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RESEARCH PAPER · Chemistry of Materials · 2016

Crystalline Mixed Halide Halobismuthates and Their Induced Second Harmonic Generation

Xiaoxin Zheng, Yang Liu, Guangfeng Liu, Jie Liu, Xin Ye, Quanxiang Han, Chao Ge, Xutang Tao

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Crystalline Mixed Halide Halobismuthates and Their Induced Second Harmonic GenerationOriginalChemical engineering of mixed halide hexaborates as nonlinear optical materials5An alkaline tin(II) halide compound Na 3 Sn 2 F 6 Cl: Synthesis, structure, and characterization10Structure and Characterization of a Zero-Dimensional Alkali Tin Dihalides Compound Cs3Sn3F2Cl7 with the [Sn2F2Cl4]2– Clusters13Structural Evolution in BaSn2F5X (X = Cl, Br, I): A Family of Alkaline Earth Metal Tin Mixed Halides15Nonlinear Optical Crystal Rb 4 Sn 3 Cl 2 Br 8 : Synthesis, Structure, and Characterization32Above-room-temperature switching of quadratic nonlinear optical properties in a Bi–halide organic–inorganic hybrid44A novel bismuth-based hybrid material with highly activity for fast removal of rhodamine B under dark conditions27Photonics and Optoelectronics of 2D Metal‐Halide Perovskites228Recent advances of low-dimensional materials in lasing applications16Exploring Anisotropy on Oriented Wafers of MAPbBr3 Crystals Grown by Controlled Antisolvent Diffusion100Recent advances and future perspectives on infrared nonlinear optical metal halides223Successive near-room-temperature dielectric phase transitions in a lead-free hybrid perovskite-like compound17[(( R )-C8H12N)4][Bi2Br10] and [(( S )-C8H12N)4][Bi2Br10]: Chiral Hybrid Bismuth Bromides Templated by Chiral Organic Cations74Structural phase transition and dielectric anisotropy properties of a lead-free organic–inorganic hybrid20Halide Perovskites for Nonlinear Optics355Synthesis and crystal structure of copper(I) halide complexes with 1-allyl-4-cyanopyridinium cation0Growth Regulation of Pentacene-Doped p-Terphenyl Crystals on Their Physical Properties for Promising Maser Gain Medium28A Series of Organic–Inorganic Hybrid Compounds [(C2H5)4N]InCl4–xBrx (x = 0, 2, 4): Synthesis, Crystal Structure, and Nonlinear Optical Properties37Incorporation of nitrate ions into halobismuthates1Structural Evolution and Optical Property Tunability by Halogen Substitution in [N(CH3)4]MX2 (M = Ga+, In+, X = Cl, Br): A Family of Organically Templated Metal Halides8Fluorine Substitution in Ethylamine Triggers Second Harmonic Generation in Noncentrosymmetric Crystalline [NH3CH2CH2F]3BiCl632Syntheses, structure and properties of a new series of organic–inorganic Hg-based halides: adjusting halogens resulted in huge performance mutations15Synthesis and first-principles study of structural, electronic and optical properties of tetragonal hybrid halobismuthathes [Py 2 (XK)] 2 [Bi 2 Br 10− x I x ]7Shedding light on the nature of the catalytically active species in photocatalytic reactions using Bi2O3 semiconductor92Using a Porphyrin Diacid Cation to Stabilize a Square-Pyramidal BiX5 (X = Br, Cl/Br) Unit4Acentric Organic–Inorganic Hybrid Halide [N(CH3)4]2HgBr2I2 Featuring an Isolated [HgBr2I2]2– Tetrahedron and Second-Order Nonlinearity18Formation of a Stable Guanidinium–Formamidinium Phase in Bismuth Chloride Perovskites with Broadband Emission28Lead-free halide perovskites, beyond solar cells and LEDs28Tunable phase transition, band gap and SHG properties by halogen replacement of hybrid perovskites [(thiomorpholinium)PbX3, X = Cl, Br, I]75Broad Photoluminescence and Second-Harmonic Generation in the Noncentrosymmetric Organic–Inorganic Hybrid Halide (C6H5(CH2)4NH3)4MX7·H2O (M = Bi, In, X = Br or I)830D chiral hybrid indium( iii ) halides for second harmonic