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RESEARCH PAPER · Chemistry of Materials · 2024

Structural Evolution and Optical Properties of Hydroxyfluorooxoborates MM′2n-1[B3O3F4(OH)]n (M = K, Cs, and Rb; M′ = K, NH4, and Cs; n = 1, 2, and 3)

Huan Pei, Luyong Zhang, Huanhuan Cheng, Shi‐Bin Wang, Zhihua Yang, Fangfang Zhang, Shilie Pan

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Structural Evolution and Optical Properties of Hydroxyfluorooxoborates MM′2n-1[B3O3F4(OH)]n (M = K, Cs, and Rb; M′ = K, NH4, and Cs; n = 1, 2, and 3)OriginalCation tuning in anionic framework hydroborates: tailored deep-ultraviolet optical crystals with large birefringence1Na 2 PbB 6 O 10 SO 4 and Ca 2.58 Pb 0.42 B 6 O 11 SO 4 : first borate–sulfates featuring 3D porous borate anionic frameworks0RbB 7 O 10 (OH) 2 and NaB 11 O 16 (OH) 2 : alkali metal hydroxyborates with two-dimensional layered structures and large birefringence1Na[B3IO7(OH)] and Na2[B4IO9](IO3): Explorations of Boroiodates with Strong Second Harmonic Generation Response and Large Birefringence54Enhancement of Birefringence in Alkali Metal Sulfates Induced by Rare Earth Metal-Centered Polyhedra and Structure Regulation via Cations2Cation regulation achieves symmetry breaking: from centrosymmetric M 2 Cs 2 B 10 O 17 (M = Na, K) to noncentrosymmetric Na 3 CsB 10 O 172Significant Enhancement of Birefringence Resulting from the Introduction of [BO 2 (OH)] Groups into Borosulfates0F−/OH− terminal modification of [B3O6] clusters: Constructing deep-ultraviolet hydroxyfluorooxoborates with tunable optical performance0Breaking Inversion Symmetry via Vanadium Coordination Engineering in Bismuth Vanadium Selenites0Topological structural chemistry of fluorooxoborates: From fundamental building blocks to macroscopic optical performance regulation0Parallel arrangement of functional building blocks: toward performance synergy in oxalate borate ultraviolet nonlinear optical crystals0Fluorination‐Driven Molecular Polarization Engineering in Hydroxyfluorooxoborates for Generating Strong Short‐Wavelength Nonlinear Optical Responses0

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  1. Cation tuning in anionic framework hydroborates: tailored deep-ultraviolet optical crystals with large birefringence

    New Journal of Chemistry · 2025-01-01

    Yansheng Jiang, Hangwei Jia, Wenhu Wang, Muhammad Arif, Xiuling Yan, Xueling Hou

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  2. Na 2 PbB 6 O 10 SO 4 and Ca 2.58 Pb 0.42 B 6 O 11 SO 4 : first borate–sulfates featuring 3D porous borate anionic frameworks

    Inorganic Chemistry Frontiers · 2025-01-01

    Huan Pei, Zi‐Jian Li, Shaohuan Liu, Xueling Hou, Fangfang Zhang

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  3. RbB 7 O 10 (OH) 2 and NaB 11 O 16 (OH) 2 : alkali metal hydroxyborates with two-dimensional layered structures and large birefringence

    Dalton Transactions · 2025-01-01

    Yujing Zheng, Ke Li, Ling Huang, Fangfang Zhang

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  4. Na[B3IO7(OH)] and Na2[B4IO9](IO3): Explorations of Boroiodates with Strong Second Harmonic Generation Response and Large Birefringence

    Journal of the American Chemical Society · 2025-04-07

    Ya-Lan Deng, Chun‐Li Hu, Xiang Xu, Mingzhi Zhang, Jiang‐Gao Mao

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  5. Enhancement of Birefringence in Alkali Metal Sulfates Induced by Rare Earth Metal-Centered Polyhedra and Structure Regulation via Cations

    Chemistry of Materials · 2025-10-23

    Luyong Zhang, Zhencheng Wu, Jingdong Yan, Shibin Wang, Zilong Chen, Zhihua Yang, Fangfang Zhang, Shilie Pan

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  6. Cation regulation achieves symmetry breaking: from centrosymmetric M 2 Cs 2 B 10 O 17 (M = Na, K) to noncentrosymmetric Na 3 CsB 10 O 17

    Journal of Materials Chemistry C · 2025-12-18

    X. Ma, Jiafu Wang, Xiaona Li, Yabo Wu, Zhihua Yang, Fangfang Zhang, Shujuan Han, Shilie Pan

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  7. Significant Enhancement of Birefringence Resulting from the Introduction of [BO 2 (OH)] Groups into Borosulfates

    Chemistry of Materials · 2026-03-04

    Luyong Zhang, Jianyi Zuo, Guangsheng Xu, Jinbin Fan, Xue Bai, Zhihua Yang, Fangfang Zhang, Shilie Pan

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  8. F−/OH− terminal modification of [B3O6] clusters: Constructing deep-ultraviolet hydroxyfluorooxoborates with tunable optical performance

    Materials Today Chemistry · 2026-05-06

    Dahong Peng, Hongkang Su, Ziting Yan, chenxu li, Shilie Pan, Min Zhang

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  9. Breaking Inversion Symmetry via Vanadium Coordination Engineering in Bismuth Vanadium Selenites

    Small · 2026-05-07

    Chanhee Ko, Congcong Jin, Taek Rim Kim, Seung Han Shin, Yunseung Kuk, Jiachen Lu, Chong‐An Chen, Wei Zeng, Joon Ik Jang, Kang Min Ok

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  10. Topological structural chemistry of fluorooxoborates: From fundamental building blocks to macroscopic optical performance regulation

    Coordination Chemistry Reviews · 2026-05-20

    Wenqing Sun, Congwei Xie, Xueling Hou, Zhihua Yang, Shilie Pan

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  11. Parallel arrangement of functional building blocks: toward performance synergy in oxalate borate ultraviolet nonlinear optical crystals

    Science China Chemistry · 2026-07-13

    Juhui Cui, Minqiang Gai, Ke Li, Z L Yang, Xueling Hou, Shilie Pan, Miriding Mutailipu

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  12. Fluorination‐Driven Molecular Polarization Engineering in Hydroxyfluorooxoborates for Generating Strong Short‐Wavelength Nonlinear Optical Responses

    Advanced Functional Materials · 2026-10-09

    Hongkang Su, Juhui Cui, chenxu li, Xiaona Li, Minqiang Gai, Zhihua Yang, Shilie Pan, Min Zhang

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