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RESEARCH PAPER · Advanced Optical Materials · 2022

BaSi7P10 and SrSi7P10: Two Infrared Nonlinear Optical Phosphides with T2 Supertetrahedra Exhibiting Strong Second‐Harmonic Generation Effects

Xin Lei Zhao, Chensheng Lin, Jindong Chen, Feng Xu, Shunda Yang, Guang Peng, Haotian Tian, Yinglei Han, Bingxuan Li, Min Luo, Ning Ye

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BaSi7P10 and SrSi7P10: Two Infrared Nonlinear Optical Phosphides with T2 Supertetrahedra Exhibiting Strong Second‐Harmonic Generation EffectsOriginalAIn 3 Si 4 P 9 (A = Ca, Sr): quaternary phosphides with double-helix structures exhibiting high laser-induced damage thresholds19High-Performance Flexible Broadband Photothermoelectric Photodetectors Based on Tellurium Films42Cs 3 In(In 4 Se 7 )(P 2 Se 6 ): A Multi‐Chromophore Chalcogenide with Excellent Nonlinear Optical Property Designed by Group Grafting55Cs3In(In4Se7)(P2Se6): A Multi‐Chromophore Chalcogenide with Excellent Nonlinear Optical Property Designed by Group Grafting2Achieving strong optical nonlinearity and wide bandgap of pnictides via ionic motif–driven directed assembly of covalent groups39AI2Mg3Ga12S22 (AI = K, Rb): T2-type supertetrahedra coupled with [MgS6] octahedra for designing wide-band gap infrared nonlinear optical materials with well-balanced properties16Assembly between diverse polycations and diamond-like anionic frameworks in salt-inclusion phosphides enables excellent nonlinear optical properties4Two-in-one: assembling hybrid supertetrahedra chromophores and achieving high-performance “hexagonal warriors” in nonlinear optical crystals6Reinforced Nonlinear Optical Performances Induced by P‐P Homoatomic Bond in Phosphide SrIn 3 Si 4 P 1131Reinforced Nonlinear Optical Performances Induced by P‐P Homoatomic Bond in Phosphide SrIn 3 Si 4 P 116In and Out: Shuttling Atoms in Covalent Nanocrystals, from Synthesis in Molten Salts to Water-Splitting Electrocatalysis5[Rb 4 Cl][Cd 11 In 9 Se 26 ]: a salt inclusion chalcogenide with a diamond-like framework for infrared nonlinear optics0CaM 3 Si 4 As 11 (M = Ga, In): arsenide infrared nonlinear optical crystals enforced by novel [As 2 ] linear motifs0Topology-Guided Discovery of BaIn 2 Si 7 P 12 : A Quaternary Diamond-like Framework Phosphide with Giant Second-Harmonic Generation and High Laser-Induced Damage Threshold22Mid-Infrared Transparent Materials: from Mechanisms to Cutting-Edge Applications9Cs X Si 15 P 21 ( X = Sn or Pb): Polar Noncentrosymmetric Si–P Frameworks Stabilized by Covalent X –P Bonding3BaM2Si7As12 (M = Ga, In): Arsenide infrared nonlinear optical crystals via an adding phase strategy0A New Infrared Nonlinear Optical Crystal Ba 5 Zn 3 Ga 2 Sn 2 Se 15 with Congruent Melting Behavior Based on Mixed-Metal T2-Supertetrahedral Units1Topology‐Preserving Ionic‐Unit Substitution Enables Sphalerite‐Like Phosphides Achieving Superior Infrared Optical Nonlinearity0Topology‐Preserving Ionic‐Unit Substitution Enables Sphalerite‐Like Phosphides Achieving Superior Infrared Optical Nonlinearity0Variation of Tetrahedrons and Cations Regulates LIDTs in 3D‐DL Structure MIR‐NLO Crystals0Beyond the bandgap bottleneck: structure–property design principles for infrared nonlinear optical phosphides0

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  1. AIn 3 Si 4 P 9 (A = Ca, Sr): quaternary phosphides with double-helix structures exhibiting high laser-induced damage thresholds

