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RESEARCH PAPER · Inorganic Chemistry · 2019

Facile Growth of an Ultraviolet Hydroisocyanurate Crystal with Strong Nonlinearity and a Wide Phase-Matching Region from π-Conjugated (HC3N3O3)2– Groups

Xianghe Meng, Fei Liang, Kaijin Kang, Jian Tang, Tixian Zeng, Zheshuai Lin, Mingjun Xia

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Facile Growth of an Ultraviolet Hydroisocyanurate Crystal with Strong Nonlinearity and a Wide Phase-Matching Region from π-Conjugated (HC3N3O3)2– GroupsOriginalLiO 4 tetrahedra lock the alignment of π-conjugated layers to maximize optical anisotropy in metal hydroisocyanurates44RbNa(HC 3 N 3 O 3 )·2H 2 O exhibiting a strong second harmonic generation response and large birefringence as a new potential UV nonlinear optical material69“Old dog, new tricks”: the lone pair effect inducing divergent optical responses in lead cyanurates containing π-bonds18Rb3Na(H2C3N3O3)4·3H2O with Large Birefringence28Structural Diversity and Giant Birefringence in Cyanates BaCNOX (X = Cl, Br, I, and CNO) Containing Linear π-Conjugated Units: A Combined Experimental and Theoretical Study13Hydroisocyanurates X 2 Y(H 2 C 3 N 3 O 3 ) 4 ·4H 2 O (X = K, Cs; Y = Zn, Cd) with large birefringence stemming from π-conjugated (H 2 C 3 N 3 O 3 ) − anions28Inorganic planar π-conjugated groups in nonlinear optical crystals: review and outlook145Second-order nonlinear optical materials with a benzene-like conjugated π system49An Optimal Arrangement of (H2C4N2O3)2– Groups in the First Non-Centrosymmetric Alkali Barbiturate Li2(H2C4N2O3)·2H2O Inducing a Giant Second Harmonic Generation Response and a Striking Birefringence43A UV birefringent crystal: RbNH4(H2C3N3O3)2·2H2O14Mechanochemical Preparation and Solid-State Characterization of 1:1 and 2:1 Ionic Cocrystals of Cyanuric Acid with Alkali Halides12Explorations of Second-Order Nonlinear Optical Materials in the Alkaline Earth Barbiturate System: Noncentrosymmetric Ca(H3C4N2O3)2·H2O and Centrosymmetric Sr(H5C8N4O5)2·4H2O23Mechanochemical Synthesis of an Ionic Cocrystal with Large Birefringence Resulting from Neutral Planar π-Conjugated Groups26Co-crystal AX·(H 3 C 3 N 3 O 3 ) (A = Na, Rb, Cs; X = Br, I): a series of strongly anisotropic alkali halide cyanurates with a planar structural motif and large birefringence13K 2 Pb(H 2 C 3 N 3 O 3 ) 4 (H 2 O) 4 : a potential UV nonlinear optical material with large birefringence50The First Positive Uniaxial Cyanurate Crystals Containing a Crown-like Anionic Group Arrangement and Strengthened Optical Anisotropy17Cyanurates consisting of intrinsic planar π-conjugated 6-membered rings: An emerging source of optical functional materials111Discovery of First Magnesium Fluorooxoborate with Stable Fluorine Terminated Framework for Deep‐UV Nonlinear Optical Application167Discovery of First Magnesium Fluorooxoborate with Stable Fluorine Terminated Framework for Deep‐UV Nonlinear Optical Application18Structure-performance relationship in tri-coordinated nonlinear optical materials toward optimal second harmonic generation and phase matching31An Overview on Recent Trends in Deep‐Ultraviolet (DUV) and Ultraviolet (UV) Nonlinear Optical Crystals25Highly polarized [GeOTe 3 ] motif-driven structural order promotion and an enhanced second harmonic generation response in the new nonlinear optical oxytelluride Ba 3 Ge 2 O 4 Te 334Synergistic Effect of π-Conjugated [C(NH 2 ) 3 ] Cation and Sb(III) Lone Pair Stereoactivity on Structural Transformation and Second Harmonic Generation58Synthesis and Characterization of New-Type Ionic Cocrystals with Cyanuric Acid and Alkali Halides: AX·(H3C3N3O3)2 (A = Rb, Cs; X = Cl, Br)6A flexible functional module to regulate ultraviolet optical nonlinearity for achieving a balance between a second-harmonic generation response and birefringence43Power-Dependent Optical Limiting Behaviour of ‘Star-Type’ Chromophore Via Z-Scan Measurement Under 532 Nm Excitation0Crystal Growth and Physical Properties of the Nonlinear Optical Crystal KLi(HC3N3O3)·2H2O15Perfectly Encoding π‐Conjugated Anions in the RE5(C3N3O3)(OH)12 (RE=Y, Yb, Lu) Family with Strong Second Harmonic Generation Response and Balanced Birefringence91Perfectly Encoding π‐Conjugated Anions in the RE5(C3N3O3)(OH)12 (RE=Y, Yb, Lu) Family with Strong Second Harmonic Generation Response and Balanced Birefringence18Compounds consisting of coplanar π-conjugated B3O6-typed structures: An emerging source of ultraviolet nonlinear optical materials20Recent progress of newly developed functional building units and corresponding nonlinear optical materials14α- and β-(C4H5N2O)(IO3)·HIO3: Two SHG Materials Based on Organic–Inorganic Hybrid Iodates14A review of the relationship between the structure and nonlinear optical properties of organic-inorganic hybrid materials149New Functional Groups Design toward High Performance Ultraviolet Nonlinear Optical Materials95Achieving strong second harmonic generation effects induced via dimensional increase of PbX 6 octahedra and halogen substitutes in (C 10 H 11 N 3 )PbX 4 (X = Cl or Br)26Alkali-metal isocyanurate Cs 3 (H 2 C 3 N 3 O 3 ) 3 (H 3 C 3 N 3 O 3 )·3H 2 O: synthesis and characterization0N 2 H 4 Zn(HC 3 N 3 O 3 ): exceptionally strong second harmonic generation and ultra-long phosphorescence16Recent advances in rational structure design for nonlinear optical crystals: leveraging advantageous templates153Designing Strong Polarity and High Configurational Entropy Flexible Units toward Excellent Ultraviolet Nonlinear Optical Materials42Two Mixed Alkali Metal Isocyanurates with Wide Band Gap and Giant Birefringence2Nonlinear optical cyanurate crystals15“Three functions in one”: multifunctional rare-earth cyamelurates with magnetism, luminescence, and giant optical nonlinearity6Enhanced second harmonic generation in a Fdd 2 polymorph of C 12 H 8 N 2 O 4 Zn for UV nonlinear optical applications1大尺寸RbLi（HC3N3O3）·2H2O晶体生长和光学性能研究（特邀）2An alkali and rare earth metal mixed cyanurate KLa2(C3N3O3)2Cl with large birefringence: Synthesis and characterization2

