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RESEARCH PAPER · Advanced Functional Materials · 2022

Achieving Large Second Harmonic Generation Effects via Optimal Planar Alignment of Triangular Units

Xinyu Li, Qi Wei, Chun‐Li Hu, Jie Pan, Bingxuan Li, Zhen‐Zhen Xue, Xiao‐Yu Li, Jinhua Li, Jiang‐Gao Mao, Guo‐Ming Wang

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Achieving Large Second Harmonic Generation Effects via Optimal Planar Alignment of Triangular UnitsOriginalFrom H 12 C 4 N 2 CdI 4 to H 11 C 4 N 2 CdI 3 : a highly polarizable CdNI 3 tetrahedron induced a sharp enhancement of second harmonic generation response and birefringence50Organic–inorganic haloargentate hybrids of [Me-dabco]Ag 2 X 3 (X = I or Br) with halide ions manipulating the crystal structure, phase transition, and dielectric behavior7Preparation and spectroscopic characteristics of Tm:YPO4 crystal26Unbiased Screening of Novel Infrared Nonlinear Optical Materials with High Thermal Conductivity: Long‐neglected Nitrides and Popular Chalcogenides12Unbiased Screening of Novel Infrared Nonlinear Optical Materials with High Thermal Conductivity: Long‐neglected Nitrides and Popular Chalcogenides48[C(NH2)2NHNO2][C(NH2)3](NO3)2: A Mixed Organic Cationic Hybrid Nitrate with an Unprecedented Nonlinear-Optical-Active Unit30KCs2[GaB5O10](OH): A Zeolitic Galloborate Framework with a Nonlinear Optical Property13Sb4O3(TeO3)2(HSO4)(OH): An Antimony Tellurite Sulfate Exhibiting Large Optical Anisotropy Activated by Lone Pair Stereoactivity30Recent progress of newly developed functional building units and corresponding nonlinear optical materials14Two New Aluminoborates with 3D Porous-Layered Frameworks2Pb(OH)I: A lead(II)-based oxyhalide with a large birefringence5Improved Birefringence Activated by Tetrahedra Decorated with a Single Linear Unit38Improved Birefringence Activated by Tetrahedra Decorated with a Single Linear Unit1YSO4F·H2O: A Deep-Ultraviolet Birefringent Rare-Earth Sulfate Fluoride with Enhanced Birefringence Induced by Fluorinated Y-Centered Polyhedra19Crystal growth and spectral properties of a mixed crystal Nd3+:LuYPO49Outstanding nonlinear optical properties of all-inorganic perovskite CsPbX3 (X=Cl, Br, I) precursor solutions and polycrystalline films19In Situ Chiral Template Approach to Synthesize Homochiral Lead Iodides for Second‐Harmonic Generation11In Situ Chiral Template Approach to Synthesize Homochiral Lead Iodides for Second‐Harmonic Generation68A-site cation manipulation of exemplary second harmonic generation response and optical anisotropy in rare-earth borates18Electromagnetic Detection Design in Liquid Crystals Janus Metastructures Based on Second Harmonic Generation32Halide-driven polarity tuning and optimized SHG-bandgap balance in (C 4 H 11 N 2 )ZnX 3 (X = Cl, Br, I)34Two chiral Co III and Ni II complexes with identical ligands presenting different nonlinear optical responses4Polysulfide Anions [S x ] 2− ( x = 2, 3, 4, 5): Promising Functional Building Units for Infrared Nonlinear Optical Materials22Guanidinium Vanadate [C(NH2)3]3VO4·2H2O Revealing Enhanced Second-Harmonic Generation and Wide Band Gaps13AYSO4F2 (A = K, Rb): [YO4F4] Polyhedra Enhancement of Birefringence in Non-π-Conjugated Sulfate Systems9Three types of promising functional building units for designing metal halide nonlinear optical crystals20Layered (C5H6ON)2[Sb2O(C2O4)3] with a large birefringence derived from the uniform arrangement of π-conjugated units11A Noncentrosymmetric Metal‐Free Borophosphate: Achieving a Large Birefringence and Excellent Stability by Covalent‐Linkage27Multiple Functions of l -Thioproline in the Synthesis of Chiral Metal Bromides Showing Second-Harmonic-Generation Responses18Polarized spectroscopic properties of Tm3+/Ho3+:YPO4 single crystal: A potential gain medium for tunable and ultrafast pulse laser at 2.0 μm2A Chlorinated Indolium‐Based Nonlinear Optical Crystal Achieving Effective Terahertz‐Wave Generation and Highly Sensitive Detection19Intramolecular Hydrogen Bonds