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RESEARCH PAPER · Chemistry of Materials · 2014

Semiconducting Properties and Phase-Matching Nonlinear Optical Response of the One-Dimensional Selenophosphates ANb2PSe10 (A = K, Rb, and Cs)

Jonathan C. Syrigos, Daniel J. Clark, Felix O. Saouma, Samantha M. Clarke, Lei Fang, Joon Ik Jang, Mercouri G. Kanatzidis

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Semiconducting Properties and Phase-Matching Nonlinear Optical Response of the One-Dimensional Selenophosphates ANb2PSe10 (A = K, Rb, and Cs)OriginalChemInform Abstract: Semiconducting Properties and Phase‐Matching Nonlinear Optical Response of the One‐Dimensional Selenophosphates ANb2PSe10 (A: K, Rb, and Cs).0Metal Thiophosphates with Good Mid-infrared Nonlinear Optical Performances: A First-Principles Prediction and Analysis441Beyond Single-Wavelength SHG Measurements: Spectrally-Resolved SHG Studies of Tetraphosphonate Ester Coordination Polymers31Syntheses, crystal structures and physical properties of three new chalcogenides: NaGaGe 3 Se 8 , K 3 Ga 3 Ge 7 S 20 , and K 3 Ga 3 Ge 7 Se 2018Syntheses, Structures, and Nonlinear Optical Properties of Two Sulfides Na2In2MS6 (M = Si, Ge)53Phase Transition, Conformational Exchange, and Nonlinear Optical Third Harmonic Generation of ACsP2Se8 (A = K, Rb, Cs)19Scandium Selenophosphates: Structure and Properties of K 4 Sc 2 (PSe 4 ) 2 (P 2 Se 6 )8Na 2 BaMQ 4 (M=Ge, Sn; Q=S, Se): Infrared Nonlinear Optical Materials with Excellent Performances and that Undergo Structural Transformations202Na2BaMQ4 (M=Ge, Sn; Q=S, Se): Infrared Nonlinear Optical Materials with Excellent Performances and that Undergo Structural Transformations44Non‐centrosymmetric Selenides AZn4In5Se12 (A=Rb, Cs): Synthesis, Characterization and Nonlinear Optical Properties47Recent achievements on middle and far-infrared second-order nonlinear optical materials433Ba 6 Li 2 CdSn 4 S 16 : lithium substitution simultaneously enhances band gap and SHG intensity44Two excellent phase-matchable infrared nonlinear optical materials based on 3D diamond-like frameworks: RbGaSn 2 Se 6 and RbInSn 2 Se 639Superpolyhedron-Built Second Harmonic Generation Materials Exhibit Large Mid-Infrared Conversion Efficiencies and High Laser-Induced Damage Thresholds101ABi2(IO3)2F5 (A=K, Rb, and Cs): A Combination of Halide and Oxide Anionic Units To Create a Large Second‐Harmonic Generation Response with a Wide Bandgap140ABi2(IO3)2F5 (A=K, Rb, and Cs): A Combination of Halide and Oxide Anionic Units To Create a Large Second‐Harmonic Generation Response with a Wide Bandgap36A review on structure-performance relationship toward the optimal design of infrared nonlinear optical materials with balanced performances253A 2 SrM IV S 4 (A = Li, Na; M IV = Ge, Sn) concurrently exhibiting wide bandgaps and good nonlinear optical responses as new potential infrared nonlinear optical materials78Ba 6 In 6 Zn 4 Se 19 : a high performance infrared nonlinear optical crystal with [InSe 3 ] 3− trigonal planar functional motifs22[ABa2Cl][Ga4S8] (A = Rb, Cs): Wide-Spectrum Nonlinear Optical Materials Obtained by Polycation-Substitution-Induced Nonlinear Optical (NLO)-Functional Motif Ordering270Chalcophosphates: A Treasure House of Infrared Nonlinear Optical Materials75Design and synthesis of Ba 3 SiSe 5 with suitable birefringence modulated via M IV atoms in the Ba–M IV –Q (M IV = Si, Ge; Q = S, Se) system3Synthesis, crystal growth and characterization of semi-organic NLO materials: L-valine copper chloride as optoelectronic sensor9Synthesis, structure, linear and nonlinear optical properties of noncentrosymmetric quaternary diamond-like semiconductors, Cu2ZnGeSe4 (CZGSe) and the novel Cu4ZnGe2Se720Investigation into Structural Variation from 3D to 1D and Strong Second Harmonic Generation of the AHgPS4 (A+ = Na+, K+, Rb+, Cs+) Family26Structural modification from centrosymmetric Rb 4 Hg 2 Ge 2 S 8 to noncentrosymmetric (Na 3 Rb)Hg 2 Ge 2 S 8 : mixed alkali metals strategy for infrared nonlinear optical material design28Cs 3 In(In 4 Se 7 )(P 2 Se 6 ): A Multi‐Chromophore Chalcogenide with Excellent Nonlinear Optical Property Designed by Group Grafting55Cs3In(In4Se7)(P2Se6): A Multi‐Chromophore Chalcogenide with Excellent Nonlinear Optical Property Designed by Group Grafting2Vacancy‐Induced Extraordinary Second Harmonic Generation Response for Diamond‐Like Cu3PS49Carbonatoperoxovanadates with Strong Second‐Harmonic Generation: Insights from First‐Principles Calculations on Anisotropic Structures and Optical Parameters0Design of a high-performance infrared birefringent crystal Ba 4 HgP 2 Se 10 via a low-dimensional motif intercalation strategy2Growth, structural characterization, enhanced NLO and optoelectronic properties of L-valine-based semi-organic crystals doped with CdCl2 and CuCl22NbGa 2 S 4 (S 2 ): A Rare Linear [S 2 ] 2− Coordination to Niobium Resulting in Simultaneously Large SHG Effect and Giant Birefringence20NbGa 2 S 4 (S 2 ): A Rare Linear [S 2 ] 2− Coordination to Niobium Resulting in Simultaneously Large SHG Effect and Giant Birefringence6ANb 2 (PS 4 )(S 2 ) 3 (A = K, Rb, Cs): the first Nb-based NLO thiophosphates with [NbS 2 (S 2 ) 3 ] and [Nb 2 PS 6 (S 2 ) 4 ] units exhibiting tri-state structural transformation and high performance6