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  1. LiO 4 tetrahedra lock the alignment of π-conjugated layers to maximize optical anisotropy in metal hydroisocyanurates

    Inorganic Chemistry Frontiers · 2019-01-01

    Xianghe Meng, Fei Liang, Jian Tang, Kaijin Kang, Wenlong Yin, Tixian Zeng, Bin Kang, Zheshuai Lin, Mingjun Xia

    Read original paper ↗ ·

  2. RbNa(HC 3 N 3 O 3 )·2H 2 O exhibiting a strong second harmonic generation response and large birefringence as a new potential UV nonlinear optical material

    Inorganic Chemistry Frontiers · 2019-10-14

    Yunxia Song, Donghong Lin, Min Luo, Chensheng Lin, Qiaoling Chen, Ning Ye

    Read original paper ↗ ·

  3. “Old dog, new tricks”: the lone pair effect inducing divergent optical responses in lead cyanurates containing π-bonds

    Dalton Transactions · 2019-12-11

    Xianghe Meng, Kaijin Kang, Fei Liang, Jian Tang, Zheshuai Lin, Wenlong Yin, Mingjun Xia

    Read original paper ↗ ·

  4. Rb3Na(H2C3N3O3)4·3H2O with Large Birefringence

    ACS Omega · 2019-12-13

    Mukeremu Aibibula, Li Wang, Shuzhao Huang

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  5. Structural Diversity and Giant Birefringence in Cyanates BaCNOX (X = Cl, Br, I, and CNO) Containing Linear π-Conjugated Units: A Combined Experimental and Theoretical Study

    Crystal Growth & Design · 2019-12-27

    Jian Tang, Xianghe Meng, Fei Liang, Kaijin Kang, Tixian Zeng, Mingjun Xia, Wenlong Yin, Zheshuai Lin, Bin Kang

