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RESEARCH PAPER · Angewandte Chemie International Edition · 2018

Employing an Unsaturated Th 4+ Site in a Porous Thorium–Organic Framework for Kr/Xe Uptake and Separation

Yanlong Wang, Wei Liu, Zhuanling Bai, Tao Zheng, Mark A. Silver, Yuxiang Li, Yaxing Wang, Xia Wang, Juan Diwu, Zhifang Chai, Shuao Wang

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Employing an Unsaturated Th 4+ Site in a Porous Thorium–Organic Framework for Kr/Xe Uptake and SeparationOriginalHighly efficient Pb( ii ) and Cu( ii ) removal using hollow Fe 3 O 4 @PDA nanoparticles with excellent application capability and reusability93Nanospace within metal–organic frameworks for gas storage and separation121Enhanced removal of uranium(VI) from aqueous solution by a novel LDH@MOF-76 composite8Adsorption of uranium by phosphorylated graphene oxide1Plasma-enhanced amidoxime/magnetic graphene oxide for efficient enrichment of U(VI) investigated by EXAFS and modeling techniques65Highly Porous Covalent Triazine Frameworks for Reversible Iodine Capture and Efficient Removal of Dye88Conformational 2-Fold Interpenetrated Uranyl Supramolecular Isomers Based on (6,3) Sheet Topology: Structure, Luminescence, and Ion Exchange37A stable mixed lanthanide metal–organic framework for highly sensitive thermometry77In situ nitroso formation induced structural diversity of uranyl coordination polymers21Radionuclide sequestration by metal-organic frameworks5Time-controlled synthesis of the 3D coordination polymer U(1,2,3-Hbtc) 2 followed by the formation of molecular poly-oxo cluster {U 14 } containing hemimellitate uranium( iv )14Uranyl Compounds Involving a Weakly Bonded Pseudorotaxane Linker: Combined Effect of pH and Competing Ligands on Uranyl Coordination and Speciation33High Uptake of ReO 4 − and CO 2 Conversion by a Radiation‐Resistant Thorium–Nickle [Th 48 Ni 6 ] Nanocage‐Based Metal–Organic Framework148High Uptake of ReO4− and CO2 Conversion by a Radiation‐Resistant Thorium–Nickle [Th48Ni6] Nanocage‐Based Metal–Organic Framework21Opportunities of Porous Organic Polymers for Radionuclide Sequestration141A Thorium Metal‐Organic Framework with Outstanding Thermal and Chemical Stability50A Uranyl-Organic Framework Featuring Two-Dimensional Graphene-like Layered Topology for Efficient Iodine and Dyes Capture76A Metal–Organic Framework Based Methane Nano‐trap for the Capture of Coal‐Mine Methane289A Metal–Organic Framework Based Methane Nano‐trap for the Capture of Coal‐Mine Methane33Synthesis of novel nanomaterials and their application in efficient removal of radionuclides365A Double-Walled Thorium-Based Metal–Organic Framework as a Promising Dual-Function Absorbent for Efficiently Capturing Iodine and Dyes54Selective extraction of thorium from uranium and rare earth elements using sulfonated covalent organic framework and its membrane derivate175Unexpected structural complexity of thorium coordination polymers and polyoxo cluster built from simple formate ligands34Separation of Xe from Kr with Record Selectivity and Productivity in Anion‐Pillared Ultramicroporous Materials by Inverse Size‐Sieving137Separation of Xe from Kr with Record Selectivity and Productivity in Anion‐Pillared Ultramicroporous Materials by Inverse Size‐Sieving59Noncomplexed Cucurbituril-Mediated Structural Evolution of Layered Uranyl Terephthalate Compounds13Grafting functional groups in metal–organic frameworks for U( vi ) sorption from aqueous solutions47Modulated synthesis and isoreticular expansion of Th-MOFs with record high pore volume and surface area for iodine adsorption128Four luminescent metal-organic chain compounds based on semi-rigid N-donor ligands and 3-hydroxy-2-naphthoic acid for recognition of Fe3+ and Cr2O72− ions11Reticular exploration of uranium-based metal—organic frameworks with hexacarboxylate building units37Thorium–Organic Framework Constructed with a Semirigid Triazine Hexacarboxylic Acid Ligand: Unique Structure with Thorium Oxide Wheel Clusters and Iodine Adsorption Behavior74Ultrastable Thorium Metal–Organic Frameworks for Efficient Iodine Adsorption162Ultrafast Luminescent Light-Up Guest Detection Based on the Lock of the Host Molecular Vibration282Creating uniform pores for xenon/ krypton and acetylene/ethylene separation