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RESEARCH PAPER · Nature Sustainability · 2024

Chain-length-controllable upcycling of polyolefins to sulfate detergents

Nuwayo Eric Munyaneza, Ruiyang Ji, Adrian DiMarco, Joel Miscall, Lisa Stanley, Nicholas A. Rorrer, Rui Qiao, Guoliang Liu

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Chain-length-controllable upcycling of polyolefins to sulfate detergentsOriginalUpcycling of polyolefins into detergents2Upcycling of poly(ethylene terephthalate) waste plastics to terephthalonitrile6Anionic Surfactants from Reactive Separation of Hydrocarbons Derived from Polyethylene Upcycling8Advances and Challenges in Low‐Temperature Upcycling of Waste Polyolefins via Tandem Catalysis25Advances and Challenges in Low‐Temperature Upcycling of Waste Polyolefins via Tandem Catalysis2Upgrading polyolefin plastics: experiences from petroleum refining and distinct characteristics19Hydrocracking of Polyethylene to Gasoline-Range Hydrocarbons over a Ruthenium-Zeolite Bifunctional Catalyst System with Optimal Synergy of Metal and Acid Sites9Relay Catalysis Enabling the Value‐Added Upgrading of Plastic Wastes2Pore‐Gradient, Flexible, and Fully‐Degradable Foam with Outstanding Noise Absorption and Thermal Insulation13Synergistic Co‐Recycling: Selective Oxidation of Polyethylene to Dicarboxylic Acids over Spent LiCoO 2 Cathodes22Synergistic Co‐Recycling: Selective Oxidation of Polyethylene to Dicarboxylic Acids over Spent LiCoO 2 Cathodes3Electrochemical Degradation of Plastic Waste Coupled with Hydrogen Evolution in Seawater Using Rosette‐Like High‐Entropy Oxides13Mechanistic alteration of polyethylene oxidation via heterogenous catalysis for enhanced fatty di-carboxylic acid yields6Circular economy strategies for converting waste plastics into surfactants633 Unresolved Questions in Nanoscience and Nanotechnology57Pyrolysis kinetics, volatile evolution, and backbone degradation mechanisms of typical nitrogen-containing plastics based on TG-FTIR-GC/MS and density functional theory8Deep cracking of polyethylene to light olefins0Advancing chemical recycling for waste plastic conversion1Well-defined polysaccharide graft (Co)polymers: Synthesis, applications, and structure-property relationships3Laser-induced pyrolysis of waste polyethylene to long-chain terminal alkenes and amphiphilic functionalization for anti-fouling film application0Fractionated degradation and valorization of polypropylene waste into sulfonate surfactants2Transforming Waste Cooking Oil into Linear and Branched Polyethylene Mimics9Thermodynamically driven closed-loop recyclable bridged polymers: from molecular design to high-performance materials0Chemical recycling of polyolefin wastes: recent advances and insights into recycling routes0Catalytic Oxidation of Commodity Plastics: Advances in Polyethylene and Polystyrene Valorization5Oligomeric surfactants facilitating superior cleaning with minimal foam1Contaminant-Tolerant Conversion of Polyethylene Waste to α-Olefins6Pyrolysis kinetics and backbone decomposition mechanisms of nylon 6/6: insights from TG-FTIR-GC/MS and density functional theory0Dynamic decrosslinking enables self-healing, reprocessability, and upcycling in polyurethane networks13Thermoplastic elastomer foams: Anti-shrinkage strategies toward dimensionally stable lightweight materials3Taming Sulfate Radical for Anti-Markovnikov Alkene Hydrosulfation2Electrochemically mediated disproportionation for selective formaldehyde upcycling in acid2Oxidative Extrusion of Polypropylene Melts: Impact of Chain-End and In-Chain Functionalization on Thermal Properties, Crystal Structure, and Crystallization Kinetics1Selective solar wax refining with nanoscale zero-valent iron1Recent advances in the directed degradation of polyolefins into oligomers0Synthesis of bimetallic Mn–Co stearate catalyst for the conversion of plastic waste to surfactant via chemical upcycling and its application1Highly Selective Conversion of Polyolefins to Methane via Mechanochemical Hydrogenolysis0Selective Oxidative Upcycling of Polyethylene Pyrolyzed Wax to High‐Performance Surfactants Using Synthesized Co and Mn–Co Stearate Catalysts0Upcycling of polyvinyl chloride into polyalphaolefin lubricants0Deep aromatic reduction in linear alkylbenzene raffinate by hydrodearomatization using Ni-based catalysts for jet and rocket fuel applications0Solar-driven programmable polystyrene upcycling to aromatic hydrocarbons via plasmonic iron nanoparticles0

