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RESEARCH PAPER · Chemistry of Materials · 2010

Polarity and Chirality in Uranyl Borates: Insights into Understanding the Vitrification of Nuclear Waste and the Development of Nonlinear Optical Materials

Shuao Wang, Evgeny V. Alekseev, Jie Ling, Guokui Liu, Wulf Depmeier, Thomas E. Albrecht‐Schmitt

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Polarity and Chirality in Uranyl Borates: Insights into Understanding the Vitrification of Nuclear Waste and the Development of Nonlinear Optical MaterialsOriginalCubic and rhombohedral heterobimetallic networks constructed from uranium, transition metals, and phosphonoacetate: new methods for constructing porous materials113Further insights into intermediate- and mixed-valency in neptunium oxoanion compounds: structure and absorption spectroscopy of K2[(NpO2)3B10O16(OH)2(NO3)2]52Comparison of Thorium(IV) and Uranium(VI) Carboxyphosphonates80Crystal Chemistry of the Potassium and Rubidium Uranyl Borate Families Derived from Boric Acid Fluxes49ChemInform Abstract: Polarity and Chirality in Uranyl Borates: Insights into Understanding the Vitrification of Nuclear Waste and the Development of Nonlinear Optical Materials.0Boronic Acid Flux Synthesis and Crystal Growth of Uranium and Neptunium Boronates and Borates: A Low-Temperature Route to the First Neptunium(V) Borate41Structure−Property Relationships in Lithium, Silver, and Cesium Uranyl Borates47Synthesis, structural and emission studies of a bis (carbamoyl methyl) sulfone complex of uranyl nitrate11Recent progress in actinide borate chemistry94Role of Anions and Reaction Conditions in the Preparation of Uranium(VI), Neptunium(VI), and Plutonium(VI) Borates56From Layered Structures to Cubic Frameworks: Expanding the Structural Diversity of Uranyl Carboxyphosphonates via the Incorporation of Cobalt55Surprising Coordination for Plutonium in the First Plutonium(III) Borate53Hydrothermal Synthesis and Structural Characterization of Organically Templated Uranyl Diphosphonate Compounds72Uranyl carboxyphosphonates that incorporate Cd(II)20K(NpO2)3(H2O)Cl4: A Channel Structure Assembled by Two- and Three-Center Cation–Cation Interactions of Neptunyl Cations23Functionalization of Borate Networks by the Incorporation of Fluoride: Syntheses, Crystal Structures, and Nonlinear Optical Properties of Novel Actinide Fluoroborates51Sr2[C6H3(CO2)3(NO3)]·DMF: One-Dimensional Nano-Channel in a New Non-Centrosymmetric Strontium–Organic Framework with High Thermal Stability31Structural Complexity of Barium Uranyl Arsenates: Synthesis, Structure, and Topology of Ba4[(UO2)2(As2O7)3], Ba3[(UO2)2(AsO4)2(As2O7)], and Ba5Ca[(UO2)8(AsO4)4O8]11Incorporation of iodate into uranyl borates and its implication for the immobilization of 129I in nuclear waste repositories10Bonding Changes in Plutonium(III) and Americium(III) Borates60Th2[BO4][PO4]: A RARE EXAMPLE OF AN ACTINIDE BORATE-PHOSPHATE9Interstitial Incorporation of Plutonium into a Low-Dimensional Potassium Borate6New Neptunium(V) Borates That Exhibit the Alexandrite Effect20Complex clover cross-sectioned nanotubules exist in the structure of the first uranium borate phosphate28In-Situ Raman Spectroscopy Studies of Room-Temperature and Hydrothermal Reactions13-Fold-Interpenetrated Uranium–Organic Frameworks: New Strategy for Rationally Constructing Three-Dimensional Uranyl Organic Materials76Steric Effects on Uranyl Complexation: Synthetic, Structural, and Theoretical Studies of Carbamoyl Pyrazole Compounds of the Uranyl(VI) Ion25Barium uranyl diphosphonates16Differentiating between Trivalent Lanthanides and Actinides115Syntheses, structures and luminescent properties of two one-dimensional uranium