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RESEARCH PAPER · Angewandte Chemie International Edition · 2019

High Uptake of ReO 4 − and CO 2 Conversion by a Radiation‐Resistant Thorium–Nickle [Th 48 Ni 6 ] Nanocage‐Based Metal–Organic Framework

Hang Xu, Chun‐Shuai Cao, Han‐Shi Hu, Shibin Wang, Jincheng Liu, Peng Cheng, Nikolas Kaltsoyannis, Jun Li, Bin Zhao

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High Uptake of ReO 4 − and CO 2 Conversion by a Radiation‐Resistant Thorium–Nickle [Th 48 Ni 6 ] Nanocage‐Based Metal–Organic FrameworkOriginalA Zn( ii ) metal–organic framework based on bimetallic paddle wheels as a luminescence indicator for carcinogenic organic pollutants: phthalate esters8Fast and Robust Synthesis of Metalated PCN-222 and Their Catalytic Performance in Cycloaddition Reactions with CO271An Ultrastable Matryoshka [Hf 13 ] Nanocluster as a Luminescent Sensor for Concentrated Alkali and Acid51An Ultrastable Matryoshka [Hf13] Nanocluster as a Luminescent Sensor for Concentrated Alkali and Acid9Water-Tolerant DUT-Series Metal–Organic Frameworks: A Theoretical–Experimental Study for the Chemical Fixation of CO2 and Catalytic Transfer Hydrogenation of Ethyl Levulinate to γ-Valerolactone66A novel water-stable MOF Zn(Py)(Atz) as heterogeneous catalyst for chemical conversion of CO2 with various epoxides under mild conditions95Unexpected structural complexity of thorium coordination polymers and polyoxo cluster built from simple formate ligands34Temperature/Solvent-Induced Two Magnetic Nickel Coordination Compounds with 5-Aminodiacetic Isophthalate0Novel cage-like MOF for gas separation, CO 2 conversion and selective adsorption of an organic dye131Cationic Cd(II) metal − organic framework based on tetrakis(1,2,4-triazol-1-yl)methane2A mixed-ligand strategy regulates thorium-based MOFs55A first new porous d–p HMOF material with multiple active sites for excellent CO 2 capture and catalysis132Highly efficient synergistic CO 2 conversion with epoxide using copper polyhedron-based MOFs with Lewis acid and base sites64Highly stable 3D porous HMOF with enhanced catalysis and fine color regulation by the combination of d- and p-ions when compared with those of its monometallic MOFs70Metal–organic frameworks for the energy-related conversion of CO 2 into cyclic carbonates86MOFs-Based Catalysts Supported Chemical Conversion of CO254Rational Stepwise Construction of Different Heterometallic–Organic Frameworks (HMOFs) for Highly Efficient CO2 Conversion25Fine-Tuning the Porosities of the Entangled Isostructural Zn(II)-Based Metal–Organic Frameworks with Active Sites by Introducing Different N-Auxiliary Ligands: Selective Gas Sorption and Efficient CO2 Conversion24Ultrastable Thorium Metal–Organic Frameworks for Efficient Iodine Adsorption162Cationic Metal–Organic Frameworks Based on Linear Zwitterionic Ligands for Cr2O72– and Ammonia Sensing58Highly Efficient Separation of Anionic Organic Pollutants from Water via Construction of Functional Cationic Metal–Organic Frameworks and Mechanistic Study17Metal–Organic Framework-Based Catalysts with Single Metal Sites1233Potassium organoaluminate: Synthesis, structure, and catalytic activity for the conversion of CO2 into cyclic carbonates6A stable Co(II)-based metal-organic framework with dual-functional pyrazolate-carboxylate ligand: Construction and CO2 selective adsorption and fixation38Cluster/cage-based coordination polymers with tetrazole derivatives66Anion-exchanged and quaternary ammonium functionalized MIL-101-Cr metal-organic framework (MOF) for ReO4−/TcO4− sequestration from groundwater39Metal–Organic Frameworks Based on Group 3 and 4 Metals140Constructing a 3D porous Co(II)-organic framework: Synthesis, characterization and chemical transformation of epoxide and CO2 into cyclic carbonate15Metal-organic frameworks as a versatile platform for radionuclide management163Boosting the Iodine Adsorption and Radioresistance of Th‐UiO‐66 MOFs via Aromatic Substitution11899TcO4− removal from legacy defense nuclear waste by an alkaline-stable 2D cationic metal organic framework223Construction of Hybrid Bimetallic Uranyl Compounds Based on a Preassembled Terpyridine Metalloligand22Potassium Ions Induced Framework Interpenetration for Enhancing the Stability of Uranium-Based Porphyrin MOF with