generation27K6Sn4F12I2•0.5H2O: a zero-dimensional alkali metal tin mixed halide compound exhibiting color change due to crystal water loss0Thermally-driven unusual dual SHG switching with wide SHG-active steps triggered by inverse symmetry breaking45Cooperative Enhancement of Second Harmonic Generation in an Organic–Inorganic Hybrid Antimony Halide63Organic Cation Modulation Triggered Second Harmonic Response in Manganese Halides with Bright Fluorescence46Remarkable Infrared Nonlinear Optical, Dielectric, and Strong Diamagnetic Characteristics of Semiconducting K3[BiS3]5Scintillation properties of ((CH3)4N)3BiCl6 as a novel lead-free perovskite halide crystal6Achieving Large Second Harmonic Generation Effects via Optimal Planar Alignment of Triangular Units64Second harmonic generation from symmetry breaking stimulated by mixed organic cations in zero-dimensional hybrid metal halides7Unusual isostructural Br/I substitution effect on the crystal structure and optical properties of hybrid halobismuthates3Uncovering the Role of Electronic Doping in Lead‐free Perovskite (CH3NH3)2CuCl4‐xBrx and Solar Cells Fabrication15A review of the relationship between the structure and nonlinear optical properties of organic-inorganic hybrid materials150Experimental analysis of methylammonium and Formamidinium-based halide perovskite properties for optoelectronic applications4Photoluminescence and Nonlinear Optical Properties of Two Terpyridine-Based Hybrid Zn/Cd Halides25Improved growth technique for high-quality trans-stilbene single crystals achieving a record PSD performance11Nonlinear Optical Effects of Hybrid Antimony(III) Halides Induced by Stereoactive 5s 2 Lone Pairs and Trimethylammonium Cations23Designing Zero-Dimensional Cadmium-Based Organic–Inorganic Hybrids: The Role of Halogen Doping in Modulating Multifunctional Properties9Polar Thiazole Derivative-Induced Second Harmonic Response in Hybrid Bismuth Chlorate with Reversible Photochromism9Layered and Low-Dimensional Lead, Silver, and Bismuth Halide Perovskites Directed by Halogen-Substituted Spacer Cations12Antimony vs. bismuth: structural differences in Cat{[MCl 5 ](I 2 )} halogen bond-linked supramolecular complexes5Three antimony-based organic–inorganic hybrid perovskites (1,4-3.2.2-H 2 dabcn)SbX 5 (X = Cl, Br, I) show progressively decreasing phase transition temperatures and bandgaps7Designing Polar Covalent Hybrid Cadmium‐Based Chalcohalides Ultraviolet Nonlinear Optical Crystal with Strong Optical Anisotropy via Double‐Site Dual FBUs Tailoring25Impact of Halide Substitution in the Inorganic Framework on the Optical Activity of Chiral Metal-Halide Perovskites4Crystal structure and optical properties of a new 0D organic-inorganic compound, (3-picolylammonium)2[Bi2Cl10]·2H2O: Experimental and theoretical insights4Alloying Small‐Cation into Low‐Dimensional Perovskite Motif Gives Multiaxial Ferroelectrics with Enhanced Photo‐Pyroelectricity3A universal synthetic strategy for noncentrosymmetric lead oxyhalide frameworks with strong second-harmonic generation0Nonlinear optical-dielectric dual switching and narrow band gap in a one-dimensional hybrid compound: [(CH 3 ) 2 S(CH 2 ) 3 NH 3 ][SbBr 5 ]0Atom-Response-Theory-Guided Design of Chiral Niobium Halides with both a Large Nonlinear Coefficient and Strong Chiroptical Nonlinearity3Dual‐Functional Ultraviolet Nonlinear Optics and Bright Luminescence Achieved in the First Fluorine‐Containing Hybrid Lone‐Pair Metal Mixed Halides8Chiral Trigonal Pyramidal Germanium Halides for Enhanced Second Harmonic Generation0Chiral Trigonal Pyramidal Germanium Halides for Enhanced Second Harmonic Generation0Tuning Chiroptical Properties of Two-Dimensional Hybrid Perovskites through Organic Spacer and Halide Composition0

