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RESEARCH PAPER · Journal of the American Chemical Society · 2019

Thermodynamics and Electronic Properties of Heterometallic Multinuclear Actinide-Containing Metal–Organic Frameworks with “Structural Memory”

Otega A. Ejegbavwo, Corey R. Martin, Oyindamola A. Olorunfemi, Gabrielle A. Leith, Richard T. Ly, Allison M. Rice, Ekaterina A. Dolgopolova, Mark D. Smith, S. Karakalos, Nancy R. Birkner, Brian A. Powell, Shubham Pandey, Robert J. Koch, Scott T. Misture, Hans‐Conrad zur Loye, Simon Robert Phillpot, Kyle S. Brinkman, Natalia B. Shustova

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Thermodynamics and Electronic Properties of Heterometallic Multinuclear Actinide-Containing Metal–Organic Frameworks with “Structural Memory”OriginalTetranuclear oxido-bridged thorium( iv ) clusters obtained using tridentate Schiff bases18Sequestration of Radionuclides in Metal–Organic Frameworks from Density Functional Theory Calculations15Unexpected structural complexity of thorium coordination polymers and polyoxo cluster built from simple formate ligands34Heterometallic multinuclear nodes directing MOF electronic behavior28Improving the Cd 2+ detection capability of a new anionic rare earth metal–organic framework based on a [RE 6 (μ 3 -OH) 8 ] 10+ secondary building unit: an ion-exchange approach towards more efficient sensors11Structural properties of ultra-small thorium and uranium dioxide nanoparticles embedded in a covalent organic framework45Oligonuclear Actinoid Complexes with Schiff Bases as Ligands—Older Achievements and Recent Progress52Ultrastable Thorium Metal–Organic Frameworks for Efficient Iodine Adsorption162Electrically Conductive Metal–Organic Frameworks1999Supramolecular Assembly of U(IV) Clusters and Superatoms with Unconventional Countercations51From Isolated Molecular Complexes to Extended Networks: Synthesis and Characterization of Thorium Furanmono‐ and Dicarboxylates2Electronic structures and magnetism of Zr-, Th-, and U-based metal-organic frameworks (MOFs) by density functional theory38Rational Design of a Uranyl Metal–Organic Framework for the Capture and Colorimetric Detection of Organic Dyes22Let the light be a guide: Chromophore communication in metal-organic frameworks60Three-Dimensional Polycatenation of a Uranium-Based Metal–Organic Cage: Structural Complexity and Radiation Detection124Metal–Organic Frameworks Based on Group 3 and 4 Metals140Metal-organic frameworks as a versatile platform for radionuclide management162Boosting the Iodine Adsorption and Radioresistance of Th‐UiO‐66 MOFs via Aromatic Substitution118Destruction of Metal–Organic Frameworks: Positive and Negative Aspects of Stability and Lability662Programmable Triboelectric Nanogenerators Dependent on the Secondary Building Units in Cadmium Coordination Polymers31A cationic thorium–organic framework with triple single-crystal-to-single-crystal transformation peculiarities for ultrasensitive anion recognition29Beyond structural motifs: the frontier of actinide-containing metal–organic frameworks65Emergence of a thorium–organic framework as a radiation attenuator for selective X-ray dosimetry20Achieving UV and X-ray Dual Photochromism in a Metal–Organic Hybrid via Structural Modulation38Heterometallic Actinide‐Containing Photoresponsive Metal‐Organic Frameworks: Dynamic and Static Tuning of Electronic Properties78Heterometallic Actinide‐Containing Photoresponsive Metal‐Organic Frameworks: Dynamic and Static Tuning of Electronic Properties11Interpenetration Control in Thorium Metal–Organic Frameworks: Structural Complexity toward Iodine Adsorption35Evaluating the Robustness of Metal–Organic Frameworks for Synthetic Chemistry66Conductive