on a strontium-based metal-organic framework11Efficient elimination of environmental pollutants through sorption-reduction and photocatalytic degradation using nanomaterials196Zinc and Cadmium Complexes of Pyridinemethanol Carboxylates: Metal Carboxylate Zwitterions and Metal–Organic Frameworks11Thhorium Metal–Organic Framework Showing Proton Transformation from [NH2(CH3)2]+ to the Carboxyl Group to Enhance Porosity for Selective Adsorption of D2 over H2 and Ammonia Capture7From Isolated Molecular Complexes to Extended Networks: Synthesis and Characterization of Thorium Furanmono‐ and Dicarboxylates2A robust Th-azole framework for highly efficient purification of C2H4 from a C2H4/C2H2/C2H6 mixture302Ultramicroporous organic materials for selective separation of xenon from krypton15Unprecedented Radiation Resistant Thorium–Binaphthol Metal–Organic Framework86Boosting Selective Adsorption of Xe over Kr by Double-Accessible Open-Metal Site in Metal–Organic Framework: Experimental and Theoretical Research60Tunable Metal–Organic Frameworks Based on 8‐Connected Metal Trimers for High Ethane Uptake28Metal-organic frameworks as a versatile platform for radionuclide management163Boosting the Iodine Adsorption and Radioresistance of Th‐UiO‐66 MOFs via Aromatic Substitution118Variability of Uranyl Carboxylates from Rigid Terophenyldicarboxylic Acid Ligands17Auxiliary Ligand-Dependent Adaptive Regulation of Uranyl Coordination in Mixed-Ligand Uranyl Compounds of Flexible Biphenyltetracarboxylic Acid16Docking of Cu I and Ag I in Metal–Organic Frameworks for Adsorption and Separation of Xenon195Docking of CuI and AgI in Metal–Organic Frameworks for Adsorption and Separation of Xenon15High Adsorption Capacity and Selectivity of SO2 over CO2 in a Metal–Organic Framework42Robust metal–organic framework with multiple traps for trace Xe/Kr separation102Highly effective and selective adsorption of thorium(Ⅳ) from aqueous solution using mesoporous graphite carbon nitride prepared by sol–gel template method108A cationic thorium–organic framework with triple single-crystal-to-single-crystal transformation peculiarities for ultrasensitive anion recognition29A microporous Ce-based MOF with the octahedron cage for highly selective adsorption towards xenon over krypton19Beyond structural motifs: the frontier of actinide-containing metal–organic frameworks65Emergence of a thorium–organic framework as a radiation attenuator for selective X-ray dosimetry20Synthesis of luminescent thorium-based metal–organic frameworks with 1,2,4,5-tetrakis(4-carboxyphenyl)benzene10U=O activation in uranyl-organic framework through solid-liquid reaction: A powerful tool to modulate electronic and magnetic structure4Speciation of Ionic Uranyl-Containing Complexes in in Situ Formed Dicyanonitrosomethanide-Based Ionic Liquids3Enhanced Adsorption and Separation of Xenon over Krypton via an Unsaturated Calcium Center in a Metal–Organic Framework20High‐Silica CHA Zeolite Membrane with Ultra‐High Selectivity and Irradiation Stability for Krypton/Xenon Separation70High‐Silica CHA Zeolite Membrane with Ultra‐High Selectivity and Irradiation Stability for Krypton/Xenon Separation12Interpenetration Control in Thorium Metal–Organic Frameworks: Structural Complexity toward Iodine Adsorption35Relationship Between Structure and Separation Property0Relationship Between Structure and Separation Property0The Structures of Metal–Organic Frameworks1The Structures of Metal–Organic Frameworks1The Structures of Metal–Organic Frameworks3Constructing Well-Defined and Robust Th-MOF-Supported Single-Site Copper for Production and Storage of Ammonia from Electroreduction of Nitrate131Proximity Effect in Uranyl Coordination of the Cucurbit[6]uril-Bipyridinium Pseudorotaxane Ligand for Promoting Host–Guest Synergistic Chelating11An updated status and trends in actinide metal-organic frameworks (An-MOFs): From synthesis to application145Tuning surface inductive electric field in microporous organic polymers for Xe/Kr separation26Rational tuning of thorium-organic frameworks by reticular chemistry for boosting radionuclide sequestration43A robust metal-organic framework showing two distinct pores for effective separation of xenon and krypton12Metal-organic frameworks as superior porous adsorbents for radionuclide