-Matching Second-Harmonic Generation and Enhanced Laser-Induced Damage Threshold Induced by Cs Substitution: Cu 3 PSe 4 vs Cs 2 CuP 3 S 94Effect of pressure on the structure, elasticity and optical properties of AgGaSe2 crystal3Exploring new horizons in mid-to-far infrared nonlinear optical crystals: the significant potential of trigonal pyramidal [TeS 3 ] 2− functional units18Large-area thin-film synthesis of photoactive Cu 3 PS 4 thiophosphate semiconductor with 0–14 pH stability range5Symmetry over Chemistry: Harmonic Generation of Low-Dimensional Alkali Chalcopnictates RbMP2S6 (M = Sb, Bi)6Structure-property relationships in IR nonlinear optical chalcogenides with stereochemically active lone pairs29Vacancy-driven tetrahedral distortion leading to exceptional second harmonic generation3Maximizing the second-harmonic generation response via coordination-induced localization of nonbonding electrons12Diamond-like Ag x Cu 3− x PS 4 ( x = 1 and 2) synthesized by the metal oxide–boron–chalcogen (MOBQ) routine: local high-entropy engineering for balanced infrared nonlinear optical performance1van der Waals layered CuInP 2 S 6 as infrared nonlinear optical material1Achieving phase matching in infrared nonlinear optical crystal Cd3ZnSiS6 via isovalent substitution from Cd4SiS60From AgGaSe2 to MIIGa2Se4 (MII = Zn, Cd): Heterovalent Substitution Creates Ordered Vacancies for Balanced IR-NLO Performance0Variation of Tetrahedrons and Cations Regulates LIDTs in 3D‐DL Structure MIR‐NLO Crystals0Phase-Selective Synthesis of Copper Phosphosulfide Nanocrystals0

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  1. Aliovalent-cation-substitution-induced structure transformation: a new path toward high-performance IR nonlinear optical materials

    Journal of Materials Chemistry C · 2021-01-01

    Chang Liu, Shenghua Zhou, Yu Xiao, Chao Zhang, Hua Lin, Yi Liu

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  2. Transition-metal-based chalcogenides: A rich source of infrared nonlinear optical materials

    Coordination Chemistry Reviews · 2021-08-26

    Hong Chen, Wenbo Wei, Hua Lin, Xintao Wu

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  3. AAg 2 PS 4 (A = K, Na/K): the first-type of noncentrosymmetric alkali metal Ag-based thiophosphates exhibiting excellent second-order nonlinear optical performances

    Inorganic Chemistry Frontiers · 2022-01-01

    Wenfeng Zhou, Bingxuan Li, Wenlong Liu, Sheng‐Ping Guo

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  4. Rational design via dual-site aliovalent substitution leads to an outstanding IR nonlinear optical material with well-balanced comprehensive properties

    Chemical Science · 2022-01-01

    Hedi Yang, Mao‐Yin Ran, Shenghua Zhou, Xin‐Tao Wu, Hua Lin, Qi‐Long Zhu

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  5. Two Nonlinear Optical Thiophosphates Cu 5 Hg 0.5 P 2 S 8 and AgHg 3 PS 6 Activated by Their Tetrahedra-Stacking Architecture

    Inorganic Chemistry · 2022-01-11

    Yang Wang, Yuqiang Fang, Yunzhen Cao, Fuqiang Huang

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  6. The Kurtz-Perry powder technique revisited: A case study on the importance of reference quality and broadband nonlinear optical measurements using LiInSe2

    Journal of Alloys and Compounds · 2022-05-13

    Daniel J. Clark, Jian‐Han Zhang, Andrew J. Craig, Ashley Weiland, Jacilynn A. Brant, Jeong Bin Cho, Yong Soo Kim, Joon Ik Jang, Jennifer A. Aitken

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  7. First Investigation of Nonlinear Optical Oxychalcogenide with Three‐Dimensional Anionic Framework and Special Windmill‐Like Functional Motifs †

    Chinese Journal of Chemistry · 2022-07-14

    Jia-Nuo Li, Xiaohui Li, Ying‐Xuan Xu, Wenlong Liu, Sheng‐Ping Guo

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  8. Recent progress in the design of IR nonlinear optical materials by partial chemical substitution: Structural evolution and performance optimization

    Coordination Chemistry Reviews · 2023-02-08

    Mao‐Yin Ran, A-Yang Wang, Wenbo Wei, Xintao Wu, Hua Lin, Qi‐Long Zhu

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  9. Recent advances in IR nonlinear optical chalcogenides with well-balanced comprehensive performance

    Materials Today Physics · 2023-05-26

    Hedi Yang, Mao‐Yin Ran, Wenbo Wei, Xin‐Tao Wu, Hua Lin, Qi‐Long Zhu

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  10. Modulation of the Band Gap and Redox Properties by Mixed Addenda in Sandwich Polyoxometalates

    Inorganic Chemistry · 2023-11-20

    Ganga Singh, Debaprasad Mandal

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  11. ACu4AsS4 (A = K, Rb): Two infrared nonlinear optical crystals with strong second-harmonic generation responses originating from multiple chromophores

    Scripta Materialia · 2023-12-20

    Xin Lei Zhao, Chensheng Lin, Chao Wang, Haotian Tian, Pengxiang Dong, Tao Yan, Bingxuan Li, Ning Ye, Min Luo

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  12. Phosphosulfide semiconductors for optoelectronics and solar energy conversion

