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RESEARCH PAPER · Angewandte Chemie International Edition · 2023

A Two‐Dimensional Hybrid Perovskite With Heat Switching Birefringence

Ziyi Wang, Chen Xu, Yipeng Song, Zhipeng Du, Zhou Yang, Minjuan Li, Weiqi Huang, Qian-Ting Xu, Yanqiang Li, Sangen Zhao, Junhua Luo

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A Two‐Dimensional Hybrid Perovskite With Heat Switching BirefringenceOriginalA highly birefringent metal-free crystal assembled by cooperative non-covalent interactions30Broadband blue light emissions of one-dimensional hybrid Cu( i ) halides with ultrahigh anti -water stability12Pressure-induced giant emission enhancement, large band gap narrowing and rich polymorphism in two-dimensional 1,2,4-triazolium lead bromide perovskite12Research progress in optical materials with cationic organic planar π-conjugated groups containing CN bonds34Revisiting a (001)-oriented layered lead chloride templated by 1,2,4-triazolium: structural phase transitions, lattice dynamics and broadband photoluminescence6Synthesis, Structure, and Optical Properties of a 0D Hybrid Organic–Inorganic Metal Halide (C 5 N 2 H 14 Cl)GeCl 317A Highly Optical Anisotropic Hybrid Perovskite for Efficient Manipulation of Light Polarization64Nonlinear Optical Properties of Cs2AgIn1–xBixCl6 Single Crystals9Unprecedented Silver‐Based Hybrid Pyroelectric Enabling Wide Spectral Photo‐Pyroelectricity for Birefringence Photomodulation7Unprecedented Silver‐Based Hybrid Pyroelectric Enabling Wide Spectral Photo‐Pyroelectricity for Birefringence Photomodulation1Unusual Triple-State Switching of Thermally Induced Birefringence in a Two-Dimensional Perovskite Ferroelectric45A Highly Optical Anisotropic Hybrid Metal Halide for Modulation and Generation of Polarized Light44[C(NH2)3]2S2O6: A SBBO-Like Dithionate Crystal with Large Optical Anisotropy14Strategically designed anisotropic organic–inorganic metal halides (OIMHs) with superior balance between bandgap and birefringence121D–2D composite perovskite films with self-assembled chiral structure for non-reciprocal circularly polarized emission modulation2Highly stable and reversible birefringence switching triggered by thermally stimulated phase transition1Large birefringence switching in a new zero-dimensional cyanide perovskite ferroelastic material3Zero-dimensional organic–inorganic hybrid cadmium halides with broadband blue light emission3BaFS: Birefringence Enhanced by the Transformation from Optical Isotropy to Anisotropy via Interlayer Anion Substitution8From (C6H5N2)2CdCl4 to (C6H5N2)2ZnCl4, Chirality Transformation to Realize a Nonlinear Optical Organic–Inorganic Hybrid Halide with Balanced Comprehensive Performance19A 3D Hybrid Perovskite Ferroelastic with Triclinic‐to‐Cubic Phase Transition Boosts Temperature/Pressure Dual On/Off Switchable Birefringence4A 3D Hybrid Perovskite Ferroelastic with Triclinic‐to‐Cubic Phase Transition Boosts Temperature/Pressure Dual On/Off Switchable Birefringence19Unearthing Hydrogen Bonded Metal‐Free Crystal with Remarkable Optical Anisotropy9Halide Perovskites for Supercapacitors and Photosupercapacitors: Recent Developments and Future Perspectives27Dual Chemical Scissors Strategy Enables 1D Antimony Selenates with Ultraviolet Nonlinear Optical Properties35Dual Chemical Scissors Strategy Enables 1D Antimony Selenates with Ultraviolet Nonlinear Optical Properties6Low‐Dimensional Organic–Inorganic Hybrid Metal Halide with Large Optical Anisotropy9Local Symmetry Breaking and Hidden Spin Polarization in 2D Hybrid Perovskites with Nonprimary Ammonium Cations14Exceptional Enhancement of Optical Anisotropy Achieved via the Strategy of Combining Rigid Groups with High Symmetry and π‐Conjugated Organic Groups in Hybrid Fluorides33Chiral Bismuth Halide Crystals: Polarizability-Driven Birefringence and Wave Plate Functionality4Proton Alloying in an Organic‐Inorganic Hybrid Material Enables Unusual Dynamic Birefringence and Martensitic Actuation7Supramolecular Rotor Assemblies Exhibiting Thermally Driven Shear‐Dominated Transformation and Birefringence Switching1Molecular pseudo-halogen engineering enables remarkable birefringence enhancement in hybrid perovskites0The condensation of π-conjugated units: a new paradigm for designing high-performance optical crystals4Hybrid Cd 2+ -Based Halide Birefringent Crystals Achieving Tunable Dual-Color Emission for Multifunctional LED and Anticounterfeiting Applications2[C(NH 2 ) 3 ]SbCl 4 : An NLO Material with Enhanced Second Harmonic Response and Birefringence3Perovskite Nanocrystals: An Emerging Nano‐Fluorophore for Stimuli‐Responsive Photoluminescence0Significant Birefringence Enhancement via Cs + Alloying in Layered Perovskites: Synergistic Alignment of Organic Cations and Inorganic Framework1Organosilicon cluster goes ferroelectric0Halogen Bond‐Driven Reversible Thermochromism in a Two‐Dimensional Hybrid Perovskite0Redox‐Driven Strategy Enabling Leapfrog Enhancement of Birefringence in Layered Tin‐Based Optical Crystals1The novel Zn-based ultraviolet birefringent crystals combined both large birefringence and wide bandgap2Heavy‐Halide Coordination and Lattice‐Confined Molecular Alignment Enable Giant Birefringence in Hybrid Metal Halides0Lateral‐Site Unblocking Enables Bilateral π ‐Chromophore Organization for Giant Birefringence in One‐Dimensional Lead Hybrids0Steric‐Guided Coordination Engineering Enables Significantly Optimized Optical Anisotropy via Sulfur‐Driven [C 5 H 5 NS] Birefringence‐Active Groups0Local Aromatic Overlap Microregulation Enables Birefringence Enhancement in Isocompositional Hybrid Antimony Halides1A Dynamic Hydrogen‐Bonded Organic Framework With Giant OFF–ON Birefringence0