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  1. Upcycling of polyolefins into detergents

    Nature Sustainability · 2024-11-18

    Fei Huang, Fan Zhang

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  2. Upcycling of poly(ethylene terephthalate) waste plastics to terephthalonitrile

    Green Chemistry · 2025-01-01

    Phuc T.T. Nguyen, Jiong Cheng, Junyu Mi, Ning Yan

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  3. Anionic Surfactants from Reactive Separation of Hydrocarbons Derived from Polyethylene Upcycling

    Langmuir · 2025-02-04

    Yu-Hsuan Lee, Alexandra Heuston, Enze Jin, Jia‐Kai Sun, Xichen Liang, Yangying Zhu, Matthew E. Helgeson, Eric R. Masanet, Susannah L. Scott, Mahdi M. Abu‐Omar

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  4. Advances and Challenges in Low‐Temperature Upcycling of Waste Polyolefins via Tandem Catalysis

    Angewandte Chemie International Edition · 2025-03-13

    Wei Zhang, Sung Min Kim, Michele L. Sarazen, Mingyuan He, Jingguang G. Chen, Johannes A. Lercher

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  5. Advances and Challenges in Low‐Temperature Upcycling of Waste Polyolefins via Tandem Catalysis

    Angewandte Chemie · 2025-03-13

    Wei Zhang, Sung Min Kim, Michele L. Sarazen, Mingyuan He, Jingguang G. Chen, Johannes A. Lercher

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  6. Upgrading polyolefin plastics: experiences from petroleum refining and distinct characteristics

    Science China Chemistry · 2025-03-19

    Rongxin Zhang, Guangchao Deng, Zhuoyang Jiang, Yiyi Fan, Yanqi Guo, Zhongwen Dong, Wenjun Chen, Bo Peng, Fan Zhang

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  7. Hydrocracking of Polyethylene to Gasoline-Range Hydrocarbons over a Ruthenium-Zeolite Bifunctional Catalyst System with Optimal Synergy of Metal and Acid Sites

    Catalysts · 2025-03-31

    Qing Bo Du, Xin Chun Shang, Yangyang Yuan, Xiong Su, Yanqiang Huang

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  8. Relay Catalysis Enabling the Value‐Added Upgrading of Plastic Wastes

    ChemCatChem · 2025-03-31

    Kaizhi Wang, Zehui Sun, Ting Yang, Wendi Guo, Feifan Gao, Mugeng Chen, Yongmei Liu, Heyong He, Yong Cao

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  9. Pore‐Gradient, Flexible, and Fully‐Degradable Foam with Outstanding Noise Absorption and Thermal Insulation

    Advanced Functional Materials · 2025-04-09

    Zhaozhi Wang, Guilong Wang, Zhaorui Xu, Chengyun Ma, Guoqun Zhao

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  10. Synergistic Co‐Recycling: Selective Oxidation of Polyethylene to Dicarboxylic Acids over Spent LiCoO 2 Cathodes

    Angewandte Chemie International Edition · 2025-04-15

    Shengming Li, Qianyue Feng, Qingye Li, Yeping Xie, Panpan Xu, Zhao Wang, Qiming Sun, Muhan Cao, Qiao Zhang, Jinxing Chen

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  11. Synergistic Co‐Recycling: Selective Oxidation of Polyethylene to Dicarboxylic Acids over Spent LiCoO 2 Cathodes

    Angewandte Chemie · 2025-04-15

    Shengming Li, Qianyue Feng, Qingye Li, Yeping Xie, Panpan Xu, Zhao Wang, Qiming Sun, Muhan Cao, Qiao Zhang, Jinxing Chen

