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RESEARCH PAPER · Inorganic Chemistry Frontiers · 2024

Hg 3 AsS 4 X (X = Cl and Br): two Hg-based chalcogenides as long-wave infrared nonlinear optical crystals with superior comprehensive performances

Feng Xu, Xiang Xu, Bingxuan Li, Ge Zhang, Chan Zheng, Jindong Chen, Ning Ye

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Hg 3 AsS 4 X (X = Cl and Br): two Hg-based chalcogenides as long-wave infrared nonlinear optical crystals with superior comprehensive performancesOriginalNoncentrosymmetric tellurite halides created by a depolymerization strategy: toward strong SHG intensity and wide bandgap16RbPbPS 4 : a promising IR nonlinear optical material achieved by lone-pair-cation-substitution-induced structure transformation23Salt-inclusion chalcogenides with d-orbital components: unveiling remarkable nonlinear optical properties and dual-band photoluminescence10A congruent-melting rubidium zinc vanadium oxychloride exhibiting strong mid-infrared second-harmonic generation and high laser-induced damage threshold6Recent advances and future perspectives on rare-earth-based nonlinear optical materials with π-conjugated [XO3] (X = B, C, N) units66A Congruent-Melt Infrared Nonlinear Optical Crystal Na4SrAs2S83Crystal Engineering of Three Novel 1-D Chalcogenidostannates Using Lanthanide Complexes as Structure-Directing Agents: Synthesis, Structure, and Photoelectric Performance Evaluation5Exploring new horizons in mid-to-far infrared nonlinear optical crystals: the significant potential of trigonal pyramidal [TeS 3 ] 2− functional units18Structural diversity and photocurrent responses of multi-component chalcogenidometalates8Surfactant-assisted synthesis of semiconductor hybrid Cd/Hg-selenidostannates with enhanced optoelectronic and piezoelectric properties0First-Principles High-Throughput Screening and Experimental Verification of III-VIB Transition Metal Chalcogenides Nonlinear Optical Crystals16From Orthorhombic Cu8GeS6 to Cubic Cu6HgGeS6: Second-Harmonic Generation and Photocurrent Responses7Recent progress in structural design strategies of high-birefringence optical crystals55Syntheses and characterisation of two lanthanide compounds with upconversion luminescence0Syntheses, structures and properties of two co-crystallized complexes constructed from lanthanide isonicotinates and mercury halides0[TeSeS 2 ] 2− : The First Heterotriple‐Chalcogenide Motifs Decode Giant Mid‐Far Infrared Birefringence18[TeSeS 2 ] 2− : The First Heterotriple‐Chalcogenide Motifs Decode Giant Mid‐Far Infrared Birefringence4Cd 7 I 12 Q·As 4 Q n (Q = S, Se; n = 3, 4): In Situ Alteration of Functional Molecules in Polar Metal Inorganic Framework Tailoring High‐Performance Infrared Nonlinear Optical Crystals9Research progress and future prospect of chalcogenides with large optical anisotropy46Nonlinear Optical Series A(VO2)3(SeO3)2 (A = NH4+, K+, and H3O+) with Large Birefringence Derived from High-Anisotropic VO6 Octahedra and SeO3 Pyramids9Diamond-Like HgIn2Q4 (Q = Se, Te) Synthesized by Flux-Assisted Boron-Chalcogen Method Exhibit Noteworthy Nonlinear Optical Properties Contributed by Three Types of Tetrahedral Motifs9Dual‐Sided Multidentate Coordination Strategy Enables Record Birefringence in UV‐Transparent Antimony‐Based Hybrid Crystals37Dual‐Sided Multidentate Coordination Strategy Enables Record Birefringence in UV‐Transparent Antimony‐Based Hybrid Crystals12Controlling d10 Metal in Phenylthiourea‐Based Hybrid Metal Halides to Actualize Dimensional Transformation and Significantly Improve the Birefringence11Structure-property relationships in IR nonlinear optical chalcogenides with stereochemically active lone pairs29SrZnSiS4: Shattering the 4.0 eV Threshold toward Dual-Optimized Bandgap and Second-Harmonic Generation7Five-Membered [C 5 O 5 ] 2 – Rings as Birefringence-Active Genes for Ultrabirefringent Crystals28Achieving giant optical anisotropy in the mid-far infrared region via ideal alignment of dual functional motifs0van der Waals layered CuInP 2 S 6 as infrared nonlinear optical material1Cd/V Ratio-Driven Centrosymmetric Transition of Crystal Structures in Cesium Cadmium Vanadate Oxychlorides Cs 3 CdV 4 O 12 Cl and CsCdV 2 O 6 Cl0Thermo-mechanical stability and strong optical absorption in quaternary chalcogenides ACdCu3Se4 (A = Sc, Y): a first-principles study0Cation-substitution-driven electronic, nonlinear optical, elastic, and thermal transport properties of layered AeHgGeSe4 (Ae = Ba, Sr): A first-principles study0Domino‐Effect Amplification via Covalent‐Chain Engineering for Giant Birefringence in NaAsQ 2 (Q = S, Se) Crystals0