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  1. ChemInform Abstract: Semiconducting Properties and Phase‐Matching Nonlinear Optical Response of the One‐Dimensional Selenophosphates ANb2PSe10 (A: K, Rb, and Cs).

    ChemInform · 2015-03-01

    Jonathan C. Syrigos, Daniel J. Clark, Felix O. Saouma, Samantha M. Clarke, Lei Fang, Joon Ik Jang, Mercouri G. Kanatzidis

    Read original paper ↗ ·

  2. Metal Thiophosphates with Good Mid-infrared Nonlinear Optical Performances: A First-Principles Prediction and Analysis

    Journal of the American Chemical Society · 2015-09-23

    Lei Kang, Molin Zhou, Jiyong Yao, Zheshuai Lin, Yicheng Wu, Chuangtian Chen

    Read original paper ↗ ·

  3. Beyond Single-Wavelength SHG Measurements: Spectrally-Resolved SHG Studies of Tetraphosphonate Ester Coordination Polymers

    Inorganic Chemistry · 2015-10-22

    Jan K. Zaręba, Michał J. Białek, Jan Janczak, Marcin Nyk, Jerzy Zoń, Marek J. Samoc

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  4. Syntheses, crystal structures and physical properties of three new chalcogenides: NaGaGe 3 Se 8 , K 3 Ga 3 Ge 7 S 20 , and K 3 Ga 3 Ge 7 Se 20

