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RESEARCH PAPER · Inorganic Chemistry · 2014

Borate Fluoride and Fluoroborate in Alkali-Metal Borate Prepared by an Open High-Temperature Solution Method

Hongping Wu, Hongwei Yu, Qiang Bian, Zhihua Yang, Shujuan Han, Shilie Pan

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Borate Fluoride and Fluoroborate in Alkali-Metal Borate Prepared by an Open High-Temperature Solution MethodOriginalChemInform Abstract: Borate Fluoride and Fluoroborate in Alkali‐Metal Borate Prepared by an Open High‐Temperature Solution Method.0Frequency-Doubling Oxide Fluorides, Borate Fluorides, and Fluorooxoborates9New fluoroborate Cd 8 B 5 O 15 F with two different isolated borate anions prepared by an open high-temperature solution method7K5Ba10(BO3)8F: A New Potassium Barium Borate Fluoride with a Perovskite-Like Structure43The plane-wave DFT investigations into the structure and the 11B solid-state NMR parameters of lithium fluorooxoborates5Na2B6O9F2: A Fluoroborate with Short Cutoff Edge and Deep-Ultraviolet Birefringent Property Prepared by an Open High-Temperature Solution Method106The structural diversity of halogen-centered secondary building units: two new mixed-metal borate halides with deep-ultraviolet cut-off edges16Interaction of B 2 O 3 with molten KF-AlF 3 and KF-NaF-AlF 326CsB 4 O 6 F: A Congruent‐Melting Deep‐Ultraviolet Nonlinear Optical Material by Combining Superior Functional Units184CsB4O6F: A Congruent‐Melting Deep‐Ultraviolet Nonlinear Optical Material by Combining Superior Functional Units895Insight on the growth and property studies of inorganic hydrated borate (Na6 [B4O5 (OH)4]3. 8H2O) single crystal – An effective third order nonlinear optical (NLO) material for optical limiting application20BaBOF 3 : a new aurivillius-like borate containing two types of F atoms32Ion-induced structural and optical performance evolution in LBO-like crystals: experimental and theoretical investigation13A Member of Fluorooxoborates: Li2Na0.9K0.1B5O8F2 with the Fundamental Building Block B5O10F2 and a Short Cutoff Edge27Cation‐Tuned Synthesis of Fluorooxoborates: Towards Optimal Deep‐Ultraviolet Nonlinear Optical Materials191Cation‐Tuned Synthesis of Fluorooxoborates: Towards Optimal Deep‐Ultraviolet Nonlinear Optical Materials714Pb8M(BO3)6 (M = Mg, Ca): Two new borates with large birefringence activated by the ∞[Pb8B6O18]2- double layers6K3B6O9F3: A New Fluorooxoborate with Four Different Anionic Units42CaB5O7F3: A Beryllium-Free Alkaline-Earth Fluorooxoborate Exhibiting Excellent Nonlinear Optical Performances192From LiB3O5 to NaRbB6O9F2: Fluorine‐Directed Evolution of Structural Chemistry33Sn[B2O3F2]—The First Tin Fluorooxoborate as Possible NLO Material102Fluorooxoborates: Ushering in a New Era of Deep Ultraviolet Nonlinear Optical Materials102BaB8O12F2: a promising deep-UV birefringent material60A new barium fluorooxoborate BaB 5 O 8 F· x H 2 O with large birefringence and a wide UV transparency window25Ba 3 B 10 O 17 F 2 ·0.1KF: the first