    Inorganic Chemistry Frontiers · 2022-12-19

    Ming‐Shu Zhang, Bin‐Wen Liu, Xiao‐Ming Jiang, Guo‐Cong Guo

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  2. High-Performance Flexible Broadband Photothermoelectric Photodetectors Based on Tellurium Films

    ACS Applied Materials & Interfaces · 2024-01-25

    Mingcong Zhang, Yunjie Liu, Fuhai Guo, Bo Zhang, Bing Hu, Siqi Li, Weizhuo Yu, Lanzhong Hao

    Read original paper ↗ ·

  3. Cs 3 In(In 4 Se 7 )(P 2 Se 6 ): A Multi‐Chromophore Chalcogenide with Excellent Nonlinear Optical Property Designed by Group Grafting

    Angewandte Chemie International Edition · 2024-02-01

    Zhen Qian, Hongping Wu, Zhanggui Hu, Jiyang Wang, Yicheng Wu, Hongwei Yu

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  4. Cs3In(In4Se7)(P2Se6): A Multi‐Chromophore Chalcogenide with Excellent Nonlinear Optical Property Designed by Group Grafting

    Angewandte Chemie · 2024-02-02

    Zhen Qian, Hongping Wu, Zhanggui Hu, Jiyang Wang, Yicheng Wu, Hongwei Yu

    Read original paper ↗ ·

  5. Achieving strong optical nonlinearity and wide bandgap of pnictides via ionic motif–driven directed assembly of covalent groups

    Science Advances · 2024-11-13

    Lihua Gao, Jindong Chen, Xuemei Shi, Yan Xiao, Yinglei Han, Chensheng Lin, Huikang Jiang, Guangsai Yang, Guang Peng, Ning Ye

    Read original paper ↗ ·

  6. AI2Mg3Ga12S22 (AI = K, Rb): T2-type supertetrahedra coupled with [MgS6] octahedra for designing wide-band gap infrared nonlinear optical materials with well-balanced properties

    Science China Materials · 2025-01-22

    Mengmeng Chen, Xu Liu, Abudukadi Tudi, Cui Chen, Qixian Ren, Zhihua Yang, Yabo Wu, Shilie Pan

    Read original paper ↗ ·

  7. Assembly between diverse polycations and diamond-like anionic frameworks in salt-inclusion phosphides enables excellent nonlinear optical properties

    Science China Chemistry · 2025-02-11

    Ming‐Shu Zhang, Shao‐Min Pei, Bin‐Wen Liu, Xiao‐Ming Jiang, Guo‐Cong Guo

    Read original paper ↗ ·

  8. Two-in-one: assembling hybrid supertetrahedra chromophores and achieving high-performance “hexagonal warriors” in nonlinear optical crystals

    Science China Chemistry · 2025-02-20

    Zhen Qian, Hongping Wu, Zhanggui Hu, Jiyang Wang, Yicheng Wu, Hongwei Yu

    Read original paper ↗ ·

  9. Reinforced Nonlinear Optical Performances Induced by P‐P Homoatomic Bond in Phosphide SrIn 3 Si 4 P 11

    Angewandte Chemie International Edition · 2025-02-26

    Shao‐Min Pei, Ming‐Shu Zhang, Xiao‐Ming Jiang, Bin‐Wen Liu, Guo‐Cong Guo

    Read original paper ↗ ·

  10. Reinforced Nonlinear Optical Performances Induced by P‐P Homoatomic Bond in Phosphide SrIn 3 Si 4 P 11

    Angewandte Chemie · 2025-02-26

    Shao‐Min Pei, Ming‐Shu Zhang, Xiao‐Ming Jiang, Bin‐Wen Liu, Guo‐Cong Guo

    Read original paper ↗ ·

  11. In and Out: Shuttling Atoms in Covalent Nanocrystals, from Synthesis in Molten Salts to Water-Splitting Electrocatalysis

    Journal of the American Chemical Society · 2025-06-04

    Yang Song, Anissa Ghoridi, Fernando Igoa, Isabel Gómez‐Recio, Daniel Janisch, Edouard de Rolland Dalon, Dominique Thiaudière, M. Luisa Ruiz‐González, José María González-Calbet, Benedikt Lassalle‐Kaiser, Andrea Zitolo, Christel Laberty‐Robert, David Portehault