Metal‐Organic Frameworks: Electronic Structure and Electrochemical Applications54Keggin-type polyoxometalates molecularly loaded in Zr-ferrocene metal organic framework nanosheets for solar-driven CO2 cycloaddition128Visible colorimetric dosimetry of UV and ionizing radiations by a dual-module photochromic nanocluster109An Azobenzene-Modified Photoresponsive Thorium–Organic Framework: Monitoring and Quantitative Analysis of Reversible trans–cis Photoisomerization30An updated status and trends in actinide metal-organic frameworks (An-MOFs): From synthesis to application145Fluorite-like hydrolyzed hexanuclear coordination clusters of Zr(IV) and Hf(IV) with syn-syn bridging N,N,N-trimethylglycine in soft crystal structures exhibiting cold-crystallization8Tuning and Directing Energy Transfer in the Whole Visible Spectrum through Linker Installation in Metal–Organic Frameworks72Tuning and Directing Energy Transfer in the Whole Visible Spectrum through Linker Installation in Metal–Organic Frameworks11MOF‐Based Sustainable Memory Devices63Unveiling the Unique Roles of Metal Coordination and Modulator in the Polymorphism Control of Metal‐Organic Frameworks202-Dimensional rare earth metal–organic frameworks based on a hexanuclear secondary building unit as efficient detectors for vapours of nitroaromatics and volatile organic compounds20A semiconducting uranium–organic framework based on a tetrathiafulvalene derivative4Recent advances in the applications of thorium-based metal–organic frameworks and molecular clusters50Recent advances in uranium-containing polyoxometalates58A New Concept of Radiation Detection Based on a Fluorochromic and Piezochromic Nanocluster70Playing “Jenga” with MOFs: De-interpenetration for pore opening4A Structure–Activity Study of Aromatic Acid Modulators for the Synthesis of Zirconium-Based Metal–Organic Frameworks78Multi-step Phase Transformation from Metal–Organic Frameworks to Inorganic Compounds for High-Purity Th(IV) Generation5Application of MOFs and COFs for photocatalysis in CO2 reduction, H2 generation, and environmental treatment476Capture Instead of Release: Defect-Modulated Radionuclide Leaching Kinetics in Metal–Organic Frameworks35Energetic Systematics of Metal–Organic Frameworks: A Case Study of Al(III)-Trimesate MOF Isomers16Extremely Stable Thorium‐MOF Assembly of Tetraphenylethylene Derivative With Tunable AIE Property and Highly Selective Detection of Nitro Aromatic Compounds28Achieving High Photo/Thermocatalytic Product Selectivity and Conversion via Thorium Clusters with Switchable Functional Ligands87Creating High-Number Defect Sites through a Bimetal Approach in Metal–Organic Frameworks for Boosting Trace SO2 Removal7f‐block MOFs: A Pathway to Heterometallic Transuranics29f‐block MOFs: A Pathway to Heterometallic Transuranics1Stepwise Crystallization of Millimeter Scale Thorium Cluster Single Crystals as a Bifunctional Platform for X‐ray Detection and Shielding9A robust thorium–organic framework as a bifunctional platform for iodine adsorption and Cr( vi ) sensitization9Energy–structure–property relationships in uranium metal–organic frameworks32The Capture Performance of An-Mof for Fission Gases: Insight from Dft and Aimd Calculations0Topological control of metal–organic frameworks toward highly sensitive and selective detection of chromate and dichromate32Ortho Effects of Tricarboxylate Linkers in Regulating Topologies of Rare-Earth Metal–Organic Frameworks34Adsorption and Detection of Iodine Species by a Thorium-Based Metal–Organic Framework46Assembling a Heterobimetallic Actinide Metal‐Organic Framework by a Reaction‐Induced Preorganization Strategy21Assembling a Heterobimetallic Actinide Metal‐Organic Framework by a Reaction‐Induced