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RESEARCH PAPER · Inorganic Chemistry · 2014

Origin of Ferroelectricity in a Family of Polar Oxides: The Dion—Jacobson Phases

Nicole A. Benedek

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Origin of Ferroelectricity in a Family of Polar Oxides: The Dion—Jacobson PhasesOriginalMagnetic‐Structure‐Stabilized Polarization in an Above‐Room‐Temperature Ferrimagnet50Magnetic‐Structure‐Stabilized Polarization in an Above‐Room‐Temperature Ferrimagnet12Ferroelectricity in Dion–Jacobson ABiNb 2 O 7 (A = Rb, Cs) compounds68Piezoelectricity enhancement in Dion-Jacobson RbBiNb 2 O 7 via negative pressure16Tuning the ferroelectric polarization in AA′MnWO 6 double perovskites through A cation substitution35Synthesis and characterization of the rare-earth Dion–Jacobson layered perovskites, APrNb 2 O 7 (A = Rb, Cs and CuCl)20Understanding ferroelectricity in layered perovskites: new ideas and insights from theory and experiments290Anharmonic lattice interactions in improper ferroelectrics for multiferroic design72Proper Ferroelectricity in the Dion–Jacobson Material CsBi2Ti2NbO10: Experiment and Theory56Improper Inversion Symmetry Breaking and Piezoelectricity through Oxygen Octahedral Rotations in Layered Perovskite Family, LiRTiO4 (R = Rare Earths)34NdBaScO 4 : aristotype of a new family of geometric ferroelectrics?16Emergent Noncentrosymmetry and Piezoelectricity Driven by Oxygen Octahedral Rotations in n = 2 Dion–Jacobson Phase Layer Perovskites43Dielectric Properties2Two New Non-centrosymmetric n = 3 Layered Dion–Jacobson Perovskites: Polar RbBi2Ti2NbO10 and Nonpolar CsBi2Ti2TaO1057La 2 SrCr 2 O 7 : Controlling the Tilting Distortions of n = 2 Ruddlesden–Popper Phases through A-Site Cation Order32Persistence of strong and switchable ferroelectricity despite vacancies8Aperiodic topological order in the domain configurations of functional materials83Electronic structure and phase transition in polar ScFeO3 from first principles calculations17Phase Transition Behavior of the Layered Perovskite CsBi0.6La0.4Nb2O7: A Hybrid Improper Ferroelectric12Systematic Thermodynamics of Layered Perovskites: Ruddlesden–Popper Phases32Direct observation of charged domain walls in hybrid improper ferroelectric (Ca,Sr) 3 Ti 2 O 711Retention Characteristics of Five‐Layered Aurivillus Films With Large Polarization8Theory and Neutrons Combine To Reveal a Family of Layered Perovskites without Inversion Symmetry47New Type of 2D Perovskites with Alternating Cations in the Interlayer Space, (C(NH 2 ) 3 )(CH 3 NH 3 ) n Pb n I 3 n +1 : Structure, Properties, and Photovoltaic Performance521Crystal Structure of Electroceramics0Nanoarchitectonics in dielectric/ferroelectric layered perovskites: from bulk 3D systems to 2D nanosheets62Bibliography0Insights into the polymorphism of Bi 2 W 2 O 9 : single crystal growth and a complete survey of the variable-temperature thermal and dielectric properties11Microstructure and Electric Properties of (Sr1−xCax)3Sn2O7 Ceramics with Ruddlesden-Popper Structure2High-throughput first-principles search for new ferroelectrics50Ferroelectric Sr 3 Zr 2 O 7 : Competition between Hybrid Improper Ferroelectric and Antiferroelectric Mechanisms132Hybrid Improper Ferroelectricity in (Sr,Ca) 3 Sn 2 O 7 and Beyond: Universal Relationship between Ferroelectric Transition Temperature and Tolerance Factor in n = 2 Ruddlesden–Popper Phases123Cation Exchange as a Mechanism To Engineer Polarity in Layered Perovskites33Polarization rotation in Bi4Ti3O12 by isovalent doping at the fluorite sublattice24Persistent spin helix in Rashba-Dresselhaus ferroelectric CsBiNb2O764Temperature-Induced Structural Transformations in Undoped and Eu3+-Doped Ruddlesden–Popper Phases Sr2SnO4 