Visible-Light-Driven Photocatalytic Activity68A cationic thorium–organic framework with triple single-crystal-to-single-crystal transformation peculiarities for ultrasensitive anion recognition29A copper( ii )-based porous metal–organic framework for the efficient and rapid capture of toxic oxo-anion pollutants from water19A new multi-functional Cu( ii )-organic framework as a platform for selective carbon dioxide chemical fixation and separation of organic dyes9Beyond structural motifs: the frontier of actinide-containing metal–organic frameworks65Charge separation in hybrid metal–organic framework films for enhanced catalytic CO 2 conversion32Emergence of a thorium–organic framework as a radiation attenuator for selective X-ray dosimetry20Multifunctional properties of {CuII2LnIII2} systems involving nitrogen-rich nitronyl nitroxide: single-molecule magnet behavior, luminescence, magnetocaloric effects and heat capacity85Solvent-controlled metal coordination polymers of Co( ii ) with different topological structures and properties4Three Mn( ii ) metal–organic frameworks with the same chemical composition, but different topological structures and properties5Anion binding in metal-organic frameworks51Highly Selective Separation Intermediate‐Size Anionic Pollutants from Smaller and Larger Analogs via Thermodynamically and Kinetically Cooperative‐Controlled Crystallization5Interpenetration Control in Thorium Metal–Organic Frameworks: Structural Complexity toward Iodine Adsorption35Microporous Cd(II) Metal–Organic Framework for CO 2 Catalysis, Luminescent Sensing, and Absorption of Methyl Green38Metal-organic frameworks as functional materials for implantable flexible biochemical sensors41Ultrastable Zirconium-Based Cationic Metal–Organic Frameworks for Perrhenate Removal from Wastewater34Effective and selective adsorption of uranyl ions by porous polyethylenimine-functionalized carboxylated chitosan/oxidized activated charcoal composite19A Porous Copper–Organic Framework Assembled by [Cu 12 ] Nanocages: Highly Efficient CO 2 Capture and Chemical Fixation and Theoretical DFT Calculations70Constructing Well-Defined and Robust Th-MOF-Supported Single-Site Copper for Production and Storage of Ammonia from Electroreduction of Nitrate131An Azobenzene-Modified Photoresponsive Thorium–Organic Framework: Monitoring and Quantitative Analysis of Reversible trans–cis Photoisomerization30A multi-responsive luminescent indicator based on a Zn(II) metal-organic framework with “Turn on” sensing of pyridine and “Turn off” sensing of Fe3+, Cr2O72− and antibiotics in aqueous media24Eco-friendly co-catalyst-free cycloaddition of CO2 and aziridines activated by a porous MOF catalyst48An updated status and trends in actinide metal-organic frameworks (An-MOFs): From synthesis to application145Rational tuning of thorium-organic frameworks by reticular chemistry for boosting radionuclide sequestration43Non-Noble-Metal Metal–Organic-Framework-Catalyzed Carboxylative Cyclization of Propargylic Amines with Atmospheric Carbon Dioxide under Ambient Conditions59A Facile Strategy for Constructing a Carbon‐Particle‐Modified Metal–Organic Framework for Enhancing the Efficiency of CO2 Electroreduction into Formate119A Facile Strategy for Constructing a Carbon‐Particle‐Modified Metal–Organic Framework for Enhancing the Efficiency of CO2 Electroreduction into Formate21Highly efficient metal/solvent-free chemical fixation of CO2 at atmospheric pressure conditions using functionalized porous covalent organic frameworks63Stepwise Assembly of a Multicomponent Heterometallic Metal–Organic Framework via Th6-Based Metalloligands15Cooperation between microporous frameworks and micron-sized channel in crystals for excellent chromate removal7Efficient Cycloaddition of CO2 and Aziridines Activated by a Quadruple-Interpenetrated Indium–Organic Framework as a Recyclable Catalyst59Reticular frameworks and their derived materials for CO2 conversion by thermo−catalysis87Constructing Cationic Metal–Organic Framework Materials Based on Pyrimidyl as a Functional Group for Perrhenate/Pertechnetate Sorption44MOF-Based Chemical Fixation of Carbon Dioxide into Value-Added Fine Chemicals2Water-stable metal–organic framework–based nanomaterials for removal of heavy metal ions and radionuclides4Radiation-Induced Solid-State