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  1. A highly birefringent metal-free crystal assembled by cooperative non-covalent interactions

    Materials Horizons · 2024-01-01

    Yanqiang Li, Zhou Yang, Belal Ahmed, Qian-Ting Xu, Weiqi Huang, Yipeng Song, Xianyu Song, Bin Chen, Junhua Luo, Sangen Zhao

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  2. Broadband blue light emissions of one-dimensional hybrid Cu( i ) halides with ultrahigh anti -water stability

    Dalton Transactions · 2024-01-01

    Na Lin, Yunxia Li, Yu Liu, Kai-Qi Sun, Hong-Yan Zhang, Xiao‐Wu Lei, Zhiwei Chen

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  3. Pressure-induced giant emission enhancement, large band gap narrowing and rich polymorphism in two-dimensional 1,2,4-triazolium lead bromide perovskite

    RSC Advances · 2024-01-01

    Mirosław Mączka, Filip Dybała, Artur P. Herman, Waldeci Paraguassu, Antonio José Barros dos Santos, R. Kudrawiec

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  4. Research progress in optical materials with cationic organic planar π-conjugated groups containing CN bonds

    Inorganic Chemistry Frontiers · 2024-01-01

    Hangwei Jia, Xueling Hou, Shilie Pan

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  5. Revisiting a (001)-oriented layered lead chloride templated by 1,2,4-triazolium: structural phase transitions, lattice dynamics and broadband photoluminescence

    Dalton Transactions · 2024-01-01

    Mirosław Mączka, Szymon Sobczak, Maciej Ptak, Szymon Smółka, Katarzyna Fedoruk, Filip Dybała, Artur P. Herman, Waldeci Paraguassu, Jan K. Zaręba, R. Kudrawiec, Adam Sieradzki, Andrzej Katrusiak

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  6. Synthesis, Structure, and Optical Properties of a 0D Hybrid Organic–Inorganic Metal Halide (C 5 N 2 H 14 Cl)GeCl 3

    Inorganic Chemistry · 2024-02-21

    Y Li, Nan He, Bohui Xu, Linfeng Dong, Xingyu Zhang, Jing J. Xu, Pifu Gong, Zheshuai Lin

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  7. A Highly Optical Anisotropic Hybrid Perovskite for Efficient Manipulation of Light Polarization

    Advanced Functional Materials · 2024-05-08

    Jieyu Zheng, Xianyu Song, Yiran Wu, Yulong Lian, Yanqiang Li, Qian-Ting Xu, Yang Zhou, Ziyi Wang, Lei Wang, Junhua Luo, Sangen Zhao

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  8. Nonlinear Optical Properties of Cs2AgIn1–xBixCl6 Single Crystals