Preorganization Strategy0Exploration and Application of the Self-Optimization Phenomenon of a Trimetal-Based MOF Electrocatalyst in the Oxygen Evolution Reaction18Near-Unity Energy Transfer from Uranyl to Europium in a Heterobimetallic Organic Framework with Record-Breaking Quantum Yield135Synthetic Control of Thorium Metal‐Organic Frameworks for Sequencing and Sensing of Radioiodine Species20Integrating Metal Complex Units and Redox Sites into Thorium‐Based Metal–Organic Frameworks for Selective Photocatalytic Oxidation of Sulfides37Binding of uranyl cations to a Zr-based metal-organic framework by density functional theory3The capture performance of An-MOF for fission gases: Insight from DFT and AIMD calculations6Linker installation transformations in a 2-D rare earth MOF: increase of the dimensionality and turn on of the temperature sensing capability11Mechanistic synthesis of a sequential calcium-carboxylate-based linker (Ca-MOFs) and rapid assessment of chemical stability through XRD analysis12Quest for Multifunctionality: Current Progress in the Characterization of Heterometallic Metal–Organic Frameworks42Friends or Foes: Fundamental Principles of Th-Organic Scaffold Chemistry Using Zr-Analogs as a Guide22Semiconductive Behavior and Photoconductivity of Uranyl Dithiophosphinate Single Crystal1Unraveling the role of coordinated water in the capture of americium and toxic gases by an ultrastable uranyl phosphonate framework12Mining for Metal–Organic Systems: Chemistry Frontiers of Th-, U-, and Zr-Materials18Constructing Functional Radiation-Resistant Thorium Clusters for Catalytic Redox Reactions31Rod-Like Tetraphenylethylene-Based Metal–Organic Framework for Ultrasensitive Detection of Neuron-Specific Enolase9Application of Hard and Soft Acid‐base Theory to Construct Heterometallic Materials with Metal‐oxo Clusters52Application of Hard and Soft Acid‐base Theory to Construct Heterometallic Materials with Metal‐oxo Clusters5Are MOFs ready for environmental applications: Assessing stability against natural stressors?74Stability of Metal–Organic Frameworks in Organic Media with Acids and Bases49Shaping the future of solar-driven photocatalysis by reticular framework materials45Investigation of Metal-Organic Frameworks (MOFs): Synthesis, Properties, and Applications - An In-Depth Review181Crystallographic Evidence for Formation of M 6 O 8 /M 6 O 9 f-Element Clusters in Hydrolysis Reactions6Visible‐Light‐Driven TiO 2 /Pt Nanozyme‐Embedded Dressings: Integrating PDT, Oxygenation, and Biomechanical Support for Pressure Ulcer Repair3Rational design of a rare N-coordinated thorium organic framework for efficient CO2 capture and catalytic conversion2Electronic structures and gas adsorption behaviors of 12–coordinated Th (U)–based metal–organic frameworks0An electrochemiluminescence immunosensor for neuron-specific enolase detection based on resonance energy transfer between europium-based metal-organic frameworks and GO-Au composites0Thermodynamics of metal–organic frameworks: from fundamentals to advanced applications4Metal-organic frameworks for nuclear waste remediation: A review of cutting-edge advances and applications11Highly Water-Stable Uranyl-Cluster Based Metal–Organic Framework for Thermal Adaptive Scintillator5The phase and energy-level evolutions in seven distinct sequential states and their hierarchical memory effect of isomeric MOFs2Computational Investigation of the Effect of Transition Metal Coordination in Bimetallic Uranylpyridine-Dicarboxylate Complexes0Approximating Standard Formation Enthalpies of Porous Metal–Organic Frameworks: Extending a Gas-Phase Approach to Porous Solids0Intrinsic Large‐Unit‐Cell Systems for Advanced Thermoelectrics and Thermal Management0

