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RESEARCH PAPER · Chemistry of Materials · 2022

Polarity and Ferromagnetism in Two-Dimensional Hybrid Copper Perovskites with Chlorinated Aromatic Spacers

Ceng Han, Alasdair J. Bradford, Jason A. McNulty, Weiguo Zhang, P. Shiv Halasyamani, Alexandra M. Z. Slawin, Finlay D. Morrison, Stephen Lee, Philip Lightfoot

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Polarity and Ferromagnetism in Two-Dimensional Hybrid Copper Perovskites with Chlorinated Aromatic SpacersOriginalZero-Dimensional (Piperidinium)2MnBr4: Ring Puckering-Induced Isostructural Transition and Strong Electron–Phonon Coupling-Mediated Self-Trapped Exciton Emission24Magnetic Properties of Layered Hybrid Organic‐Inorganic Metal‐Halide Perovskites: Transition Metal, Organic Cation and Perovskite Phase Effects59Photoemission spectral analysis of (Benzylammonium)$_{2}$CuCl$_{4}$ 2D-perovskite and confirmation of sustainable thermochromism via encapsulation5Organic-inorganic hybrid perovskites and their heterostructures45Tailoring the Optical and Electronic Properties of 2D Hybrid Dion–Jacobson Copper Chloride Perovskites7Structural Insights into Layered Tetrahalocuprates(II) Based on Small Unsaturated and Cyclic Primary Ammonium Cations3One‐Dimensional Chiral Copper Iodide Chain‐Like Structure Cu 4 I 4 ( R / S ‐3‐quinuclidinol) 3 with Near‐Unity Photoluminescence Quantum Yield and Efficient Circularly Polarized Luminescence46A notable reversible thermochromic (3,3-difluoropyrrolidinium)2[CuCl4] with ferroelectricity and ferroelasticity22First-principles calculations to investigate role of 4d electrons spin (Mo/Tc) in half metallic ferromagnetism, and thermoelectric characteristics of Rb2(Tc, Mo)X6 (X =Cl, Br)21Structure-Related Evolution of Magnetic Order in Anisidinium Tetrachlorocuprates(II)4Multifunctional properties of a polar spin chain compound [N(C3H7)4][Cu(C8H4NO4)]·H2O exhibiting both one-dimensional magnetism and nonlinear optical activity15Electron Spin Decoherence Dynamics in Magnetic Manganese Hybrid Organic–Inorganic Crystals: The Effect of Lattice Dimensionality35Ferroics in Hybrid Organic–Inorganic Perovskites: Fundamentals, Design Strategies, and Implementation42Ultraviolet–Visible-Near-Infrared Photoresponses Realized in a Polar Dion–Jacobson Hybrid Perovskite through Light-Induced Pyroelectric Effects18Bromination of organic spacer impacts on the structural arrangement, phase transitions, and optical and electrical properties of a hybrid halide compound:[(CH 3 ) 3 N(CH 2 ) 3 Br] 2 PdBr 45Controllable Magnetic Properties of Centimeter-Sized 2D (C4H9NH3)2CuCl4–xBrx Hybrid Perovskite Single-Crystalline Nanosheets for Spintronics Applications3Crystal structure, semiconducting and photoluminescence (PL) properties of hybrid tin perovskite-like materials: [Cl–(CH 2 ) 2 –NH 3 ] 2 SnCl 6 and [Cl–(CH 2 ) 2 –NH 3 ] 2 SnBr 5.65 Cl 0.359Synthesis, optical, electronic and magnetic studies of air-stable chiral Cu( ii ) chlorides3Chiral multiferroicity in two-dimensional hybrid organic-inorganic perovskites59Crystal structure, ferromagnetic coupling and antibacterial activity of a new family of dicopper(II) complexes supported by auxiliary para-substituted benzoate linkers4Stronger polar ferromagnetism and narrower optical band gaps in two-dimensional hybrid copper perovskites induced by bromine-substitution9Engineering magnetism in hybrid organic–inorganic metal halide perovskites27Novel lead-free bismuth-based perovskite-like (BrC 5 H 13 N) 3 Bi 2 Br 9 : synthesis, structural investigations and optoelectronic properties5IrxPb1–xO2 Oxygen Evolution Interlayers for Enhancing the Electrochemical Stability of Dimensionally Stable Anodes3Coexistence of Ferroelectricity and Antiferromagnetism in Manganese-Based Hybrid Organic–Inorganic Perovskites0Exciton Diffusion in Two‐dimentional Chiral Perovskites8Mixed A-Site Organic Cation Copper Chloride Perovskite-like: From Thermochromism to Mixed-Valence Cu for Redox Switching5Tailoring Monofluoride Substitution in a 2D Copper Chloride Perovskite Showing Thermochromism and High‐Temperature Dielectric Switching0Magnetic Organic–Inorganic Hybrid Halide Perovskites: Fundamental Physics, Properties, and Applications14The two-halide super exchange pathway in Cu(II) chains: synthesis, structure, and magnetic behavior of (2-X-3-methylpyridinium) 2 [CuX′ 4 ] (X, X′ = Cl, Br)2Lead-free halide perovskite memristors for scalable crossbar arrays14Doping Effects on Magnetic Layered Hybrid Organic–Inorganic Transition Metal Halide Perovskites5Magnetocaloric Effect in a Microporous Material Using a Rare-Earth-Free, Hybrid Perovskite0Observation of a Polar Compound with Halide Ordering in the Compositional Series (CH 3 NH 3 ) 2 Te(Br x Cl 1– x ) 60Raman Spectroscopic Signatures of Piezochromism in Organic‐Inorganic Hybrid Compound (p‐bromoanilinium) 2 CuCl 41Syntheses, Structures, and Properties of Copper(II) and Cobalt(II) Complexes with 1-(4-Chlorophenyl)Piperazinium Cations0Coupling structural phase transition, thermochromism and magnetic circular dichroism in a Cu( ii )-based hybrid perovskite0Nonlinear optical-dielectric dual switching and narrow band gap in a one-dimensional hybrid compound: [(CH 3 ) 2 S(CH 2 ) 3 NH 3 ][SbBr 5 ]0Thermally driven isosymmetric phase transitions and structure–bioactivity relationships in a hybrid tetrachlorocuprate( ii )0Optical Magnetoelectric Effect in a Polar Ferromagnetic Two-Dimensional Organic–Inorganic Hybrid Perovskite1Polar Oxalate Fluoride KMn(C 2 O 4 )F with Triangular Arrangements of Mn 2+ –F–Mn 2+ Spin Chains: Nonlinear Optical and Magnetic Properties0Composition-Driven Control of Magnetic Anisotropy in Hybrid Organic–Inorganic Metal Halides0Electrochemical Behavior and Cycling-Induced Structural Changes in Benzylammonium Copper Chloride Electrodes for Lithium-Ion Batteries0Unveiling Jahn-Teller-Modulated Structural Reversibility in Organic–Inorganic Hybrid Compound ( p -Bromoanilinium)2CuCl4 (PBrAnCuCl) with Temperature by Raman Spectroscopy and X-ray Diffraction Studies0Dion-Jacobson copper-based perovskite (BDA)CuBr4 with narrow interlayer spacing for highly Stable and sensitive X-ray detection0Halide Substitution and π-Conjugated Cation Engineering Enable Large-Hysteresis Phase-Transition-Induced Thermochromic Luminescence in Zero-Dimensional Hybrid Manganese(II) Halides0Multiferroic Semiconducting Behavior in Quasi-2D Cu-Based Hybrid Perovskites0