    Read original paper ↗ ·

  6. Hydroisocyanurates X 2 Y(H 2 C 3 N 3 O 3 ) 4 ·4H 2 O (X = K, Cs; Y = Zn, Cd) with large birefringence stemming from π-conjugated (H 2 C 3 N 3 O 3 ) − anions

    CrystEngComm · 2020-01-01

    Kaijin Kang, Xianghe Meng, Fei Liang, Jian Tang, Tixian Zeng, Wenlong Yin, Zheshuai Lin, Mingjun Xia

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  7. Inorganic planar π-conjugated groups in nonlinear optical crystals: review and outlook

    Inorganic Chemistry Frontiers · 2020-01-01

    Pifu Gong, Xiaomeng Liu, Lei Kang, Zheshuai Lin

    Read original paper ↗ ·

  8. Second-order nonlinear optical materials with a benzene-like conjugated π system

    Chemical Communications · 2020-01-01

    Hongkun Liu, Bingbing Zhang, Ying Wang

    Read original paper ↗ ·

  9. An Optimal Arrangement of (H2C4N2O3)2– Groups in the First Non-Centrosymmetric Alkali Barbiturate Li2(H2C4N2O3)·2H2O Inducing a Giant Second Harmonic Generation Response and a Striking Birefringence

    Crystal Growth & Design · 2020-07-24

    Donghong Lin, Min Luo, Chensheng Lin, Liling Cao, Ning Ye

    Read original paper ↗ ·

  10. A UV birefringent crystal: RbNH4(H2C3N3O3)2·2H2O

    Inorganic Chemistry Communications · 2020-07-27

    Mukeremu Aibibula, Li Wang

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  11. Mechanochemical Preparation and Solid-State Characterization of 1:1 and 2:1 Ionic Cocrystals of Cyanuric Acid with Alkali Halides

    Crystal Growth & Design · 2020-09-24

    Oleksii Shemchuk, Fabrizia Grepioni, Dario Braga

    Read original paper ↗ ·

  12. Explorations of Second-Order Nonlinear Optical Materials in the Alkaline Earth Barbiturate System: Noncentrosymmetric Ca(H3C4N2O3)2·H2O and Centrosymmetric Sr(H5C8N4O5)2·4H2O

    Inorganic Chemistry · 2020-10-12

    Yiyi Xu, Chensheng Lin, Donghong Lin, Min Luo, Dan Zhao, Liling Cao, Ning Ye

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  13. Mechanochemical Synthesis of an Ionic Cocrystal with Large Birefringence Resulting from Neutral Planar π-Conjugated Groups

    Crystal Growth & Design · 2020-11-10

    Xianghe Meng, Kaijin Kang, Youquan Liu, Jian Tang, Xingxing Jiang, Wenlong Yin, Zheshuai Lin, Mingjun Xia

    Read original paper ↗ ·

  14. Co-crystal AX·(H 3 C 3 N 3 O 3 ) (A = Na, Rb, Cs; X = Br, I): a series of strongly anisotropic alkali halide cyanurates with a planar structural motif and large birefringence

    Dalton Transactions · 2021-01-01

    Jinhui Wang, Xinyuan Zhang, Fei Liang, Zhanggui Hu, Yicheng Wu

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  15. K 2 Pb(H 2 C 3 N 3 O 3 ) 4 (H 2 O) 4 : a potential UV nonlinear optical material with large birefringence

    Inorganic Chemistry Frontiers · 2021-01-01

    Yan Chen, Chun‐Li Hu, Zhi Gang Fang, Jiang‐Gao Mao

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  16. The First Positive Uniaxial Cyanurate Crystals Containing a Crown-like Anionic Group Arrangement and Strengthened Optical Anisotropy

    Crystal Growth & Design · 2021-02-25

    Dandan Wang, Fei Liang, Xinyuan Zhang, Zhanggui Hu, Yicheng Wu

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  17. Cyanurates consisting of intrinsic planar π-conjugated 6-membered rings: An emerging source of optical functional materials

    Coordination Chemistry Reviews · 2021-04-14

    Xianghe Meng, Wenlong Yin, Mingjun Xia

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  18. Discovery of First Magnesium Fluorooxoborate with Stable Fluorine Terminated Framework for Deep‐UV Nonlinear Optical Application