oxyfluorides12Tailor-Made Zinc Uranyl Diphosphonates from Layered to Framework Structures46Effect of pH and Reaction Time on the Structures of Early Lanthanide(III) Borate Perchlorates16Elucidation of Tetraboric Acid with a New Borate Fundamental Building Block in a Chiral Uranyl Fluoroborate13From 1D Chain to 3D Framework Uranyl Diphosphonates: Syntheses, Crystal Structures, and Selective Ion Exchange82Bisactinyl halogenated complexes: relativistic density functional theory calculation and experimental synthesis9Crystal Chemistry of Uranium Oxides and Minerals27Mono- and dinuclear uranyl(VI) complexes with chiral Schiff base ligand30Uranium(VI) solubility in carbonate-free WIPP brine11High Structural Complexity of Potassium Uranyl Borates Derived from High-Temperature/High-Pressure Reactions32Facile Assembly of an Unusual Lead Borate with Different Cluster Building Units via a Hydrothermal Process38Novel Fundamental Building Blocks and Site Dependent Isomorphism in the First Actinide Borophosphates11Dissolution of uranyl and plutonyl borates: Influences of crystalline structures and aqueous ligands4MOFs of Uranium and the Actinides95Two New Barium Borate Fluorides ABa12(BO3)7F4 (A = Li and Na)41Synthetic, structural, extraction and theoretical studies of uranyl nitrate dithio-diglycolamide compounds11Tris(acrylato)uranylates as a scaffold for NLO materials21Beryllium-free Li4Sr(BO3)2 for deep-ultraviolet nonlinear optical applications462Highly Distorted Uranyl Ion Coordination and One/Two-Dimensional Structural Relationship in the Ba2[UO2(TO4)2] (T = P, As) System: An Experimental and Computational Study19Microbial dissolution and reduction of uranyl crystals by Shewanella oneidensis MR-19Design, synthesis and structure of uranyl coordination polymers from 2-D layer to 3-D network structure2A family of uranyl-aromatic dicarboxylate (pht-, ipa-, tpa-) framework hybrid materials: photoluminescence, surface photovoltage and dye adsorption31Design and synthesis of a chiral uranium-based microporous metal organic framework with high SHG efficiency and sequestration potential for low-valent actinides58Steric effects in complexes of diphenyl(2-pyridyl)phosphine oxide with the uranyl ion. Synthetic, structural and theoretical studies10Multifunctional Uranyl Hybrid Materials: Structural Diversities as a Function of pH, Luminescence with Potential Nitrobenzene Sensing, and Photoelectric Behavior as p-type Semiconductors56The structural effects of alkaline- and rare-earth element incorporation into thorium molybdates8Potassium uranyl borate 3D framework compound resulted from temperature directed hydroborate condensation: structure, spectroscopy, and dissolution studies7Evaluation of f-element borate chemistry76Entangled Uranyl Organic Frameworks with (10,3)-b Topology and Polythreading Network: Structure, Luminescence, and Computational Investigation43BiFSeO 3 : An Excellent SHG Material Designed by Aliovalent Substitution207Novel Uranyl Coordination Polymers Based on Quinoline-Containing Dicarboxylate by Altering Auxiliary Ligands: From 1D Chain to 3D Framework31Influence of Synthetic Conditions on Chemistry and Structural Properties of Alkaline Earth Uranyl Borates23Solvent‐Dependent Synthesis of Porous Anionic Uranyl–Organic Frameworks Featuring a Highly Symmetrical (3,4)‐Connected ctn or bor Topology for Selective Dye Adsorption64Inorganic Synthesis of Actinides3Formation of co-racemic uranyl chromate constructed from chiral layers of different topology10Efficient tetracycline adsorption and photocatalytic degradation of rhodamine B by uranyl coordination polymer49Morphotropy in alkaline uranyl methacrylate complexes9Syntheses, Crystal Structures, and Nonlinear Optical Activity of