    Dalton Transactions · 2015-11-09

    Xiaoshuang Li, Chao Li, Pifu Gong, Zheshuai Lin, Jiyong Yao, Yicheng Wu

    Read original paper ↗ ·

  5. Syntheses, Structures, and Nonlinear Optical Properties of Two Sulfides Na2In2MS6 (M = Si, Ge)

    Inorganic Chemistry · 2016-02-04

    Shu‐Fang Li, Bin‐Wen Liu, Mingjian Zhang, Yuhang Fan, Hui‐Yi Zeng, Guo‐Cong Guo

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  6. Phase Transition, Conformational Exchange, and Nonlinear Optical Third Harmonic Generation of ACsP2Se8 (A = K, Rb, Cs)

    Chemistry of Materials · 2016-03-17

    Alyssa S. Haynes, Abhishek Banerjee, Felix O. Saouma, Calford Odhiambo Otieno, Joon Ik Jang, Mercouri G. Kanatzidis

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  7. Scandium Selenophosphates: Structure and Properties of K 4 Sc 2 (PSe 4 ) 2 (P 2 Se 6 )

    Inorganic Chemistry · 2016-04-14

    Jonathan C. Syrigos, Mercouri G. Kanatzidis

    Read original paper ↗ ·

  8. Na 2 BaMQ 4 (M=Ge, Sn; Q=S, Se): Infrared Nonlinear Optical Materials with Excellent Performances and that Undergo Structural Transformations

    Angewandte Chemie International Edition · 2016-04-21

    Kui Wu, Zhihua Yang, Shilie Pan

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  9. Na2BaMQ4 (M=Ge, Sn; Q=S, Se): Infrared Nonlinear Optical Materials with Excellent Performances and that Undergo Structural Transformations

    Angewandte Chemie · 2016-04-21

    Kui Wu, Zhihua Yang, Shilie Pan

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  10. Non‐centrosymmetric Selenides AZn4In5Se12 (A=Rb, Cs): Synthesis, Characterization and Nonlinear Optical Properties

    Chemistry - An Asian Journal · 2016-12-01

    Hua Lin, Yu‐Jun Zheng, Xiaoning Hu, Hong Chen, Ju‐Song Yu, Li‐Ming Wu

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  11. Recent achievements on middle and far-infrared second-order nonlinear optical materials

    Coordination Chemistry Reviews · 2016-12-27

    Sheng‐Ping Guo, Yang Chi, Guo‐Cong Guo

    Read original paper ↗ ·

  12. Ba 6 Li 2 CdSn 4 S 16 : lithium substitution simultaneously enhances band gap and SHG intensity

    Journal of Materials Chemistry C · 2017-01-01

    Ruihuan Duan, Pengfei Liu, Hua Lin, Yi‐Wen Zheng, Ju‐Song Yu, Xin‐Tao Wu, Shangxiong Huangfu, Ling Chen

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  13. Two excellent phase-matchable infrared nonlinear optical materials based on 3D diamond-like frameworks: RbGaSn 2 Se 6 and RbInSn 2 Se 6

    Dalton Transactions · 2017-01-01

    Hua Lin, Hong Chen, Yujun Zheng, Ju‐Song Yu, Xin‐Tao Wu, Li‐Ming Wu

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  14. Superpolyhedron-Built Second Harmonic Generation Materials Exhibit Large Mid-Infrared Conversion Efficiencies and High Laser-Induced Damage Thresholds

    Chemistry of Materials · 2017-01-30

    Shu‐Fang Li, Xiao‐Ming Jiang, Bin‐Wen Liu, Dong Yan, Chensheng Lin, Hui‐Yi Zeng, Guo‐Cong Guo

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  15. ABi2(IO3)2F5 (A=K, Rb, and Cs): A Combination of Halide and Oxide Anionic Units To Create a Large Second‐Harmonic Generation Response with a Wide Bandgap