mixed alkali/alkaline-earth metal fluorooxoborate with unprecedented double-layered B–O/F anionic arrangement17Band structure engineering of boron–oxygen-based materials for efficient charge separation12Fluoroborophosphates: a family of potential deep ultraviolet NLO materials43Designing Three Fluorooxoborates with a Wide Transmittance Window by Anionic Group Substitution15BaB 2 O 3 F 2 : A Barium Fluorooxoborate with a Unique [B 2 O 3 F] − Layer and Short Cutoff Edge38K9[B4O5(OH)4]3(CO3)X·7H2O (X = Cl, Br): Syntheses, Characterizations, and Theoretical Studies of Noncentrosymmetric Halogen Borate–Carbonates with Short UV Cutoff Edges16Cation Modulation on the Crystal Structure and Band Gap of Fluorooxoborates A3B3O3F6 (A = Alkali and Mixed Alkali Metal)17Pb 3 Ba 3 Zn 6 (BO 3 ) 8 and α-BaZn 2 (BO 3 ) 2 : new members of the zincoborates containing two different dimensional Zn–O units8From BaAl 2 (BO 3 ) 2 O to SnAl 2 (BO 3 ) 2 F 2 : structure transformation based on ion regulation3Noncentrosymmetric Fluorooxoborates A10B13O15F19 (A = K and Rb) with Unexpected [B10O12F13]7– Units and Deep-Ultraviolet Cutoff Edges26Enhanced nonlinear optical functionality in birefringence and refractive index dispersion of the deep-ultraviolet fluorooxoborates123Cs3B3O3F6 with a Deep-Ultraviolet Cutoff Edge and a Suitable Birefringence as the Potential Zero-Order Waveplate Material31NaKB 6 O 9 F 2 : a new complex alkali metal fluorooxoborate with puckered layers10Newly emerging borate-based nonlinear optical materials for organic pollutant degradation: A review33NaRbB3O4F3: A New Fluorooxoborate with a Short UV Cutoff Edge Enriching the Structural Chemistry of Borate7MM′B3O4F3 (M = K; M′ = Na, K, Cs): Alkali-Metal Fluorooxoborates with ∞1[B3O4F3] Chains and Deep-Ultraviolet Cutoff Edges12LiNaB6O9F2: A Promising UV NLO Crystal Having Fluorine‐Directed Optimal Performances and Double Interpenetrating 3[B6O9F2]∞ Networks33Li2AB5O8F2 (A = Na and K): two new deep-ultraviolet transparent fluorooxoborates with moderate birefringence designed by targeted dimensional modulation7SYNTHESIS AND CRYSTAL STRUCTURE OF TWO NEW TETRAFLUOROBORATE CRYSTALLOHYDRATES M(BF4)2·3H2O, M = Sr, Ba2Ba2B9O13F4·BF4: first fluorooxoborate with unprecedented infinite [B18O26F8] tubes and deep-ultraviolet cutoff edge14CaB2O2F4: A Novel [BOF2]∞-Based Structural Template with a Strong Second Harmonic Generation Response and Large Band Gap2Two Ultraviolet Optical Crystals K6B12O19F4 and K12B28O48: The Effects of Metal Cations Size and the F Ions on the Structure6Melting Behavior and Densities of K2B2OF6 Melts Containing KReO41Fluorine-driven materials design of novel deep-ultraviolet nonlinear optical crystal materials: Research progress and challenges6Structural Evolution and Optical Properties of Hydroxyfluorooxoborates MM′2n-1[B3O3F4(OH)]n (M = K, Cs, and Rb; M′ = K, NH4, and Cs; n = 1, 2, and 3)12Electrodeposition of Iridium and Rhenium Layers from Molten Salts and Behavior of Ir/Re-based Coatings under High-Temperature Oxidation Conditions1