Enhance Structure Coplanarity, Resulting in Significant Birefringence in Bridged-Bipyridine Halides7Near Ultraviolet‐Excitable Cyan‐Emissive Hybrid Copper(I) Halides Nonlinear Optical Crystals with Near‐Unity Photoluminescence Quantum Yield and High‐Efficiency X‐ray Scintillation82Near Ultraviolet‐Excitable Cyan‐Emissive Hybrid Copper(I) Halides Nonlinear Optical Crystals with Near‐Unity Photoluminescence Quantum Yield and High‐Efficiency X‐ray Scintillation13NaK5La2(SO4)6: Enhanced Birefringence of Multiple-Alkali Metal Sulfate Systems via Rare Earth Metal-Centered Polyhedra5A layered Janus metastructure for multi-physical quantity detection based on the second harmonic wave0Two l -Proline Cadmium Thiocyanates with Moderate Second-Harmonic-Generation Responses and Large Birefringences13Cationic Coordination Modification Drives Birefringence and Nonlinear Effect Double Lifting in Sulfate4Ligand substitution in organic–inorganic hybrid zinc iodides for second-harmonic generation7Strong second-harmonic generation response in an organic–inorganic hybrid antimony bromide1Designing Polar Covalent Hybrid Cadmium‐Based Chalcohalides Ultraviolet Nonlinear Optical Crystal with Strong Optical Anisotropy via Double‐Site Dual FBUs Tailoring25Extendable Synthesis of Organic Cations for In Situ Construction of Hybrid Metal Halides with Near‐Unity Photoluminescence and Strong Second Harmonic Generation22Extendable Synthesis of Organic Cations for In Situ Construction of Hybrid Metal Halides with Near‐Unity Photoluminescence and Strong Second Harmonic Generation8Na3Y2F3P2O8 and K4Y3F5P4O14: [YOF] Polyhedra Inducing Birefringence Enhancement in Non-π-Conjugated Phosphate Systems3Toward the Strongest Nonlinear Optical Response and Largest Birefringence in Solvent‐Free Organic–Inorganic Metal Halides by Hydrogen Bond Engineering39Phase-Matching Second-Harmonic Generation in Zero-Dimensional Zinc Thiocyanates Ligated with Chiral Amino Acids6Bridging the Interlayer Binding to Ordered π‐Conjugated Units for Constructing High‐Performing Light Polarization Crystals8Bridging the Interlayer Binding to Ordered π‐Conjugated Units for Constructing High‐Performing Light Polarization Crystals48Spectral characteristics of Nd3+/Yb3+:LuPO4 crystal applied to multi-wavelength emission in 1.0 μm2Structural Evolution of Hybrid Bismuth-Based Halides toward Enhanced Second-Harmonic Generation Response and Birefringence through Multisite Chemical Substitution7High‐Efficient Switchable Third Harmonic Generation on Thin Film Phase Change Materials0Remarkable Birefringence Enhancement Enabled by π-Conjugated Cyanoguanidine Group Based on Anisotropic Molecule Coordination Approach8pH‐Regulated Ring‐Opening/Closing Transformation in Polyoxometalates Enables High‐Performance Nonlinear Optical Crystals1pH‐Regulated Ring‐Opening/Closing Transformation in Polyoxometalates Enables High‐Performance Nonlinear Optical Crystals13Dual-anion synergy drives remarkable birefringence in sulfate–nitrate crystals1Anionic configuration extension induced birefringence enhancement in vanadium iodate oxyfluorides0Internally and externally induced chiral hybrid metal halide materials for advanced chiroptoelectronic applications23Unlocking Strong SHG Response and Large Birefringence in Hybrid Antimony Halides via a Three-in-One Strategy7Nonlinear Optical Responses in One-Dimensional Zinc Thiocyanates Functionalized with Natural Amino Acids8In-situ organic cation evolution driven sequential crystal transformation in hybrid metal halides1Engineering Multiple Hydrogen‐Bond Sites With D‐π‐A Motifs for Strong Optical Nonlinearity and Giant Birefringence in Organic‐Inorganic Halides4Engineering Multiple Hydrogen‐Bond Sites With D‐π‐A Motifs for Strong Optical Nonlinearity and Giant Birefringence in Organic‐Inorganic Halides1The novel Zn-based ultraviolet birefringent crystals combined both large birefringence and wide bandgap2Mid‐ to Far‐Infrared Nonlinear Optical Crystals: Design Strategies, Structure–Property Relationships and Engineering Prospects0

