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RESEARCH PAPER · Chemical Science · 2024

A bifunctional primitive strategy induces enhancements of large second harmonic generation and wide UV transmittance in rare-earth borates containing [B 5 O 10 ] groups

Shuaifeng Li, Weiming Li, Xiang Li, Guangsai Yang, Ning Ye, Zhanggui Hu, Yicheng Wu, Conggang Li

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A bifunctional primitive strategy induces enhancements of large second harmonic generation and wide UV transmittance in rare-earth borates containing [B 5 O 10 ] groupsOriginalLarge second harmonic generation and birefringence from extended octupolar π-conjugated structures35A Rare-Earth-Based Borate Optical Crystal with Enlarged Dihedral Angles of Distinct [BO3] Groups Exhibiting a Wide UV Transparent Range8Chemical substitution towards a rare-earth borate ultraviolet NLO crystal exhibiting a strong SHG response17K6NaCaRe2(B5O10)3 (Re = Y, Lu): Two NLO Compounds Exhibiting a Short Absorption Edge in the A7–xA’xAeRe2(B5O10)3 (x = 0, 1) Family4A new structure type of the Na3Yb(BO3)2: Synthesis, crystal structure, thermal behavior, ionic conductivity, and spectroscopy2Designing rare earth borates as UV nonlinear optical crystals exhibiting strong second-harmonic generation responses15KNa 2 Y 2 B 2 O 6 F 3 : a beryllium free deep-UV nonlinear optical crystal with well-balanced properties2Synthesising a series of promising ultraviolet nonlinear optical materials with the aid of the flexibility of isolated [B 5 O 10 ] groups3Two alkali metal borates built by {Li@B 14 } and {B 15 } cluster units1Assembly of π-conjugated [B3O7] groups by unprecedented antiparallel triangles [ZnO3] to tailor a deep-UV zinc borate birefringent crystal6Tuning Birefringence in Supramolecular Mg-PDA Frameworks: Modulating Bonding and Layer Connectivity0Syntheses, structural characterization, and nonlinear optical properties of mixed alkaline/alkaline earth metal borophosphates1Promising UV/DUV nonlinear optical materials with X-membered (X = multiples of 6) rings in anhydrous inorganic borates20Design and Synthesis of a Rare Earth Borate Ultraviolet Nonlinear Optical Crystal K 3 Lu 2 (BO 3 ) 38Investigation on growth, structural, spectral and nonlinear properties of novel Mannich base material 1-((benzylamino)(phenyl)methyl) napthalen-2-ol0Tailoring ordered structures with distorted [TeO 3 ] and aligned [ScO 6 ] motifs for balanced nonlinear optical properties in rare-earth tellurate crystals5Halogen-ion-driven polymorphs for high-performance nonlinear optical crystalline materials3Two scandium borate UV NLO crystals designed through chemical element substitution1Pyrazole‐Protected Heteronuclear Rare‐Earth Boron‐Oxo Cluster Cage With Tunable Luminescence0Covalent Interlayer Engineering Enables Ideal Birefringence and Strong SHG in Beryllium‐Free Deep‐UV NLO Borates2A Rare-Earth Borophosphate Ultraviolet Nonlinear Optical Crystal Featuring P–O–P Linkages0Cation‐Regulated [CH 3 BO 2 F]‐Derived Borates: Synergistic Fluorination and Organic Functionalization for High‐Birefringence UV NLO Materials0

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  1. Large second harmonic generation and birefringence from extended octupolar π-conjugated structures

    Chemical Science · 2024-01-01

    Danyang Dou, Bingbing Zhang, Daqing Yang, Ying Wang

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  2. A Rare-Earth-Based Borate Optical Crystal with Enlarged Dihedral Angles of Distinct [BO3] Groups Exhibiting a Wide UV Transparent Range

    Inorganic Chemistry · 2024-07-26

    Jie Song, Xianghao Kong, Conggang Li, Jinmiao Jiao, Yuheng She, Ning Ye, Zhanggui Hu, Yicheng Wu

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  3. Chemical substitution towards a rare-earth borate ultraviolet NLO crystal exhibiting a strong SHG response

    Inorganic Chemistry Frontiers · 2024-11-21

    Xianghao Kong, Jing Chai, Huijian Zhao, Ning Ye, Zhanggui Hu, Yicheng Wu, Conggang Li

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  4. K6NaCaRe2(B5O10)3 (Re = Y, Lu): Two NLO Compounds Exhibiting a Short Absorption Edge in the A7–xA’xAeRe2(B5O10)3 (x = 0, 1) Family

    Inorganic Chemistry · 2024-12-19

    Wencong Li, Zhaowei Hu, Yanyan Ding, Yueting Zhu, Qun Jing, Lili Liu

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  5. A new structure type of the Na3Yb(BO3)2: Synthesis, crystal structure, thermal behavior, ionic conductivity, and spectroscopy

    Solid State Sciences · 2024-12-31

    Alexey Karpovich Subanakov, Evgeniy V. Kovtunets, Tatyana Sergeevna Spiridonova, Andrey Sobolev, Мaxim S. Моlokeev, Dmitry Olegovich Sofich, Alexandr Bogdanov, Баир Гармаевич Базаров

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  6. Designing rare earth borates as UV nonlinear optical crystals exhibiting strong second-harmonic generation responses