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  1. Noncentrosymmetric tellurite halides created by a depolymerization strategy: toward strong SHG intensity and wide bandgap

    Chemical Science · 2024-01-01

    Dandan Zhou, Chun‐Li Hu, Xinwei Zhang, Jiang‐Gao Mao, Fang Kong

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  2. RbPbPS 4 : a promising IR nonlinear optical material achieved by lone-pair-cation-substitution-induced structure transformation

    Inorganic Chemistry Frontiers · 2024-01-01

    A-Yang Wang, Sheng-Hua Zhou, Mao‐Yin Ran, Bingxuan Li, Xin‐Tao Wu, Hua Lin, Qi‐Long Zhu

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  3. Salt-inclusion chalcogenides with d-orbital components: unveiling remarkable nonlinear optical properties and dual-band photoluminescence

    Chemical Science · 2024-01-01

    Shao‐Min Pei, Ming‐Shu Zhang, Fan Wu, Yan Guo, Xiao‐Ming Jiang, Bin‐Wen Liu, Guo‐Cong Guo

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  4. A congruent-melting rubidium zinc vanadium oxychloride exhibiting strong mid-infrared second-harmonic generation and high laser-induced damage threshold

    Journal of Alloys and Compounds · 2024-04-14

    Lei Geng, Wenfei Li, Chang‐Yu Meng, You‐Zhao Lan, Baozhu Zhu, Shihua Ma, Qi Wu

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  5. Recent advances and future perspectives on rare-earth-based nonlinear optical materials with π-conjugated [XO3] (X = B, C, N) units

    Coordination Chemistry Reviews · 2024-07-03

    Bo Zhang, Mao‐Yin Ran, Xin‐Tao Wu, Hua Lin, Qi‐Long Zhu

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  6. A Congruent-Melt Infrared Nonlinear Optical Crystal Na4SrAs2S8

    Inorganic Chemistry · 2024-07-31

    Zhihui Xiong, Aoge Yao, Zhixi Li, Xianghe Meng, Qian Wu, Guowei Deng, Lei Kang, Mingjun Xia

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  7. Crystal Engineering of Three Novel 1-D Chalcogenidostannates Using Lanthanide Complexes as Structure-Directing Agents: Synthesis, Structure, and Photoelectric Performance Evaluation

    Crystal Growth & Design · 2024-08-09

    Huiling Zhao, Lirong Zhang, Xin Liu, Gele Teri, E. Namila, Menghe Baiyin

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  8. Exploring new horizons in mid-to-far infrared nonlinear optical crystals: the significant potential of trigonal pyramidal [TeS 3 ] 2− functional units

    Chemical Science · 2025-01-01

    Bo Zhang, Sheng-Hua Zhou, Bingxuan Li, Xin‐Tao Wu, Hua Lin, Qi‐Long Zhu

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  9. Structural diversity and photocurrent responses of multi-component chalcogenidometalates

