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RESEARCH PAPER · Inorganic Chemistry Frontiers · 2021

Applying band gap engineering to tune the linear optical and nonlinear optical properties of noncentrosymmetric chalcogenides La 4 Ge 3 Se x S 12− x ( x = 0, 2, 4, 6, 8, 10)

Gary Cicirello, Kui Wu, Bingbing Zhang, Jian Wang

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Applying band gap engineering to tune the linear optical and nonlinear optical properties of noncentrosymmetric chalcogenides La 4 Ge 3 Se x S 12− x ( x = 0, 2, 4, 6, 8, 10)OriginalA 2 P 2 S 6 (A = Ba and Pb): a good platform to study the polymorph effect and lone pair effect to form an acentric structure28Synthesis, Crystal and Electronic Structures, and Nonlinear Optical Properties of Y4Si3S1212Shedding Light on the Structure and Characterization of K2ZnGe2O6: A Phase-Matchable Nonlinear Optical Crystal19Synthesis, Crystal and Electronic Structures, Nonlinear Optical Properties, and Magnetic Properties of Two Thiophosphates: KInP2S7 and KCrP2S79d6versus d10, Which Is Better for Second Harmonic Generation Susceptibility? A Case Study of K2TGe3Ch8 (T = Fe, Cd; Ch = S, Se)18Revisiting two thiophosphate compounds constituting d 0 transition metal HfP 2 S 6 and d 10 transition metal α-Ag 4 P 2 S 6 as multifunctional materials for combining second harmonic generation response and photocurrent response12Visualizing the alignment of lone pair electrons in La 3 AsS 5 Br 2 and La 5 As 2 S 9 Cl 3 to form an acentric or centrosymmetric structure10Synthesis, crystal and electronic structures, linear and nonlinear optical properties, and photocurrent response of oxyhalides CeHaVIO 4 (Ha = Cl, Br; VI = Mo, W)10Chemical perspectives on heteroanionic compounds: a potential playground for multiferroics7Evaluation and prospect of Mid-Infrared nonlinear optical materials in f0 rare earth (RE = Sc, Y, La) chalcogenides45A Rare Earth Chalcogenide Nonlinear Optical Crystal KLaGeS4: Achieving Good Balance among Band Gap, Second Harmonic Generation Effect, and Birefringence13Synthesis, Crystal and Electronic Structures, and Magnetic and Electrical Transport Properties of Bismuthides NdZn0.6Bi2 and (La0.5RE0.5)Zn0.6Bi2 (RE = Pr or Nd)7Synthesis, Crystal, and Electronic Structures, and Second Harmonic Generation of La4Ge3S121The Influence of Different Group Distortions on the Structure–Property Relationship of Alkali Metal Thiophosphate0Structural Evolution and Optical Tunability of Diamond-Like Semiconductors Li 2 Zn 1– x Cd x SnS 4 , Li 2 CdSn(S 1– y Se y ) 4 , and Li 2 ZnSn(S 1– y Se y ) 44Synthesis, Crystal Growth, Linear, and Nonlinear Optical Properties of Water-Grown Giant Optical Anisotropic Thiocyanates ABi(SCN) 4 (A = Rb, Cs)3Discovery of Noncentrosymmetric Sr 3 As 2 S 7 and Sr 3 As 2 Se 2.5 S 4.5 Featuring As 3+ /As 5+ Coordination and Their Strong Nonlinear Optical Response2Synthesis, Crystal Growth, and Optical and Magnetic Properties of Three Bimetallic Thiocyanates: Na 2 Zn(NCS) 4 ·8H 2 O, K 2 Zn(NCS) 4 ·3H 2 O, and (NH 4 ) 2 Co(NCS) 4 ·3H 2 O4Pr4-m-nTbmErnGe3S12: From structure to properties0Achieving Excellent Nonlinear Optics in α ‑Ba 2 Ge 4 S 10 via Flux‑Induced Symmetry Breaking1Mixed‐Valence Engineering in Ge 2+ Chalcogenides: Structural Modulation for Balanced Infrared Nonlinear Optics0