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  1. From H 12 C 4 N 2 CdI 4 to H 11 C 4 N 2 CdI 3 : a highly polarizable CdNI 3 tetrahedron induced a sharp enhancement of second harmonic generation response and birefringence

    Chemical Science · 2023-01-01

    Huai‐Yu Wu, Chun‐Li Hu, Miao‐Bin Xu, Qianqian Chen, Nan Ma, Xiao‐Ying Huang, Ke‐Zhao Du, Jin Chen

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  2. Organic–inorganic haloargentate hybrids of [Me-dabco]Ag 2 X 3 (X = I or Br) with halide ions manipulating the crystal structure, phase transition, and dielectric behavior

    Dalton Transactions · 2023-01-01

    Xue−Wei Pan, Qingqing Li, Lu Zhai, Jin Zhang, Wenlong Liu, Xiao‐Ming Ren

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  3. Preparation and spectroscopic characteristics of Tm:YPO4 crystal

    Journal of Luminescence · 2023-02-15

    Lijie Sun, Lijie Sun, Jingyao Lu, Jingyao Lu, Shikun Su, Yanfei Zou, Ronghui Liu, Zonghao Lei, Degao Zhong, Jianhong Li, Jia Gao, Shijia Sun, Bing Teng

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  4. Unbiased Screening of Novel Infrared Nonlinear Optical Materials with High Thermal Conductivity: Long‐neglected Nitrides and Popular Chalcogenides

    Angewandte Chemie · 2023-02-20

    Dongdong Chu, Yi Huang, Congwei Xie, Evgenii Tikhonov, Ivan A. Kruglov, Guangmao Li, Shilie Pan, Zhihua Yang

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  5. Unbiased Screening of Novel Infrared Nonlinear Optical Materials with High Thermal Conductivity: Long‐neglected Nitrides and Popular Chalcogenides

    Angewandte Chemie International Edition · 2023-02-20

    Dongdong Chu, Yi Huang, Congwei Xie, Evgenii Tikhonov, Ivan A. Kruglov, Guangmao Li, Shilie Pan, Zhihua Yang

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  6. [C(NH2)2NHNO2][C(NH2)3](NO3)2: A Mixed Organic Cationic Hybrid Nitrate with an Unprecedented Nonlinear-Optical-Active Unit

    Inorganic Chemistry · 2023-03-14

    Dong Yan, Meng-Meng Ren, Qian Liu, Fei‐Fei Mao, Yu Ma, Ru‐Ling Tang, Hongbo Huang, Bingbing Zhang, Xiu‐Du Zhang, Shu‐Fang Li

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  7. KCs2[GaB5O10](OH): A Zeolitic Galloborate Framework with a Nonlinear Optical Property

    Crystal Growth & Design · 2023-04-04

    Wenfang Liu, Chong‐An Chen, Xuyan Li, Guo‐Yu Yang

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  8. Sb4O3(TeO3)2(HSO4)(OH): An Antimony Tellurite Sulfate Exhibiting Large Optical Anisotropy Activated by Lone Pair Stereoactivity