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  1. ChemInform Abstract: Borate Fluoride and Fluoroborate in Alkali‐Metal Borate Prepared by an Open High‐Temperature Solution Method.

    ChemInform · 2015-02-16

    Hongping Wu, Hongwei Yu, Qiang Bian, Zhihua Yang, Shujuan Han, Shilie Pan

    Read original paper ↗ ·

  2. Frequency-Doubling Oxide Fluorides, Borate Fluorides, and Fluorooxoborates

    Elsevier eBooks · 2016-01-01

    Shilie Pan, Y. Wang, Kenneth Reinhard Poeppelmeier

    Read original paper ↗ ·

  3. New fluoroborate Cd 8 B 5 O 15 F with two different isolated borate anions prepared by an open high-temperature solution method

    Dalton Transactions · 2016-01-01

    Yun Mo Yang, Xiaoyu Dong, Shilie Pan

    Read original paper ↗ ·

  4. K5Ba10(BO3)8F: A New Potassium Barium Borate Fluoride with a Perovskite-Like Structure

    The Journal of Physical Chemistry C · 2016-08-01

    Lili Liu, Yun Mo Yang, Qun Jing, Xiaoyu Dong, Zhihua Yang, Shilie Pan, Kui Wu

    Read original paper ↗ ·

  5. The plane-wave DFT investigations into the structure and the 11B solid-state NMR parameters of lithium fluorooxoborates

    Chemical Physics Letters · 2016-10-28

    Jiřı́ Czernek, Jiřı́ Brus

    Read original paper ↗ ·

  6. Na2B6O9F2: A Fluoroborate with Short Cutoff Edge and Deep-Ultraviolet Birefringent Property Prepared by an Open High-Temperature Solution Method

    Inorganic Chemistry · 2016-12-14

    Guoqiang Q. Shi, Fangfang Zhang, Bingbing Zhang, Dianwei Hou, Xinglong Chen, Zhihua Yang, Shilie Pan

    Read original paper ↗ ·

  7. The structural diversity of halogen-centered secondary building units: two new mixed-metal borate halides with deep-ultraviolet cut-off edges

    Dalton Transactions · 2017-01-01

    Miriding Mutailipu, Min Zhang, Yanna Chen, Xiaoquan Lu, Shilie Pan

    Read original paper ↗ ·

  8. Interaction of B 2 O 3 with molten KF-AlF 3 and KF-NaF-AlF 3

    Journal of Molecular Liquids · 2017-02-07

    Alexander A. Kataev, Olga Yu. Tkacheva, Irina D. Zakirýanova, Alexey A. Apisarov, Alexander S. Dedyukhin, Yu. P. Zaikov

    Read original paper ↗ ·

  9. CsB 4 O 6 F: A Congruent‐Melting Deep‐Ultraviolet Nonlinear Optical Material by Combining Superior Functional Units

    Angewandte Chemie · 2017-09-12

    Xuefei Wang, Ying Wang, Bingbing Zhang, Fangfang Zhang, Zhihua Yang, Shilie Pan

    Read original paper ↗ ·

  10. CsB4O6F: A Congruent‐Melting Deep‐Ultraviolet Nonlinear Optical Material by Combining Superior Functional Units

    Angewandte Chemie International Edition · 2017-09-12

    Xuefei Wang, Ying Wang, Bingbing Zhang, Fangfang Zhang, Zhihua Yang, Shilie Pan

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  11. Insight on the growth and property studies of inorganic hydrated borate (Na6 [B4O5 (OH)4]3. 8H2O) single crystal – An effective third order nonlinear optical (NLO) material for optical limiting application

    Materials Chemistry and Physics · 2017-11-08

    Ramki Chakaravarthy, R. Ezhil Vizhi

    Read original paper ↗ ·

  12. BaBOF 3 : a new aurivillius-like borate containing two types of F atoms

    Dalton Transactions · 2018-01-01

    Dequan Jiang, Ying Wang, Hao Li, Zhihua Yang, Shilie Pan

    Read original paper ↗ ·

  13. Ion-induced structural and optical performance evolution in LBO-like crystals: experimental and theoretical investigation