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  1. Zero-Dimensional (Piperidinium)2MnBr4: Ring Puckering-Induced Isostructural Transition and Strong Electron–Phonon Coupling-Mediated Self-Trapped Exciton Emission

    Inorganic Chemistry · 2022-07-12

    Debendra Prasad Panda, Diptikanta Swain, Athinarayanan Sundaresan

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  2. Magnetic Properties of Layered Hybrid Organic‐Inorganic Metal‐Halide Perovskites: Transition Metal, Organic Cation and Perovskite Phase Effects

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  3. Photoemission spectral analysis of (Benzylammonium)$$_{2}$$CuCl$$_{4}$$ 2D-perovskite and confirmation of sustainable thermochromism via encapsulation

    Journal of Materials Science Materials in Electronics · 2022-10-22

    Ancy Albert, C.O. Sreekala

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  4. Organic-inorganic hybrid perovskites and their heterostructures

    Matter · 2022-12-01

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  5. Tailoring the Optical and Electronic Properties of 2D Hybrid Dion–Jacobson Copper Chloride Perovskites

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    Muhammad Haris Mahyuddin, Arramel Arramel, Lina Jaya Diguna, Mohammad Kemal Agusta, Irma Mulyani, Djulia Onggo, Muhandis Shiddiq, Chi Sin Tang, Xinmao Yin, Caozheng Diao, Muhammad Danang Birowosuto, Andrew T. S. Wee, Andrivo Rusydi