and Sr3Sn2O7: Relation to the Impedance and Luminescence Behaviors13Magneto-electric multiferroics: designing new materials from first-principles calculations10Experimental and theoretical determination of physical properties of Sm 2 Bi 2 Fe 4 O 12 ferromagnetic semiconductors19Photocatalytic activity of 2D nanosheets of ferroelectric Dion–Jacobson compounds13Understanding the Energetics in Two-dimensional Metal Halide Perovskite Quantum Wells0Structural and optical properties of Fe-doped Ruddlesden-Popper Ca3Ti2-xFexO7-δ nanoparticles52Hidden improper ferroelectric phases for design of antiferroelectrics3Complex Structural Phase Transitions of the Hybrid Improper Polar Dion–Jacobson Oxides RbNdM 2 O 7 and CsNdM 2 O 7 (M = Nb, Ta)35Bi2W2O9 : A potentially antiferroelectric Aurivillius phase14Synergistic Influence of d0 (Nb5+) and d10 (Cd2+) Cations in Stabilizing Noncentrosymmetric Dion–Jacobson Layered Perovskites, A′Cd2Nb3O10 (A′ = Rb, Cs)12Ferroelectricity of Dion–Jacobson layered perovskites CsNdNb 2 O 7 and RbNdNb 2 O 720Study of the microstructure and the optical, electrical, and magnetic feature of the Dy2Bi2Fe4O12 ferromagnetic semiconductor10Highly Tunable Ferroelectricity in Hybrid Improper Ferroelectric Sr3Sn2O740Polar Structures of KNdNb2O7and KNdTa2O710Beyond Expectation: Advanced Materials Design, Synthesis, and Processing to Enable Novel Ferroelectric Properties and Applications1Prediction of an Extended Ferroelectric Clathrate26Phase transitions in RbPrNb2O7, a layer structured ferroelectric with a high Curie point26Tuning between Proper and Hybrid-Improper Mechanisms for Polar Behavior in Cs Ln 2Ti2NbO10 Dion-Jacobson Phases22The influence of the 6s 2 configuration of Bi 3+ on the structures of A′BiNb 2 O 7 (A′ = Rb, Na, Li) layered perovskite oxides10Orbital ordering in the layered perovskite material CsVF416Switching between Proper and Hybrid-Improper Polar Structures via Cation Substitution in A2La(TaTi)O7(A = Li, Na)17Unit-cell-thick domain in free-standing quasi-two-dimensional ferroelectric material9Layered Double Perovskites75Directed synthesis of a hybrid improper magnetoelectric multiferroic material25Heteroanionic Ruddlesden-Popper ferroelectrics from anion order and octahedral tilts8Physical–Chemical Exfoliation of n-Alkylamine Derivatives of Layered Perovskite-like Oxide H2K0.5Bi2.5Ti4O13 into Nanosheets13Review of experimental progress of hybrid improper ferroelectricity in layered perovskite oxides36Point defect induced incommensurate dipole moments in the KCa2Nb3O10 Dion-Jacobson layered perovskite4Hybrid Improper Ferroelectricity in Highly Cleavable Single Crystals of Dion‐Jacobson‐Compound CsBiNb2O76Spintronic Properties in Complex Perovskites: A Concordance Between Experiments and Ab-Initio Calculations10The crystal and defect structures of polar KBiNb 2 O 72Designing new polar materials1Exfoliation of functionalized layered oxides : synthetic approaches and advanced characterizations : toward a non-electrostatic reassembly0Prospects for obtaining perovskite-like compounds with the Dion-Jacobson structure and the influence of precursors on their phase formation, structure, and properties0Hybrid Improper Ferroelectricity: A Theoretical, Computational, and Synthetic Perspective45Local atomic structure distortions in the Dion-Jacobson ferroelectric CsBiNb2O71Interplay between Oxygen Octahedral Rotation and Deformation in the Acentric ARTiO4 Series toward Negative Thermal Expansion19Rare-earth ferrobismuthites: ferromagnetic ceramic semiconductors with applicability in spintronic devices3Syntheses, structures, and optical properties of n = 3 layered Dion–Jacobson perovskites, RbEu2-Bi Ti2NbO10 (0 ≤ x ≤ 2)1Recent Advances in Ferroelectric‐Enhanced Low‐Dimensional Optoelectronic