    Inorganic Chemistry Frontiers · 2018-01-01

    Yun Mo Yang, Shilie Pan

    Read original paper ↗ ·

  14. A Member of Fluorooxoborates: Li2Na0.9K0.1B5O8F2 with the Fundamental Building Block B5O10F2 and a Short Cutoff Edge

    Inorganic Chemistry · 2018-01-02

    Shujuan Han, Ying Wang, Bingbing Zhang, Zhihua Yang, Shilie Pan

    Read original paper ↗ ·

  15. Cation‐Tuned Synthesis of Fluorooxoborates: Towards Optimal Deep‐Ultraviolet Nonlinear Optical Materials

    Angewandte Chemie · 2018-01-10

    Ying Wang, Bingbing Zhang, Zhihua Yang, Shilie Pan

    Read original paper ↗ ·

  16. Cation‐Tuned Synthesis of Fluorooxoborates: Towards Optimal Deep‐Ultraviolet Nonlinear Optical Materials

    Angewandte Chemie International Edition · 2018-01-10

    Ying Wang, Bingbing Zhang, Zhihua Yang, Shilie Pan

    Read original paper ↗ ·

  17. Pb8M(BO3)6 (M = Mg, Ca): Two new borates with large birefringence activated by the ∞[Pb8B6O18]2- double layers

    Journal of Alloys and Compounds · 2018-02-22

    Chen Zhou, Hui Zhang, Jianian Cheng, Hongyi Li, Sadeh Beysen

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  18. K3B6O9F3: A New Fluorooxoborate with Four Different Anionic Units

    Chemistry - A European Journal · 2018-02-24

    Guopeng Han, Guoqiang Q. Shi, Ying Wang, Bingbing Zhang, Shujuan Han, Fangfang Zhang, Zhihua Yang, Shilie Pan

    Read original paper ↗ ·

  19. CaB5O7F3: A Beryllium-Free Alkaline-Earth Fluorooxoborate Exhibiting Excellent Nonlinear Optical Performances

    Inorganic Chemistry · 2018-04-17

    Zhizhong Zhang, Ying Wang, Bingbing Zhang, Zhihua Yang, Shilie Pan

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  20. From LiB3O5 to NaRbB6O9F2: Fluorine‐Directed Evolution of Structural Chemistry

    Chemistry - A European Journal · 2018-06-04

    Shujuan Han, Bingbing Zhang, Zhihua Yang, Shilie Pan

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  21. Sn[B2O3F2]—The First Tin Fluorooxoborate as Possible NLO Material

    Advanced Optical Materials · 2018-06-25

    Stephan G. Jantz, Marwin Dialer, Lkhamsuren Bayarjargal, Björn Winkler, Leo van Wüllen, Florian Pielnhofer, Jakoah Brgoch, Richard Weihrich, Henning A. Höppe

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  22. Fluorooxoborates: Ushering in a New Era of Deep Ultraviolet Nonlinear Optical Materials

    Chemistry - A European Journal · 2018-07-19

    Guopeng Han, Ying Wang, Bingbing Zhang, Shilie Pan

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  23. BaB8O12F2: a promising deep-UV birefringent material

    Inorganic Chemistry Frontiers · 2018-12-25

    Zhizhong Zhang, Ying Wang, Hao Li, Zhihua Yang, Shilie Pan

    Read original paper ↗ ·

  24. A new barium fluorooxoborate BaB 5 O 8 F· x H 2 O with large birefringence and a wide UV transparency window

    Dalton Transactions · 2019-01-01

    Chunmei Huang, Guopeng Han, Hao Li, Fangfang Zhang, Zhihua Yang, Shilie Pan

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  25. Ba 3 B 10 O 17 F 2 ·0.1KF: the first mixed alkali/alkaline-earth metal fluorooxoborate with unprecedented double-layered B–O/F anionic arrangement

    Chemical Communications · 2019-01-01

    Yahui Li, Hongwei Yu, Guopeng Han, Hao Li, Zhihua Yang, Shilie Pan

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  26. Band structure engineering of boron–oxygen-based materials for efficient charge separation

    Materials Chemistry Frontiers · 2019-01-01

    Xiaoyun Fan, Kangdi Zhong, Yang Zhang, Jiao Yin, Yufei Zhai

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  27. Fluoroborophosphates: a family of potential deep ultraviolet NLO materials