Cs 2 Ba[AnO 2 (C 2 H 5 COO) 3 ] 4 (An = U, Np, Pu) and Unprecedented Octanuclear Complex Units in KR 2 (H 2 O) 8 [UO 2 (C 2 H 5 COO) 3 ] 5 (R = Sr, Ba)21Syntheses, Structures, and Comparisons of Heterometallic Uranyl Iodobenzoates with Monovalent Cations27Mild Periodic Acid Flux and Hydrothermal Methods for the Synthesis of Crystalline f-Element-Bearing Iodate Compounds20Divergent Structural Chemistry of Uranyl Borates Obtained from Solid State and Hydrothermal Conditions19Interpenetrated Uranyl–Organic Frameworks with bor and pts Topology: Structure, Spectroscopy, and Computation40A hydrolytically stable uranyl organic framework for highly sensitive and selective detection of Fe 3+ in aqueous media70Heat capacity, thermal expansion, and thermal diffusivity of NaUO2BO32An Anionic Uranium-Based Metal–Organic Framework with Ultralarge Nanocages for Selective Dye Adsorption67Na2(UO2)(BO3): An All-Uranium(V) Borate Synthesized under Mild Hydrothermal Conditions18Conformational 2-Fold Interpenetrated Uranyl Supramolecular Isomers Based on (6,3) Sheet Topology: Structure, Luminescence, and Ion Exchange37Flux crystal growth: a versatile technique to reveal the crystal chemistry of complex uranium oxides49Multi-colour uranyl emission efficiently tuned by hexacyanidometallates within hybrid coordination frameworks37Overview of nuclear waste treatment and management5Inorganic X-ray Scintillators Based on a Previously Unnoticed but Intrinsically Advantageous Metal Center17Speciation Change of Uranyl in Lithium Borate Glasses31Mg3Pt(BO3)2O2: The first platinum borate from the flux technique13Introducing Uranium as the Activator toward Highly Stable Narrow-Band Green Emitters with Near-Unity Quantum Efficiency35Occurrence of polyoxouranium motifs in uranyl organic networks constructed by using silicon-centered carboxylate linkers: structures, spectroscopy and computation11Crystal Growth of Alkali Uranyl Borates from Molten Salt Fluxes: Characterization and Ion Exchange Behavior of A2(UO2)B2O5 (A = Cs, Rb, K)13Borates: A Rich Source for Optical Materials1090Alkali Uranyl Borates: Bond Length, Equatorial Coordination and 5f States11Hydrothermal Synthesis and Structural Investigation of a Crystalline Uranyl Borosilicate3Спектроскопическое исследование структурных и магнитных свойств TbCr-=SUB=-3-=/SUB=-(BO-=SUB=-3-=/SUB=-)-=SUB=-4-=/SUB=-0Synthetic uranium oxide hydrate materials: Current advances and future perspectives30Progress in solid state and coordination chemistry of actinides in China5Energy–structure–property relationships in uranium metal–organic frameworks32Flux Crystal Growth of the Extended Structure Pu(V) Borate Na2(PuO2)(BO3)11Constructing stable uranyl-copper(II) bimetallic organic frameworks using rigid thiophenedicarboxylic acid1Structural variation in Uranyl-Phosphonate networks utilizing tetrahedral Silicon-Centered phosphonate linkers2Spectroscopic Investigation of Structural and Magnetic Properties of TbCr3(BO3)43Molecular properties in the linear response regime and beyond with relativistic coupled-cluster0Frequency-Dependent Quadratic Response Properties and Two-Photon Absorption from Relativistic Equation-of-Motion Coupled Cluster Theory6Molecular properties in the linear response regime and beyond with relativistic coupled-cluster0Arene-, Chlorido-, and Imido-Uranium Bis- and Tris(boryloxide) Complexes5Mild Hydrothermal Crystal Growth of Two Luminescing Uranyl Phosphates Exhibiting an Autunite-Type Sheet Structure3Extending the Chemistry of Scheelite‐type Oxides with Borates8Extending the Chemistry of Scheelite‐type Oxides with Borates2Unveiling the hidden risk: Cryo-TRLFS identifies critically elusive UO2 alteration phases under chemically complex conditions1