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  12. Electrochemical Degradation of Plastic Waste Coupled with Hydrogen Evolution in Seawater Using Rosette‐Like High‐Entropy Oxides

    Advanced Science · 2025-07-02

    Zhenhao Xu, Yuchen Wang, Zhikeng Zheng, Xiaodie Zhang, Bin Liu, Karen Wilson, Kai Yan

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  13. Mechanistic alteration of polyethylene oxidation via heterogenous catalysis for enhanced fatty di-carboxylic acid yields

    Science China Chemistry · 2025-07-10

    Huidong Lv, Yi Ji, Wenjun Chen, Yuan Xiang, Yue Liu, Jianrong Zeng, Fei Huang, Fan Zhang

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  14. Circular economy strategies for converting waste plastics into surfactants

    Journal of environmental chemical engineering · 2025-08-29

    Muhammad Faizan, Abdul Aziz Jallow, Mohammad Nahid Siddiqui

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  15. 33 Unresolved Questions in Nanoscience and Nanotechnology

    ACS Nano · 2025-09-04

    Chad Alexander Mirkin, Sarah Hurst Petrosko, Natalie Artzi, Koray Aydın, Austin Biaggne, C. Jeffrey Brinker, Katherine E. Bujold, Y. Charles Cao, Rachel R. Chan, Chaojian Chen, Pengcheng Chen, Xiaodong Chen, Olivier J. G. L. Chevalier, Chung Hang Jonathan Choi, Richard M. Crooks, Vinayak P. Dravid, Jingshan S. Du, Sasha B. Ebrahimi, Hongyou Fan, Omar K. Farha, C. Adrian Figg, Tanner D. Fink, Connor M. Forsyth, Harald Fuchs, Franz M. Geiger, Nathan C. Gianneschi, Kyle J. Gibson, David S. Ginger, Sishi Guo, Justin S. Hanes, Liang Hao, Jin Shan Huang, Bryan Michael Hunter, Fengwei Huo, Jeongmin Hwang, Rongchao M. Jin, Shana O. Kelley, Thomas J. Kempa, Youngeun Kim, Sergej Kudruk, Sneha Kumari, Kaitlin M. Landy, Ki‐Bum Lee, Noel J. Leon, Jun Li, Yuanwei Li, Zhiwei Li, Bin Liu, Guoliang Liu, Xiaogang Liu, Luis M. Liz‐Marzán, Jochen H. Lorch, Taokun Luo, Robert J. Macfarlane, Jill E. Millstone, Milan Mrksich, Catherine Jones Murphy, Rajesh R. Naik, André E. Nel, Christopher Oetheimer, Jenny Orbeck, So‐Jung Park, Benjamin E. Partridge, Nicholas A. Peppas, Michelle L. Personick, Arindam Raj, Namrata Ramani, Michael B. Ross, Susan E. Ross, Edward Hartley Sargent, Tanushri Sengupta, George Chappell Schatz, Dwight S. Seferos, Tamar Seideman, Soyoung E. Seo, Bo Shen, Wooyoung Shim, Donghoon Shin, Ulrich Simon, Andrew J. Sinegra, Peter T. Smith, Alexander M. Spokoyny, Peter J. Stang, Alexander H. Stegh, James Fraser Stoddart, Dayne F. Swearer, Weihong Tan, Michelle H. Teplensky, Colby Shad Thaxton, David R. Walt, Mary X. Wang, Zhe Wang, Wei David Wei, Paul S. Weiss, Peter H. Winegar, Younan Xia, Yi Xie, Xiaoyang Xu, Peidong Yang, Yiming Yang

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  16. Pyrolysis kinetics, volatile evolution, and backbone degradation mechanisms of typical nitrogen-containing plastics based on TG-FTIR-GC/MS and density functional theory

    Journal of Analytical and Applied Pyrolysis · 2025-10-04

    Donghua Xu, Yibing Wei, Haoyu Xiao, Tengyue Zhang, Zichun Sheng, Haiping Yang, Yingquan Chen, Xianhua Wang, Hanping Chen

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  17. Deep cracking of polyethylene to light olefins