    Journal of Physics Materials · 2024-04-01

    Lena Angelika Mittmann, Andrea Crovetto

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  13. Vacancy‐Induced Extraordinary Second Harmonic Generation Response for Diamond‐Like Cu3PS4

    Advanced Optical Materials · 2024-04-10

    Weiping Guo, Yudi Fu, Hong‐Hua Cui, Lingyun Li, Yan Yu, Zhong‐Zhen Luo, Zhigang Zou

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  14. Ag 2 GeS 3 : A Diamond‐Like Chalcogenide as an IR Nonlinear Optical Material with Outstanding Second‐Harmonic Generation Response

    Advanced Optical Materials · 2024-07-04

    Hong Chen, Mao‐Yin Ran, Shenghua Zhou, Xin‐Tao Wu, Hua Lin

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  15. Phase-Matching Second-Harmonic Generation and Enhanced Laser-Induced Damage Threshold Induced by Cs Substitution: Cu 3 PSe 4 vs Cs 2 CuP 3 S 9

    Inorganic Chemistry · 2024-09-19

    Mingyang Li, Chen‐Yi Zhao, Haiping Xu, Wenfeng Zhou, Wenlong Liu, Jing Zhu, Sheng‐Ping Guo

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  16. Effect of pressure on the structure, elasticity and optical properties of AgGaSe2 crystal

    Physica B Condensed Matter · 2024-10-28

    Zhen Fan, Guangyong Jin, Hongxu Liu, Ye Li

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  17. Exploring new horizons in mid-to-far infrared nonlinear optical crystals: the significant potential of trigonal pyramidal [TeS 3 ] 2− functional units

    Chemical Science · 2025-01-01

    Bo Zhang, Sheng-Hua Zhou, Bingxuan Li, Xin‐Tao Wu, Hua Lin, Qi‐Long Zhu

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  18. Large-area thin-film synthesis of photoactive Cu 3 PS 4 thiophosphate semiconductor with 0–14 pH stability range

    Chemical Science · 2025-01-01

    Lena Angelika Mittmann, Josep Enric Peris Rodrigo, Eugene P. Bertin, Giulia Dalmonte, J.‐C. Grivel, Ivano E. Castelli, Andrea Crovetto

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  19. Symmetry over Chemistry: Harmonic Generation of Low-Dimensional Alkali Chalcopnictates RbMP2S6 (M = Sb, Bi)

    Chemistry of Materials · 2025-03-21

    Benjamin M. Oxley, Joshua Lim, Kyeong‐Hyeon Lee, Jeong-Bin Cho, Saugata Sarker, Jadupati Nag, Michael J. Waters, James M. Rondinelli, Venkatraman Gopalan, Joon Ik Jang, Mercouri G. Kanatzidis

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  20. Structure-property relationships in IR nonlinear optical chalcogenides with stereochemically active lone pairs

    Coordination Chemistry Reviews · 2025-09-03

    Hong Chen, Xin‐Tao Wu, Hua Lin

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  21. Vacancy-driven tetrahedral distortion leading to exceptional second harmonic generation

    Science China Materials · 2025-09-03

    Weiping Guo, Yongjia Zhang, Hong‐Hua Cui, Xin‐Xiong Li, Lingyun Li, Yan Yu, Zhong‐Zhen Luo, Zhigang Zou

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  22. Maximizing the second-harmonic generation response via coordination-induced localization of nonbonding electrons

    Chemical Science · 2025-11-17

    Jia-Xiang Zhang, A-Lan Xu, Yang Chi, Xin-Tao Wu, Hua Lin, Qi‐Long Zhu

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  23. Diamond-like Ag x Cu 3− x PS 4 ( x = 1 and 2) synthesized by the metal oxide–boron–chalcogen (MOBQ) routine: local high-entropy engineering for balanced infrared nonlinear optical performance

    Inorganic Chemistry Frontiers · 2026-01-01

    Ao Guo, Rong-Ling Zhu, Zi-Nan Chen, Zhi Deng, Zong-Ze Li, Shao-Peng Gui, Mao‐Yin Ran, Sheng‐Ping Guo

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  24. van der Waals layered CuInP 2 S 6 as infrared nonlinear optical material

    Chemical Communications · 2026-01-01

    Zheng-Tao Hu, 马祖驹, Xin‐Tao Wu, Qi‐Long Zhu, Hua Lin

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  25. Achieving phase matching in infrared nonlinear optical crystal Cd3ZnSiS6 via isovalent substitution from Cd4SiS6

    Journal of Solid State Chemistry · 2026-04-02

    Ya Yang, Yan Xiao, Ying Zhang, Weiping Guo, Ziwei Li, Bingbing Zhang, Guoqiang Wang, Naifeng Zhuang, Zhong‐Zhen Luo, Zhigang Zou

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  26. From AgGaSe2 to MIIGa2Se4 (MII = Zn, Cd): Heterovalent Substitution Creates Ordered Vacancies for Balanced IR-NLO Performance

    Chinese Journal of Structural Chemistry · 2026-09-01

    Hong Chen, Zheng-Tao Hu, Mao‐Yin Ran, 马祖驹, Xin-Tao Wu, Hua Lin

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  27. Variation of Tetrahedrons and Cations Regulates LIDTs in 3D‐DL Structure MIR‐NLO Crystals

    ChemistrySelect · 2026-09-01

    Chaoyi Zhu

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  28. Phase-Selective Synthesis of Copper Phosphosulfide Nanocrystals

    Inorganic Chemistry · 2026-10-07

    Haley L. Young, Danushki N. Suriyawansa, Raymond E. Schaak

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