    Angewandte Chemie International Edition · 2021-04-19

    Ming Xia, Fuming Li, Miriding Mutailipu, Shujuan Han, Zhihua Yang, Shilie Pan

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  19. Discovery of First Magnesium Fluorooxoborate with Stable Fluorine Terminated Framework for Deep‐UV Nonlinear Optical Application

    Angewandte Chemie · 2021-04-19

    Ming Xia, Fuming Li, Miriding Mutailipu, Shujuan Han, Zhihua Yang, Shilie Pan

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  20. Structure-performance relationship in tri-coordinated nonlinear optical materials toward optimal second harmonic generation and phase matching

    Coordination Chemistry Reviews · 2021-06-08

    Fengjuan Hou, Dajiang Mei, Mingjun Xia, Yuandong Wu

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  21. An Overview on Recent Trends in Deep‐Ultraviolet (DUV) and Ultraviolet (UV) Nonlinear Optical Crystals

    ChemistrySelect · 2021-10-18

    Sekar Anand, M. Usha Rani, S. Kalainathan

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  22. Highly polarized [GeOTe 3 ] motif-driven structural order promotion and an enhanced second harmonic generation response in the new nonlinear optical oxytelluride Ba 3 Ge 2 O 4 Te 3

    Journal of Materials Chemistry C · 2021-11-18

    Mengran Sun, Xingyu Zhang, Chunxiao Li, Wenhao Liu, Zheshuai Lin, Jiyong Yao

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  23. Synergistic Effect of π-Conjugated [C(NH 2 ) 3 ] Cation and Sb(III) Lone Pair Stereoactivity on Structural Transformation and Second Harmonic Generation

    Inorganic Chemistry · 2021-11-19

    Man Zhang, Bingbing Zhang, Daqing Yang, Ying Wang

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  24. Synthesis and Characterization of New-Type Ionic Cocrystals with Cyanuric Acid and Alkali Halides: AX·(H3C3N3O3)2 (A = Rb, Cs; X = Cl, Br)

    Crystal Growth & Design · 2021-11-19

    Jinhui Wang, Xinyuan Zhang, Fei Liang, Zhanggui Hu, Yicheng Wu

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  25. A flexible functional module to regulate ultraviolet optical nonlinearity for achieving a balance between a second-harmonic generation response and birefringence

    Chemical Science · 2022-01-01

    Liling Cao, Haotian Tian, Donghong Lin, Chensheng Lin, Feng Xu, Yinglei Han, Tao Yan, Jindong Chen, Bingxuan Li, Ning Ye, Min Luo

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  26. Power-Dependent Optical Limiting Behaviour of ‘Star-Type’ Chromophore Via Z-Scan Measurement Under 532 Nm Excitation

    SSRN Electronic Journal · 2022-01-01

    Muhammad Izz Rosli, M. Abdullah, G. Krishnan, N. Basar, M.S. Aziz, Sulaiman Wadi Harun, R. Awang, Fatin Saiha Omar

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  27. Crystal Growth and Physical Properties of the Nonlinear Optical Crystal KLi(HC3N3O3)·2H2O

    Crystal Growth & Design · 2022-04-24

    Feng Xu, Bingxuan Li, Tao Yan, Lingxiong Huang, Ge Zhang, Ning Ye, Min Luo

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  28. Perfectly Encoding π‐Conjugated Anions in the RE5(C3N3O3)(OH)12 (RE=Y, Yb, Lu) Family with Strong Second Harmonic Generation Response and Balanced Birefringence

    Angewandte Chemie International Edition · 2022-11-08

    Xianghe Meng, Xingyu Zhang, Qingxiong Liu, Zhengyang Zhou, Xingxing Jiang, Yonggang Wang, Zheshuai Lin, Mingjun Xia

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  29. Perfectly Encoding π‐Conjugated Anions in the RE5(C3N3O3)(OH)12 (RE=Y, Yb, Lu) Family with Strong Second Harmonic Generation Response and Balanced Birefringence

    Angewandte Chemie · 2022-11-08

    Xianghe Meng, Xingyu Zhang, Qingxiong Liu, Zhengyang Zhou, Xingxing Jiang, Yonggang Wang, Zheshuai Lin, Mingjun Xia

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  30. Compounds consisting of coplanar π-conjugated B3O6-typed structures: An emerging source of ultraviolet nonlinear optical materials

    Chinese Journal of Structural Chemistry · 2023-01-01

    Lingli Wu, Huixin Fan, Chensheng Lin, Min Luo

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  31. Recent progress of newly developed functional building units and corresponding nonlinear optical materials