Devices32Second Harmonic Generation in the Polar A′SmNb2O7 (A′ = Rb, Cs) Dion–Jacobson Layered Perovskites11Ferroelectric switching pathways and domain structure of SrBi2(Ta,Nb)2O9 from first principles8Hybrid Improper Ferroelectricity in Columnar (NaY)MnMnTi4O125Hybrid Improper Ferroelectricity in Columnar (NaY)MnMnTi4O120Pressure-Induced Phase Transformations of Quasi-2D Sr3Hf2O73MnCaTa2O7─A Magnetically Ordered Polar Phase Prepared via Cation Exchange4Emerging ceramic nanosheets: From tailored synthesis to electronic applications1Out-of-plane ferroelectricity and robust magnetoelectricity in quasi-two-dimensional materials15Tunable ferroelectricity in oxygen-deficient perovskites with Grenier structure10A new class of single-phase multiferroics: Bismuth-based layered supercell oxide thin films—Current progress and future perspectives5Magnetoelectric coupling in the multiferroic hybrid-improper ferroelectric Ca3Mn1.9Ti0.1O710Atomic Layer Engineering of Ferroelectricity in Dion–Jacobson Perovskites12Structural frustration effects by mixed alkali ions in ferroelectric Dion–Jacobson layered perovskites (Cs,Rb)NdNb 2 O 76Suppression of Ferroelectric Transitions by Symmetry Trapping in Dion–Jacobson-Layered Perovskites Cs(La,Nd)Nb2O74Lattice dynamical properties and interatomic force constants of transition metal oxide perovskite superlattices4Recent Progress of Hybrid Improper Ferroelectrics with Ruddlesden-Popper Structure1Structural chemistry of the n = 3 Dion–Jacobson phases: controlling polarity and band gap3Structural Mechanisms of Quasi-2D Perovskites for Next-Generation Photovoltaics43Dion–Jacobson (n = 2) Layered Perovskites (A′SmTa2O7; A′ = Rb, Cs) As Potential Ferroelectric Materials6Structural distortions leading to potential polar materials in n $=$ 3 and 4 Dion–Jacobson-layered perovskite series1A DFT analysis on the electronic, mechanical, optical, elastic, structural and thermodynamic properties of XBiNb2O7 (X = Cs, Rb, K and Na) for photovoltaic applications24Structural Distortions and Uniaxial Negative Thermal Expansion in the Polar Dion–Jacobson Oxide RbNdTa 2 O 70Structural Phase Transitions in Layered Perovskite CsFeF4${\rm CsFeF}_{4}$ and Weak Polar Response in CsFeF4${\rm CsFeF}_{4}$/RbFeF4${\rm RbFeF}_{4}$ Superlattice0Cation Exchange as a Route to Introduce Magnetism to Hybrid-Improper Polar Phases0Ruddlesden-Popper chalcogenides push the limit of mechanical stiffness and glass-like thermal conductivity in single crystals6Theoretical Evaluation of Multifunctional Properties of Thermodynamically Stable Dion Jacobson Family Members LiBiNb 2 O 7 and FrBiNb 2 O 7 for Optoelectronic Devices1A study focusing on the influence of multiple cationic substitutions in Dion–Jacobson ( n = 2) layered perovskite oxides0Revival of Layered Ferroelectrics in Thin Films2Theoretical multifunctional investigations for CsXNb2O7 (X = La, Lu, In and Ga) for next-generation optical devices under visible and UV radiations4Theoretical investigations of 2D Dion–Jacobson-type materials for energy storage applications: A DFT+U study3Two‐Dimensional La 2 CoO 4 Perovskite Oxide Enabled by Phonon‐Resonance‐Driven Exfoliation for High‐Performance Gas Sensing18Atomic-Scale Visualization of Competing Polar Orders in Dion–Jacobson Layered Perovskites2Unexpected Structural Complexity in Pseudo-Ruddlesden–Popper Phases02D dielectrics and ferroelectrics: emerging materials, physics and design principles0Record‐Low Coercive Field and Stable Curie Temperature in Bulk Hybrid Improper Ferroelectrics via Synergistic A / B ‐Site Co‐Substitution0Neutron Diffraction for Structural Characterisation of Inorganic Materials0Layer Alignment via Short Strong Hydrogen Bonding in the Dion–Jacobson Perovskite Solid Acid HLaNb2O70

