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RESEARCH PAPER · Advanced Materials · 2020

Metal–Organic Frameworks Based on Group 3 and 4 Metals

Liang Feng, Jiandong Pang, Ping She, Jia‐Luo Li, Jun‐Sheng Qin, Dong‐Ying Du, Hong-Cai “Joe” Zhou

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Metal–Organic Frameworks Based on Group 3 and 4 MetalsOriginalCr2O72− inside Zr/Hf-based metal–organic frameworks: highly sensitive and selective detection and crystallographic evidence43A Series of Mesoporous Rare‐Earth Metal–Organic Frameworks Constructed from Organic Secondary Building Units76A Series of Mesoporous Rare‐Earth Metal–Organic Frameworks Constructed from Organic Secondary Building Units1Crystal engineering of porous coordination networks for C3 hydrocarbon separation66Alkyl decorated metal–organic frameworks for selective trapping of ethane from ethylene above ambient pressures21The coordination chemistry of benzhydrazide with lanthanide( iii ) ions: hydrothermal in situ ligand formation, structures, magnetic and photoluminescence sensing properties14Linker Desymmetrization: Access to a Series of Rare-Earth Tetracarboxylate Frameworks with Eight-Connected Hexanuclear Nodes125Selective Crystallization of Rare‐Earth Ions into Cationic Metal‐Organic Frameworks for Rare‐Earth Separation93Selective Crystallization of Rare‐Earth Ions into Cationic Metal‐Organic Frameworks for Rare‐Earth Separation6Structural and Hydrolytic Stability of Coordinatively Unsaturated Metal–Organic Frameworks M3(BTC)2 (M = Cu, Co, Mn, Ni, and Zn): A Combined DFT and Experimental Study33The forgotten chemistry of group(IV) metals: A survey on the synthesis, structure, and properties of discrete Zr(IV), Hf(IV), and Ti(IV) oxo clusters91Pyrazolate-based porphyrinic metal-organic frameworks as catechol oxidase mimic enzyme for fluorescent and colorimetric dual-mode detection of dopamine with high sensitivity and specificity55Incorporating Photochromic Triphenylamine into a Zirconium–Organic Framework for Highly Effective Photocatalytic Aerobic Oxidation of Sulfides102A Showcase of Green Chemistry: Sustainable Synthetic Approach of Zirconium‐Based MOF Materials78A Review of MOFs and Their Composites‐Based Photocatalysts: Synthesis and Applications540Metal-organic frameworks in cooling and water desalination: Synthesis and application58High Enhancement in Proton Conductivity by Incorporating Sulfonic Acids into a Zirconium-Based Metal–Organic Framework via “Click” Reaction38An updated status and trends in actinide metal-organic frameworks (An-MOFs): From synthesis to application145Structure, Luminescent Sensing and Proton Conduction of a Boiling-Water-Stable Zn(II) Metal-Organic Framework7Fiber Surface/Interfacial Engineering on Wearable Electronics45Topology-guided synthesis and construction of amide-functionalized rare-earth metal–organic frameworks11Aqueous Stability of Zirconium Clusters, Including the Zr(IV) Hexanuclear Hydrolysis Complex [Zr 6 O 4 (OH) 4 (H 2 O) 24 ] 12+ , from Density Functional Theory22Constructing Cationic Metal–Organic Framework Materials Based on Pyrimidyl as a Functional Group for Perrhenate/Pertechnetate Sorption44Synthesis of metal–organic-frameworks on polydopamine modified cellulose nanofibril hydrogels: constructing versatile vehicles for hydrophobic drug delivery56Novel cerium-based MOFs photocatalyst for photocarrier collaborative performance under visible light62Design of ultra-stable Yttrium-organic framework adsorbents for efficient methane purification and storage20Effect of the Defect Modulator and Ligand Length of Metal–Organic Frameworks on Carbon Dioxide Photoreduction53Amino group induced structural diversity and near-infrared emission of yttrium-tetracarboxylate frameworks38Novel lanthanide nanoparticle frameworks for highly efficient photoluminescence and hypersensitive detection20Which factors govern the adsorption of peptides to Zr( iv )-based metal–organic frameworks?23Zirconium oxo clusters as discrete molecular catalysts for the direct amide bond formation40Zr 4+ -terephthalate MOFs with 6-connected structures, highly efficient As( iii / v ) sorption and superhydrophobic properties11Tumor acidity and near-infrared light responsive drug delivery MoS2-based nanoparticles for chemo-photothermal therapy27The Chemistry of Zirconium/Carboxylate Clustering Process: Acidic Conditions to Promote Carboxylate-Unsaturated Octahedral Hexamers and Pentanuclear Species29A Multifunctional Porous Uranyl Phosphonate Framework for Cyclic Utilization: Salvages, Uranyl Leaking Prevention, and Fluorescent Sensing44Mixed-Linker Strategy for the Construction of Metal–Organic Framework Combined with Dyes toward Alcohol Detection13Customized Synthesis: Solvent- and Acid-Assisted Topology Evolution in Zirconium-Tetracarboxylate Frameworks33Subnanometric Cu clusters on atomically Fe-doped MoO2 for furfural upgrading to aviation biofuels51Cage‐Ligand Strategy for the Construction of Zr4(embonate)6–Based MOFs with Third‐Order Nonlinear‐Optical Properties14Four new coordination polymers constructed by (3-carboxyl-phenyl)-(4-(2’-carboxyl-phenyl)-benzyl) ether and 2,2'-bipyridine6Highly Porous Materials as Potential Components of Natural Gas Storage Systems: Part 2 (A Review)7Construction of Co/Fe co-embedded in benzene tricarboxylic acid with modulated coordination environment for accelerated oxygen evolution reaction6Metal-organic framework-derived