    Inorganic Chemistry Frontiers · 2025-01-01

    Chang Liu, Wen-Jing Tian, Mao‐Yin Ran, Pan Gao, Panpan Jing, Yi Liu, Hua Lin

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  10. Surfactant-assisted synthesis of semiconductor hybrid Cd/Hg-selenidostannates with enhanced optoelectronic and piezoelectric properties

    Inorganic Chemistry Frontiers · 2025-01-01

    Mohamed Saber Lassoued, Yue‐Qiao Hu, Faizan Ahmad, Yan‐Zhen Zheng

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  11. First-Principles High-Throughput Screening and Experimental Verification of III-VIB Transition Metal Chalcogenides Nonlinear Optical Crystals

    Chemistry of Materials · 2025-01-23

    Miao Song, Hongbo Huang, Baoli Gao, Yumiao Niu, Ying Wang, Daqing Yang, Bingbing Zhang

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  12. From Orthorhombic Cu8GeS6 to Cubic Cu6HgGeS6: Second-Harmonic Generation and Photocurrent Responses

    Inorganic Chemistry · 2025-04-24

    Qiu-Yang Du, Shanshan Han, Wen‐Dong Yao, Xu-Bin Ni, Wenfeng Zhou, Wenlong Liu, Sheng‐Ping Guo

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  13. Recent progress in structural design strategies of high-birefringence optical crystals

    Coordination Chemistry Reviews · 2025-05-08

    A-Lan Xu, Mao‐Yin Ran, Xintao Wu, Hua Lin, Qi‐Long Zhu

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  14. Syntheses and characterisation of two lanthanide compounds with upconversion luminescence

    Emerging Materials Research · 2025-05-29

    Hao-Dong Liu, Xi-Yu Shao, Yu-Yue Xu, Long-Hua Zeng, Wen‐Tong Chen, Cheng Liu

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  15. Syntheses, structures and properties of two co-crystallized complexes constructed from lanthanide isonicotinates and mercury halides

    Inorganic Chemistry Communications · 2025-05-31

    Xi-Yu Shao, Hao-Dong Liu, Hao-Dong Liu, Long-Hua Zeng, Wei Wang, Chang-Wang Pan, Cheng Liu, Wen‐Tong Chen

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  16. [TeSeS 2 ] 2− : The First Heterotriple‐Chalcogenide Motifs Decode Giant Mid‐Far Infrared Birefringence

    Angewandte Chemie International Edition · 2025-06-17

    Bo Zhang, Wei‐Qi Huang, Jiaxiang Zhang, Xintao Wu, Hua Lin, Qi‐Long Zhu

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  17. [TeSeS 2 ] 2− : The First Heterotriple‐Chalcogenide Motifs Decode Giant Mid‐Far Infrared Birefringence

    Angewandte Chemie · 2025-06-17

    Bo Zhang, Wei‐Qi Huang, Jiaxiang Zhang, Xintao Wu, Hua Lin, Qi‐Long Zhu

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  18. Cd 7 I 12 Q·As 4 Q n (Q = S, Se; n = 3, 4): In Situ Alteration of Functional Molecules in Polar Metal Inorganic Framework Tailoring High‐Performance Infrared Nonlinear Optical Crystals

    Laser & Photonics Review · 2025-06-20

    Huikang Jiang, Xuemei Shi, Lihua Gao, Guangsai Yang, Guang Peng, Ning Ye, Jindong Chen

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  19. Research progress and future prospect of chalcogenides with large optical anisotropy

    Coordination Chemistry Reviews · 2025-06-20

    Zhen-Cheng Wu, Sheng‐Ping Guo

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  20. Nonlinear Optical Series A(VO2)3(SeO3)2 (A = NH4+, K+, and H3O+) with Large Birefringence Derived from High-Anisotropic VO6 Octahedra and SeO3 Pyramids

    Inorganic Chemistry · 2025-06-23

    Qian Wu, Tianyu Wang, Jingfang Zhou, Pifu Gong, Haochen Li, Haotian Tian, Mingjun Xia