    Inorganic Chemistry · 2023-04-21

    Xiaofei Li, Kui Wang, Chao He, Jinhua Li, Xing‐Tao An, Jie Pan, Qi Wei, Guo‐Ming Wang, Guo‐Yu Yang

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  9. Recent progress of newly developed functional building units and corresponding nonlinear optical materials

    Chinese Journal of Structural Chemistry · 2023-05-11

    Wenjing Tan, Chenyang Zhang, Chenyang Zhang, Tingting Huang, Bingbing Zhang

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  10. Two New Aluminoborates with 3D Porous-Layered Frameworks

    Molecules · 2023-05-27

    Chen Wang, Juan Chen, Chong‐An Chen, Zhenwen Wang, Guo‐Yu Yang

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  11. Pb(OH)I: A lead(II)-based oxyhalide with a large birefringence

    Inorganic Chemistry Communications · 2023-06-25

    Xiaofei Li, Huili Zhang, Dong‐Xue Jiao, Chao He, Yu-Xue Guo, Xing‐Tao An, Qi Wei

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  12. Improved Birefringence Activated by Tetrahedra Decorated with a Single Linear Unit

    Angewandte Chemie International Edition · 2023-06-29

    Wenlong Xie, Fuming Li, Jianbang Chen, Zhihuang Yang, Guangmao Li, Shilie Pan

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  13. Improved Birefringence Activated by Tetrahedra Decorated with a Single Linear Unit

    Angewandte Chemie · 2023-06-29

    Wenlong Xie, Fuming Li, Jianbang Chen, Zhihuang Yang, Guangmao Li, Shilie Pan

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  14. YSO4F·H2O: A Deep-Ultraviolet Birefringent Rare-Earth Sulfate Fluoride with Enhanced Birefringence Induced by Fluorinated Y-Centered Polyhedra

    Inorganic Chemistry · 2023-10-12

    Dong‐Xue Jiao, Huili Zhang, Xiao-Fei Li, Chao He, Jinhua Li, Qi Wei, Guo‐Yu Yang

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  15. Crystal growth and spectral properties of a mixed crystal Nd3+:LuYPO4

    Journal of Luminescence · 2023-11-15

    Lijie Sun, Jingyao Lu, Qingtang Xu, Shikun Su, Ronghui Liu, Zonghao Lei, Kai Xu, Yanfei Zou, Bingtao Zhang, Jianhong Li, Jia Gao, Bing Teng, Shijia Sun, Degao Zhong

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  16. Outstanding nonlinear optical properties of all-inorganic perovskite CsPbX3 (X=Cl, Br, I) precursor solutions and polycrystalline films

    iScience · 2023-11-22

    Yue Chun Fu, Srinivasa Rao Konda, Rashid Ashirovich Ganeev, Vyacheslav V. Kim, Ganjaboy S. Boltaev, Ran Wang, Weili Yu, Wei Li

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  17. In Situ Chiral Template Approach to Synthesize Homochiral Lead Iodides for Second‐Harmonic Generation

    Angewandte Chemie · 2023-12-21

    Juan Cheng, Gangji Yi, Zhizhuan Zhang, Ying Long, Hongmei Zeng, Ling Huang, Guohong Zou, Zhien Lin

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  18. In Situ Chiral Template Approach to Synthesize Homochiral Lead Iodides for Second‐Harmonic Generation

    Angewandte Chemie International Edition · 2023-12-21

    Juan Cheng, Gangji Yi, Zhizhuan Zhang, Ying Long, Hongmei Zeng, Ling Huang, Guohong Zou, Zhien Lin

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  19. A-site cation manipulation of exemplary second harmonic generation response and optical anisotropy in rare-earth borates

    Chemical Science · 2024-01-01

    Jie Song, Huijian Zhao, Conggang Li, Ning Ye, Zhanggui Hu, Yicheng Wu

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  20. Electromagnetic Detection Design in Liquid Crystals Janus Metastructures Based on Second Harmonic Generation