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  1. Tetranuclear oxido-bridged thorium( iv ) clusters obtained using tridentate Schiff bases

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  2. Sequestration of Radionuclides in Metal–Organic Frameworks from Density Functional Theory Calculations

    The Journal of Physical Chemistry C · 2019-10-14

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  3. Unexpected structural complexity of thorium coordination polymers and polyoxo cluster built from simple formate ligands

    Inorganic Chemistry Frontiers · 2019-10-29

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  4. Heterometallic multinuclear nodes directing MOF electronic behavior

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  5. Improving the Cd 2+ detection capability of a new anionic rare earth metal–organic framework based on a [RE 6 (μ 3 -OH) 8 ] 10+ secondary building unit: an ion-exchange approach towards more efficient sensors

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  6. Structural properties of ultra-small thorium and uranium dioxide nanoparticles embedded in a covalent organic framework

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  7. Oligonuclear Actinoid Complexes with Schiff Bases as Ligands—Older Achievements and Recent Progress

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  8. Ultrastable Thorium Metal–Organic Frameworks for Efficient Iodine Adsorption

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  9. Electrically Conductive Metal–Organic Frameworks

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  10. Supramolecular Assembly of U(IV) Clusters and Superatoms with Unconventional Countercations

    Journal of the American Chemical Society · 2020-04-22

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  11. From Isolated Molecular Complexes to Extended Networks: Synthesis and Characterization of Thorium Furanmono‐ and Dicarboxylates

    European Journal of Inorganic Chemistry · 2020-06-19

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  12. Electronic structures and magnetism of Zr-, Th-, and U-based metal-organic frameworks (MOFs) by density functional theory

    Computational Materials Science · 2020-07-09

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  13. Rational Design of a Uranyl Metal–Organic Framework for the Capture and Colorimetric Detection of Organic Dyes

    Chemistry - A European Journal · 2020-07-18

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  14. Let the light be a guide: Chromophore communication in metal-organic frameworks

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  15. Three-Dimensional Polycatenation of a Uranium-Based Metal–Organic Cage: Structural Complexity and Radiation Detection

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  16. Metal–Organic Frameworks Based on Group 3 and 4 Metals

    Advanced Materials · 2020-09-09

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  17. Metal-organic frameworks as a versatile platform for radionuclide management

    Coordination Chemistry Reviews · 2020-09-15

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  18. Boosting the Iodine Adsorption and Radioresistance of Th‐UiO‐66 MOFs via Aromatic Substitution

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  19. Destruction of Metal–Organic Frameworks: Positive and Negative Aspects of Stability and Lability

    Chemical Reviews · 2020-10-13

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  20. Programmable Triboelectric Nanogenerators Dependent on the Secondary Building Units in Cadmium Coordination Polymers

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  21. A cationic thorium–organic framework with triple single-crystal-to-single-crystal transformation peculiarities for ultrasensitive anion recognition

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  22. Beyond structural motifs: the frontier of actinide-containing metal–organic frameworks

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  23. Emergence of a thorium–organic framework as a radiation attenuator for selective X-ray dosimetry

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  24. Achieving UV and X-ray Dual Photochromism in a Metal–Organic Hybrid via Structural Modulation

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  25. Heterometallic Actinide‐Containing Photoresponsive Metal‐Organic Frameworks: Dynamic and Static Tuning of Electronic Properties

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  26. Heterometallic Actinide‐Containing Photoresponsive Metal‐Organic Frameworks: Dynamic and Static Tuning of Electronic Properties

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  27. Interpenetration Control in Thorium Metal–Organic Frameworks: Structural Complexity toward Iodine Adsorption

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  28. Evaluating the Robustness of Metal–Organic Frameworks for Synthetic Chemistry

    ACS Applied Materials & Interfaces · 2021-04-06

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  29. Conductive Metal‐Organic Frameworks: Electronic Structure and Electrochemical Applications

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  30. Keggin-type polyoxometalates molecularly loaded in Zr-ferrocene metal organic framework nanosheets for solar-driven CO2 cycloaddition

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  31. Visible colorimetric dosimetry of UV and ionizing radiations by a dual-module photochromic nanocluster

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  32. An Azobenzene-Modified Photoresponsive Thorium–Organic Framework: Monitoring and Quantitative Analysis of Reversible trans–cis Photoisomerization

