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RESEARCH PAPER · Chemistry of Materials · 2022

Difluoro(oxalato)borates as Short-Wavelength Optical Crystals with Bifunctional [BF 2 C 2 O 4 ] Units

Congcong Jin, Fuming Li, Xingqi Li, Juanjuan Lu, Zhihua Yang, Shilie Pan, Miriding Mutailipu

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Difluoro(oxalato)borates as Short-Wavelength Optical Crystals with Bifunctional [BF 2 C 2 O 4 ] UnitsOriginalZrF2(IO3)2 and RbGaF3(IO3): Two Promising Birefringent Crystals Featuring 1D Metal-Fluoride Cationic Chains and Wide Bandgaps22Na 2 (C 4 O 4 )(H 3 BO 3 )(H 2 O) 4 ·H 3 BO 3 : the first borate-squarate with strong SHG response obtained by superior synergy11Noncentrosymmetric versus Centrosymmetric: Halogen Induced Variable Coordination Modes of Sn2+ and Structural Transition in Sn3B3O7X (X = Cl and Br)17C 10 H 6 NO 2 Cd(NO 3 )·2H 2 O: a birefringent crystal with an enlarged band-gap derived from covalent edge-sharing connection4Discovery of SrZn 2 B 6 O 12 with an unprecedented quadruple-layered configuration0LiCs 3 AlB 7 O 14 : achieving enhanced optical anisotropy via [AlO 4 ] tetrahedron introduction to rearrange the anionic framework5Recent progress on sulfide infrared nonlinear optical materials with large SHG response and wide band gap26HgB2S4: A d10 Metal Thioborate with Giant Birefringence and Wide Band Gap31Target-Oriented Synthesis of Borate Derivatives Featuring Isolated [B3O3] Six-Membered Rings as Structural Features20Recent Progress in Crystalline Borates with Edge-Sharing BO4 Tetrahedra21Multifunctional properties of a polar spin chain compound [N(C3H7)4][Cu(C8H4NO4)]·H2O exhibiting both one-dimensional magnetism and nonlinear optical activity15(NH 4 ) 2 (I 5 O 12 )(IO 3 ) and K 1.03 (NH 4 ) 0.97 (I 5 O 12 )(IO 3 ): Mixed‐Valent Polyiodates with Unprecedented I 5 O 12 − Unit Exhibiting Strong Second‐Harmonic Generation Responses and Giant Birefringence22Centrosymmetric Rb2Sb(C2O4)2.5(H2O)3 and Noncentrosymmetric RbSb2(C2O4)F5: Two Antimony (III) Oxalates as UV Optical Materials20Achieving great optical anisotropy with the well-directed alignment of π-conjugated groups due to hydrogen bonds9Exploring short-wavelength birefringent crystals via triggering cooperative arrangement between different π-conjugated groups8Optimized arrangement of non-π-conjugated PO 3 NH 3 units leads to enhanced ultraviolet optical nonlinearity in NaPO 3 NH 328Sr2[B5O8(OH)]2 ⋅ [B(OH)3] ⋅ H2O: A Strontium Borate That Shows Deep‐Ultraviolet‐Transparent Nonlinear Optical Properties17Designing Strong Polarity and High Configurational Entropy Flexible Units toward Excellent Ultraviolet Nonlinear Optical Materials42Structure‐Prediction‐Oriented Synthesis of Thiophosphates as Promising Infrared Nonlinear Optical Materials24Structure‐Prediction‐Oriented Synthesis of Thiophosphates as Promising Infrared Nonlinear Optical Materials1A new ultraviolet-transparent molybdate featuring a layered structure and moderate birefringence0Inch‐sized K[NH2(CH2COO)2]: a High‐Performance UV Nonlinear Optical Crystal Enabled by Novel Flexible π‐Conjugated Building Units, [NH2(CH2COO)2]−13Engineering an Excellent β ‐BaB 2 O 4 ‐Inspired UV Nonlinear Optical Material Through Secondary Building Unit Substitution21Engineering an Excellent β ‐BaB 2 O 4 ‐Inspired UV Nonlinear Optical Material Through Secondary Building Unit Substitution6Investigation of Optical Properties and Biological Activities of Antimony(III) Halide Templated by 2,2′-Bipyridinium for Optoelectronic Devices5Improving the Performance of Birefringent Crystals by Molecular Assembly Strategy in the Solar‐Blind UV Region14Breaking the Birefringence Barrier in B–O Crystals via B–C π-scaffolding36Descriptors Assisted in Design High-performance Nonlinear Optical Materials with Donor-Acceptor Framework Systems0[C(NH2)3]Pb(C2O4)Cl·H2O: A halogen- and lone-pair-tuned UV crystal with large birefringence originated from cooperative π-conjugation6[HgX 2 ] Linear Group Enabled Ultraviolet Birefringent Crystal RbHg 5 Br 11 with Strong Optical Anisotropy and Wide Bandgap12Quantum chemical investigation of Z-shaped Diradicaloid heptazethrene derivatives towards linear and nonlinear optical polarizability2Counterion engineering in open-framework crystals: dual enhancement of birefringence and UV transparency in Cd–oxalate framework via cation substitution0Transition metal (Co, Ni, Cu) 1-vinylimidazole templated borates as high-efficiency oxygen reduction catalysts for zinc–air battery0From [C(NH2)3]2[Sn2(C2O4)3]·2H2O to [C(NH2)3]4[Sn(C2O4)2]2·H2O: Uneven-substitution-activated polar stannous oxalate with balanced bandgap and birefringence0Designing Novel Solar‐Blind Ultraviolet Nonlinear Optical Crystals Based on Local Proton Distribution Complementary Effect0Designing Novel Solar‐Blind Ultraviolet Nonlinear Optical Crystals Based on Local Proton Distribution Complementary Effect0A novel tetrafluoroborate with giant birefringence assembled from biocompatible adenine0Dual‐Role BF 3 Anchoring Enables Giant Birefringence in Short‐Wave UV‐Transparent Fluoroborates0