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  1. A 2 P 2 S 6 (A = Ba and Pb): a good platform to study the polymorph effect and lone pair effect to form an acentric structure

    Dalton Transactions · 2022-01-01

    Bingheng Ji, Arka Sarkar, Kui Wu, Andrew Swindle, Jian Wang

    Read original paper ↗ ·

  2. Synthesis, Crystal and Electronic Structures, and Nonlinear Optical Properties of Y4Si3S12

    Zeitschrift für anorganische und allgemeine Chemie · 2022-03-21

    Stefano Bardelli, Zhengyang Ye, Fei Wang, Bingbing Zhang, Jian Wang

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  3. Shedding Light on the Structure and Characterization of K2ZnGe2O6: A Phase-Matchable Nonlinear Optical Crystal

    Inorganic Chemistry · 2022-07-13

    Jinmiao Jiao, Fei Liang, Conggang Li, Tao Han, Wenli Zhao, Yuheng She, Ning Ye, Zhanggui Hu, Yicheng Wu

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  4. Synthesis, Crystal and Electronic Structures, Nonlinear Optical Properties, and Magnetic Properties of Two Thiophosphates: KInP2S7 and KCrP2S7

    Crystals · 2022-10-22

    Craig Cropek, Vivian Nguyen, Santosh Karki Chhetri, Jin Hu, Sheng‐Ping Guo, Jian Wang

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  5. d6versus d10, Which Is Better for Second Harmonic Generation Susceptibility? A Case Study of K2TGe3Ch8 (T = Fe, Cd; Ch = S, Se)

    Inorganic Chemistry · 2022-12-27

    Bingheng Ji, Fei Wang, Kui Wu, Bingbing Zhang, Jian Wang

    Read original paper ↗ ·

  6. Revisiting two thiophosphate compounds constituting d 0 transition metal HfP 2 S 6 and d 10 transition metal α-Ag 4 P 2 S 6 as multifunctional materials for combining second harmonic generation response and photocurrent response

    CrystEngComm · 2023-01-01

    Craig Cropek, Bingheng Ji, Arka Sarkar, Fei Wang, Tajamul Hussain Syed, Wei Wei, Sheng‐Ping Guo, Jian Wang

    Read original paper ↗ ·

  7. Visualizing the alignment of lone pair electrons in La 3 AsS 5 Br 2 and La 5 As 2 S 9 Cl 3 to form an acentric or centrosymmetric structure

    CrystEngComm · 2023-01-01

    Gary Cicirello, Andrew Swindle, Jian Wang

    Read original paper ↗ ·

  8. Synthesis, crystal and electronic structures, linear and nonlinear optical properties, and photocurrent response of oxyhalides CeHaVIO 4 (Ha = Cl, Br; VI = Mo, W)

    Dalton Transactions · 2023-12-15

    Zixian Jiao, Jasmine Quah, Tajamul Hussain Syed, Wei Wei, Bingbing Zhang, Fei Wang, Jian Wang

    Read original paper ↗ ·

  9. Chemical perspectives on heteroanionic compounds: a potential playground for multiferroics

    Materials Chemistry Frontiers · 2024-01-01

    Karishma Prasad, Vivian Nguyen, Bingheng Ji, Jasmine Quah, Danielle Goodwin, Jian Wang

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  10. Evaluation and prospect of Mid-Infrared nonlinear optical materials in f0 rare earth (RE = Sc, Y, La) chalcogenides

    Coordination Chemistry Reviews · 2024-03-22

    Linfeng Dong, Shengzi Zhang, Pifu Gong, Lei Kang, Zheshuai Lin

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  11. A Rare Earth Chalcogenide Nonlinear Optical Crystal KLaGeS4: Achieving Good Balance among Band Gap, Second Harmonic Generation Effect, and Birefringence

    Inorganic Chemistry · 2024-06-03

    Yang Liu, Xiangming Li, Shuchang Wu, Mengjie Ma, Xiao‐Ming Jiang, Yuandong Wu, Dajiang Mei