    IEEE Transactions on Instrumentation and Measurement · 2024-01-01

    Cheng Yang, Chu-Ming Guo, Yu-Xin Wei, Haifeng Zhang

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  21. Halide-driven polarity tuning and optimized SHG-bandgap balance in (C 4 H 11 N 2 )ZnX 3 (X = Cl, Br, I)

    Inorganic Chemistry Frontiers · 2024-01-01

    Jin Chen, Huai-Yu Wu, Miao‐Bin Xu, Mingchang Wang, Qianqian Chen, Bingxuan Li, Chun‐Li Hu, Ke‐Zhao Du

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  22. Two chiral Co III and Ni II complexes with identical ligands presenting different nonlinear optical responses

    New Journal of Chemistry · 2024-01-01

    Taoyu Wang, Yanhong Peng, Zhiqiang Zhang, Congli Gao, Xi-Li Li

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  23. Polysulfide Anions [S x ] 2− ( x = 2, 3, 4, 5): Promising Functional Building Units for Infrared Nonlinear Optical Materials

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  24. Guanidinium Vanadate [C(NH2)3]3VO4·2H2O Revealing Enhanced Second-Harmonic Generation and Wide Band Gaps

    Inorganic Chemistry · 2024-02-05

    Zhiyong Bai, Yunseung Kuk, Jihyun Lee, Heewon Kim, Kang Min Ok

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  25. AYSO4F2 (A = K, Rb): [YO4F4] Polyhedra Enhancement of Birefringence in Non-π-Conjugated Sulfate Systems

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    Zhencheng Wu, Huimin Li, Xueling Hou, Zhihua Yang, Hongsheng Shi

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  26. Three types of promising functional building units for designing metal halide nonlinear optical crystals

    Chinese Journal of Structural Chemistry · 2024-04-01

    Jiajing Wu, Ru‐Ling Tang, Sheng‐Ping Guo

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  27. Layered (C5H6ON)2[Sb2O(C2O4)3] with a large birefringence derived from the uniform arrangement of π-conjugated units

    Chinese Journal of Structural Chemistry · 2024-04-13

    Dong‐Xue Jiao, Huili Zhang, Chao He, Siyu Chen, Ke Wang, Xiaohan Zhang, Li Wei, Qi Wei

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  28. A Noncentrosymmetric Metal‐Free Borophosphate: Achieving a Large Birefringence and Excellent Stability by Covalent‐Linkage

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    Hui‐Li Zhang, Dong‐Xue Jiao, Xiaofei Li, Chao He, Xi‐Ming Dong, Kai Huang, Jinhua Li, Xing‐Tao An, Qi Wei, Guo‐Ming Wang

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  29. Multiple Functions of l -Thioproline in the Synthesis of Chiral Metal Bromides Showing Second-Harmonic-Generation Responses

    Inorganic Chemistry · 2024-04-23

    Peiqi Qian, Ying Li, Juan Cheng, Jing Li, Hongmei Zeng, Ling Huang, Guohong Zou, Zhien Lin

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  30. Polarized spectroscopic properties of Tm3+/Ho3+:YPO4 single crystal: A potential gain medium for tunable and ultrafast pulse laser at 2.0 μm

    Journal of Luminescence · 2024-05-16

    Lijie Sun, Chunxiao Nie, Zonghao Lei, Qingtang Xu, Shikun Su, Xinyue Shi, Ronghui Liu, Yanfei Zou, Jianhong Li, Jia Gao, Degao Zhong, Bing Teng, Shijia Sun

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  31. A Chlorinated Indolium‐Based Nonlinear Optical Crystal Achieving Effective Terahertz‐Wave Generation and Highly Sensitive Detection

    Advanced Functional Materials · 2024-05-25

    Hebin Liang, Qiaoqiao Fu, Yicheng Wu, Xinyuan Zhang, Pengxiang Liu

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  32. Intramolecular Hydrogen Bonds Enhance Structure Coplanarity, Resulting in Significant Birefringence in Bridged-Bipyridine Halides