    Read original paper ↗ ·

  12. [Rb 4 Cl][Cd 11 In 9 Se 26 ]: a salt inclusion chalcogenide with a diamond-like framework for infrared nonlinear optics

    Dalton Transactions · 2026-01-01

    Pengzhi Xie, Qixian Ren, Junwei Feng, Hong Lei Du, Shuyi Mi

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  13. CaM 3 Si 4 As 11 (M = Ga, In): arsenide infrared nonlinear optical crystals enforced by novel [As 2 ] linear motifs

    Chemical Science · 2026-01-01

    Shusen Yang, Qichao Zhao, Xuemei Shi, Guang Peng, Ning Ye, Jindong Chen

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  14. Topology-Guided Discovery of BaIn 2 Si 7 P 12 : A Quaternary Diamond-like Framework Phosphide with Giant Second-Harmonic Generation and High Laser-Induced Damage Threshold

    Journal of the American Chemical Society · 2026-02-16

    Jiazheng Zhou, Yu Chu, Xin Su, Le Luo, Miriding Mutailipu, Shilie Pan, Junjie Li

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  15. Mid-Infrared Transparent Materials: from Mechanisms to Cutting-Edge Applications

    Nano-Micro Letters · 2026-02-28

    Hanyuan Zhang, Zhenhui Huang, Changyuan Chen, Yi Long, Weilin Xu, Zhengui Zhou, Jun Wan

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  16. Cs X Si 15 P 21 ( X = Sn or Pb): Polar Noncentrosymmetric Si–P Frameworks Stabilized by Covalent X –P Bonding

    Chemistry of Materials · 2026-03-31

    Philip Yox, Victoria Kyveryga, Ernesto Soto, Jessica Warner, Gayatri Viswanathan, Eranga H. Gamage, Kui Wu, Bingbing Zhang, Victor Trinquet, Geoffroy Hautier, Gian‐Marco Rignanese, Kirill A. Kovnir

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  17. BaM2Si7As12 (M = Ga, In): Arsenide infrared nonlinear optical crystals via an adding phase strategy

    Chinese Journal of Structural Chemistry · 2026-05-26

    Shusen Yang, Xuemei Shi, Bo Li, Guang Peng, Ning Ye, Jindong Chen

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  18. A New Infrared Nonlinear Optical Crystal Ba 5 Zn 3 Ga 2 Sn 2 Se 15 with Congruent Melting Behavior Based on Mixed-Metal T2-Supertetrahedral Units

    Crystal Growth & Design · 2026-06-29

    Huichang Wang, Miao Song, Guili Wang, Pifu Gong, Siyang Luo, Jiyong Yao

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  19. Topology‐Preserving Ionic‐Unit Substitution Enables Sphalerite‐Like Phosphides Achieving Superior Infrared Optical Nonlinearity

    Angewandte Chemie · 2026-08-26

    Qichao Zhao, Bingxuan Li, Guang Peng, Ning Ye, Jindong Chen

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  20. Topology‐Preserving Ionic‐Unit Substitution Enables Sphalerite‐Like Phosphides Achieving Superior Infrared Optical Nonlinearity

    Angewandte Chemie International Edition · 2026-08-26

    Qichao Zhao, Bingxuan Li, Guang Peng, Ning Ye, Jindong Chen

    Read original paper ↗ ·

  21. Variation of Tetrahedrons and Cations Regulates LIDTs in 3D‐DL Structure MIR‐NLO Crystals

    ChemistrySelect · 2026-09-01

    Chaoyi Zhu

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  22. Beyond the bandgap bottleneck: structure–property design principles for infrared nonlinear optical phosphides

    Coordination Chemistry Reviews · 2026-09-22

    Zichang Wang, Dajiang Mei, Ximeng Lv, Shuchang Wu, Yang Liu, Jingdong Yan, Xiangran Kong, Hongwei Leng, Zuotao Lei, Chunhui Yang

    Read original paper ↗ ·
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