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  1. Magnetic‐Structure‐Stabilized Polarization in an Above‐Room‐Temperature Ferrimagnet

    Angewandte Chemie International Edition · 2014-08-11

    Man‐Rong Li, M. Retuerto, David Walker, Tapati Sarkar, Peter W. Stephens, Swarnakamal Mukherjee, Tanusri Saha‐Dasgupta, Jason P. Hodges, Mark Croft, Christoph P. Grams, J. Hemberger, Javier Sánchez-Benítez, Ashfia Huq, Felix O. Saouma, Joon Ik Jang, M. Greenblatt

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  2. Magnetic‐Structure‐Stabilized Polarization in an Above‐Room‐Temperature Ferrimagnet

    Angewandte Chemie · 2014-08-11

    Man‐Rong Li, M. Retuerto, David Walker, Tapati Sarkar, Peter W. Stephens, Swarnakamal Mukherjee, Tanusri Saha‐Dasgupta, Jason P. Hodges, Mark Croft, Christoph P. Grams, J. Hemberger, Javier Sánchez-Benítez, Ashfia Huq, Felix O. Saouma, Joon Ik Jang, M. Greenblatt

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  3. Ferroelectricity in Dion–Jacobson ABiNb 2 O 7 (A = Rb, Cs) compounds

    Journal of Materials Chemistry C · 2014-11-04

    Chen Chen, Huanpo Ning, Serban Lepadatu, Markys G. Cain, Haixue Yan, Mike John Reece

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  4. Piezoelectricity enhancement in Dion-Jacobson RbBiNb 2 O 7 via negative pressure

    Europhysics Letters (EPL) · 2014-12-01

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  5. Tuning the ferroelectric polarization in AA′MnWO 6 double perovskites through A cation substitution

    Dalton Transactions · 2014-12-23

    Joshua Young, Alessandro Stroppa, Silvia Picozzi, James M. Rondinelli

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  6. Synthesis and characterization of the rare-earth Dion–Jacobson layered perovskites, APrNb 2 O 7 (A = Rb, Cs and CuCl)

    Dalton Transactions · 2015-01-01

    Dariush Montasserasadi, Mark Granier, Leonard Spînu, Satish Chandra Rai, Weilie L Zhou, John B. Wiley

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  7. Understanding ferroelectricity in layered perovskites: new ideas and insights from theory and experiments

    Dalton Transactions · 2015-01-01

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  8. Anharmonic lattice interactions in improper ferroelectrics for multiferroic design

    Journal of Physics Condensed Matter · 2015-06-30

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  9. Proper Ferroelectricity in the Dion–Jacobson Material CsBi2Ti2NbO10: Experiment and Theory

    Chemistry of Materials · 2015-11-04

    Emma E. McCabe, Éric Bousquet, Christopher P. J. Stockdale, Charles A. Deacon, T. Thao Tran, P. Shiv Halasyamani, Martin Christopher. Stennett, Neil Christian Hyatt

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  10. Improper Inversion Symmetry Breaking and Piezoelectricity through Oxygen Octahedral Rotations in Layered Perovskite Family, LiRTiO4 (R = Rare Earths)

    Advanced Electronic Materials · 2015-12-07

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  11. NdBaScO 4 : aristotype of a new family of geometric ferroelectrics?