    The Journal of Physical Chemistry Letters · 2024-05-25

    Xu Hai, Junzi Li, Tai Luo, Wenjing Zhang, Hao Jin, Yang Gao, Tingchao He

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  9. Unprecedented Silver‐Based Hybrid Pyroelectric Enabling Wide Spectral Photo‐Pyroelectricity for Birefringence Photomodulation

    Angewandte Chemie International Edition · 2024-09-09

    Xi Rui Zeng, Li Ming Fu, Yi Liu, Yu Ma, Yaoyao Chen, Yang Zhou, Pengfei Zhu, Hongbin Zhang, Junhua Luo, Zhihua Sun

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  10. Unprecedented Silver‐Based Hybrid Pyroelectric Enabling Wide Spectral Photo‐Pyroelectricity for Birefringence Photomodulation

    Angewandte Chemie · 2024-09-09

    Xi Rui Zeng, Li Ming Fu, Yi Liu, Yu Ma, Yaoyao Chen, Yang Zhou, Pengfei Zhu, Hongbin Zhang, Junhua Luo, Zhihua Sun

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  11. Unusual Triple-State Switching of Thermally Induced Birefringence in a Two-Dimensional Perovskite Ferroelectric

    Journal of the American Chemical Society · 2024-09-30

    Yu Ma, Beibei Wang, Wenjing Li, Yi Liu, Wuqian Guo, Haojie Xu, Liwei Tang, Qingshun Fan, Junhua Luo, Zhihua Sun

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  12. A Highly Optical Anisotropic Hybrid Metal Halide for Modulation and Generation of Polarized Light

    Advanced Functional Materials · 2024-10-10

    Qian-Ting Xu, Ziyi Wang, Zhou Yang, Weiqi Huang, Yipeng Song, Jieyu Zheng, Yanqiang Li, Linxi Hou, Junhua Luo, Sangen Zhao

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  13. [C(NH2)3]2S2O6: A SBBO-Like Dithionate Crystal with Large Optical Anisotropy

    Inorganic Chemistry · 2024-12-11

    Siyu Li, Danyang Dou, Cheng Chen, Qi Shi, Bingbing Zhang, Ying Wang

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  14. Strategically designed anisotropic organic–inorganic metal halides (OIMHs) with superior balance between bandgap and birefringence

    Inorganic Chemistry Frontiers · 2024-12-16

    Mingchang Wang, Huaiyu Wu, Miao‐Bin Xu, Jiajia Li, Ke‐Zhao Du, Jin Chen

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  15. 1D–2D composite perovskite films with self-assembled chiral structure for non-reciprocal circularly polarized emission modulation

    Chemical Communications · 2025-01-01

    Yu Xiao, Ruxi Zhang, Hongxu Li, Qiang Zhang, Yin Xiao

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  16. Highly stable and reversible birefringence switching triggered by thermally stimulated phase transition

    Inorganic Chemistry Frontiers · 2025-01-01

    Cheng Chen, Yunjie Bai, Qi Wu Shi, Mingye Han, Bingbing Zhang, Ying Wang

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  17. Large birefringence switching in a new zero-dimensional cyanide perovskite ferroelastic material

    Inorganic Chemistry Frontiers · 2025-01-01

    Jun-Si Zhou, Luan-Ying Ji, Shuyi Liu, Xiao‐Gang Chen

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  18. Zero-dimensional organic–inorganic hybrid cadmium halides with broadband blue light emission

    CrystEngComm · 2025-01-01

    Jiapeng Li, Yuan Li, Ping Li, Ming Wu, Yong-Tai Xie, Xiao‐Wu Lei, Zhihong Jing, Zhongliang Gong

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  19. BaFS: Birefringence Enhanced by the Transformation from Optical Isotropy to Anisotropy via Interlayer Anion Substitution

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    Chao‐Hong Xie, Xiao‐Ming Jiang, Bin‐Wen Liu, Guo‐Cong Guo

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  20. From (C6H5N2)2CdCl4 to (C6H5N2)2ZnCl4, Chirality Transformation to Realize a Nonlinear Optical Organic–Inorganic Hybrid Halide with Balanced Comprehensive Performance

    Inorganic Chemistry · 2025-02-13

    Die-Xue Yang, Yi‐Lei Lv, Jiandong Guo, Wen-Ye Gao, Wenlong Liu, Ru‐Ling Tang

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  21. A 3D Hybrid Perovskite Ferroelastic with Triclinic‐to‐Cubic Phase Transition Boosts Temperature/Pressure Dual On/Off Switchable Birefringence

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  22. A 3D Hybrid Perovskite Ferroelastic with Triclinic‐to‐Cubic Phase Transition Boosts Temperature/Pressure Dual On/Off Switchable Birefringence