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  1. Cubic and rhombohedral heterobimetallic networks constructed from uranium, transition metals, and phosphonoacetate: new methods for constructing porous materials

    Chemical Communications · 2010-01-01

    A.N. Alsobrook, Brad G. Hauser, Joseph T. Hupp, Evgeny V. Alekseev, Wulf Depmeier, Thomas E. Albrecht‐Schmitt

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  2. Further insights into intermediate- and mixed-valency in neptunium oxoanion compounds: structure and absorption spectroscopy of K2[(NpO2)3B10O16(OH)2(NO3)2]

    Chemical Communications · 2010-01-01

    Shuao Wang, Evgeny V. Alekseev, Wulf Depmeier, Thomas E. Albrecht‐Schmitt

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  3. Comparison of Thorium(IV) and Uranium(VI) Carboxyphosphonates

    Inorganic Chemistry · 2010-05-13

    Pius O. Adelani, Thomas E. Albrecht‐Schmitt

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  4. Crystal Chemistry of the Potassium and Rubidium Uranyl Borate Families Derived from Boric Acid Fluxes

    Inorganic Chemistry · 2010-06-18

    Shuao Wang, Evgeny V. Alekseev, Jared T. Stritzinger, Wulf Depmeier, Thomas E. Albrecht‐Schmitt

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  5. ChemInform Abstract: Polarity and Chirality in Uranyl Borates: Insights into Understanding the Vitrification of Nuclear Waste and the Development of Nonlinear Optical Materials.

    ChemInform · 2010-07-24

    Shuao Wang, Evgeny V. Alekseev, Jie Ling, Guokui Liu, Wulf Depmeier, Thomas E. Albrecht‐Schmitt

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  6. Boronic Acid Flux Synthesis and Crystal Growth of Uranium and Neptunium Boronates and Borates: A Low-Temperature Route to the First Neptunium(V) Borate

    Inorganic Chemistry · 2010-10-04

    Shuao Wang, Evgeny V. Alekseev, Hannah Marie Miller, Wulf Depmeier, Thomas E. Albrecht‐Schmitt

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  7. Structure−Property Relationships in Lithium, Silver, and Cesium Uranyl Borates

    Chemistry of Materials · 2010-10-13

    Shuao Wang, Evgeny V. Alekseev, Jared T. Stritzinger, Guokui Liu, Wulf Depmeier, Thomas E. Albrecht‐Schmitt

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  8. Synthesis, structural and emission studies of a bis (carbamoyl methyl) sulfone complex of uranyl nitrate

    Inorganic Chemistry Communications · 2010-10-31

    Shanmugaperumal Kannan, Sadhan Bijoy Deb, M.G.B. Drew

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  9. Recent progress in actinide borate chemistry

    Chemical Communications · 2011-01-01

    Shuao Wang, Evgeny V. Alekseev, Wulf Depmeier, Thomas E. Albrecht‐Schmitt

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  10. Role of Anions and Reaction Conditions in the Preparation of Uranium(VI), Neptunium(VI), and Plutonium(VI) Borates

    Inorganic Chemistry · 2011-02-03

    Shuao Wang, Eric M. Villa, Juan Diwu, Evgeny V. Alekseev, Wulf Depmeier, Thomas E. Albrecht‐Schmitt

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  11. From Layered Structures to Cubic Frameworks: Expanding the Structural Diversity of Uranyl Carboxyphosphonates via the Incorporation of Cobalt

    Crystal Growth & Design · 2011-02-08

    A.N. Alsobrook, Brad G. Hauser, Joseph T. Hupp, Evgeny V. Alekseev, Wulf Depmeier, Thomas E. Albrecht‐Schmitt

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  12. Surprising Coordination for Plutonium in the First Plutonium(III) Borate

    Inorganic Chemistry · 2011-02-22

    Shuao Wang, Evgeny V. Alekseev, Wulf Depmeier, Thomas E. Albrecht‐Schmitt

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  13. Hydrothermal Synthesis and Structural Characterization of Organically Templated Uranyl Diphosphonate Compounds

    Crystal Growth & Design · 2011-03-09

    Pius O. Adelani, Allen G. Oliver, Thomas E. Albrecht‐Schmitt

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  14. Uranyl carboxyphosphonates that incorporate Cd(II)

