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RESEARCH PAPER · Advanced Materials · 2025

Advanced Catalysts for the Chemical Recycling of Plastic Waste

Jibo Qin, Feiyan Wu, Yibo Dou, Dan Zhao, Claus Hélix‐Nielsen, Wenjing Angela Zhang

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Advanced Catalysts for the Chemical Recycling of Plastic WasteOriginalA revolutionary paradigm in chemistry and materials science research: self-driving laboratories8Electrothermal upcycling of plastic waste18Turning plastic trash into Energy: Converted MOFs and carbon for energy storage18NaOH-Catalyzed Alcoholysis of Polylactide7Microwave-Assisted Catalytic Upcycling of Plastic Wastes over Heterojunction-Structured Layered Triple Oxides8Transforming waste to energy: nanocatalyst innovations driving green hydrogen production22Mixed plastics turned into valuable chemicals1Solar-driven plastic waste conversion: A mini-review on photoreforming for Co-producing hydrogen and chemical feedstocks7Upcycling waste plastics into hierarchically ordered macro/meso-microporous carbon-encapsulated FeNi alloy for efficient periodate oxidation4Industrial-grade electrocatalytic valorization of waste plastics via reconstructed Ni 2+ -CoOOH nanosheet arrays55NiFe-Loaded Self-Supporting Carbon Nanotubes Electrode for Hydrogen Evolution Reaction Via in Situ Catalytic Carbonization of Waste Polypropylene0Upcycling waste plastics into monolithic catalysts for micropollutant removal via dual-pathway peroxymonosulfate activation9Zinc oxide-mediated C H activation of polypropylene waste for thermochemical valorization1AI-accelerated innovations in photodegradation and depolymerization of waste plastics: a critical review on mechanistic insights, environmental impact, and future perspectives6Zn Gallate Catalysts Activated in Nanoporous Silica Nanoparticles for the Depolymerization of Poly(propylene carbonate) to Cyclic Carbonate under Mild Conditions1Lanthanide contraction effect of PdPr nanosheets boosting PET electrocatalytic value‐added conversion3Toward Sustainable Plastic Waste Valorization: Green Synergistic Catalytic Strategies for Plastic Upcycling12Plasma Catalysis for Plastic Waste Conversion into Value‐Added Products: Advancements and Perspectives11Recent advances in chemical upcycling of plastic waste: microwave-assisted heating and heterogeneous catalysis11Transforming Waste Polyvinyl Chloride into Strong Adhesives by NiCl 2 ‐Catalyzed Amination at Near‐Ambient Temperature0A review of recent advances in thermal-catalytic cracking of plastic waste8Energy‐Saving Microwave‐Assisted Catalysis Over SiC@NiFe for Selective Valorization of Plastic Wastes Into H 2 and Carbon Nanotubes4Tandem depolymerization-electrocatalysis for plastic waste upcycling6Advances and Insights in Electrocatalytic Upcycling of Polyethylene Terephthalate Plastic Wastes23Electrochemical recovery and regeneration of polyethylene terephthalate materials7Waste PVC-derived Co-N-C catalysts for antibiotic degradation via non-radical PMS activation: Synthesis and mechanism of singlet oxygen generation5Promoting effects of gaseous CO2 and supercritical CO2 on the degradation of plastics: A review2Spinel NiCo2O4@CeO2-x/NF with abundant oxygen vacancies and heterogeneous interfaces for efficient polyethylene terephthalate electrocatalytic conversion2Photothermal Revolution in Plastic Upcycling24Beyond mechanical recycling: artificial photosynthesis enables polyester plastic upcycling into valuable chemicals5Catalytic transfer reductive conversion of plastic wastes into fuel and chemicals0Highly efficient photoreforming of plastic waste for hydrogen production: recent advances and prospects1Highly selective hydrocracking of polypropylene to gasoline-range fuels over the Pt/MCM-22 catalyst0Integration of Transport, Energy, and Materials Based on Immunological Insights1Microwave-assisted catalytic upcycling of medical polypropylene to BTX aromatics under mild conditions0Tailoring surface chemistry via Cr doping: modulating Ni(OH) 2 for high-efficiency electrocatalytic plastic upcycling0Structurally Tuned Citric Acid–Based Polyester Thermoset with Balanced Barrier, Durability, and Biodegradation Performance1Engineering Microporous Zn-Functionalized Carbon Catalysts for Controllable Chain Cracking and Aromatization in Polyethylene Upcycling1A dual-function bio-crosslinked recyclable thermosetting polyimide integrating strong adhesion and lubrication1Acid Site Engineering of Ni/BEA Zeolites Enables Efficient Upcycling of Polyolefin Plastics to Liquid Fuels1Synergistic bifunctional catalysis and plasma activation for valorizing polypropylene and CO2 to gasoline-range olefins1Thermo-chemical upgrading of waste polyethylene and polypropylene plastics0Perovskite oxide catalysts: Molecular-level design, structure–activity relationships, and reaction mechanisms0Enhancing carbon nanotubes production from pyrolysis–catalysis of plastic waste through monolithic heating18Efficient degradation of polycarbonate via collaborative alcoholysis and