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  1. ZrF2(IO3)2 and RbGaF3(IO3): Two Promising Birefringent Crystals Featuring 1D Metal-Fluoride Cationic Chains and Wide Bandgaps

    Inorganic Chemistry · 2022-10-26

    Jin Chen, Ke‐Zhao Du

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  2. Na 2 (C 4 O 4 )(H 3 BO 3 )(H 2 O) 4 ·H 3 BO 3 : the first borate-squarate with strong SHG response obtained by superior synergy

    Chemical Communications · 2022-12-01

    Dong Yan, Yao Ma, Hongbo Huang, Bingbing Zhang, Ru‐Ling Tang, Liang Hu, Fei‐Fei Mao, Jie Zheng, Xiu‐Du Zhang, Shu‐Fang Li

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  3. Noncentrosymmetric versus Centrosymmetric: Halogen Induced Variable Coordination Modes of Sn2+ and Structural Transition in Sn3B3O7X (X = Cl and Br)

    Inorganic Chemistry · 2022-12-30

    Jingyu Guo, Abudukadi Tudi, Xiaoquan Lu, Shujuan Han

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  4. C 10 H 6 NO 2 Cd(NO 3 )·2H 2 O: a birefringent crystal with an enlarged band-gap derived from covalent edge-sharing connection

    Dalton Transactions · 2023-01-01

    Yu Wang, Yaoguo Shen, Weiqi Huang, Sangen Zhao

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  5. Discovery of SrZn 2 B 6 O 12 with an unprecedented quadruple-layered configuration

    New Journal of Chemistry · 2023-01-01

    Xiangyu Long, Yan An Lv, Xueyan Wu

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  6. LiCs 3 AlB 7 O 14 : achieving enhanced optical anisotropy via [AlO 4 ] tetrahedron introduction to rearrange the anionic framework

    Dalton Transactions · 2023-01-01

    Xingqi Li, Dongdong Chu, Haotian Qiu, Yabo Wu, Xueling Hou

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  7. Recent progress on sulfide infrared nonlinear optical materials with large SHG response and wide band gap