Transformations of Uranyl Peroxides16A semiconducting uranium–organic framework based on a tetrathiafulvalene derivative4Highly effective CS 2 conversion with aziridines catalyzed by novel [Dy 24 ] nano-cages in MOFs under mild conditions27Progress in anion receptor chemistry154Recent advances in the applications of thorium-based metal–organic frameworks and molecular clusters50Selective perrhenate/pertechnetate removal by a MOF-based molecular trap18Stepwise assembly and reversible structural transformation of ligated titanium coated bismuth-oxo cores: shell morphology engineering for enhanced chemical fixation of CO 224Synthesis, structure and highly selective C 3 H 8 /CH 4 and C 2 H 6 /CH 4 adsorption of a (4,8)-c ternary flu -metal–organic framework based upon both [Sc 4 O 2 (COO) 8 ] and [Cu 4 OCl 6 ] clusters16A New Concept of Radiation Detection Based on a Fluorochromic and Piezochromic Nanocluster70Efficient organic iodide capture by a mesoporous bimetallic-organic framework35A novel 2D zinc(II)-organic framework for efficient catalytic cycloaddition of CO2 with epoxides18Potential Applications of Nickel‐Based Metal‐Organic Frameworks and their Derivatives83Leveraging Nitrogen Linkages in the Formation of a Porous Thorium–Organic Nanotube Suitable for Iodine Capture24Effects of High Gamma Doses on the Structural Stability of Metal–Organic Frameworks54Th-MOF showing six-fold imide-sealed pockets for middle-size-separation of propane from natural gas34Progress in solid state and coordination chemistry of actinides in China5Synthesis of TBAB‐based Deep Eutectic Solvents as the Catalyst in the Coupling Reaction between CO 2 and Epoxides under Ambient Temperature11Achieving High Photo/Thermocatalytic Product Selectivity and Conversion via Thorium Clusters with Switchable Functional Ligands87A Pentanuclear Cu(II)-based 2D Bilayer Coordination Polymer for CO2 Fixation Under Mild Conditions4Slow magnetic relaxation and selective luminescent probe in a 2p–3d–4f heterotrispin chain25Four unprecedented V14 clusters as highly efficient heterogeneous catalyst for CO2 fixation with epoxides and oxidation of sulfides26Selective Sequestration of Perrhenate by Cationic Polymeric Networks Based on Elongated Pyridyl Ligands28Tailored Persistent Radical‐containing Heterotrimetal‐Organic Framework for Boosting Efficiency of Visible/NIR Light‐driven Photocatalytic CO 2 Reduction47Highly Efficient Conversion of Aziridines and CO2 Catalyzed by Microporous [Cu12] Nanocages27Rare earth-based MOFs for photo/electrocatalysis146Two novel Ln 8 clusters bridged by CO 3 2− effectively convert CO 2 into oxazolidinones and cyclic carbonates26Selective Crystallization of a Highly Radiation-Resistant Isonicotinic Acid-Based Metal–Organic Framework as a Primary Actinide Waste Form23Expanding the Structural Topologies of Rare-Earth Porphyrinic Metal–Organic Frameworks through Ligand Modulation11Advanced porous adsorbents for radionuclides elimination207A multifunctional Eu2-cluster coordination polymer as a luminescent probe of imidacloprid and renewable catalyst for the fixation of CO2 with epoxides9Structural flexibility in cationic metal–organic framework for boosting ReO4− capture6Assembling a Heterobimetallic Actinide Metal‐Organic Framework by a Reaction‐Induced Preorganization Strategy21Assembling a Heterobimetallic Actinide Metal‐Organic Framework by a Reaction‐Induced Preorganization Strategy0Removal of radionuclide 99Tc from aqueous solution by various adsorbents: A review53Synthetic Control of Thorium Metal‐Organic Frameworks for Sequencing and Sensing of Radioiodine Species20Single Atom Environmental Catalysis: Influence of Supports and Coordination Environments117Integrating Metal Complex Units and Redox Sites into Thorium‐Based Metal–Organic Frameworks for Selective Photocatalytic Oxidation of Sulfides37A comprehensive overview of the catalytic pathway for CO2 utilization with epoxide to cyclic carbonate99A bis-aromatic MOF system constructed with a copper iodine cluster and porphyrinic ligand for enhancing near-infrared photothermal conversion5Building robust metal-organic frameworks with premade ligands53Effective Reduction of CO 2 with Aromatic Amines into N‐Formamides Triggered by Noble‐Free Metal–Organic Framework Catalysts Under Mild Conditions17Designed assembly