    Nature Chemical Engineering · 2025-10-14

    Guoliang Liu

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  18. Advancing chemical recycling for waste plastic conversion

    Cell Reports Physical Science · 2025-10-21

    Meng Zhang, Yadong Wu

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  19. Well-defined polysaccharide graft (Co)polymers: Synthesis, applications, and structure-property relationships

    Progress in Polymer Science · 2025-11-20

    Jeffrey E. Thompson, John B. Matson, Kevin J. Edgar

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  20. Laser-induced pyrolysis of waste polyethylene to long-chain terminal alkenes and amphiphilic functionalization for anti-fouling film application

    Sustainable materials and technologies · 2025-11-21

    Lun Chen, Fu‐Lu Chang, Zi‐Yang Hua, Fu-Rui Chen, Han Earl Yang, Sheng Wang, Xianwu Cao, Xiaochun Yin, Guangjian He

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  21. Fractionated degradation and valorization of polypropylene waste into sulfonate surfactants

    Nature Communications · 2025-11-25

    Zhen Xu, Yang Zhang, Tao Wang, Rong Yang, Hao Sun, Meiling Chen, Feng Liu, Jianjun Xu, Kai‐Jie Chen, Qikun Zhang, Fuping Pan

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  22. Transforming Waste Cooking Oil into Linear and Branched Polyethylene Mimics

    Journal of the American Chemical Society · 2025-11-28

    Nagarjuna A. Mahadas, Lucas A. H. Sanchez, Amir Suhail, Jacob Price, Arefin M. Anik, Matthew W. Kanan, Olga Kuksenok, Chuanbing Tang

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  23. Thermodynamically driven closed-loop recyclable bridged polymers: from molecular design to high-performance materials

    Scientia Sinica Chimica · 2025-12-04

    Xiangyu Miao, Wencan Li, Changxia Shi

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  24. Chemical recycling of polyolefin wastes: recent advances and insights into recycling routes

    Scientia Sinica Chimica · 2025-12-10

    Sen Wang, Qingyue Wang, Weiqiang Gao, Yinlong Chang, Jijiang Hu, Pingwei Liu, Wen-Jun Wang, Bo-Geng Li

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  25. Catalytic Oxidation of Commodity Plastics: Advances in Polyethylene and Polystyrene Valorization

    Chemistry - A European Journal · 2025-12-12

    Shuhua Chen, Yeping Xie, Shengming Li, Jinxing Chen

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  26. Oligomeric surfactants facilitating superior cleaning with minimal foam

    Chemical Engineering Journal · 2025-12-29

    Fulin Qiao, Tengda Wang, Zeyu Zhao, Ziqi Zhang, Jie Wang, Bing Qin, Jianlin Jiang, Lili Zhou, Yaxun Fan, Yilin Wang

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  27. Contaminant-Tolerant Conversion of Polyethylene Waste to α-Olefins

    ACS Sustainable Chemistry & Engineering · 2026-01-01

    Carlos Posada, Hongwei Sun, Adrian DiMarco, Nuwayo Eric Munyaneza, Oscar Valenzuela, Candace E. Wall, Guoliang Liu

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  28. Pyrolysis kinetics and backbone decomposition mechanisms of nylon 6/6: insights from TG-FTIR-GC/MS and density functional theory

    Progress in Reaction Kinetics and Mechanism · 2026-01-01

    Donghua Xu, Haoyu Xiao, Shengwei Feng, Yingquan Chen, Xianhua Wang, Hanping Chen, Haiping Yang

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  29. Dynamic decrosslinking enables self-healing, reprocessability, and upcycling in polyurethane networks

    Nature Communications · 2026-01-06

    Qingming Kong, Yu Tan, Kaiqiang Zhang, Haiyang Zhang, Tengyang Zhu, Xu Wang

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  30. Thermoplastic elastomer foams: Anti-shrinkage strategies toward dimensionally stable lightweight materials

    Composites Part B Engineering · 2026-01-19

    Qiqi Sun, Yang Sun, Xiaoyu Zhang, Zhaozhi Wang

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  31. Taming Sulfate Radical for Anti-Markovnikov Alkene Hydrosulfation