    Chemical Communications · 2025-01-01

    Mengru Liu, Xianghao Kong, Shuaifeng Li, Ning Ye, Zhanggui Hu, Yicheng Wu, Conggang Li

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  7. KNa 2 Y 2 B 2 O 6 F 3 : a beryllium free deep-UV nonlinear optical crystal with well-balanced properties

    Chemical Communications · 2025-01-01

    Huijian Zhao, Mengru Liu, Weina Nan, Ning Yang, Conggang Li, Ning Ye, Zhanggui Hu

    Read original paper ↗ ·

  8. Synthesising a series of promising ultraviolet nonlinear optical materials with the aid of the flexibility of isolated [B 5 O 10 ] groups

    Dalton Transactions · 2025-01-01

    Yixin Song, Hongwei Yu, Hongping Wu, Zhanggui Hu, Jiyang Wang, Yicheng Wu

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  9. Two alkali metal borates built by {Li@B 14 } and {B 15 } cluster units

    Dalton Transactions · 2025-01-01

    Mian Li, Dan Qin, Juan Chen, Qi Wei, Guo‐Yu Yang

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  10. Assembly of π-conjugated [B3O7] groups by unprecedented antiparallel triangles [ZnO3] to tailor a deep-UV zinc borate birefringent crystal

    Chinese Chemical Letters · 2025-01-07

    Ning Yang, Huijian Zhao, Wenli Zhao, Yuheng She, Ning Ye, Zhanggui Hu, Conggang Li

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  11. Tuning Birefringence in Supramolecular Mg-PDA Frameworks: Modulating Bonding and Layer Connectivity

    Inorganic Chemistry · 2025-03-21

    Miao‐Bin Xu, Ning Yu, Jiajia Li, Mingchang Wang, Mo-Fan Zhuo, Ke‐Zhao Du, Jin Chen, Yan Chen

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  12. Syntheses, structural characterization, and nonlinear optical properties of mixed alkaline/alkaline earth metal borophosphates

    Journal of Solid State Chemistry · 2025-08-19

    Yang Pan, Jian Qiu Deng, Yucheng Hao, Xi Zhao, Yuanyuan Bao, Zixuan Fang, Chonghai Deng, Kunhong Hu, Wei Cheng, Yuan Hua Lin

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  13. Promising UV/DUV nonlinear optical materials with X-membered (X = multiples of 6) rings in anhydrous inorganic borates

    Coordination Chemistry Reviews · 2025-08-26

    Bailin Chen, Shuai An, Xueling Hou, Shilie Pan

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  14. Design and Synthesis of a Rare Earth Borate Ultraviolet Nonlinear Optical Crystal K 3 Lu 2 (BO 3 ) 3

    Inorganic Chemistry · 2025-10-20

    Mingyue Gu, Xianchao Zhu, Zhanggui Hu, Yicheng Wu

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  15. Investigation on growth, structural, spectral and nonlinear properties of novel Mannich base material 1-((benzylamino)(phenyl)methyl) napthalen-2-ol

    Journal of Molecular Structure · 2025-11-06

    M. Shankar, A. Dennis Raj, Mani Jeeva, R. Purusothaman, I. Vetha Potheher

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  16. Tailoring ordered structures with distorted [TeO 3 ] and aligned [ScO 6 ] motifs for balanced nonlinear optical properties in rare-earth tellurate crystals

    Chemical Science · 2025-11-18

    Xiaoxu Wang, Tinghui Zhang, Huijian Zhao, Ning Jia, Hongjun Liu, Ning Ye, Zhanggui Hu, Conggang Li

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  17. Halogen-ion-driven polymorphs for high-performance nonlinear optical crystalline materials

    Chemical Science · 2026-01-01

    Yuwei Kang, Can Hui Yang, Yunjie Wang, Qi Wu

    Read original paper ↗ ·

  18. Two scandium borate UV NLO crystals designed through chemical element substitution

    Chemical Communications · 2026-01-01

    Zelong Liu, Huijian Zhao, Longyun Xu, Ning Jia, Ning Ye, Zhanggui Hu, Conggang Li

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  19. Pyrazole‐Protected Heteronuclear Rare‐Earth Boron‐Oxo Cluster Cage With Tunable Luminescence

    Small · 2026-03-18

    Jiang‐Hong Fu, Pan‐Pan Zhao, Xiang‐Ming Zhang, J. B. Chen, Hai-Xia Zhang, Jian Zhang

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  20. Covalent Interlayer Engineering Enables Ideal Birefringence and Strong SHG in Beryllium‐Free Deep‐UV NLO Borates

    Advanced Functional Materials · 2026-07-10

    Huijian Zhao, Kangyan Fan, Conggang Li, Zelong Liu, Pifu Gong, Ning Ye, Zhanggui Hu

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  21. A Rare-Earth Borophosphate Ultraviolet Nonlinear Optical Crystal Featuring P–O–P Linkages

    Inorganic Chemistry · 2026-08-08

    Hanjing Huang, Huijian Zhao, Wenli Zhao, Xianchao Zhu, Ning Ye, Zhanggui Hu, Conggang Li

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  22. Cation‐Regulated [CH 3 BO 2 F]‐Derived Borates: Synergistic Fluorination and Organic Functionalization for High‐Birefringence UV NLO Materials

    Small · 2026-10-11

    Haoran Wang, Haotian Qiu, chenxu li, Xue Bai, Qingyu Liu, Zhihua Yang, Min Zhang

    Read original paper ↗ ·
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