    Crystal Growth & Design · 2024-05-30

    Wenjie He, Xin Liu, Ling Chen, Li‐Ming Wu

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  33. Near Ultraviolet‐Excitable Cyan‐Emissive Hybrid Copper(I) Halides Nonlinear Optical Crystals with Near‐Unity Photoluminescence Quantum Yield and High‐Efficiency X‐ray Scintillation

    Angewandte Chemie International Edition · 2024-07-09

    Jing‐Li Qi, Yue Guo, Jiajing Wu, Jiajing Wu, Qiao‐Feng Huang, Junjie Xu, Shufang Yan, Wenlong Liu, Sheng‐Ping Guo

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  34. Near Ultraviolet‐Excitable Cyan‐Emissive Hybrid Copper(I) Halides Nonlinear Optical Crystals with Near‐Unity Photoluminescence Quantum Yield and High‐Efficiency X‐ray Scintillation

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    Jing‐Li Qi, Yue Guo, Jiajing Wu, Qiao‐Feng Huang, Junjie Xu, Shufang Yan, Wenlong Liu, Sheng‐Ping Guo

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  35. NaK5La2(SO4)6: Enhanced Birefringence of Multiple-Alkali Metal Sulfate Systems via Rare Earth Metal-Centered Polyhedra

    Inorganic Chemistry · 2024-07-22

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  36. A layered Janus metastructure for multi-physical quantity detection based on the second harmonic wave

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    Yu‐Xin Wei, Jun-Yang Sui, Chuanqi Wu, Chu-Ming Guo, Xiang Li, Haifeng Zhang

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  37. Two l -Proline Cadmium Thiocyanates with Moderate Second-Harmonic-Generation Responses and Large Birefringences

    Inorganic Chemistry · 2024-11-27

    Yue Zhou, Juan Cheng, Daibing Luo, Hongmei Zeng, Ling Huang, Guohong Zou, Zhien Lin

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  38. Cationic Coordination Modification Drives Birefringence and Nonlinear Effect Double Lifting in Sulfate

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    Jiahao Wan, Ping Wang, Zhenhua Li, Chunxiang Wu, Weining Zheng, Lehui Liu, Hongming Liu

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  39. Ligand substitution in organic–inorganic hybrid zinc iodides for second-harmonic generation

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  40. Strong second-harmonic generation response in an organic–inorganic hybrid antimony bromide

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  41. Designing Polar Covalent Hybrid Cadmium‐Based Chalcohalides Ultraviolet Nonlinear Optical Crystal with Strong Optical Anisotropy via Double‐Site Dual FBUs Tailoring

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  42. Extendable Synthesis of Organic Cations for In Situ Construction of Hybrid Metal Halides with Near‐Unity Photoluminescence and Strong Second Harmonic Generation

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  43. Extendable Synthesis of Organic Cations for In Situ Construction of Hybrid Metal Halides with Near‐Unity Photoluminescence and Strong Second Harmonic Generation

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  44. Na3Y2F3P2O8 and K4Y3F5P4O14: [YOF] Polyhedra Inducing Birefringence Enhancement in Non-π-Conjugated Phosphate Systems

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  45. Toward the Strongest Nonlinear Optical Response and Largest Birefringence in Solvent‐Free Organic–Inorganic Metal Halides by Hydrogen Bond Engineering

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  46. Phase-Matching Second-Harmonic Generation in Zero-Dimensional Zinc Thiocyanates Ligated with Chiral Amino Acids

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  47. Bridging the Interlayer Binding to Ordered π‐Conjugated Units for Constructing High‐Performing Light Polarization Crystals

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  48. Bridging the Interlayer Binding to Ordered π‐Conjugated Units for Constructing High‐Performing Light Polarization Crystals

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  49. Spectral characteristics of Nd3+/Yb3+:LuPO4 crystal applied to multi-wavelength emission in 1.0 μm

    Optical Materials · 2025-06-02

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  50. Structural Evolution of Hybrid Bismuth-Based Halides toward Enhanced Second-Harmonic Generation Response and Birefringence through Multisite Chemical Substitution

    Inorganic Chemistry · 2025-07-28

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