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RESEARCH PAPER · Matter · 2021

Unusual ferroelectric-dependent birefringence in 2D trilayered perovskite-type ferroelectric exploited by dimensional tailoring

Jiaqi Wang, Yu Ma, Zujian Wang, Xitao Liu, Shiguo Han, Yi Liu, Wuqian Guo, Junhua Luo, Zhihua Sun

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Unusual ferroelectric-dependent birefringence in 2D trilayered perovskite-type ferroelectric exploited by dimensional tailoringOriginalChemical design of homochiral heterocyclic organic ferroelectric crystals8cis/trans-Isomeric Cation Tuning Photoluminescence and Photodetection in 2D Perovskites21Cooperative Enhancement of Second Harmonic Generation in an Organic–Inorganic Hybrid Antimony Halide63Organic Cation Modulation Triggered Second Harmonic Response in Manganese Halides with Bright Fluorescence46Emerging Halide Perovskite Ferroelectrics161Structural dimension engineering and high-temperature dielectric–optical switching in fluorine-substituted lead bromide hybrid perovskites5Nonlinear Optical Glass‐Ceramic From a New Polar Phase‐Transition Organic‐Inorganic Hybrid Crystal12Nonlinear Optical Glass‐Ceramic From a New Polar Phase‐Transition Organic‐Inorganic Hybrid Crystal35Acquiring Bulk Anomalous Photovoltaic Effect in Single Crystals of a Lead‐Free Double Perovskite with Aromatic and Alkali Mixed‐Cations28Synergy of 3D and 2D Perovskites for Durable, Efficient Solar Cells and Beyond249Broadband Achromatic Quarter-Waveplate Using 2D Hybrid Copper Halide Single Crystals18Electron Spin Decoherence Dynamics in Magnetic Manganese Hybrid Organic–Inorganic Crystals: The Effect of Lattice Dimensionality35Polarization‐Dependent Large Photorefractive Effect In A Wide Bandgap 2D Metal Halide Ferroelectric14A Two‐Dimensional Hybrid Perovskite With Heat Switching Birefringence47A Two‐Dimensional Hybrid Perovskite With Heat Switching Birefringence7Ultraviolet–Visible-Near-Infrared Photoresponses Realized in a Polar Dion–Jacobson Hybrid Perovskite through Light-Induced Pyroelectric Effects18Large Enhancement of Polarization in a Layered Hybrid Perovskite Ferroelectric Semiconductor via Molecular Engineering29Ferroelectricity and Related Properties of Nitratecadmate(II) Hybrid with Metal‐Vacancy0H/F substitution activating tunable dimensions and dielectric–optical properties in organic lead-bromide hybrids19The effect of precursor concentrations on the structure and optoelectronic properties of quasi low-dimensional hybrid 2-methylpyridinium lead bromide crystalline phases11Organic‐Inorganic Hybrid Ferroelectric and Antiferroelectric with Afterglow Emission49Organic‐Inorganic Hybrid Ferroelectric and Antiferroelectric with Afterglow Emission10Phase Transitions and Dynamics in Mixed Three- and Low-Dimensional Lead Halide Perovskites134C9H7NBrX (X = Cl, Br, NO3): Three Excellent Birefringent Crystals with Distinct Optical Anisotropy Regulated by Anions34Ferroic Characteristics of Metal‐Halide Perovskites0Unprecedented Silver‐Based Hybrid Pyroelectric Enabling Wide Spectral Photo‐Pyroelectricity for Birefringence Photomodulation7Unprecedented Silver‐Based Hybrid Pyroelectric Enabling Wide Spectral Photo‐Pyroelectricity for Birefringence Photomodulation1Anomalous Polarons in Two‐Dimensional Organometallic Perovskite Ferroelectric7Unusual Triple-State Switching of Thermally Induced Birefringence in a Two-Dimensional Perovskite Ferroelectric45DFT insight into electronic structure of quasi 2D hybrid lead iodide perovskites with linear unsaturated diamines based on