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    Huan‐Huan Chen, Xiao‐Gang Chen, Zhe‐Kun Xu, Hang Peng, Yan Fang Qin, Hui‐Peng Lv, Xian‐Jiang Song, Sheng-Qian Hu, Luan-Ying Ji, Jun-Si Zhou, Ren‐Gen Xiong, Wei‐Qiang Liao

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  23. Unearthing Hydrogen Bonded Metal‐Free Crystal with Remarkable Optical Anisotropy

    Advanced Optical Materials · 2025-04-11

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  24. Halide Perovskites for Supercapacitors and Photosupercapacitors: Recent Developments and Future Perspectives

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  25. Dual Chemical Scissors Strategy Enables 1D Antimony Selenates with Ultraviolet Nonlinear Optical Properties

    Angewandte Chemie International Edition · 2025-06-20

    Xuehua Dong, Ling Huang, Hongmei Zeng, Zhien Lin, Kang Min Ok, Guohong Zou

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  26. Dual Chemical Scissors Strategy Enables 1D Antimony Selenates with Ultraviolet Nonlinear Optical Properties

    Angewandte Chemie · 2025-06-20

    Xuehua Dong, Ling Huang, Hongmei Zeng, Zhien Lin, Kang Min Ok, Guohong Zou

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  27. Low‐Dimensional Organic–Inorganic Hybrid Metal Halide with Large Optical Anisotropy

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  28. Local Symmetry Breaking and Hidden Spin Polarization in 2D Hybrid Perovskites with Nonprimary Ammonium Cations

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  29. Exceptional Enhancement of Optical Anisotropy Achieved via the Strategy of Combining Rigid Groups with High Symmetry and π‐Conjugated Organic Groups in Hybrid Fluorides

    Advanced Science · 2025-10-06

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  30. Chiral Bismuth Halide Crystals: Polarizability-Driven Birefringence and Wave Plate Functionality

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  31. Proton Alloying in an Organic‐Inorganic Hybrid Material Enables Unusual Dynamic Birefringence and Martensitic Actuation

    Angewandte Chemie International Edition · 2025-10-18

    Hao‐Fei Ni, Lei Pan, Cha‐Hui Du, Lifu Xu, J. Lou, Peiyao Liu, Hui‐Nan Wang, Changfeng Wang, Zhi‐Xu Zhang, Da‐Wei Fu, Yi Zhang

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  32. Supramolecular Rotor Assemblies Exhibiting Thermally Driven Shear‐Dominated Transformation and Birefringence Switching

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  33. Molecular pseudo-halogen engineering enables remarkable birefringence enhancement in hybrid perovskites

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  34. The condensation of π-conjugated units: a new paradigm for designing high-performance optical crystals

    Chemical Society Reviews · 2026-01-01

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  35. Hybrid Cd 2+ -Based Halide Birefringent Crystals Achieving Tunable Dual-Color Emission for Multifunctional LED and Anticounterfeiting Applications

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  36. [C(NH 2 ) 3 ]SbCl 4 : An NLO Material with Enhanced Second Harmonic Response and Birefringence

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  37. Perovskite Nanocrystals: An Emerging Nano‐Fluorophore for Stimuli‐Responsive Photoluminescence

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  38. Significant Birefringence Enhancement via Cs + Alloying in Layered Perovskites: Synergistic Alignment of Organic Cations and Inorganic Framework

    Advanced Optical Materials · 2026-02-25

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  39. Organosilicon cluster goes ferroelectric

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  40. Halogen Bond‐Driven Reversible Thermochromism in a Two‐Dimensional Hybrid Perovskite

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  41. Redox‐Driven Strategy Enabling Leapfrog Enhancement of Birefringence in Layered Tin‐Based Optical Crystals

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  42. The novel Zn-based ultraviolet birefringent crystals combined both large birefringence and wide bandgap

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  43. Heavy‐Halide Coordination and Lattice‐Confined Molecular Alignment Enable Giant Birefringence in Hybrid Metal Halides

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  44. Lateral‐Site Unblocking Enables Bilateral π ‐Chromophore Organization for Giant Birefringence in One‐Dimensional Lead Hybrids

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  45. Steric‐Guided Coordination Engineering Enables Significantly Optimized Optical Anisotropy via Sulfur‐Driven [C 5 H 5 NS] Birefringence‐Active Groups

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  46. Local Aromatic Overlap Microregulation Enables Birefringence Enhancement in Isocompositional Hybrid Antimony Halides

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  47. A Dynamic Hydrogen‐Bonded Organic Framework With Giant OFF–ON Birefringence

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