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RESEARCH PAPER · Crystal Growth & Design · 2018

Six New Members of the A2MIIMIV3Q8 Family and Their Structural Relationship

Xiao-Ning Hu, Lin Xiong, Li‐Ming Wu

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Six New Members of the A2MIIMIV3Q8 Family and Their Structural RelationshipOriginalK 2 MnGe 3 S 8 : a new multifunctional semiconductor featuring [MnGe 3 S 8 ] 2− layers and demonstrating interesting nonlinear optical response and antiferromagnetic properties33BaM2As2S6 (M = Cd, Hg): Synthesis, crystal structure, optical and electronic properties16K2ZnGe3S8: A Congruent-Melting Infrared Nonlinear-Optical Material with a Large Band Gap41Partial Congener Substitution Induced Centrosymmetric to Noncentrosymmetric Transformation Witnessed by K3Ga3(Ge7–xMx)Se20 (M = Si, Sn) and Their Nonlinear Optical Properties51Rational design of infrared nonlinear optical chalcogenides by chemical substitution287New quaternary chalcogenide Ba 4 HgAs 2 S 10 originating from the combination of linear [HgS 2 ] 2− and tetrahedral [AsS 4 ] 3− modules8AGaSnS4 (A = Rb, Cs): Three sulfides and their structure diversity8Functional Chalcogenide Na2HgSn2Se6 and K2MnGe2Se6 Exhibiting Flexible Chain Structure and Intriguing Birefringence Tunability16Syntheses, structural variants and characterization of A2ZnSn3S8 (A = Cs, Rb) and A2CdSn3S8 (A = Cs, Rb, K, Na) compounds18Intriguing Dimensional Transition Inducing Variable Birefringence in K2Na2Sn3S8 and Rb3NaSn3Se828Applying band gap engineering to tune the linear optical and nonlinear optical properties of noncentrosymmetric chalcogenides La 4 Ge 3 Se x S 12− x ( x = 0, 2, 4, 6, 8, 10)21Centrosymmetric or Noncentrosymmetric? Transition Metals Talking in K 2 TGe 3 S 8 (T = Co, Fe)25Triclinic Layered A2ZnSi3S8 (A = Rb and Cs) with Large Optical Anisotropy and Systematic Research on the Inherent Structure–Performance Relationship in the A2MIIBMIV3Q8 Family11Transition-metal-based chalcogenides: A rich source of infrared nonlinear optical materials184Rb2MGe3S8 (M=Zn, Cd): Non-Centrosymmetry Transformation Led by Structure Change of [MGe3S8]2- Unit※4Rb2FeGe3S8 and Cs2FeGe3S8: New layered chalcogenides in A2MIIMIV3Q8 family with antiferromagnetic property6d6versus d10, Which Is Better for Second Harmonic Generation Susceptibility? A Case Study of K2TGe3Ch8 (T = Fe, Cd; Ch = S, Se)18{[In2S7]8–}∞ Chain and Isolated HgS4 Planar Unit Constructed One-Dimensional Pentanary Sulfide K2Ba7HgIn4S16 Exhibiting Nonlinear-Optical Activity10Recent advances in IR nonlinear optical chalcogenides with well-balanced comprehensive performance57Alkali halide flux synthesis, crystal structure, and photoelectric response of quaternary thiosilicates K 3 Ga 3 Si 7 S 20 and K 2 ZnSi 3 S 81K2HgGe3Se8: A Quaternary Hg-Based Selenide with Nonlinear Optical Properties6Alkali metal/mercury dual-metal sulfides as infrared nonlinear optical materials with high laser-induced damage thresholds5Cationic substitution engineering induces a new quaternary chalcogenide in the A–M IIIA –M IVA –Q system for optical crystal applications1Isovalent cation substitution drives structural transformation and infrared nonlinear optical activity in Eu-based chalcogenides11Rb 2 ZnGe 3 Se 8 : A Large-Birefringence Layered Chalcogenide Enabled by Anisotropic Electrons in Tetrahedral Units0Isothermal sections Tl2Se–CdSe–DIVSe2 (DIV – Si, Ge), quasi-binary systems Tl2DIVSe3–CdSe, Tl2CdGeSe4–GeSe2 and the crystal structure, electronic and optical properties of novel quaternary selenides Tl2CdDIV3Se80

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  1. K 2 MnGe 3 S 8 : a new multifunctional semiconductor featuring [MnGe 3 S 8 ] 2− layers and demonstrating interesting nonlinear optical response and antiferromagnetic properties