sequestration: Current status and perspectives52Actinide Coordination Chemistry on Surfaces: Synthesis, Manipulation, and Properties of Thorium Bis(porphyrinato) Complexes17Stepwise Assembly of a Multicomponent Heterometallic Metal–Organic Framework via Th6-Based Metalloligands15Thorium(IV) adsorption onto multilayered Ti3C2Tx MXene: a batch, X-ray diffraction and EXAFS combined study9Unveiling the Unique Roles of Metal Coordination and Modulator in the Polymorphism Control of Metal‐Organic Frameworks20State-of-the-art progress for the selective crystallization of actinides, synthesis of actinide compounds and their functionalization20A Trivalent Americium Organic Framework with Decent Structural Stability against Self‐Irradiation14Lanthanide–uranyl phosphonates constructed from diethyl ((phenylsulfonyl)methyl)phosphonate4A semiconducting uranium–organic framework based on a tetrathiafulvalene derivative4Enhanced Xe/Kr separation via the pore size confinement effect of a microporous thorium-based metal–organic framework9Recent advances in microporous metal–organic frameworks as promising adsorbents for gas separation83Recent advances in the applications of thorium-based metal–organic frameworks and molecular clusters50Coordination-Adaptive Polydentate Pseudorotaxane Ligand for Capturing Multiple Uranyl Species11Robust and Radiation-Resistant Hofmann-Type Metal–Organic Frameworks for Record Xenon/Krypton Separation168Encapsulation of Polymetallic Oxygen Clusters in a Mesoporous/Microporous Thorium-Based Porphyrin Metal–Organic Framework for Enhanced Photocatalytic CO2 Reduction38Unlocking the limits of diffusion and adsorption of metal-crosslinked reduced graphene oxide membranes for gas separation15Dinuclear Nickel–Oxygen Cluster-Based Metal–Organic Frameworks with Octahedral Cages for Efficient Xe/Kr Separation23Professor Zhifang Chai: Scientific contributions and achievements2Microwave-Assisted Synthesis of Porous Composites MOF–Textile for the Protection against Chemical and Nuclear Hazards76Multi-step Phase Transformation from Metal–Organic Frameworks to Inorganic Compounds for High-Purity Th(IV) Generation5Efficient Xe/Kr Separation Based on a Lanthanide–Organic Framework with One-Dimensional Local Positively Charged Rhomboid Channels45Orbital Trap of Xenon: Driving Force Distinguishing between Xe and Kr Found at a Single Ag(I) Site in MFI Zeolite at Room Temperature11Microporous Metal–Organic Framework with Cage-within-Cage Structures for Xenon/Krypton Separation16Double-Accessible Open Metal Sites in Metal–Organic Frameworks with Suitable Pore Size for Efficient Xe/Kr Separation29Utilization of cationic microporous metal-organic framework for efficient Xe/Kr separation56Constructing dual-functional porphyrin-based thorium metal-organic framework toward photocatalytic uranium(VI) reduction integrated with organic oxidation28Selective krypton uptake through trap confinement, formation of Kr2 dimer, and light response in a photochromic and radiation-resistant thorium-diarylethene-framework16Progress in solid state and coordination chemistry of actinides in China5Extremely Stable Thorium‐MOF Assembly of Tetraphenylethylene Derivative With Tunable AIE Property and Highly Selective Detection of Nitro Aromatic Compounds28Achieving High Photo/Thermocatalytic Product Selectivity and Conversion via Thorium Clusters with Switchable Functional Ligands87Dense packing of xenon in an ultra-microporous metal–organic framework for benchmark xenon capture and separation33Fabrication of a Cd( ii ) metal–organic framework as a dual functional material: efficient iodine capture and selective adsorption of a cationic dye24Porous organic cages for gas separations74Covalent organic frameworks (COF) materials for selective radionuclides removal from water10Advanced porous nanomaterials as superior adsorbents for environmental pollutants removal from aqueous solutions147Boosting Xe/Kr separation by a Mixed-linker strategy in Radiation-Resistant Aluminum-Based Metal − Organic frameworks17A Tetravalent Plutonium Organic Framework Containing [ Pu2O16 ] Dimers as Secondary Building Units: Synthesis, Structure, and Radiation Stability9Unveiling the Structure–Modulator Relationships in Thorium-Based Metal–Organic Framework Crystallization18Uranium(IV) and Thorium(IV) Coordination