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  12. Synthesis, Crystal and Electronic Structures, and Magnetic and Electrical Transport Properties of Bismuthides NdZn0.6Bi2 and (La0.5RE0.5)Zn0.6Bi2 (RE = Pr or Nd)

    Inorganic Chemistry · 2024-09-19

    Karishma Prasad, Dinesh Upreti, Md Rafique Un Nabi, Richeal Oppong, Fei Wang, Manish Shinde, Jin Hu, Jian Wang

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  13. Synthesis, Crystal, and Electronic Structures, and Second Harmonic Generation of La4Ge3S12

    Zeitschrift für anorganische und allgemeine Chemie · 2025-04-07

    Hiroya Ohtsuki, Suguru Nakata, Yu Yamane, Ryunosuke Takahashi, Koichi Kusakabe, Hiroki Wadati

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  14. The Influence of Different Group Distortions on the Structure–Property Relationship of Alkali Metal Thiophosphate

    Crystal Growth & Design · 2025-06-11

    Jiafu Ding, Zhihao He, Yunjie Wang, Xin Su, Yu Chu

    Read original paper ↗ ·

  15. Structural Evolution and Optical Tunability of Diamond-Like Semiconductors Li 2 Zn 1– x Cd x SnS 4 , Li 2 CdSn(S 1– y Se y ) 4 , and Li 2 ZnSn(S 1– y Se y ) 4

    Chemistry of Materials · 2025-10-16

    Pritam Das, Diganta Sarkar, Vidyanshu Mishra, Mengran Sun, Dundappa Mumbaraddi, Mohammed Jomaa, Vladimir K. Michaelis, Jiyong Yao, Arthur Mar

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  16. Synthesis, Crystal Growth, Linear, and Nonlinear Optical Properties of Water-Grown Giant Optical Anisotropic Thiocyanates ABi(SCN) 4 (A = Rb, Cs)

    Crystal Growth & Design · 2025-12-30

    Vivian Nguyen, Chu Chu, Monique Sutherlin, Bingbing Zhang, Jian Wang

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  17. Discovery of Noncentrosymmetric Sr 3 As 2 S 7 and Sr 3 As 2 Se 2.5 S 4.5 Featuring As 3+ /As 5+ Coordination and Their Strong Nonlinear Optical Response

    Chemistry of Materials · 2026-01-27

    Vidyanshu Mishra, Jinseong Kim, Joshua Lim, Manya Rishi, Joon Ik Jang, Abishek K. Iyer

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  18. Synthesis, Crystal Growth, and Optical and Magnetic Properties of Three Bimetallic Thiocyanates: Na 2 Zn(NCS) 4 ·8H 2 O, K 2 Zn(NCS) 4 ·3H 2 O, and (NH 4 ) 2 Co(NCS) 4 ·3H 2 O

    Inorganic Chemistry · 2026-02-26

    David Rich, Dinesh Upreti, Eric A. Gabilondo, P. Shiv Halasyamani, Jin Hu, Fei Wang, Mrittika Sarkar, Jian Wang

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  19. Pr4-m-nTbmErnGe3S12: From structure to properties

    Journal of Alloys and Compounds · 2026-04-24

    N.M. Blashko, О.V. Marchuk, Vasyl Kordan, Roksoliana Bukliv, Vasyl M. Hreb

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  20. Achieving Excellent Nonlinear Optics in α ‑Ba 2 Ge 4 S 10 via Flux‑Induced Symmetry Breaking

    Small · 2026-06-24

    Ying Guo, Guo‐Qiang Wang, Yan Guo, Xiao‐Ming Jiang, B C Liu, Guo‐Cong Guo

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  21. Mixed‐Valence Engineering in Ge 2+ Chalcogenides: Structural Modulation for Balanced Infrared Nonlinear Optics

    Advanced Optical Materials · 2026-09-23

    Chunlan Tang, Aoge Yao, Wenhao Xing, Cihai Hong, Jian Tang, Lei Kang, Jiang Huang, Jieyun Wu, Wenlong Yin, Bin Kang

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