of heterometallic cluster organic frameworks based on Th6 cluster14Recent progress in separation of technetium-99 from spent nuclear fuel and radioactive waste. Challenges and prospects55Highly Stable 72-Nuclearity Nanocages for Efficient Synthesis of Aryl Nitriles via Ni/Cu Synergistic Catalysis19The self-assembly of tetranuclear [Gd4] cluster: Magnetic refrigeration and efficient CO2 chemical fixation2Friends or Foes: Fundamental Principles of Th-Organic Scaffold Chemistry Using Zr-Analogs as a Guide22A four-fold interpenetrated MOF for efficient perrhenate/pertechnetate removal from alkaline nuclear effluents14Metal Hydrogen-Bonded Organic Frameworks as Open Lewis Acid Catalysts for Two Types of CO2 Transformations28Conversion of Propargylic Amines with CO2 Catalyzed by a Highly Stable Copper(I) Iodide Thorium-Based Heterometal–Organic Framework31Thorium Cluster Synthesized by a Solvent-Free Flux Approach: The Richest Coordination Diversity and Application Exploration5A Robust Zn-Hydroxamate Metal–Organic Framework Constructed from an Unsymmetrical Ligand for Iodine Capture6A novel Eu8 cluster for efficiently catalyzing CO2 cycloaddition and Knoevenagel condensation5Recent progress of radionuclides separation by porous materials265Metal-organic framework-based fibers for next-generation wearable applications17A [Zn 3 ]-cluster-based MOF catalyst for highly efficient and recyclable CO 2 conversion into cyclic carbonates2Adsorption of nuclides (Cs, Sr, Co, U, and Tc) by various adsorbents0Correlation between coordination environments and sorption selectivity to 99 TcO 4 − in two-dimensional metal–organic frameworks2Linear trinuclear and tetranuclear Ln( iii ) compounds aggregated by multidentate Schiff base ligands: insights into the magnetocaloric effect, slow magnetic relaxation behavior and catalytic CO 2 conversion3Two novel tetranuclear Yb( iii )-based compounds for highly efficient conversion of CO 2 to cyclic carbonates2Recent progress in metal-organic frameworks (Part II—material application)57Chemistry of uranium and thorium complexes towards challenging transformation: A recent trends1Crystallographic Evidence for Formation of M 6 O 8 /M 6 O 9 f-Element Clusters in Hydrolysis Reactions6Nickel Ion Induced Multistage Assembly of Th13 Cluster4Modulating metal nodes in metal hydrogen-bonded organic frameworks for catalytic CO2 fixation to synthesize high-value-added oxazolidinones3Uranyl Clusters Based on 1,10-Phenanthroline Derivative Ligands: Synthesis, Crystal Structures, and Iodine Capture1CO2 Chemical Fixation into Value-Added Heterocycles Catalyzed by Non-Noble-Metal Metal-Organic Frameworks37Enhanced Photocatalytic Activity in Thorium-Based Metal–Organic Frameworks (MOFs) via Solvent Induced π–π Stacking of Photoactive Ligands4Metal-organic frameworks for clean water21Framework materials for nuclear waste treatment19Three-Component CO 2 Conversion to Carbonyl Carboxylates Catalyzed by a Copper-Based Metal–Organic Framework under Mild Conditions4Highly Efficient Multicomponent CO 2 Conversion Facilitated by Synergistic Catalysis from N‐Heterocyclic Carbene and Copper in Metal–Organic Framework under Mild Conditions1Regulating the topology and pore size of covalent metal-organic frameworks for boosting catalytic CO2 conversion6Application of computational tools for experimental data analysis of homogeneous catalytic systems in the synthesis of cyclic carbonates1Atomically precise ferrocene-based Fe/Mn nanocluster for solar-driven cycloaddition of epoxides with carbon dioxide2Self-assembled novel Ln6 clusters showing efficient cycloaddition of CO2 into cyclic carbonates and magnetic behaviors2Construction of an Amino-Functionalized Thorium MOF for Bifunctional Catalysis toward CO2 Cycloaddition and N-Formylation0Functionalized metal organic frameworks for thorium (IV) adsorption: Mechanisms, speciation, and practical challenges0Controlled Synthesis of High‐Nuclearity Th 38 Cluster for Efficient Photocatalytic Dehydrogenative Cross‐Coupling0The tautomerism induced by the number of hydroxyl groups in COFs and its contribution to thorium adsorption0A novel linear-shaped octanuclear Ni(II)-based cluster formed by one-pot condensation and coordination self-assembly: crystal structure and highly efficient conversion of CO2 into cyclic carbonates0

