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RESEARCH PAPER · Angewandte Chemie · 2022

An Optically Anisotropic Crystal with Large Birefringence Arising from Cooperative π Orbitals

Yanqiang Li, Xu Zhang, Zhou Yang, Weiqi Huang, Yipeng Song, Han Wang, Minjuan Li, Maochun Hong, Junhua Luo, Sangen Zhao

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An Optically Anisotropic Crystal with Large Birefringence Arising from Cooperative π OrbitalsOriginalA hybrid halide lead-free pseudo-perovskite with large birefringence37Discovery of SrZn 2 B 6 O 12 with an unprecedented quadruple-layered configuration0A Second‐Order Nonlinear Optical Material Consisting of Two π‐Conjugated Groups10Cd2Nb2Te4O15: A Novel Pseudo‐Aurivillius‐Type Tellurite with Unprecedented Nonlinear Optical Properties and Excellent Stability40Designing a Hybrid Perovskite with Enlarged Birefringence and Bandgap for Modulation of Light Polarization32A highly stable cerium–organic framework: an efficient catalyst for the cycloaddition of CO 2 and aziridines under mild-pressure6K 2 MgMoP 2 O 10 and K 3 Mg 2 MoP 3 O 14 : two new molybdophosphates exhibiting different optical anisotropies induced by variable dimensionality of the anion framework4Giant ab‐Plane Birefringence in Quasi‐1D Fibrous Red Phosphorus13Giant ab‐Plane Birefringence in Quasi‐1D Fibrous Red Phosphorus0Bi(SO4)F·H2O and Bi(SO4)(NO3)·3H2O: Chemical Substitution-Induced Birefringence Enhancement in Bismuth Sulfates6A novel sodium manganese fluorooxalate crystal Na2Mn2(C2O4)2.5F·2H2O: Synthesis, structure, optical and thermal properties2CdF(C 6 H 4 NO 2 )(H 2 O): a UV nonlinear optical material with unprecedented SHG and birefringence via π-conjugated rings and a unique “Warren truss structure”11Four noncentrosymmetric molybdophosphates discovered by a chemical substitution strategy4Realizing large birefringence via S-substitution and anisotropic arrangement optimization4Significant enhancement in the birefringence of metal phosphite halides via the introduction of π-conjugated cations17Unveiling two-photon absorption dynamic in melt grown 2,4-dihydroxybenzophenone (DHBP) single crystal: Insights from bridgman method using double-zone glass furnace0Five-Membered [C 5 O 5 ] 2 – Rings as Birefringence-Active Genes for Ultrabirefringent Crystals27Unveiling the Superior Birefringence Property of a Record‐Birefringent Crystal with Unique Building Block4(C 5 H 7 N 2 ) (C 8 H 4 O 4 ) PbBr: Jahn–Teller Distortion‐Induced Tilting of π‐Conjugated Planes Resolving the Second‐Order Polarizability–Structural Anisotropy Conflicts1Lock‐and‐Key Assembly Enables Record Birefringence in Monocyclic π‐Conjugated Crystals via Spatial Confinement of Linear Polyhalide0Designing Novel Solar‐Blind Ultraviolet Nonlinear Optical Crystals Based on Local Proton Distribution Complementary Effect0A Dynamic Hydrogen‐Bonded Organic Framework With Giant OFF–ON Birefringence0

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  1. A hybrid halide lead-free pseudo-perovskite with large birefringence

    Inorganic Chemistry Frontiers · 2023-01-01

    Weiqi Huang, Xiaolong Wu, Belal Ahmed, Yanqiang Li, Zhou Yang, Han Wang, Yipeng Song, Xiaojun Kuang, Junhua Luo, Sangen Zhao

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  2. Discovery of SrZn 2 B 6 O 12 with an unprecedented quadruple-layered configuration

    New Journal of Chemistry · 2023-01-01

    Xiangyu Long, Yan An Lv, Xueyan Wu

    Read original paper ↗ ·

  3. A Second‐Order Nonlinear Optical Material Consisting of Two π‐Conjugated Groups

    ChemPlusChem · 2023-03-01

    Minjuan Li, Ziyi Wang, Belal Ahmed, Yanqiang Li, Han Wang, Yipeng Song, Xianyu Song, Xiaojun Kuang, Junhua Luo, Sangen Zhao

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  4. Cd2Nb2Te4O15: A Novel Pseudo‐Aurivillius‐Type Tellurite with Unprecedented Nonlinear Optical Properties and Excellent Stability

    Small · 2023-05-28

    Qiang Wang, Xuehua Dong, Ling Huang, Kang Min Ok, Zhien Lin, Guohong Zou

    Read original paper ↗ ·

  5. Designing a Hybrid Perovskite with Enlarged Birefringence and Bandgap for Modulation of Light Polarization

    Small · 2023-10-20

    Weiqi Huang, Xianyu Song, Yanqiang Li, Zhou Yang, Qian-Ting Xu, Yipeng Song, Han Wang, Minjuan Li, Sangen Zhao, Junhua Luo

    Read original paper ↗ ·

  6. A highly stable cerium–organic framework: an efficient catalyst for the cycloaddition of CO 2 and aziridines under mild-pressure

    CrystEngComm · 2024-01-01

    Tong-Ji Liu, Hang Xu, Ying Shi, Bin Zhao

    Read original paper ↗ ·

  7. K 2 MgMoP 2 O 10 and K 3 Mg 2 MoP 3 O 14 : two new molybdophosphates exhibiting different optical anisotropies induced by variable dimensionality of the anion framework