    Chinese Journal of Structural Chemistry · 2023-01-01

    Linan Wang, Qi Sun, Junjie Li

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  8. HgB2S4: A d10 Metal Thioborate with Giant Birefringence and Wide Band Gap

    Chemistry of Materials · 2023-05-24

    Yi Huang, Yong an Zhang, Dongdong Chu, Zhihua Yang, Guangmao Li, Shilie Pan

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  9. Target-Oriented Synthesis of Borate Derivatives Featuring Isolated [B3O3] Six-Membered Rings as Structural Features

    Inorganic Chemistry · 2023-05-31

    Meng Cheng, Congcong Jin, Wenqi Jin, Xueling Hou

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  10. Recent Progress in Crystalline Borates with Edge-Sharing BO4 Tetrahedra

    Molecules · 2023-06-28

    Jinɡjinɡ Li, Weifeng Chen, You‐Zhao Lan, Jian‐Wen Cheng

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  11. Multifunctional properties of a polar spin chain compound [N(C3H7)4][Cu(C8H4NO4)]·H2O exhibiting both one-dimensional magnetism and nonlinear optical activity

    Chinese Chemical Letters · 2023-07-06

    Ang Li, Yanhong Wang, Haotian Tian, Alimujiang Yalikun, Yves Journaux, Min Luo, Hongcheng Lu

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  12. (NH 4 ) 2 (I 5 O 12 )(IO 3 ) and K 1.03 (NH 4 ) 0.97 (I 5 O 12 )(IO 3 ): Mixed‐Valent Polyiodates with Unprecedented I 5 O 12 − Unit Exhibiting Strong Second‐Harmonic Generation Responses and Giant Birefringence

    Small · 2023-07-25

    Nan Ma, Jin Chen, Bingxuan Li, Chun‐Li Hu, Jiang‐Gao Mao

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  13. Centrosymmetric Rb2Sb(C2O4)2.5(H2O)3 and Noncentrosymmetric RbSb2(C2O4)F5: Two Antimony (III) Oxalates as UV Optical Materials

    Inorganic Chemistry · 2023-08-02

    Weiyi Wang, Xinyue Wang, Lu Xiong Xu, Die Zhang, Jiale Xue, Shuyao Wang, Xuehua Dong, Liling Cao, Ling Huang, Guohong Zou

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  14. Achieving great optical anisotropy with the well-directed alignment of π-conjugated groups due to hydrogen bonds

    Journal of Saudi Chemical Society · 2023-12-16

    Chenhui Hu, Junjie Liu, Jiale Qu, Jinghui Hu, Xiangzhan Jiang

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  15. Exploring short-wavelength birefringent crystals via triggering cooperative arrangement between different π-conjugated groups

    Chemical Communications · 2024-01-01

    Xiao Wang, Tingwen Han, Kenneth Reinhard Poeppelmeier, Xueling Hou, Shilie Pan, Fangfang Zhang

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  16. Optimized arrangement of non-π-conjugated PO 3 NH 3 units leads to enhanced ultraviolet optical nonlinearity in NaPO 3 NH 3

    Inorganic Chemistry Frontiers · 2024-01-01

    Lingli Wu, Haotian Tian, Chensheng Lin, Xin Yi Zhao, Huixin Fan, Pengxiang Dong, Shunda Yang, Ning Ye, Min Luo

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  17. Sr2[B5O8(OH)]2 ⋅ [B(OH)3] ⋅ H2O: A Strontium Borate That Shows Deep‐Ultraviolet‐Transparent Nonlinear Optical Properties

    Chemistry - A European Journal · 2024-03-18

    Weifeng Chen, J. Lu, Jingjing Li, You‐Zhao Lan, Jian‐Wen Cheng, Guo‐Yu Yang

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  18. Designing Strong Polarity and High Configurational Entropy Flexible Units toward Excellent Ultraviolet Nonlinear Optical Materials

    Advanced Functional Materials · 2024-04-15

    Haotian Tian, Chensheng Lin, Bingxuan Li, Xin Lei Zhao, Tao Yan, Ning Ye, Min Luo