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  1. Chemical engineering of mixed halide hexaborates as nonlinear optical materials

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  2. An alkaline tin(II) halide compound Na 3 Sn 2 F 6 Cl: Synthesis, structure, and characterization

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  3. Structure and Characterization of a Zero-Dimensional Alkali Tin Dihalides Compound Cs3Sn3F2Cl7 with the [Sn2F2Cl4]2– Clusters

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  4. Structural Evolution in BaSn2F5X (X = Cl, Br, I): A Family of Alkaline Earth Metal Tin Mixed Halides

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  5. Nonlinear Optical Crystal Rb 4 Sn 3 Cl 2 Br 8 : Synthesis, Structure, and Characterization

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  6. Above-room-temperature switching of quadratic nonlinear optical properties in a Bi–halide organic–inorganic hybrid

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  7. A novel bismuth-based hybrid material with highly activity for fast removal of rhodamine B under dark conditions

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  8. Photonics and Optoelectronics of 2D Metal‐Halide Perovskites

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  9. Recent advances of low-dimensional materials in lasing applications

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  10. Exploring Anisotropy on Oriented Wafers of MAPbBr3 Crystals Grown by Controlled Antisolvent Diffusion

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  11. Recent advances and future perspectives on infrared nonlinear optical metal halides

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  12. Successive near-room-temperature dielectric phase transitions in a lead-free hybrid perovskite-like compound

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  13. [(( R )-C8H12N)4][Bi2Br10] and [(( S )-C8H12N)4][Bi2Br10]: Chiral Hybrid Bismuth Bromides Templated by Chiral Organic Cations

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  14. Structural phase transition and dielectric anisotropy properties of a lead-free organic–inorganic hybrid

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  15. Halide Perovskites for Nonlinear Optics

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  16. Synthesis and crystal structure of copper(I) halide complexes with 1-allyl-4-cyanopyridinium cation

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  17. Growth Regulation of Pentacene-Doped p-Terphenyl Crystals on Their Physical Properties for Promising Maser Gain Medium

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  18. A Series of Organic–Inorganic Hybrid Compounds [(C2H5)4N]InCl4–xBrx (x = 0, 2, 4): Synthesis, Crystal Structure, and Nonlinear Optical Properties

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  19. Incorporation of nitrate ions into halobismuthates

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  20. Structural Evolution and Optical Property Tunability by Halogen Substitution in [N(CH3)4]MX2 (M = Ga+, In+, X = Cl, Br): A Family of Organically Templated Metal Halides

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  21. Fluorine Substitution in Ethylamine Triggers Second Harmonic Generation in Noncentrosymmetric Crystalline [NH3CH2CH2F]3BiCl6

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  22. Syntheses, structure and properties of a new series of organic–inorganic Hg-based halides: adjusting halogens resulted in huge performance mutations

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  23. Synthesis and first-principles study of structural, electronic and optical properties of tetragonal hybrid halobismuthathes [Py 2 (XK)] 2 [Bi 2 Br 10− x I x ]

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  30. Broad Photoluminescence and Second-Harmonic Generation in the Noncentrosymmetric Organic–Inorganic Hybrid Halide (C6H5(CH2)4NH3)4MX7·H2O (M = Bi, In, X = Br or I)

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  32. K6Sn4F12I2•0.5H2O: a zero-dimensional alkali metal tin mixed halide compound exhibiting color change due to crystal water loss

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  34. Cooperative Enhancement of Second Harmonic Generation in an Organic–Inorganic Hybrid Antimony Halide

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  37. Scintillation properties of ((CH3)4N)3BiCl6 as a novel lead-free perovskite halide crystal

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  38. Achieving Large Second Harmonic Generation Effects via Optimal Planar Alignment of Triangular Units

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  40. Unusual isostructural Br/I substitution effect on the crystal structure and optical properties of hybrid halobismuthates

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