    Inorganic Chemistry Frontiers · 2019-01-01

    Baolin Wu, Chun‐Li Hu, Ru‐Ling Tang, Fei‐Fei Mao, Jianghe Feng, Jiang‐Gao Mao

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  28. Designing Three Fluorooxoborates with a Wide Transmittance Window by Anionic Group Substitution

    Inorganic Chemistry · 2019-03-04

    Dequan Jiang, Guopeng Han, Ying Wang, Hao Li, Zhihua Yang, Shilie Pan

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  29. BaB 2 O 3 F 2 : A Barium Fluorooxoborate with a Unique [B 2 O 3 F] − Layer and Short Cutoff Edge

    Chemistry - A European Journal · 2019-04-01

    Chunmei Huang, Fangfang Zhang, Hao Li, Zhihua Yang, Haohai Yu, Shilie Pan

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  30. K9[B4O5(OH)4]3(CO3)X·7H2O (X = Cl, Br): Syntheses, Characterizations, and Theoretical Studies of Noncentrosymmetric Halogen Borate–Carbonates with Short UV Cutoff Edges

    Inorganic Chemistry · 2019-05-01

    Xueyan Zhang, Hongping Wu, Shichao Cheng, Guopeng Han, Zhihua Yang, Shilie Pan

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  31. Cation Modulation on the Crystal Structure and Band Gap of Fluorooxoborates A3B3O3F6 (A = Alkali and Mixed Alkali Metal)

    Inorganic Chemistry · 2019-09-18

    Wenyao Zhang, Zhonglei Wei, Zhihua Yang, Shilie Pan

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  32. Pb 3 Ba 3 Zn 6 (BO 3 ) 8 and α-BaZn 2 (BO 3 ) 2 : new members of the zincoborates containing two different dimensional Zn–O units

    Inorganic Chemistry Frontiers · 2019-10-09

    Xiaobo Pan, Hongping Wu, Shichao Cheng, Zhengping Wang

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  33. From BaAl 2 (BO 3 ) 2 O to SnAl 2 (BO 3 ) 2 F 2 : structure transformation based on ion regulation

    New Journal of Chemistry · 2020-01-01

    Ya Wang, Jian Wei Han, Junben Huang, Zhihua Yang, Shuzhao Huang, Shilie Pan

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  34. Noncentrosymmetric Fluorooxoborates A10B13O15F19 (A = K and Rb) with Unexpected [B10O12F13]7– Units and Deep-Ultraviolet Cutoff Edges

    Inorganic Chemistry · 2020-02-10

    Wenyao Zhang, Zhonglei Wei, Zhihua Yang, Shilie Pan

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  35. Enhanced nonlinear optical functionality in birefringence and refractive index dispersion of the deep-ultraviolet fluorooxoborates

    Science China Materials · 2020-03-20

    Zhihua Yang, Abudukadi Tudi, Bing‐Hua Lei, Shilie Pan

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  36. Cs3B3O3F6 with a Deep-Ultraviolet Cutoff Edge and a Suitable Birefringence as the Potential Zero-Order Waveplate Material

    Inorganic Chemistry · 2020-09-11

    Meng Cheng, Wenqi Jin, Zhihua Yang, Shilie Pan

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  37. NaKB 6 O 9 F 2 : a new complex alkali metal fluorooxoborate with puckered layers

    New Journal of Chemistry · 2021-01-01

    Zilong Chen, Junwei Feng, Bin Dai, Feng Yu

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  38. Newly emerging borate-based nonlinear optical materials for organic pollutant degradation: A review

    Critical Reviews in Environmental Science and Technology · 2021-02-10

    Xiaoyun Fan

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  39. NaRbB3O4F3: A New Fluorooxoborate with a Short UV Cutoff Edge Enriching the Structural Chemistry of Borate