    Chemical Communications · 2016-01-01

    Amber K. Cochrane, Michael Telfer, Charlotte A. L. Dixon, Weiguo Zhang, P. Shiv Halasyamani, Éric Bousquet, Philip Lightfoot

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  12. Emergent Noncentrosymmetry and Piezoelectricity Driven by Oxygen Octahedral Rotations in n = 2 Dion–Jacobson Phase Layer Perovskites

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  13. Dielectric Properties

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  14. Two New Non-centrosymmetric n = 3 Layered Dion–Jacobson Perovskites: Polar RbBi2Ti2NbO10 and Nonpolar CsBi2Ti2TaO10

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    Hyung Gu Kim, T. Thao Tran, Woongjin Choi, Tae‐Soo You, P. Shiv Halasyamani, Kang Min Ok

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  15. La 2 SrCr 2 O 7 : Controlling the Tilting Distortions of n = 2 Ruddlesden–Popper Phases through A-Site Cation Order

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  16. Persistence of strong and switchable ferroelectricity despite vacancies

    Scientific Reports · 2017-01-25

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  17. Aperiodic topological order in the domain configurations of functional materials

    Nature Reviews Materials · 2017-03-07

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  18. Electronic structure and phase transition in polar ScFeO3 from first principles calculations

    Journal of Alloys and Compounds · 2017-04-10

    Bog G. Kim, Masayuki Toyoda, Janghee Park, Tamio Oguchi

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  19. Phase Transition Behavior of the Layered Perovskite CsBi0.6La0.4Nb2O7: A Hybrid Improper Ferroelectric

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  20. Systematic Thermodynamics of Layered Perovskites: Ruddlesden–Popper Phases

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  21. Direct observation of charged domain walls in hybrid improper ferroelectric (Ca,Sr) 3 Ti 2 O 7

    Japanese Journal of Applied Physics · 2017-09-08

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  22. Retention Characteristics of Five‐Layered Aurivillus Films With Large Polarization

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  23. Theory and Neutrons Combine To Reveal a Family of Layered Perovskites without Inversion Symmetry

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  24. New Type of 2D Perovskites with Alternating Cations in the Interlayer Space, (C(NH 2 ) 3 )(CH 3 NH 3 ) n Pb n I 3 n +1 : Structure, Properties, and Photovoltaic Performance

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  25. Crystal Structure of Electroceramics

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  26. Nanoarchitectonics in dielectric/ferroelectric layered perovskites: from bulk 3D systems to 2D nanosheets

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  27. Bibliography

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  28. Insights into the polymorphism of Bi 2 W 2 O 9 : single crystal growth and a complete survey of the variable-temperature thermal and dielectric properties

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  29. Microstructure and Electric Properties of (Sr1−xCax)3Sn2O7 Ceramics with Ruddlesden-Popper Structure

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  30. High-throughput first-principles search for new ferroelectrics

    Physical review. B./Physical review. B · 2018-01-31

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  31. Ferroelectric Sr 3 Zr 2 O 7 : Competition between Hybrid Improper Ferroelectric and Antiferroelectric Mechanisms

    Advanced Functional Materials · 2018-05-28

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  32. Hybrid Improper Ferroelectricity in (Sr,Ca) 3 Sn 2 O 7 and Beyond: Universal Relationship between Ferroelectric Transition Temperature and Tolerance Factor in n = 2 Ruddlesden–Popper Phases