    Journal of Solid State Chemistry · 2011-04-14

    A.N. Alsobrook, Evgeny V. Alekseev, Wulf Depmeier, Thomas E. Albrecht‐Schmitt

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  15. K(NpO2)3(H2O)Cl4: A Channel Structure Assembled by Two- and Three-Center Cation–Cation Interactions of Neptunyl Cations

    Inorganic Chemistry · 2011-05-09

    Shuao Wang, Evgeny V. Alekseev, Wulf Depmeier, Thomas E. Albrecht‐Schmitt

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  16. Functionalization of Borate Networks by the Incorporation of Fluoride: Syntheses, Crystal Structures, and Nonlinear Optical Properties of Novel Actinide Fluoroborates

    Chemistry of Materials · 2011-05-13

    Shuao Wang, Evgeny V. Alekseev, Juan Diwu, Hannah Marie Miller, Allen G. Oliver, Guokui Liu, Wulf Depmeier, Thomas E. Albrecht‐Schmitt

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  17. Sr2[C6H3(CO2)3(NO3)]·DMF: One-Dimensional Nano-Channel in a New Non-Centrosymmetric Strontium–Organic Framework with High Thermal Stability

    Crystal Growth & Design · 2011-05-18

    Dong Woo Lee, Vinna Jo, Kang Min Ok

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  18. Structural Complexity of Barium Uranyl Arsenates: Synthesis, Structure, and Topology of Ba4[(UO2)2(As2O7)3], Ba3[(UO2)2(AsO4)2(As2O7)], and Ba5Ca[(UO2)8(AsO4)4O8]

    Crystal Growth & Design · 2011-05-30

    Evgeny V. Alekseev, Sergey V. Krivovichev, Wulf Depmeier

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  19. Incorporation of iodate into uranyl borates and its implication for the immobilization of 129I in nuclear waste repositories

    Radiochimica Acta · 2011-06-09

    Shijun Wu, Shuao Wang, Antonio Simonetti, Fanrong Chen, Thomas E. Albrecht‐Schmitt

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  20. Bonding Changes in Plutonium(III) and Americium(III) Borates

    Angewandte Chemie International Edition · 2011-08-18

    Matthew J. Polinski, Shuao Wang, Evgeny V. Alekseev, Wulf Depmeier, Thomas E. Albrecht‐Schmitt

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  21. Th2[BO4][PO4]: A RARE EXAMPLE OF AN ACTINIDE BORATE-PHOSPHATE

    The Canadian Mineralogist · 2011-10-01

    Colette B. Lipp, Peter Carman Burns

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  22. Interstitial Incorporation of Plutonium into a Low-Dimensional Potassium Borate

    Environmental Science & Technology · 2011-10-03

    Shuao Wang, Juan Diwu, Antonio Simonetti, Corwin H. Booth, Thomas E. Albrecht‐Schmitt

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  23. New Neptunium(V) Borates That Exhibit the Alexandrite Effect

    Inorganic Chemistry · 2011-12-06

    Shuao Wang, Evgeny V. Alekseev, Wulf Depmeier, Thomas E. Albrecht‐Schmitt

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  24. Complex clover cross-sectioned nanotubules exist in the structure of the first uranium borate phosphate

    Chemical Communications · 2012-01-01

    Shijun Wu, Shuao Wang, Juan Diwu, Wulf Depmeier, Thomas Malcherek, Evgeny V. Alekseev, Thomas E. Albrecht‐Schmitt

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  25. In-Situ Raman Spectroscopy Studies of Room-Temperature and Hydrothermal Reactions

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  26. 3-Fold-Interpenetrated Uranium–Organic Frameworks: New Strategy for Rationally Constructing Three-Dimensional Uranyl Organic Materials

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  27. Steric Effects on Uranyl Complexation: Synthetic, Structural, and Theoretical Studies of Carbamoyl Pyrazole Compounds of the Uranyl(VI) Ion

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  28. Barium uranyl diphosphonates

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  29. Differentiating between Trivalent Lanthanides and Actinides