    Chinese Journal of Structural Chemistry · 2023-05-11

    Wenjing Tan, Chenyang Zhang, Chenyang Zhang, Tingting Huang, Bingbing Zhang

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  32. α- and β-(C4H5N2O)(IO3)·HIO3: Two SHG Materials Based on Organic–Inorganic Hybrid Iodates

    Inorganic Chemistry · 2023-08-11

    Qianqian Chen, Chun‐Li Hu, Mingzhi Zhang, Bingxuan Li, Jiang‐Gao Mao

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  33. A review of the relationship between the structure and nonlinear optical properties of organic-inorganic hybrid materials

    Coordination Chemistry Reviews · 2023-10-06

    Yuwei Kang, Qi Wu

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  34. New Functional Groups Design toward High Performance Ultraviolet Nonlinear Optical Materials

    Accounts of Chemical Research · 2023-10-27

    Huixin Fan, Ning Ye, Min Luo

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  35. Achieving strong second harmonic generation effects induced via dimensional increase of PbX 6 octahedra and halogen substitutes in (C 10 H 11 N 3 )PbX 4 (X = Cl or Br)

    Inorganic Chemistry Frontiers · 2024-01-01

    Liling Zhang, Qingran Ding, Peihan Wang, Yanqiu Zhang, Qing‐Yan Liu, Yu‐Ling Wang, Junhua Luo

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  36. Alkali-metal isocyanurate Cs 3 (H 2 C 3 N 3 O 3 ) 3 (H 3 C 3 N 3 O 3 )·3H 2 O: synthesis and characterization

    CrystEngComm · 2024-01-01

    Xinyue Wang, Dandan Wang, Yujie Liu, Jinhui Wang

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  37. N 2 H 4 Zn(HC 3 N 3 O 3 ): exceptionally strong second harmonic generation and ultra-long phosphorescence

    Chemical Science · 2024-01-01

    Can Hui Yang, Yuwei Kang, Xuefei Wang, Jie Gou, Yi Xiong, Zece Zhu, Ling Chen, Qi Wu

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  38. Recent advances in rational structure design for nonlinear optical crystals: leveraging advantageous templates

    Chemical Society Reviews · 2024-01-01

    Ziting Yan, Jinbin Fan, Shilie Pan, Min Zhang

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  39. Designing Strong Polarity and High Configurational Entropy Flexible Units toward Excellent Ultraviolet Nonlinear Optical Materials

    Advanced Functional Materials · 2024-04-15

    Haotian Tian, Chensheng Lin, Bingxuan Li, Xin Lei Zhao, Tao Yan, Ning Ye, Min Luo

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  40. Two Mixed Alkali Metal Isocyanurates with Wide Band Gap and Giant Birefringence

    Crystal Growth & Design · 2024-05-15

    Xinyue Wang, Jinhui Wang, Xinyuan Zhang, Fei Liang, Zhanggui Hu, Yicheng Wu

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  41. Nonlinear optical cyanurate crystals

    Journal of Crystal Growth · 2024-10-09

    Xianghe Meng, Haotian Tian, Qian Wu, Mingjun Xia

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  42. “Three functions in one”: multifunctional rare-earth cyamelurates with magnetism, luminescence, and giant optical nonlinearity

    Chemical Science · 2025-01-01

    Jing Zhang, Yuxiao Liu, Fangyan Wang, Pifu Gong, Zhaoyi Li, Xinyuan Zhang, Fei Liang, Shu Hai Guo, Zhanggui Hu, Yicheng Wu

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  43. Enhanced second harmonic generation in a Fdd 2 polymorph of C 12 H 8 N 2 O 4 Zn for UV nonlinear optical applications

    Dalton Transactions · 2025-01-01

    Jie Gou, Can Yang, YunJie Wang, Yaolong Zhu, Qingwen Zhu, Xin Su, Qi Wu

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  44. 大尺寸RbLi（HC3N3O3）·2H2O晶体生长和光学性能研究（特邀）

    Chinese Journal of Lasers · 2025-01-01

    颜涛 Yan Tao, 董鑫航 Dong Xinhang, 林菊 Lin Ju, 陈昱 Chen Yu, 罗敏 Luo Min

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  45. An alkali and rare earth metal mixed cyanurate KLa2(C3N3O3)2Cl with large birefringence: Synthesis and characterization

    Solid State Communications · 2025-02-05

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