    Journal of the American Chemical Society · 2018-10-23

    Suguru Yoshida, Hirofumi Akamatsu, Ryosuke Tsuji, Olivier Hernandez, Haricharan Padmanabhan, Arnab Sen Gupta, Alexandra S. Gibbs, Ko Mibu, Shunsuke Murai, James M. Rondinelli, Venkatraman Gopalan, Katsuhisa Tanaka, Koji Fujita

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  33. Cation Exchange as a Mechanism To Engineer Polarity in Layered Perovskites

    Chemistry of Materials · 2018-11-26

    Tong Zhu, Guru Khalsa, Dana M. Havas, Alexandra S. Gibbs, Weiguo Zhang, P. Shiv Halasyamani, Nicole A. Benedek, Michael A. Hayward

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  34. Polarization rotation in Bi4Ti3O12 by isovalent doping at the fluorite sublattice

    Physical review. B./Physical review. B · 2019-01-02

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  35. Persistent spin helix in Rashba-Dresselhaus ferroelectric CsBiNb2O7

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  36. Temperature-Induced Structural Transformations in Undoped and Eu3+-Doped Ruddlesden–Popper Phases Sr2SnO4 and Sr3Sn2O7: Relation to the Impedance and Luminescence Behaviors

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  37. Magneto-electric multiferroics: designing new materials from first-principles calculations

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  38. Experimental and theoretical determination of physical properties of Sm 2 Bi 2 Fe 4 O 12 ferromagnetic semiconductors

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  39. Photocatalytic activity of 2D nanosheets of ferroelectric Dion–Jacobson compounds

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  40. Understanding the Energetics in Two-dimensional Metal Halide Perovskite Quantum Wells

    Unknown journal · 2020-01-01

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  41. Structural and optical properties of Fe-doped Ruddlesden-Popper Ca3Ti2-xFexO7-δ nanoparticles

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  42. Hidden improper ferroelectric phases for design of antiferroelectrics

    Journal of Physics Condensed Matter · 2020-03-02

    Nikita V. Ter-Oganessian, V. P. Sakhnenko

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  43. Complex Structural Phase Transitions of the Hybrid Improper Polar Dion–Jacobson Oxides RbNdM 2 O 7 and CsNdM 2 O 7 (M = Nb, Ta)

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  44. Bi2W2O9 : A potentially antiferroelectric Aurivillius phase

    Physical review. B./Physical review. B · 2020-04-29

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  45. Synergistic Influence of d0 (Nb5+) and d10 (Cd2+) Cations in Stabilizing Noncentrosymmetric Dion–Jacobson Layered Perovskites, A′Cd2Nb3O10 (A′ = Rb, Cs)

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    Shalu Atri, Meenakshi Pokhriyal, S. Uma

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  46. Ferroelectricity of Dion–Jacobson layered perovskites CsNdNb 2 O 7 and RbNdNb 2 O 7

    Japanese Journal of Applied Physics · 2020-08-07

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  47. Study of the microstructure and the optical, electrical, and magnetic feature of the Dy2Bi2Fe4O12 ferromagnetic semiconductor

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  48. Highly Tunable Ferroelectricity in Hybrid Improper Ferroelectric Sr3Sn2O7

    Advanced Functional Materials · 2020-08-19

    Xianghan Xu, Yazhong Wang, Fei‐Ting Huang, Kai Du, Elizabeth Nowadnick, Sang‐Wook Cheong

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  49. Polar Structures of KNdNb2O7and KNdTa2O7

    Chemistry of Materials · 2020-08-25

    Subhadip Mallick, Alexandra S. Gibbs, Weiguo Zhang, P. Shiv Halasyamani, Nicole A. Benedek, Michael A. Hayward

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  50. Beyond Expectation: Advanced Materials Design, Synthesis, and Processing to Enable Novel Ferroelectric Properties and Applications

    MRS Advances · 2020-09-08

    Jieun Kim, Eduardo Lupi, David Pesquera, Megha Acharya, Wenbo Zhao, Gabriel A. P. Velarde, Sinéad M. Griffin, Lane W. Martin

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