    Journal of Materials Chemistry C · 2018-01-01

    Zhuang Li, Xingxing Jiang, Changjiang Yi, Molin Zhou, Yangwu Guo, Xiaoyu Luo, Zheshuai Lin, Yicheng Wu, Youguo Shi, Jiyong Yao

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  2. BaM2As2S6 (M = Cd, Hg): Synthesis, crystal structure, optical and electronic properties

    Journal of Alloys and Compounds · 2018-05-21

    Yangwu Guo, Fei Liang, Molin Zhou, Zheshuai Lin, Jiyong Yao, Yicheng Wu

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  3. K2ZnGe3S8: A Congruent-Melting Infrared Nonlinear-Optical Material with a Large Band Gap

    Inorganic Chemistry · 2018-07-13

    Xiaoyu Luo, Fei Liang, Molin Zhou, Yangwu Guo, Zhuang Li, Zheshuai Lin, Jiyong Yao, Yicheng Wu

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  4. Partial Congener Substitution Induced Centrosymmetric to Noncentrosymmetric Transformation Witnessed by K3Ga3(Ge7–xMx)Se20 (M = Si, Sn) and Their Nonlinear Optical Properties

    Inorganic Chemistry · 2019-09-25

    Xiaohui Li, Nian‐Tzu Suen, Yang Chi, Yueling Sun, Anhua Gong, Huaiguo Xue, Sheng‐Ping Guo

    Read original paper ↗ ·

  5. Rational design of infrared nonlinear optical chalcogenides by chemical substitution

    Coordination Chemistry Reviews · 2019-12-21

    Hua Lin, Wenbo Wei, Hong Chen, Xintao Wu, Qi‐Long Zhu

    Read original paper ↗ ·

  6. New quaternary chalcogenide Ba 4 HgAs 2 S 10 originating from the combination of linear [HgS 2 ] 2− and tetrahedral [AsS 4 ] 3− modules

    Dalton Transactions · 2020-01-01

    Wenhao Xing, Naizheng Wang, Zhuang Li, Wenhao Liu, Jian Tang, Wenlong Yin, Zheshuai Lin, Bin Kang, Jiyong Yao

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  7. AGaSnS4 (A = Rb, Cs): Three sulfides and their structure diversity

    Journal of Solid State Chemistry · 2020-02-04

    Qianqian Liu, Xin Liu, Ling Chen, Li‐Ming Wu

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  8. Functional Chalcogenide Na2HgSn2Se6 and K2MnGe2Se6 Exhibiting Flexible Chain Structure and Intriguing Birefringence Tunability

    Inorganic Chemistry · 2020-05-15

    Zhuang Li, Youquan Liu, Shengzi Zhang, Wenhao Xing, Wenlong Yin, Zheshuai Lin, Jiyong Yao, Yicheng Wu

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  9. Syntheses, structural variants and characterization of A2ZnSn3S8 (A = Cs, Rb) and A2CdSn3S8 (A = Cs, Rb, K, Na) compounds

    Journal of Solid State Chemistry · 2020-08-12

    Ashok Pogu, Kanamaluru Vidyasagar

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  10. Intriguing Dimensional Transition Inducing Variable Birefringence in K2Na2Sn3S8 and Rb3NaSn3Se8

    Inorganic Chemistry · 2020-12-23

    Xiao Ji, Hongping Wu, Bingbing Zhang, Hongwei Yu, Zhanggui Hu, Jiyang Wang, Yicheng Wu

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  11. Applying band gap engineering to tune the linear optical and nonlinear optical properties of noncentrosymmetric chalcogenides La 4 Ge 3 Se x S 12− x ( x = 0, 2, 4, 6, 8, 10)

    Inorganic Chemistry Frontiers · 2021-01-01

    Gary Cicirello, Kui Wu, Bingbing Zhang, Jian Wang

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  12. Centrosymmetric or Noncentrosymmetric? Transition Metals Talking in K 2 TGe 3 S 8 (T = Co, Fe)

    Inorganic Chemistry · 2021-06-29

    Bingheng Ji, Krishna Pandey, Colin P. Harmer, Fei Wang, Kui Wu, Jin Hu, Jian Wang

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  13. Triclinic Layered A2ZnSi3S8 (A = Rb and Cs) with Large Optical Anisotropy and Systematic Research on the Inherent Structure–Performance Relationship in the A2MIIBMIV3Q8 Family

    Inorganic Chemistry · 2021-07-28

    Lihua Gao, Ya Feng Yang, Bingbing Zhang, Xiaowen Wu, Kui Wu

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  14. Transition-metal-based chalcogenides: A rich source of infrared nonlinear optical materials