    Angewandte Chemie International Edition · 2017-06-20

    Hongming Liu, Qi Wu, Xingxing Jiang, Zheshuai Lin, Xiang‐Gao Meng, Xingguo Chen, Jingui Qin

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  16. ABi2(IO3)2F5 (A=K, Rb, and Cs): A Combination of Halide and Oxide Anionic Units To Create a Large Second‐Harmonic Generation Response with a Wide Bandgap

    Angewandte Chemie · 2017-06-20

    Hongming Liu, Qi Wu, Xingxing Jiang, Zheshuai Lin, Xiang‐Gao Meng, Xingguo Chen, Jingui Qin

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  17. A review on structure-performance relationship toward the optimal design of infrared nonlinear optical materials with balanced performances

    Coordination Chemistry Reviews · 2018-09-20

    Kui Wu, Shilie Pan

    Read original paper ↗ ·

  18. A 2 SrM IV S 4 (A = Li, Na; M IV = Ge, Sn) concurrently exhibiting wide bandgaps and good nonlinear optical responses as new potential infrared nonlinear optical materials

    Chemical Science · 2019-01-01

    Kui Wu, Yu Chu, Zhihua Yang, Shilie Pan

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  19. Ba 6 In 6 Zn 4 Se 19 : a high performance infrared nonlinear optical crystal with [InSe 3 ] 3− trigonal planar functional motifs

    Journal of Materials Chemistry C · 2020-01-01

    Anyi Zhou, Chensheng Lin, Bingxuan Li, Wen‐Dan Cheng, Zhengxiao Guo, Zhufeng Hou, Fang-Yu Yuan, Guoliang Chai

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  20. [ABa2Cl][Ga4S8] (A = Rb, Cs): Wide-Spectrum Nonlinear Optical Materials Obtained by Polycation-Substitution-Induced Nonlinear Optical (NLO)-Functional Motif Ordering

    Journal of the American Chemical Society · 2020-05-29

    Bin‐Wen Liu, Xiao‐Ming Jiang, Hui‐Yi Zeng, Guo‐Cong Guo

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  21. Chalcophosphates: A Treasure House of Infrared Nonlinear Optical Materials

    Crystal Growth & Design · 2020-10-23

    Zhuang Li, Jiyong Yao, Yicheng Wu

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  22. Design and synthesis of Ba 3 SiSe 5 with suitable birefringence modulated via M IV atoms in the Ba–M IV –Q (M IV = Si, Ge; Q = S, Se) system

    Dalton Transactions · 2021-01-01

    Huanhuan Cheng, Abudukadi Tudi, Peng Wang, Kewang Zhang, Zhihua Yang, Shilie Pan

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  23. Synthesis, crystal growth and characterization of semi-organic NLO materials: L-valine copper chloride as optoelectronic sensor

    Indian Journal of Physics · 2021-02-24

    N. Sheen Kumar, S. L. Rayar

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  24. Synthesis, structure, linear and nonlinear optical properties of noncentrosymmetric quaternary diamond-like semiconductors, Cu2ZnGeSe4 (CZGSe) and the novel Cu4ZnGe2Se7

    Journal of Alloys and Compounds · 2021-08-09

    Charles W. Sinagra, Felix O. Saouma, Calford Odhiambo Otieno, Saul H. Lapidus, Jian‐Han Zhang, Andrew J. Craig, P. Grima, Jacilynn A. Brant, Kimberly A. Rosmus, Kate E. Rosello, Joon Ik Jang, Jennifer A. Aitken

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  25. Investigation into Structural Variation from 3D to 1D and Strong Second Harmonic Generation of the AHgPS4 (A+ = Na+, K+, Rb+, Cs+) Family

    Inorganic Chemistry · 2021-11-12

    Wenhao Xing, Chunlan Tang, Pifu Gong, Jieyun Wu, Zheshuai Lin, Jiyong Yao, Wenlong Yin, Bin Kang