    Journal of the American Chemical Society · 2012-05-29

    Matthew J. Polinski, Daniel J. Grant, Shuao Wang, Evgeny V. Alekseev, Justin N. Cross, Eric M. Villa, Wulf Depmeier, Laura Gagliardi, Thomas E. Albrecht‐Schmitt

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  30. Syntheses, structures and luminescent properties of two one-dimensional uranium oxyfluorides

    Inorganic Chemistry Communications · 2012-06-12

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  31. Tailor-Made Zinc Uranyl Diphosphonates from Layered to Framework Structures

    Crystal Growth & Design · 2012-08-02

    Hongyue Wu, Weiting Yang, Zhong‐Ming Sun

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  32. Effect of pH and Reaction Time on the Structures of Early Lanthanide(III) Borate Perchlorates

    Inorganic Chemistry · 2012-10-09

    Matthew J. Polinski, Shuao Wang, Evgeny V. Alekseev, Justin N. Cross, Wulf Depmeier, Thomas E. Albrecht‐Schmitt

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  33. Elucidation of Tetraboric Acid with a New Borate Fundamental Building Block in a Chiral Uranyl Fluoroborate

    Inorganic Chemistry · 2012-10-22

    Shuao Wang, T. Gannon Parker, Daniel J. Grant, Juan Diwu, Evgeny V. Alekseev, Wulf Depmeier, Laura Gagliardi, Thomas E. Albrecht‐Schmitt

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  34. From 1D Chain to 3D Framework Uranyl Diphosphonates: Syntheses, Crystal Structures, and Selective Ion Exchange

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  35. Bisactinyl halogenated complexes: relativistic density functional theory calculation and experimental synthesis

    RSC Advances · 2012-11-14

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  36. Crystal Chemistry of Uranium Oxides and Minerals

    Elsevier eBooks · 2013-01-01

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  37. Mono- and dinuclear uranyl(VI) complexes with chiral Schiff base ligand

    Inorganica Chimica Acta · 2013-01-06

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  38. Uranium(VI) solubility in carbonate-free WIPP brine

    Radiochimica Acta · 2013-03-19

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  39. High Structural Complexity of Potassium Uranyl Borates Derived from High-Temperature/High-Pressure Reactions

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  40. Facile Assembly of an Unusual Lead Borate with Different Cluster Building Units via a Hydrothermal Process

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  41. Novel Fundamental Building Blocks and Site Dependent Isomorphism in the First Actinide Borophosphates

    Inorganic Chemistry · 2013-07-03

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  42. Dissolution of uranyl and plutonyl borates: Influences of crystalline structures and aqueous ligands

    Chemical Geology · 2013-08-28

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  43. MOFs of Uranium and the Actinides

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  44. Two New Barium Borate Fluorides ABa12(BO3)7F4 (A = Li and Na)

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  45. Synthetic, structural, extraction and theoretical studies of uranyl nitrate dithio-diglycolamide compounds

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  46. Tris(acrylato)uranylates as a scaffold for NLO materials

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  47. Beryllium-free Li4Sr(BO3)2 for deep-ultraviolet nonlinear optical applications

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  48. Highly Distorted Uranyl Ion Coordination and One/Two-Dimensional Structural Relationship in the Ba2[UO2(TO4)2] (T = P, As) System: An Experimental and Computational Study

    Inorganic Chemistry · 2014-07-03

    Shijun Wu, Piotr M. Kowalski, Na Yu, Thomas Malcherek, Wulf Depmeier, Dirk Bosbach, Shuao Wang, Evgeny V. Suleimanov, Thomas E. Albrecht‐Schmitt, Evgeny V. Alekseev

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  49. Microbial dissolution and reduction of uranyl crystals by Shewanella oneidensis MR-1

    Chemical Geology · 2014-08-28

    Yu Yang, Shuao Wang, Thomas E. Albrecht‐Schmitt

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  50. Design, synthesis and structure of uranyl coordination polymers from 2-D layer to 3-D network structure

    Journal of Coordination Chemistry · 2014-11-27

    Si Yue Wei, Feng‐Ying Bai, Ya Nan Hou, Xiao Xi Zhang, Xue Ting Xu, Ji Xiao Wang, Huan Zhi Zhang, Yong‐Heng Xing

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