    Coordination Chemistry Reviews · 2021-08-26

    Hong Chen, Wenbo Wei, Hua Lin, Xintao Wu

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  15. Rb2MGe3S8 (M=Zn, Cd): Non-Centrosymmetry Transformation Led by Structure Change of [MGe3S8]2- Unit※

    化学学报 · 2022-01-01

    Xiandan Chai, Wen‐Fa Chen, Qiu-Nan Yan, Binwen Liu, Xiao‐Ming Jiang, Guo‐Cong Guo

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  16. Rb2FeGe3S8 and Cs2FeGe3S8: New layered chalcogenides in A2MIIMIV3Q8 family with antiferromagnetic property

    Journal of Solid State Chemistry · 2022-06-02

    Weikang Wang, Wangzhu Cao, Ling‐Yun Zhang, Guobao Li, Yuandong Wu, Shaoguo Wen, Dajiang Mei

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  17. d6versus d10, Which Is Better for Second Harmonic Generation Susceptibility? A Case Study of K2TGe3Ch8 (T = Fe, Cd; Ch = S, Se)

    Inorganic Chemistry · 2022-12-27

    Bingheng Ji, Fei Wang, Kui Wu, Bingbing Zhang, Jian Wang

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  18. {[In2S7]8–}∞ Chain and Isolated HgS4 Planar Unit Constructed One-Dimensional Pentanary Sulfide K2Ba7HgIn4S16 Exhibiting Nonlinear-Optical Activity

    Inorganic Chemistry · 2023-05-01

    Xiao Fen Huang, Yexin Chen, Yuan Xue, Ying-Chi Wang, Qing-Hua Ren, Wenlong Liu, Jiajing Wu, Sheng‐Ping Guo

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  19. Recent advances in IR nonlinear optical chalcogenides with well-balanced comprehensive performance

    Materials Today Physics · 2023-05-26

    Hedi Yang, Mao‐Yin Ran, Wenbo Wei, Xin‐Tao Wu, Hua Lin, Qi‐Long Zhu

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  20. Alkali halide flux synthesis, crystal structure, and photoelectric response of quaternary thiosilicates K 3 Ga 3 Si 7 S 20 and K 2 ZnSi 3 S 8

    CrystEngComm · 2024-01-01

    Jia-Ting Liu, Abdusalam Ablez, Qianqian Hu, Jun-Hao Tang, Chuan Lv, Lu Yang, Mei‐Ling Feng, Xiao‐Ying Huang

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  21. K2HgGe3Se8: A Quaternary Hg-Based Selenide with Nonlinear Optical Properties

    Inorganic Chemistry · 2024-08-26

    Guili Wang, Pifu Gong, Jiyong Yao

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  22. Alkali metal/mercury dual-metal sulfides as infrared nonlinear optical materials with high laser-induced damage thresholds

    Dalton Transactions · 2025-01-01

    Guili Wang, Bohui Xu, Chunxiao Li, Pifu Gong, Zheshuai Lin, Jiyong Yao

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  23. Cationic substitution engineering induces a new quaternary chalcogenide in the A–M IIIA –M IVA –Q system for optical crystal applications

    CrystEngComm · 2025-01-01

    Yue Wang, Xuezhong Li, Zihao Lou, Yong‐Fang Shi

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  24. Isovalent cation substitution drives structural transformation and infrared nonlinear optical activity in Eu-based chalcogenides

    Inorganic Chemistry Frontiers · 2025-01-01

    Ping Feng, Shenghua Zhou, Mao‐Yin Ran, Bingxuan Li, Xin-Tao Wu, Hua Lin, Qi‐Long Zhu

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  25. Rb 2 ZnGe 3 Se 8 : A Large-Birefringence Layered Chalcogenide Enabled by Anisotropic Electrons in Tetrahedral Units

    Inorganic Chemistry · 2026-06-15

    Xinchen Chen, Yabo Wu, Wangfei Che, Shuyi Mi, Juanjuan Lu, Chen Cui

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  26. Isothermal sections Tl2Se–CdSe–DIVSe2 (DIV – Si, Ge), quasi-binary systems Tl2DIVSe3–CdSe, Tl2CdGeSe4–GeSe2 and the crystal structure, electronic and optical properties of novel quaternary selenides Tl2CdDIV3Se8

    Journal of Alloys and Compounds · 2026-07-22

    Л.В. Піскач, Andrii Selezen, Lubomir D. Gulay, Yuri Kogut, Dmytro Ivanyuk, Galyna Myronchuk, Stepan V. Syrotyuk, Yu. V. Klysko, Svitlana Bolshanina, Oleksiy Synelnychenko, Oleg Khyzhun

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