Polymers Based on Tritopic Carboxylic Acids2Pore environment modulation of metal-organic frameworks enables efficient adsorptive separation of Xe/Kr23Toward Optimal Xenon Adsorption Capacity at Low Pressure on Silver-Exchanged Zeolites4Synthetic Control of Thorium Metal‐Organic Frameworks for Sequencing and Sensing of Radioiodine Species20Integrating Metal Complex Units and Redox Sites into Thorium‐Based Metal–Organic Frameworks for Selective Photocatalytic Oxidation of Sulfides37Selective capture and separation of xenon and krypton using metal organic frameworks: a review13The capture performance of An-MOF for fission gases: Insight from DFT and AIMD calculations63D ultra-micropore organic polymers with fixed group and thieno[3,2-b]thiophene to enhance adsorption and separation of Xe/Kr8Engineering uranyl sites into MOFs for efficient and highly selective photocatalytic CO 2 reduction16Iodine capture of a two-dimensional layered uranyl–organic framework: a combined DFT and AIMD study4Designed assembly of heterometallic cluster organic frameworks based on Th6 cluster14Adsorptive separation of Xe/Kr mixtures by microporous lanthanide metal-organic frameworks with high thermal stability3Metal–Organic Frameworks Possessing Suitable Pores for Xe/Kr Separation19Effective approaches to boost Xe/Kr separation in Metal-Organic Frameworks: A review52Control of Zeolite Local Polarity toward Efficient Xenon/Krypton Separation57Metal-organic frameworks with optimal pore cages for high Xe adsorption and efficient Xe/Kr separation20Significant Enhancement of Xe Adsorption and Xe/Kr Separation of Metal–Organic Framework Induced by Pore Channel Shaping and Pore Polarity Engineering29Mining for Metal–Organic Systems: Chemistry Frontiers of Th-, U-, and Zr-Materials18Constructing Functional Radiation-Resistant Thorium Clusters for Catalytic Redox Reactions31A Microporous Hydrogen‐Bonded Organic Framework with Open Pyrene Sites Isolated by Hydrogen‐Bonded Helical Chains for Efficient Separation of Xenon and Krypton34A Microporous Hydrogen‐Bonded Organic Framework with Open Pyrene Sites Isolated by Hydrogen‐Bonded Helical Chains for Efficient Separation of Xenon and Krypton4Fluoro-functionalized metal organic frameworks with two-fold interpenetration for boosting xenon/krypton separation6Nickel Ion Induced Multistage Assembly of Th13 Cluster4Uranyl Clusters Based on 1,10-Phenanthroline Derivative Ligands: Synthesis, Crystal Structures, and Iodine Capture1Efficient Harvesting of Triplet Excitons via a T 1 ‐Blocked TADF Mechanism in Series MOFs for Optimal X‐ray Detection and Imaging4Efficient Harvesting of Triplet Excitons via a T 1 ‐Blocked TADF Mechanism in Series MOFs for Optimal X‐ray Detection and Imaging11Synergistic confinement and polar recognition in a methyl-engineered ultramicroporous MOF for boosted Xe/Kr separation4Anion‐Shielded Porous Organic Cages for High‐Performance Xenon/Krypton Separation11Effects of Phosphonic Acid Groups and Benzene Ring Content on Crystallization Behavior and Thorium(IV) Adsorption Performance4Boosting Record Xe Uptake for Efficient Xe/Kr Separation under High Humidity in a Cage-Based MOF with Open Metal Sites6A Zn-based MOF with honeycomb topology for highly efficient iodine uptake from vapor and liquid phases: synthesis, crystal structure, topology and dual-phase sorption performance4Framework materials for nuclear waste treatment19The first bimetallic Np( v ) MOF with a Np 4 Cs 2 O 8 structural unit: sorption properties and thermal and radiation stability0Bio-metal-organic framework with Nano-window traps for ultra-selective thorium separation1Engineering Dual‐Active N and O Sites in Covalent Organic Frameworks for Ultrahigh and Selective Thorium Removal0Polydopamine-Derived Ultramicroporous Carbon with a Bimodal Pore Size Distribution for Enhanced Xenon and Radon Adsorption0Machine learning potential-driven molecular dynamics study of fission gas adsorption and diffusion in thorium-based metal-organic frameworks0Metal‐Organic Frameworks for Precise Separation of Radionuclides: Our Journey and Perspective0

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  48. Docking of Cu I and Ag I in Metal–Organic Frameworks for Adsorption and Separation of Xenon

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