    Journal of the American Chemical Society · 2026-02-13

    Zeting Zhang, Pingping Yu, Chunlan Song, Jiakun Li

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  32. Electrochemically mediated disproportionation for selective formaldehyde upcycling in acid

    Nature Communications · 2026-03-18

    Yun Mi Song, Zhaohua Zhu, Tridip Das, Aarya D. Riasati, Jianjun Su, Weihua Guo, Yong Liu, Geng Li, Yinger Xin, Qiang Zhang, Mingming He, Ruixuan Wang, Rui Xue, Shenlong Zhao, Chuan Xia, Ben Zhong Tang, Marc Robert, Xin Wang, William A. Goddard, Ruquan Ye

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  33. Oxidative Extrusion of Polypropylene Melts: Impact of Chain-End and In-Chain Functionalization on Thermal Properties, Crystal Structure, and Crystallization Kinetics

    Macromolecules · 2026-03-30

    Ronard Herrera Monegro, Ioannis Mountziaris, Md Sifat Tanveer, Kira E. Gonzales, Shrishti Das, Sanat K. Kumar, Ramanan Krishnamoorti, Megan L. Robertson

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  34. Selective solar wax refining with nanoscale zero-valent iron

    Nature Communications · 2026-03-30

    Yifei Sun, Chengliang Mao, Yunjie Zou, Yuqing Hu, Di Yang, Junzhou Xu, Haopeng Pei, Yanbiao Shi, Z. D. Chen, Wendong Wei, Zhihui Ai, Lizhi Zhang

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  35. Recent advances in the directed degradation of polyolefins into oligomers

    Science China Chemistry · 2026-05-07

    Binzhi Zhao, Yi-Han Yu, Chaochun Wei, Ning Jiao

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  36. Synthesis of bimetallic Mn–Co stearate catalyst for the conversion of plastic waste to surfactant via chemical upcycling and its application

    Chemical Engineering Journal Advances · 2026-05-20

    Abdul Aziz Jallow, Usman Bello, Muhammad Faizan, Maryem Ourimi, Roa'a H. Alzoubi, Abdul Gani Abdul Jameel, Mohammad Nahid Siddiqui

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  37. Highly Selective Conversion of Polyolefins to Methane via Mechanochemical Hydrogenolysis

    ACS Sustainable Chemistry & Engineering · 2026-07-31

    Ruiqian Gu, Yue Ma, Yingnan Zhao, Rui‐Qi Yao, Tonghui Wang, Zi Wen, Gao‐Feng Han, Xingyou Lang, Qing Jiang

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  38. Selective Oxidative Upcycling of Polyethylene Pyrolyzed Wax to High‐Performance Surfactants Using Synthesized Co and Mn–Co Stearate Catalysts

    Advanced Sustainable Systems · 2026-08-01

    Abdul Aziz Jallow, Usman Bello, Muhammad Faizan, Roa'a H. Alzoubi, Maryem Ourimi, Abdul Gani Abdul Jameel, Usama Ahmed, Mohammad Nahid Siddiqui

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  39. Upcycling of polyvinyl chloride into polyalphaolefin lubricants

    Nature · 2026-08-05

    Nuwayo Eric Munyaneza, Connor Thompson, Abby Civiello, Adrian DiMarco, Jingtao Zhang, Seungjoo Lee, Gugyeong Sung, Tridip Das, Yue Zhang, Clark Vu, Shelby Koshak, John B. Matson, Ali Erdemir, William A. Goddard, Xi Chen, Guoliang Liu

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  40. Deep aromatic reduction in linear alkylbenzene raffinate by hydrodearomatization using Ni-based catalysts for jet and rocket fuel applications

    Fuel · 2026-08-14

    Alok Singh, Minakshi Garg, Savita Singh, Shailendra K. Singh

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  41. Solar-driven programmable polystyrene upcycling to aromatic hydrocarbons via plasmonic iron nanoparticles

    Applied Catalysis B: Environmental · 2026-08-23

    Yifei Sun, Xupeng Liu, Yuqing Hu, Di Yang, Zhihui Ai

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