    Dalton Transactions · 2024-01-01

    Zhixia Gao, Qiuyuan Feng, Juanjuan Lu, Hong Lei Du

    Read original paper ↗ ·

  8. Giant ab‐Plane Birefringence in Quasi‐1D Fibrous Red Phosphorus

    Angewandte Chemie International Edition · 2024-05-06

    Wu-Jia Chen, Bowen Zhang, Kezheng Tao, Qiang Li, Jia‐Lin Sun, Qingfeng Yan

    Read original paper ↗ ·

  9. Giant ab‐Plane Birefringence in Quasi‐1D Fibrous Red Phosphorus

    Angewandte Chemie · 2024-05-06

    Wujia Chen, Bowen Zhang, Kezheng Tao, Qiang Li, Jia‐Lin Sun, Qingfeng Yan

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  10. Bi(SO4)F·H2O and Bi(SO4)(NO3)·3H2O: Chemical Substitution-Induced Birefringence Enhancement in Bismuth Sulfates

    Inorganic Chemistry · 2024-07-04

    Jiachen Lu, Yang Li, Yunseung Kuk, Seung-Hun Choi, Kyungmo Kim, Chanhee Ko, Zhiyong Bai, Kang Min Ok

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  11. A novel sodium manganese fluorooxalate crystal Na2Mn2(C2O4)2.5F·2H2O: Synthesis, structure, optical and thermal properties

    Journal of Solid State Chemistry · 2024-09-27

    Sen Ji, Lei Kang, Yanyang Han, Shanshan Liu, Ye Liu, Ye Liu, Xin Yang, Kai Feng

    Read original paper ↗ ·

  12. CdF(C 6 H 4 NO 2 )(H 2 O): a UV nonlinear optical material with unprecedented SHG and birefringence via π-conjugated rings and a unique “Warren truss structure”

    Inorganic Chemistry Frontiers · 2025-01-01

    Jie Gou, Yaolong Zhu, Xin Su, Can Hui Yang, YunJie Wang, Qingwen Zhu, Yi Xiong, Qi Wu

    Read original paper ↗ ·

  13. Four noncentrosymmetric molybdophosphates discovered by a chemical substitution strategy

    Dalton Transactions · 2025-01-01

    Zhixia Gao, Ke Li, Hong Du, Tuohetijiang Baiheti

    Read original paper ↗ ·

  14. Realizing large birefringence via S-substitution and anisotropic arrangement optimization

    Inorganic Chemistry Frontiers · 2025-01-01

    Zhiwei Sun, Bingbing Wu, Zihao Yu, Qingran Ding, Yu‐Ling Wang, Ming Zhong, Sangen Zhao, Junhua Luo

    Read original paper ↗ ·

  15. Significant enhancement in the birefringence of metal phosphite halides via the introduction of π-conjugated cations

    Chemical Science · 2025-01-01

    Ru‐Ling Tang, Yue Wang, Yi‐Lei Lv, Bing-Wei Miao, Wenlong Liu, Sheng‐Ping Guo

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  16. Unveiling two-photon absorption dynamic in melt grown 2,4-dihydroxybenzophenone (DHBP) single crystal: Insights from bridgman method using double-zone glass furnace

    Optik · 2025-01-13

    Mohamad Asikali Abdul Hakkim, Rajesh Paulraj, T.C. Sabari Girisun

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  17. Five-Membered [C 5 O 5 ] 2 – Rings as Birefringence-Active Genes for Ultrabirefringent Crystals

    Journal of the American Chemical Society · 2025-09-16

    Jiachen Lu, Yang Li, Kang Min Ok

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  18. Unveiling the Superior Birefringence Property of a Record‐Birefringent Crystal with Unique Building Block

    Angewandte Chemie · 2026-01-27

    Kaijie Xie, Zhiyong Bai, Weiqi Huang, Ji Qi, Tingjuan Lin, Muhammad Zeeshan, Yanqiang Li, Yang Zhou, Junhua Luo, Sangen Zhao

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  19. (C 5 H 7 N 2 ) (C 8 H 4 O 4 ) PbBr: Jahn–Teller Distortion‐Induced Tilting of π‐Conjugated Planes Resolving the Second‐Order Polarizability–Structural Anisotropy Conflicts

    Angewandte Chemie · 2026-03-28

    Ming‐Yan Yu, Can Yang, Yun‐Jie Wang, Xin Yan Su, Jian Cui, Yao‐Long Zhu, Qing‐Wen Zhu, Qi Wu, Li‐Ming Wu, Ling Chen

    Read original paper ↗ ·

  20. Lock‐and‐Key Assembly Enables Record Birefringence in Monocyclic π‐Conjugated Crystals via Spatial Confinement of Linear Polyhalide

    Angewandte Chemie · 2026-05-26

    Yun‐Xia Hu, Huai Yu Wu, Jia‐jia Li, Ming‐Chang Wang, Jia‐Min Lian, Jin Yu Luo, Yiru Fu, Zi‐Yan Chen, Yang‐Hang Guo, Jin Chen, Ke‐Zhao Du

    Read original paper ↗ ·

  21. Designing Novel Solar‐Blind Ultraviolet Nonlinear Optical Crystals Based on Local Proton Distribution Complementary Effect

    Angewandte Chemie · 2026-08-11

    Hongyuan Sha, Dongling Yang, Lilin Yang, Fan Xiao, Xiaoming Yang, Lingfei Lv, Chao He, Zhihua Yang, Fangfang Zhang, Zujian Wang, Xifa Long

    Read original paper ↗ ·

  22. A Dynamic Hydrogen‐Bonded Organic Framework With Giant OFF–ON Birefringence

    Angewandte Chemie · 2026-09-04

    Christopher A.G. Halliwell, M.R.J. Elsegood, Qiang Zhu, Shaun Fowler, Sandra Míguez‐Lago, Kenny Jolley, Deobrat Singh, Raquel Lizárraga, Antonio Fernández

    Read original paper ↗ ·
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