nitrogen-doped carbon-coated hollow tubular In2O3/CdZnS heterojunction for efficient photocatalytic hydrogen evolution34Dual-Color 2D Lead–Organic Framework with Two-Fold Interlocking Structures for the Detection of Nitrofuran Antibiotics and 2,6-Dichloro-4-nitroaniline49Lanthanide(III)-Modified MIL-125(Ti-Ln) (Ln = Eu or Tb) for the Detection of Cu(II) and Fe(III) Ions14Supramolecular aggregate of pillar[5]arene-based Cu(II) coordination complexes as a highly selective fluorescence sensor for nitroaromatics and metal ions8Upconversion Luminescence through Cooperative and Energy‐Transfer Mechanisms in Yb 3+ ‐Metal‐Organic Frameworks67Upconversion Luminescence through Cooperative and Energy‐Transfer Mechanisms in Yb3+‐Metal‐Organic Frameworks11Fatty acid capped, metal oxo clusters as the smallest conceivable nanocrystal prototypes40A stable ultra-microporous hafnium-based metal–organic framework with high performance for CO 2 adsorption and separation6Enhanced proton conductivity by guest molecule exchange in an acylamide-functionalized metal–organic framework6The Capture Performance of An-Mof for Fission Gases: Insight from Dft and Aimd Calculations0Zr- and Ti-based metal–organic frameworks: synthesis, structures and catalytic applications84Construction of Bimetallic Co/Fe-Incorporated PTA/FDA Nanoclusters for Boosting Electrocatalytic Oxygen Evolution4Metal–organic framework-based electrocatalysts for acidic oxygen evolution reaction40Photo‐Stimuli‐Responsive Dual‐Emitting Luminescence of a Spiropyran‐Encapsulating Metal–Organic Framework for Dynamic Information Encryption195Bioinspired Framework Catalysts: From Enzyme Immobilization to Biomimetic Catalysis490Ortho Effects of Tricarboxylate Linkers in Regulating Topologies of Rare-Earth Metal–Organic Frameworks34Design of an ocu‐Metal‐Organic Framework for a Photocatalysis Reaction18Aluminum metal–organic frameworks: From structures to applications172Synthesis and Optical Properties of Copper Terephthalate Metal Organic Frame Works11Assembling a Heterobimetallic Actinide Metal‐Organic Framework by a Reaction‐Induced Preorganization Strategy21Assembling a Heterobimetallic Actinide Metal‐Organic Framework by a Reaction‐Induced Preorganization Strategy0Excitonic effect in MOFs-mediated photocatalysis: Phenomenon, characterization techniques and regulation strategies67Synthesis, Structure, and Properties of a New Tetranuclear Terbium Hydroxotrifluoroacetate1Acidic Properties of Known and New COOH‐Functionalized M(IV) Metal‐Organic Frameworks11Systematic Study on Zirconium Chelidamates: From a Molecular Complex to a M-HOF and a MOF14Porous La2O2CO3 derived from solvent-guided metal-organic frameworks for high-efficient phosphorus removal24Characterization, Structure, and Reactivity of Hydroxyl Groups on Metal‐Oxide Cluster Nodes of Metal–Organic Frameworks: Structural Diversity and Keys to Reactivity and Catalysis56Dynamically responsive photonic metal–organic frameworks23Metal/covalent-organic frameworks-based electrochemical sensors for the detection of ascorbic acid, dopamine and uric acid193The capture performance of An-MOF for fission gases: Insight from DFT and AIMD calculations6Efficient Exciton Dissociation on Ceria Chelated Cerium‐Based MOF Isogenous S‐Scheme Photocatalyst for Acetaldehyde Purification30A review on synthesis of MOF-derived carbon composites: innovations in electrochemical, environmental and electrocatalytic technologies126Heterometallic MIL-125(Ti–Al) frameworks for electrochemical determination of ascorbic acid, dopamine and uric acid16Local protons enhance photocatalytic CO 2 reduction by porphyrinic zirconium-organic frameworks15Nanoscale Metal-Organic Frameworks for Cancer-Targeted Therapy and Molecular Imaging0Phosphoester bond hydrolysis by a discrete zirconium-oxo cluster: mechanistic insights into the central role of the binuclear Zr IV –Zr IV active site16Stepwise post-synthetic linker installation in rare-earth metal–organic frameworks7Eu 3+ -Doped Anionic Zinc-Based Organic Framework Ratio Fluorescence Sensing Platform: Supersensitive Visual Identification of Prescription Drugs62Non‐Fullerene Acceptors Assisted Target Therapy for Interface Treatment Enable High Performance Inverted Perovskite Solar Cells14Three novel MOFs with various dimensions as efficient Fenton-like photocatalysts for degradation of Rhodamine B7Development of Heterometallic Annular Tetranuclear Clusters in Metal–Organic Frameworks for Methane Purification and Storage6A Multistimuli-Responsive Cd-MOF Constructed by an Extended Viologen-Based Carboxylate Ligand41Constructing Molecular Sieve Channels in Mixed Matrix Membranes for Efficient CO2 Separation12Electron-withdraw groups functionalized MOFs for efficient nitric oxide enrichment and simultaneous removal14Friends or Foes: Fundamental Principles of Th-Organic Scaffold Chemistry Using Zr-Analogs as a Guide22Immobilization of a novel d-allulose 3-epimerase from Bacillus cihuensis within metal-organic frameworks4All‐in‐One: Photo‐Responsive Lanthanide‐Organic Framework for Simultaneous Sensing, Adsorption, and Photocatalytic Reduction of Uranium80Ionic Liquid Modified Fe-Porphyrinic Metal–Organic Frameworks as Efficient and Selective Photocatalysts for CO 2 Reduction25Unraveling the role of coordinated water in the capture of americium and toxic gases by an ultrastable uranyl phosphonate framework12Mining for Metal–Organic Systems: Chemistry Frontiers