hydrolysis1Simultaneous Determination of Halogens and Metals in Waste Plastic Pyrolysis Oil by Inductively Coupled Plasma Mass Spectrometry0Bioinspired Design of F–Zn Sites in Layered Double Hydroxides for Photothermal Catalytic Upcycling of Polyethylene Terephthalate9Bioinspired Design of F–Zn Sites in Layered Double Hydroxides for Photothermal Catalytic Upcycling of Polyethylene Terephthalate0Catalytic Upcycling of Polyolefins and Polystyrene: Integrating Active Site Design With Mass Transfer Considerations4Bismuth-based oxides in piezocatalysis: Structure, mechanism, and multifunctional applications2Dynamic imine network-enabled thermal processable and degradable cellulose-based bioplastics5Engineering Interfacial Compatibility and Dynamic Active Hydrogen Pools to Accelerate Polyolefin Hydrogenolysis0Opportunities and challenges in sustainable solar fuel production from plastics0Plastic wastes facilitate Co-Mo bimetallic bond formation for selective 1O2 generation and sustainable water decontamination1A Panoramic View on Plastic Waste Recycling and Upcycling: Heterogeneous Catalytic Strategies for Diverse Plastics and Multiple Pathways6Mass transfer during HDPE autoxidation and the use of expanded bed reactor0Amyloid‐Like Protein Assembly‐Driven Functional Materials for Enabling the Sustainable Development of Light Industry1Dual redox shuttles drive efficient succinic acid electrosynthesis from plastic and biowaste1Solvent‐ and Hydrogen‐Free Upcycling of Polystyrene by Layered Double Oxides0Well‐Defined Heterocatalysts for Plastic Upcycling: From Design to Applications3Enhanced Seawater High‐Purity Uranium Extraction Coupled With Microplastic Degradation by Quaternary Amine Tuned Microenvironment of COFs0Ultrasonic Vibration‐Driven Cold Upcycling of Waste Plastics: Enabling High‐Efficiency Seawater Distillation0Waste plastic recycling and upgrading via electro- and photocatalytic C−X bond coupling1Co 1 /Ru Single‐Atom Alloy Catalyst for Sustainable Polypropylene Hydrogenolysis to Long‐Chain Liquid Products1Strategies to Improve the Compatibility of Polyethylene Terephthalate and Polyethylene Blends0Light‐Driven Coupled Upcycling of Polyethylene and CO 2 to Aromatics over Zeolite–Ni/CeO 2 Composite Catalysts0Electrothermal Strategies for Upcycling Commodity Plastics0Upcycling Real‐World Post‐Consumer Polyolefins Plastics Into Light Olefins Via Microwave‐Assisted Processing0Efficient electrosynthesis of ammonium formate from nitrate and PET waste over a Cu-doped CoP0Intramolecularly Synergic Catalysis Enables Efficient Closed‐Loop Recycling of Polyesters and Polycarbonates0Intramolecularly Synergic Catalysis Enables Efficient Closed‐Loop Recycling of Polyesters and Polycarbonates0Efficient and mild hydrogenolysis of polyethylene terephthalate to terephthalic acid over a Ni cluster catalyst0Experimental Investigation of Recycling of MLP and LDPE Plastic Waste into Cofiring Fuel and Sustainable Materials0Photoreforming and Photoelectroreforming of Waste‐Derived Feedstocks for Solar‐Driven Production of Fuels and Chemicals0Spatial Confinement Nanoreactors Enable Synergistic Catalysis for Polyethylene Terephthalate-Derived Ethylene Glycol Oxidation0Sustainable hydrogen production from aluminium waste: Reactor technologies, environmental benefits, and system‐level integration0Integrating S-scheme Heterojunctions and Photothermal Effects for Enhanced Solar-Driven Catalysis10Chemical Recycling of Polyester Wastes: Emerging Upcycling Technologies, Fundamental Mechanisms, Process Analysis, and Machine Learning1Electro‐ and Photocatalytic C─X Bond Coupling in Valorization of Waste Plastics/Biomass: Reaction Mechanism and Catalyst Engineering1Solar‐Driven Upcycling of Waste Polyethylene Terephthalate0Defect‐Engineered Microwave‐Responsive Ni@C Composites From Waste PET for Catalytic Plastic Upcycling0Constructing Ultrafine Ru Nanoclusters via a Dual‐Confinement Strategy: Synergizing Hierarchical Pores and Electronic Modulation for Efficient Lignin Hydrogenolysis0High-strength thermo-moldable cellulose-based bioplastics for sustainable 3D structured materials0Electron‐Extracting Pd Single Atoms Arrest Solar Photooxidative Upcycling of Waste Polyesters at Glycolaldehyde0Upcycling Post-Consumer Plastic Waste into Electrospun Nanofibrous Separators for Sustainable Energy Storage0Upcycling of Mixed Polyolefins via a Grafting-Dynamic Cross-Linking Strategy0Selective polypropylene recovery from a model PP/PET mixture via thermally induced phase separation and its upcycling into multifunctional porous materials0Catalytic upcycling of plastic waste under electromagnetic fields0Hydroplastic polyamides with high moisture resistance and fast water absorption enabled by sulfone interactions0Artificial Photoreforming Technology for Plastic Waste Valorization0

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  8. Solar-driven plastic waste conversion: A mini-review on photoreforming for Co-producing hydrogen and chemical feedstocks

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