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  33. An updated status and trends in actinide metal-organic frameworks (An-MOFs): From synthesis to application

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  34. Fluorite-like hydrolyzed hexanuclear coordination clusters of Zr(IV) and Hf(IV) with syn-syn bridging N,N,N-trimethylglycine in soft crystal structures exhibiting cold-crystallization

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  35. Tuning and Directing Energy Transfer in the Whole Visible Spectrum through Linker Installation in Metal–Organic Frameworks

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  36. Tuning and Directing Energy Transfer in the Whole Visible Spectrum through Linker Installation in Metal–Organic Frameworks

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  37. MOF‐Based Sustainable Memory Devices

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  38. Unveiling the Unique Roles of Metal Coordination and Modulator in the Polymorphism Control of Metal‐Organic Frameworks

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  39. 2-Dimensional rare earth metal–organic frameworks based on a hexanuclear secondary building unit as efficient detectors for vapours of nitroaromatics and volatile organic compounds

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  40. A semiconducting uranium–organic framework based on a tetrathiafulvalene derivative

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  41. Recent advances in the applications of thorium-based metal–organic frameworks and molecular clusters

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  42. Recent advances in uranium-containing polyoxometalates

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  43. A New Concept of Radiation Detection Based on a Fluorochromic and Piezochromic Nanocluster

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  44. Playing “Jenga” with MOFs: De-interpenetration for pore opening

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  45. A Structure–Activity Study of Aromatic Acid Modulators for the Synthesis of Zirconium-Based Metal–Organic Frameworks

    Chemistry of Materials · 2022-03-28

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  46. Multi-step Phase Transformation from Metal–Organic Frameworks to Inorganic Compounds for High-Purity Th(IV) Generation

    Inorganic Chemistry · 2022-05-03

    Yiwei Huang, Feng Li Han, Xiao‐Hong Xiong, Feng Luo

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  47. Application of MOFs and COFs for photocatalysis in CO2 reduction, H2 generation, and environmental treatment

    EnergyChem · 2022-06-25

    Yifeng Zhang, Hangxi Liu, Feixue Gao, Xiaoli Tan, Yawen Cai, Baowei Hu, Qifei Huang, Ming Fang, Xiangke Wang

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  48. Capture Instead of Release: Defect-Modulated Radionuclide Leaching Kinetics in Metal–Organic Frameworks

    Journal of the American Chemical Society · 2022-08-26

    Kyoung Chul Park, Corey R. Martin, Gabrielle A. Leith, Grace C. Thaggard, Gina R. Wilson, Brandon J. Yarbrough, Buddhima K. P. Maldeni Kankanamalage, Preecha Kittikhunnatham, Abhijai Mathur, Isak Jatoi, Mackenzie A. Manzi, Jaewoong Lim, Ingrid Lehman‐Andino, Alejandra Hernandez-Jimenez, Jake Amoroso, David P. DiPrete, Yuan Liu, Joseph C. Schaeperkoetter, Scott T. Misture, Simon Robert Phillpot, Shenyang Hu, Yulan Li, Antoine Leydier, Vanessa Proust, Agnès Grandjean, Mark D. Smith, Natalia B. Shustova

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  49. Energetic Systematics of Metal–Organic Frameworks: A Case Study of Al(III)-Trimesate MOF Isomers

    Inorganic Chemistry · 2022-09-13

    Jiahong Li, Vitaliy G. Goncharov, Andrew Strzelecki, Hongwu Xu, Xiaofeng Guo, Qiang Zhang

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  50. Extremely Stable Thorium‐MOF Assembly of Tetraphenylethylene Derivative With Tunable AIE Property and Highly Selective Detection of Nitro Aromatic Compounds

    Advanced Materials Interfaces · 2022-09-22

    Qing Lin Guan, Fen Xu, Yao Xiao, Zi-Xin You, Feng‐Ying Bai, Yong‐Heng Xing

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