of Th-, U-, and Zr-Materials18Unveiling the limitless potential: Exploring metal–organic frameworks (MOFs)/MXene based construction materials25High‐Entropy Metal‐Organic Frameworks (HEMOFs): A New Frontier in Materials Design for CO 2 Utilization29The Central Role of Oxo Clusters in Zirconium‐Based Esterification Catalysis12Syntheses, Crystal Structures, and Photothermal Conversion Property of Aluminum Cluster Molecular Rings-Based Heterometallic Complexes3Synthesis, Characterization and in Vitro Drug Delivery Applications of a Tin-Based Metal‒Organic Framework1Modulator engineering of bifunctional metal-organic framework for synergistic catalysis5Hourglass-shaped europium cluster-based secondary building unit in metal–organic framework for photocatalytic wastewater purification and sterilization via enhanced reactive oxygen species production22Reduced-Symmetry Ligand Constructed Y-Based Metal–Organic Framework for Inverse Propane/Propylene Separation20Recent progress in metal-organic frameworks: part I—material preparation59Low-cost, robust, and transportable devices based on Cu( i )–I cluster hybrid luminescent compounds as tetracycline sensors for contaminated waters4Synthesis, characterization and gas sensing characteristics of vanadium-based-MOFs with and without Cu doping1Synthesis, Characterization, and Gas-Sensing Characteristics of Vanadium-Based Mofs with and Without Cu Doping0Recent progress in metal-organic frameworks (Part II—material application)57Multi-Emitting Ratiometric Temperature Sensing and Tunable White Light Emitting Based on Effective Energy Transfer in a Lanthanide-Brønsted Acidic Ionic Liquid Coordination Polymer7Retrieving the Stability and Practical Performance of Activation‐Unstable Mesoporous Zr(IV)‐MOF for Highly Efficient Self‐Calibrating Acidity Sensing47Retrieving the Stability and Practical Performance of Activation‐Unstable Mesoporous Zr(IV)‐MOF for Highly Efficient Self‐Calibrating Acidity Sensing8Enhanced stability and separation resolution of gas chromatographic stationary phases via nano-MIL-103 fabrication4Metal-organic frameworks for low-concentration gases adsorption under ambient conditions: Characterization, modification, processing, shaping and applications35Enzyme‐Photocoupled Catalytic Systems Based on Zirconium‐Metal‐Organic Frameworks5Photocatalytic degradation of crystal violet and malachite green dyes using a 3D Cobalt(Ⅱ) MOF15Cluster Nuclearity Determines Substrate Adsorption/Desorption Dynamics and Peptidase Activity of UiO-66 Nanozymes6Selective-crystallization strategy for the separation of rare earth elements: A minireview29New strategies and advancements in the synthesis of metal organic frameworks for PAHs removal6Zirconium-Based Metal–Organic Frameworks for Photocatalytic CO 2 Reduction32Optimizing Multivariate Metal–Organic Frameworks for Electrochemical Sensing of Dihydroxybenzene Isomers18Cerium Metal–Organic Framework Incorporating Quinoline Sulfonic Acid for Photocatalytic Carbon Dioxide Reduction8Advanced inorganic membranes for water purification: FeZr-MOF/GO composites with optimized adsorption performance7Enhancing Photocatalytic Hydrogen Production Performance of Zr-Tetracarboxylate Frameworks through Topology/Substituent Tunings0Modulator-Induced Secondary Building Unit Control in Lanthanide–Porphyrin Metal–Organic Frameworks for Enhanced Photooxidation4Two novel polynuclear copper complexes: electrochemiluminescence from synthesis to performance exploration1Advancements in acidic OER and HER electrocatalysts: Iridium, MOF-based, and ruthenium systems for sustainable hydrogen production28Lanthanide-Based Metal–Organic Frameworks with Upconversion/Downshifting Emission for Optical Information Encryption8Anisotropic Excitation‐Modulated Multi‐Color Three‐photon Excited Luminescence in Ln‐MOF Heterostructure20Green CO2/CS2 Catalytic Fixation into High-Value Chemicals Promoted by a [Ce2] Cluster-Based Metal–Organic Framework6Multidirectional color palette of electrochromic metal–organic frameworks12Regulating the Growth Orientation of ZIF‐L Membrane for H 2 /CO 2 Separation12Microenvironment Regulation of Multivariate Metal–Organic Frameworks Facilitating the Detection of Common Oral Drugs7Control of CO 2 Electrocatalysis via Modularly Customizable Graphdiyne6High Efficient Liquid‐Phase Breakthrough of Hexane Isomers Via a Robust Heteroporous TiCo‐MOF5Mechanism-driven gas sensing in MOF and COF materials: bridging adsorption thermodynamics, electronic structure, and signal transduction0Multivariate metal–organic frameworks facilitating electrochemical detection of small biomolecules and chloramphenicol0Construction of Versatile Cascade Detection Platforms for Biomolecules Based on a Fluorescent Yttrium Metal–Organic Framework2How to Get Away With Instability: Understanding Degradation Mechanisms in Unstable Metal–Organic Frameworks6Synthesis, Crystal Structure and Intriguing Thermal Behavior of a Hydrated Erbium Pentafluoropropionate0Integrated Photosensitive Fragments and Catalytically Active Sites into Zirconium Metal–Organic Frameworks for CO 2 Photoreduction1Metal–Organic Frameworks for Hydrogen and Methane Storage0Unlocking open metal sites in Zr-MOF/MOG for efficient and rapid Se(IV) adsorption0Isostructural fcu Rare-Earth Metal–Organic Frameworks Based on a Zigzag Dicarboxylate Ligand: One-Step Ethylene Purification from C2 Mixtures and Turn-On Sensing of a Nerve Agent Simulant0

