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RESEARCH PAPER · ACS Central Science · 2024

The New Paradigm of Ligand Substitution-Driven Enhancement of Anisotropy from SO4 Units in Short-Wavelength Region

Chenhui Hu, Huimin Li, Guangsheng Xu, Zhihua Yang, Jian Wei Han, Shilie Pan

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The New Paradigm of Ligand Substitution-Driven Enhancement of Anisotropy from SO4 Units in Short-Wavelength RegionOriginal(CN 4 H 7 ) 2 SO 4 ·H 2 O: high-performance metal-free ultraviolet birefringent crystal with KBBF-like configuration5K 2 SO 4 (NH 3 SO 3 ) 2 and Cs 2 SO 4 (NH 3 SO 3 ) 3 : two deep-UV transparent sulfamate-sulfates with moderate birefringence2Structural chemistry of antimony( iii ) oxalates with lone pairs: polyhedral distortion [SbO 4 F 2 ], π-conjugation [C 2 O 4 ], and birefringence tuning1Research progress and future prospect of chalcogenides with large optical anisotropy46(CN4H7)H2C3N3S3: Trithiocyanurate Exhibiting Giant Optical Anisotropy via Weak Interaction-Mediated Functional Module Alignment3Anionic Group Trimming Strategy: Oriented Fabrication of Sulfonate UV Birefringent Crystals with High Optical Anisotropy5π-Conjugated unit bridge for giant second-harmonic generation and birefringence in hybrid materials with dual heteroleptic polyhedra5Dual-anion synergy drives remarkable birefringence in sulfate–nitrate crystals1Achieving an optimal performance balance in UV nonlinear optical crystals via hydrogen-bond regulation1Achieving record birefringence in metal-free semiorganic sulfate crystals via tetrahedral anionic group substitution0The Achievement of a Strong Second Harmonic Generation Response and a Large Birefringence in Sulfates4Synergistic Enhancement of Optical Anisotropy in Nitrate Sulfamate for UV Applications: Role of Functional Group Alignment and Hydrogen Bond Network1Cation-sulfur-driven dimensional reduction engineering for tailoring sulfonate birefringent crystals with enhanced anisotropy2(CN 4 H 7 )(NH 2 SO 3 ): A Solar‐Blind Ultraviolet Nonlinear Optical Crystal With Short UV Cutoff Edge and Full‐Wavelength Phase‐Matching0

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  1. (CN 4 H 7 ) 2 SO 4 ·H 2 O: high-performance metal-free ultraviolet birefringent crystal with KBBF-like configuration

    Inorganic Chemistry Frontiers · 2025-01-01

    Xia Hao, Sijing Xie, Ruijie Wang, Chensheng Lin, Lingli Wu, Guang Peng, Tao Yan, Ning Ye, Min Luo

    Read original paper ↗ ·

  2. K 2 SO 4 (NH 3 SO 3 ) 2 and Cs 2 SO 4 (NH 3 SO 3 ) 3 : two deep-UV transparent sulfamate-sulfates with moderate birefringence

    Dalton Transactions · 2025-01-01

    Yun Ji, Huili Zhang, Xin Wen, Jindong Chen, Guangsai Yang, Yuchen Yan, Guang Peng, Ning Ye

    Read original paper ↗ ·

  3. Structural chemistry of antimony( iii ) oxalates with lone pairs: polyhedral distortion [SbO 4 F 2 ], π-conjugation [C 2 O 4 ], and birefringence tuning

    Dalton Transactions · 2025-01-01

    Yunxiao Zhang, Guangsheng Xu, Ke Li, Wei Jia, Xiaoyu Dong

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  4. Research progress and future prospect of chalcogenides with large optical anisotropy

    Coordination Chemistry Reviews · 2025-06-20

    Zhen-Cheng Wu, Sheng‐Ping Guo

    Read original paper ↗ ·

  5. (CN4H7)H2C3N3S3: Trithiocyanurate Exhibiting Giant Optical Anisotropy via Weak Interaction-Mediated Functional Module Alignment

    Inorganic Chemistry · 2025-08-19

    Xia Hao, Y.K. Su, Chensheng Lin, Min Luo, Lingli Wu, Ruijie Wang, Xin Wen, Ning Ye

    Read original paper ↗ ·

  6. Anionic Group Trimming Strategy: Oriented Fabrication of Sulfonate UV Birefringent Crystals with High Optical Anisotropy

    ACS Applied Materials & Interfaces · 2025-09-16

    Hangwei Jia, Yaqi Jin, Shuai An, Xu Liu, Zhihua Yang, Xueling Hou, Shilie Pan

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  7. π-Conjugated unit bridge for giant second-harmonic generation and birefringence in hybrid materials with dual heteroleptic polyhedra

    Chinese Chemical Letters · 2025-11-01

    Yumei Zhang, Wen‐Dong Yao, Yifan Fu, Zhen-Cheng Wu, Zhen-Cheng Wu, Wenlong Liu, Wenlong Liu, Jiajing Wu, Sheng‐Ping Guo

    Read original paper ↗ ·

  8. Dual-anion synergy drives remarkable birefringence in sulfate–nitrate crystals

    Inorganic Chemistry Frontiers · 2025-11-24

    LeHui Liu, FeiFei Yuan, YiSheng Huang, LiZhen Zhang, ZhouBin Lin

    Read original paper ↗ ·

  9. Achieving an optimal performance balance in UV nonlinear optical crystals via hydrogen-bond regulation

    Inorganic Chemistry Frontiers · 2026-01-01

    S AN, Yaqi Jin, Wenhu Wang, Bailin Chen, Zhihua Yang, Xueling Hou, Shilie Pan

    Read original paper ↗ ·

  10. Achieving record birefringence in metal-free semiorganic sulfate crystals via tetrahedral anionic group substitution

    Chemical Science · 2026-01-01

    Yan-Zhen Xie, Hai-Yan Jiang, Yi Zhang, Hui‐Ping Xiao, Qing‐Yan Liu, Yu‐Ling Wang

    Read original paper ↗ ·

  11. The Achievement of a Strong Second Harmonic Generation Response and a Large Birefringence in Sulfates

    Advanced Functional Materials · 2026-03-16

    Qinghe Li, Lilin Yang, Hongyuan Sha, Dongling Yang, Zujian Wang, Xiaoming Yang, Rongbing Su, Bin Su, Chao He, Xifa Long

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  12. Synergistic Enhancement of Optical Anisotropy in Nitrate Sulfamate for UV Applications: Role of Functional Group Alignment and Hydrogen Bond Network

    Small · 2026-04-09

    Xiaotian Ma, Hongyuan Sha, Qianzhen Zhang, Ruyi Niu, Xiya Wen, Xifa Long, Shilie Pan, Yun Mo Yang

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  13. Cation-sulfur-driven dimensional reduction engineering for tailoring sulfonate birefringent crystals with enhanced anisotropy

    Chinese Journal of Structural Chemistry · 2026-05-02

    Hanjing Huang, Longyun Xu, Wenli Zhao, Huijian Zhao, Xianghao Kong, Ning Ye, Zhanggui Hu, Conggang Li

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  14. (CN 4 H 7 )(NH 2 SO 3 ): A Solar‐Blind Ultraviolet Nonlinear Optical Crystal With Short UV Cutoff Edge and Full‐Wavelength Phase‐Matching

    Advanced Optical Materials · 2026-07-01

    Senfu Lei, Yiting Luo, Wenjing Yang, Y N Wu, Zuju Ma, Zilong Geng, Xiaofan Tong, Ruibiao Fu

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