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  6. Structural Insights into Layered Tetrahalocuprates(II) Based on Small Unsaturated and Cyclic Primary Ammonium Cations

    Materials · 2023-03-10

    Edi Topić, Mirta Rubčić

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  7. One‐Dimensional Chiral Copper Iodide Chain‐Like Structure Cu 4 I 4 ( R / S ‐3‐quinuclidinol) 3 with Near‐Unity Photoluminescence Quantum Yield and Efficient Circularly Polarized Luminescence

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    Jian Chen, Xin Pan, Xuanyu Zhang, Chen Sun, Congcong Chen, Xiaoqin Ji, Rui Chen, Lingling Mao

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  8. A notable reversible thermochromic (3,3-difluoropyrrolidinium)2[CuCl4] with ferroelectricity and ferroelasticity

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    Shulin Jiao, Zheng Tang, Dong Li, Cuiping Xu, Yang Zhu, Peng Chen, Xiaofan Sun, Hong‐Ling Cai, Xiaoshan Wu

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  9. First-principles calculations to investigate role of 4d electrons spin (Mo/Tc) in half metallic ferromagnetism, and thermoelectric characteristics of Rb2(Tc, Mo)X6 (X =Cl, Br)

    Ceramics International · 2023-05-05

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  10. Structure-Related Evolution of Magnetic Order in Anisidinium Tetrachlorocuprates(II)

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    Edi Topić, Pavla Šenjug, Dario Barišić, Ivor Lončarić, Damir Pajić, Mirta Rubčić

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  11. Multifunctional properties of a polar spin chain compound [N(C3H7)4][Cu(C8H4NO4)]·H2O exhibiting both one-dimensional magnetism and nonlinear optical activity

    Chinese Chemical Letters · 2023-07-06

    Ang Li, Yanhong Wang, Haotian Tian, Alimujiang Yalikun, Yves Journaux, Min Luo, Hongcheng Lu

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  12. Electron Spin Decoherence Dynamics in Magnetic Manganese Hybrid Organic–Inorganic Crystals: The Effect of Lattice Dimensionality

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  13. Ferroics in Hybrid Organic–Inorganic Perovskites: Fundamentals, Design Strategies, and Implementation

    Advanced Materials · 2023-09-29

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  14. Ultraviolet–Visible-Near-Infrared Photoresponses Realized in a Polar Dion–Jacobson Hybrid Perovskite through Light-Induced Pyroelectric Effects

    Chemistry of Materials · 2023-09-29

    Zhuo Chen, Yueyue He, Yue Zhang, Xian‐Ming Zhang, Dongying Fu

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  15. Bromination of organic spacer impacts on the structural arrangement, phase transitions, and optical and electrical properties of a hybrid halide compound:[(CH 3 ) 3 N(CH 2 ) 3 Br] 2 PdBr 4

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  16. Controllable Magnetic Properties of Centimeter-Sized 2D (C4H9NH3)2CuCl4–xBrx Hybrid Perovskite Single-Crystalline Nanosheets for Spintronics Applications

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    Meihan Liu, Haoran Fu, Sijie Yang, Hongyang Zhao, Zhibin Ma, Qiuming Fu, Hong Tao, Shu‐Hua Yao, Yibo Han, Weidong Man, Zhenxiang Cheng

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  17. Crystal structure, semiconducting and photoluminescence (PL) properties of hybrid tin perovskite-like materials: [Cl–(CH 2 ) 2 –NH 3 ] 2 SnCl 6 and [Cl–(CH 2 ) 2 –NH 3 ] 2 SnBr 5.65 Cl 0.35

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  18. Synthesis, optical, electronic and magnetic studies of air-stable chiral Cu( ii ) chlorides

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  19. Chiral multiferroicity in two-dimensional hybrid organic-inorganic perovskites

    Nature Communications · 2024-07-02

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  20. Crystal structure, ferromagnetic coupling and antibacterial activity of a new family of dicopper(II) complexes supported by auxiliary para-substituted benzoate linkers

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  21. Stronger polar ferromagnetism and narrower optical band gaps in two-dimensional hybrid copper perovskites induced by bromine-substitution

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  22. Engineering magnetism in hybrid organic–inorganic metal halide perovskites

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  26. Exciton Diffusion in Two‐dimentional Chiral Perovskites

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  27. Mixed A-Site Organic Cation Copper Chloride Perovskite-like: From Thermochromism to Mixed-Valence Cu for Redox Switching

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