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  30. Which factors govern the adsorption of peptides to Zr( iv )-based metal–organic frameworks?

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  31. Zirconium oxo clusters as discrete molecular catalysts for the direct amide bond formation

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  32. Zr 4+ -terephthalate MOFs with 6-connected structures, highly efficient As( iii / v ) sorption and superhydrophobic properties

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  34. The Chemistry of Zirconium/Carboxylate Clustering Process: Acidic Conditions to Promote Carboxylate-Unsaturated Octahedral Hexamers and Pentanuclear Species

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  37. Customized Synthesis: Solvent- and Acid-Assisted Topology Evolution in Zirconium-Tetracarboxylate Frameworks

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  39. Cage‐Ligand Strategy for the Construction of Zr4(embonate)6–Based MOFs with Third‐Order Nonlinear‐Optical Properties

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  40. Four new coordination polymers constructed by (3-carboxyl-phenyl)-(4-(2’-carboxyl-phenyl)-benzyl) ether and 2,2'-bipyridine

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  41. Highly Porous Materials as Potential Components of Natural Gas Storage Systems: Part 2 (A Review)

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  42. Construction of Co/Fe co-embedded in benzene tricarboxylic acid with modulated coordination environment for accelerated oxygen evolution reaction

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  43. Metal-organic framework-derived nitrogen-doped carbon-coated hollow tubular In2O3/CdZnS heterojunction for efficient photocatalytic hydrogen evolution

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  48. Upconversion Luminescence through Cooperative and Energy‐Transfer Mechanisms in Yb3+‐Metal‐Organic Frameworks

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