hexane2Switchable planar chirality and spin texture in highly ordered ferroelectric hybrid perovskite domains21A low-dimensional ferrocenium lead-iodide perovskite ferroelastic with a narrow band gap7Co-ligand tuning of MOF structural anisotropy for giant optical birefringence7Effect of ring substituent position on the structural and optoelectronic properties of novel quasi low-dimensional hybrid 2-, 3-, and 4-(bromomethyl)pyridinium lead bromides9Highly stable and reversible birefringence switching triggered by thermally stimulated phase transition1Large birefringence switching in a new zero-dimensional cyanide perovskite ferroelastic material3A 3D Hybrid Perovskite Ferroelastic with Triclinic‐to‐Cubic Phase Transition Boosts Temperature/Pressure Dual On/Off Switchable Birefringence4A 3D Hybrid Perovskite Ferroelastic with Triclinic‐to‐Cubic Phase Transition Boosts Temperature/Pressure Dual On/Off Switchable Birefringence19Controlling Energy Flow in Perovskite Heterostructures Through Dimensionality and Phase Engineering7Research progress and future prospect of chalcogenides with large optical anisotropy46Large vertical spontaneous polarization and strong second harmonic generation in a layered perovskite ferroelectric1(C7H10N)3Bi2I9·I2: Synergistic Cooperation of π-Conjugated Cations and Distorted [BiI6] Octahedra Enabling a Large Infrared Birefringence4Proton Alloying in an Organic‐Inorganic Hybrid Material Enables Unusual Dynamic Birefringence and Martensitic Actuation0Proton Alloying in an Organic‐Inorganic Hybrid Material Enables Unusual Dynamic Birefringence and Martensitic Actuation7Supramolecular Rotor Assemblies Exhibiting Thermally Driven Shear‐Dominated Transformation and Birefringence Switching1Molecular pseudo-halogen engineering enables remarkable birefringence enhancement in hybrid perovskites0Structural and optoelectronic properties of quasi-1D hybrid 3-halogenopyridinium lead bromides0Unveiling the Superior Birefringence Property of a Record‐Birefringent Crystal with Unique Building Block13Unveiling the Superior Birefringence Property of a Record‐Birefringent Crystal with Unique Building Block4Distinct Tunable In‐Plane Birefringence via Domain Manipulation in a 2D Metal Halide Ferroelectric3Distinct Tunable In‐Plane Birefringence via Domain Manipulation in a 2D Metal Halide Ferroelectric1Dimensionality Engineering: A Pathway to Ferroelectric Halide Perovskites3Organosilicon cluster goes ferroelectric0Mixed Cation-Ordering-Driven Ferroelastic Phase Transition in Hybrid Lead Halide Enabling Large Switchable Birefringence0Redox‐Driven Strategy Enabling Leapfrog Enhancement of Birefringence in Layered Tin‐Based Optical Crystals1Recent advances in supramolecular ferroelectrics based on macrocycles and cages0Lateral‐Site Unblocking Enables Bilateral π ‐Chromophore Organization for Giant Birefringence in One‐Dimensional Lead Hybrids0Lateral‐Site Unblocking Enables Bilateral π ‐Chromophore Organization for Giant Birefringence in One‐Dimensional Lead Hybrids0Cation Locking Accelerates Exciton Recombination in Polar Two-Dimensional Hybrid Perovskites0Decoupling Contributions of Distinct Strategies for Enhancing Polarizability Anisotropy in Crystals Containing π-Conjugated Groups0Low-Dimensional Perovskites and Metal Halides across Structures and Functions: Connectivity, Dimensionality, and Emerging Principles1A Dynamic Hydrogen‐Bonded Organic Framework With Giant OFF–ON Birefringence0A Dynamic Hydrogen‐Bonded Organic Framework With Giant OFF–ON Birefringence0

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