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  26. Structural modification from centrosymmetric Rb 4 Hg 2 Ge 2 S 8 to noncentrosymmetric (Na 3 Rb)Hg 2 Ge 2 S 8 : mixed alkali metals strategy for infrared nonlinear optical material design

    Journal of Materials Chemistry C · 2021-12-15

    Chunlan Tang, Wenhao Xing, Fei Liang, Mengran Sun, Jian Tang, Zheshuai Lin, Jiyong Yao, Kaixin Chen, Jieyun Wu, Wenlong Yin, Bin Kang

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  27. Cs 3 In(In 4 Se 7 )(P 2 Se 6 ): A Multi‐Chromophore Chalcogenide with Excellent Nonlinear Optical Property Designed by Group Grafting

    Angewandte Chemie International Edition · 2024-02-01

    Zhen Qian, Hongping Wu, Zhanggui Hu, Jiyang Wang, Yicheng Wu, Hongwei Yu

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  28. Cs3In(In4Se7)(P2Se6): A Multi‐Chromophore Chalcogenide with Excellent Nonlinear Optical Property Designed by Group Grafting

    Angewandte Chemie · 2024-02-02

    Zhen Qian, Hongping Wu, Zhanggui Hu, Jiyang Wang, Yicheng Wu, Hongwei Yu

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  29. Vacancy‐Induced Extraordinary Second Harmonic Generation Response for Diamond‐Like Cu3PS4

    Advanced Optical Materials · 2024-04-10

    Weiping Guo, Yudi Fu, Hong‐Hua Cui, Lingyun Li, Yan Yu, Zhong‐Zhen Luo, Zhigang Zou

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  30. Carbonatoperoxovanadates with Strong Second‐Harmonic Generation: Insights from First‐Principles Calculations on Anisotropic Structures and Optical Parameters

    ChemPlusChem · 2024-10-11

    Jinyu Hu, Yuxin Hu, Hui Zhu, Hui‐Yan Zhao, Chao He, Xihu Wang

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  31. Design of a high-performance infrared birefringent crystal Ba 4 HgP 2 Se 10 via a low-dimensional motif intercalation strategy

    Dalton Transactions · 2025-01-01

    Zhihui Xiong, Haotian Tian, Zhixi Li, Guowei Deng, Fang Ding, Qian Wu, Mingjun Xia

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  32. Growth, structural characterization, enhanced NLO and optoelectronic properties of L-valine-based semi-organic crystals doped with CdCl2 and CuCl2

    Journal of Molecular Structure · 2025-05-27

    N. Sheen Kumar, V. Vijimon Moni, M. Gerald Arul Selvan, Bright Brailson Mansingh, Joseph Selvi Binoj

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  33. NbGa 2 S 4 (S 2 ): A Rare Linear [S 2 ] 2− Coordination to Niobium Resulting in Simultaneously Large SHG Effect and Giant Birefringence

    Angewandte Chemie International Edition · 2025-05-29

    Wenli Zhao, Rui‐Xi Wang, Shuang Zhao, Li‐Ming Wu, Ling Chen

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  34. NbGa 2 S 4 (S 2 ): A Rare Linear [S 2 ] 2− Coordination to Niobium Resulting in Simultaneously Large SHG Effect and Giant Birefringence

    Angewandte Chemie · 2025-05-29

    Wenli Zhao, Rui‐Xi Wang, Shuang Zhao, Li‐Ming Wu, Ling Chen

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  35. ANb 2 (PS 4 )(S 2 ) 3 (A = K, Rb, Cs): the first Nb-based NLO thiophosphates with [NbS 2 (S 2 ) 3 ] and [Nb 2 PS 6 (S 2 ) 4 ] units exhibiting tri-state structural transformation and high performance

    Inorganic Chemistry Frontiers · 2025-12-09

    Zong-Ze Li, Yang Chi, Yu-Xuan Zhang, Ao Guo, Hui-Zhi Gao, Zheng-Ren Chen, Mao-Yin Ran, Wenlong Liu, Sheng-Ping Guo

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