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  5. Water-Tolerant DUT-Series Metal–Organic Frameworks: A Theoretical–Experimental Study for the Chemical Fixation of CO2 and Catalytic Transfer Hydrogenation of Ethyl Levulinate to γ-Valerolactone

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  6. A novel water-stable MOF Zn(Py)(Atz) as heterogeneous catalyst for chemical conversion of CO2 with various epoxides under mild conditions

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  31. 99TcO4− removal from legacy defense nuclear waste by an alkaline-stable 2D cationic metal organic framework

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  32. Construction of Hybrid Bimetallic Uranyl Compounds Based on a Preassembled Terpyridine Metalloligand

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  33. Potassium Ions Induced Framework Interpenetration for Enhancing the Stability of Uranium-Based Porphyrin MOF with Visible-Light-Driven Photocatalytic Activity

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  34. A cationic thorium–organic framework with triple single-crystal-to-single-crystal transformation peculiarities for ultrasensitive anion recognition

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  35. A copper( ii )-based porous metal–organic framework for the efficient and rapid capture of toxic oxo-anion pollutants from water

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  36. A new multi-functional Cu( ii )-organic framework as a platform for selective carbon dioxide chemical fixation and separation of organic dyes

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  37. Beyond structural motifs: the frontier of actinide-containing metal–organic frameworks

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  38. Charge separation in hybrid metal–organic framework films for enhanced catalytic CO 2 conversion

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  39. Emergence of a thorium–organic framework as a radiation attenuator for selective X-ray dosimetry

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  40. Multifunctional properties of {CuII2LnIII2} systems involving nitrogen-rich nitronyl nitroxide: single-molecule magnet behavior, luminescence, magnetocaloric effects and heat capacity

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  42. Three Mn( ii ) metal–organic frameworks with the same chemical composition, but different topological structures and properties

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