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  19. Structure‐Prediction‐Oriented Synthesis of Thiophosphates as Promising Infrared Nonlinear Optical Materials

    Angewandte Chemie International Edition · 2024-06-03

    Yi Bo Huang, Dongdong Chu, Yong an Zhang, Congwei Xie, Guangmao Li, Shilie Pan

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  20. Structure‐Prediction‐Oriented Synthesis of Thiophosphates as Promising Infrared Nonlinear Optical Materials

    Angewandte Chemie · 2024-06-03

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  21. A new ultraviolet-transparent molybdate featuring a layered structure and moderate birefringence

    New Journal of Chemistry · 2025-01-01

    Shiyu Du, Paipai Zhang, Haozhen Liu, Donghai An, Yanna Chen

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  22. Inch‐sized K[NH2(CH2COO)2]: a High‐Performance UV Nonlinear Optical Crystal Enabled by Novel Flexible π‐Conjugated Building Units, [NH2(CH2COO)2]−

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  23. Engineering an Excellent β ‐BaB 2 O 4 ‐Inspired UV Nonlinear Optical Material Through Secondary Building Unit Substitution

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  24. Engineering an Excellent β ‐BaB 2 O 4 ‐Inspired UV Nonlinear Optical Material Through Secondary Building Unit Substitution

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  25. Investigation of Optical Properties and Biological Activities of Antimony(III) Halide Templated by 2,2′-Bipyridinium for Optoelectronic Devices

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    Eya Toumi, Sameh Sellami, Nour Elleuch, Sameh Dammak, Sergiu G. Shova, Mohamed Boujelbene

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  26. Improving the Performance of Birefringent Crystals by Molecular Assembly Strategy in the Solar‐Blind UV Region

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  27. Breaking the Birefringence Barrier in B–O Crystals via B–C π-scaffolding

    Journal of the American Chemical Society · 2025-07-04

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  28. Descriptors Assisted in Design High-performance Nonlinear Optical Materials with Donor-Acceptor Framework Systems

    Chemical Research in Chinese Universities · 2025-08-27

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  29. [C(NH2)3]Pb(C2O4)Cl·H2O: A halogen- and lone-pair-tuned UV crystal with large birefringence originated from cooperative π-conjugation

    Journal of Molecular Structure · 2025-09-08

    Chao Ma, Yu-Ming Pan, Pei Feng Han, Meihong Duan

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  30. [HgX 2 ] Linear Group Enabled Ultraviolet Birefringent Crystal RbHg 5 Br 11 with Strong Optical Anisotropy and Wide Bandgap

    Advanced Science · 2025-09-09

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  31. Quantum chemical investigation of Z-shaped Diradicaloid heptazethrene derivatives towards linear and nonlinear optical polarizability

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  32. Counterion engineering in open-framework crystals: dual enhancement of birefringence and UV transparency in Cd–oxalate framework via cation substitution

    CrystEngComm · 2026-01-01

    Chenyuan Ma, Jingyi Xie, Zhi Fang, Meihong Duan

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  33. Transition metal (Co, Ni, Cu) 1-vinylimidazole templated borates as high-efficiency oxygen reduction catalysts for zinc–air battery

    Dalton Transactions · 2026-01-01

    Jiayue Yuan, Zhen-Ping Liao, Bo-Wei Liao, Chun‐Yang Pan

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  34. From [C(NH2)3]2[Sn2(C2O4)3]·2H2O to [C(NH2)3]4[Sn(C2O4)2]2·H2O: Uneven-substitution-activated polar stannous oxalate with balanced bandgap and birefringence

    Journal of Molecular Structure · 2026-01-25

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  35. Designing Novel Solar‐Blind Ultraviolet Nonlinear Optical Crystals Based on Local Proton Distribution Complementary Effect

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  36. Designing Novel Solar‐Blind Ultraviolet Nonlinear Optical Crystals Based on Local Proton Distribution Complementary Effect

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  37. A novel tetrafluoroborate with giant birefringence assembled from biocompatible adenine

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  38. Dual‐Role BF 3 Anchoring Enables Giant Birefringence in Short‐Wave UV‐Transparent Fluoroborates

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