    Chemistry - An Asian Journal · 2021-08-20

    Rui Zhang, Jie Zhang, Zhihua Yang, Shujuan Han, Shilie Pan

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  40. MM′B3O4F3 (M = K; M′ = Na, K, Cs): Alkali-Metal Fluorooxoborates with ∞1[B3O4F3] Chains and Deep-Ultraviolet Cutoff Edges

    Inorganic Chemistry · 2022-02-02

    Zhikang Chen, Kewang Zhang, Zi‐Jian Li, Fangfang Zhang, Zhihua Yang, Shilie Pan

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  41. LiNaB6O9F2: A Promising UV NLO Crystal Having Fluorine‐Directed Optimal Performances and Double Interpenetrating 3[B6O9F2]∞ Networks

    Advanced Optical Materials · 2022-12-03

    Xiaojing Li, Zilong Chen, Fuming Li, Fangfang Zhang, Zhihua Yang, Shilie Pan

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  42. Li2AB5O8F2 (A = Na and K): two new deep-ultraviolet transparent fluorooxoborates with moderate birefringence designed by targeted dimensional modulation

    Materials Today Chemistry · 2023-01-01

    Huanhuan Cheng, Z. Li, Fromenteze Zhang, Zhihua Yang, Shilie Pan

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  43. SYNTHESIS AND CRYSTAL STRUCTURE OF TWO NEW TETRAFLUOROBORATE CRYSTALLOHYDRATES M(BF4)2·3H2O, M = Sr, Ba

    Journal of Structural Chemistry · 2023-02-01

    Dmitri O. Charkin, Sergey N. Volkov, Lev S. Manelis, Alevtina N. Gosteva, Sergey M. Aksenov, В. А. Долгих

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  44. Ba2B9O13F4·BF4: first fluorooxoborate with unprecedented infinite [B18O26F8] tubes and deep-ultraviolet cutoff edge

    Science China Chemistry · 2023-02-23

    Huan Pei, Xuefei Wang, Jie Zhang, Fangfang Zhang, Zhihua Yang, Shilie Pan

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  45. CaB2O2F4: A Novel [BOF2]∞-Based Structural Template with a Strong Second Harmonic Generation Response and Large Band Gap

    The Journal of Physical Chemistry C · 2023-03-22

    Evgenii Tikhonov, Huanhuan Cheng, Abudukadi Tudi, Congwei Xie, Shilie Pan, Zhihua Yang

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  46. Two Ultraviolet Optical Crystals K6B12O19F4 and K12B28O48: The Effects of Metal Cations Size and the F Ions on the Structure

    Inorganic Chemistry · 2023-05-09

    Shuzhao Huang, Liang Zhu, Ivan A. Kruglov, Yun Mo Yang, Zhihua Yang, Shilie Pan

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  47. Melting Behavior and Densities of K2B2OF6 Melts Containing KReO4

    Processes · 2023-11-03

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  48. Fluorine-driven materials design of novel deep-ultraviolet nonlinear optical crystal materials: Research progress and challenges

    Chinese Science Bulletin (Chinese Version) · 2024-07-01

    Zhihua Yang, Shilie Pan

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  49. Structural Evolution and Optical Properties of Hydroxyfluorooxoborates MM′2n-1[B3O3F4(OH)]n (M = K, Cs, and Rb; M′ = K, NH4, and Cs; n = 1, 2, and 3)

    Chemistry of Materials · 2024-11-25

    Huan Pei, Luyong Zhang, Huanhuan Cheng, Shi‐Bin Wang, Zhihua Yang, Fangfang Zhang, Shilie Pan

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  50. Electrodeposition of Iridium and Rhenium Layers from Molten Salts and Behavior of Ir/Re-based Coatings under High-Temperature Oxidation Conditions

    Journal of The Electrochemical Society · 2025-07-01

    Andrey V. Isakov, Olga V. Grishenkova, Yu. P. Zaikov

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