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  21. Diamond-Like HgIn2Q4 (Q = Se, Te) Synthesized by Flux-Assisted Boron-Chalcogen Method Exhibit Noteworthy Nonlinear Optical Properties Contributed by Three Types of Tetrahedral Motifs

    Inorganic Chemistry · 2025-06-24

    Jian Ping Cheng, Wen‐Dong Yao, Wenlong Liu, Sheng‐Ping Guo

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  22. Dual‐Sided Multidentate Coordination Strategy Enables Record Birefringence in UV‐Transparent Antimony‐Based Hybrid Crystals

    Angewandte Chemie International Edition · 2025-07-10

    Pu Zhang, Xuehua Dong, Ling Huang, Zhien Lin, Yuqiao Zhou, Guohong Zou

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  23. Dual‐Sided Multidentate Coordination Strategy Enables Record Birefringence in UV‐Transparent Antimony‐Based Hybrid Crystals

    Angewandte Chemie · 2025-07-10

    Pu Zhang, Xuehua Dong, Ling Huang, Zhien Lin, Yuqiao Zhou, Guohong Zou

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  24. Controlling d10 Metal in Phenylthiourea‐Based Hybrid Metal Halides to Actualize Dimensional Transformation and Significantly Improve the Birefringence

    Advanced Optical Materials · 2025-07-20

    Yi‐Lei Lv, Ru‐Ling Tang, Liang Ma, Cheng Chen, Wenlong Liu, Sheng‐Ping Guo

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  25. Structure-property relationships in IR nonlinear optical chalcogenides with stereochemically active lone pairs

    Coordination Chemistry Reviews · 2025-09-03

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  26. SrZnSiS4: Shattering the 4.0 eV Threshold toward Dual-Optimized Bandgap and Second-Harmonic Generation

    Inorganic Chemistry · 2025-09-04

    Huilin Yin, Xia Wu, Shuchang Wu, Changsheng Sun, Chengxiao Wang, Jiaman Sun, Yang Liu, Xiao‐Ming Jiang, Ximeng Lv, Dajiang Mei

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  27. Five-Membered [C 5 O 5 ] 2 – Rings as Birefringence-Active Genes for Ultrabirefringent Crystals

    Journal of the American Chemical Society · 2025-09-16

    Jiachen Lu, Yang Li, Kang Min Ok

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  28. Achieving giant optical anisotropy in the mid-far infrared region via ideal alignment of dual functional motifs

    Inorganic Chemistry Frontiers · 2026-01-01

    Yi-Wen Shan, Ming‐Zhi Zhang, C Hu, Jiang‐Gao Mao

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  29. van der Waals layered CuInP 2 S 6 as infrared nonlinear optical material

    Chemical Communications · 2026-01-01

    Zheng-Tao Hu, 马祖驹, Xin‐Tao Wu, Qi‐Long Zhu, Hua Lin

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  30. Cd/V Ratio-Driven Centrosymmetric Transition of Crystal Structures in Cesium Cadmium Vanadate Oxychlorides Cs 3 CdV 4 O 12 Cl and CsCdV 2 O 6 Cl

    Inorganic Chemistry · 2026-05-14

    Xindan Xu, Lei Geng, Baozhu Zhu, Shoubao Zhang, Yuqi Song, Changyu Meng

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  31. Thermo-mechanical stability and strong optical absorption in quaternary chalcogenides ACdCu3Se4 (A = Sc, Y): a first-principles study

    Indian Journal of Physics · 2026-06-24

    Ahmed Azzouz‐Rached, Amir Ullah, Mubashir Hussain, Eman M. Alshehri, Vineet Tirth, Ali Algahtani, Saleha Qissi, Wafa S. Aljuaid, Essam A. Al‐Ammar, Nasir Rahman, Mudasser Husain

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  32. Cation-substitution-driven electronic, nonlinear optical, elastic, and thermal transport properties of layered AeHgGeSe4 (Ae = Ba, Sr): A first-principles study

    Computational Condensed Matter · 2026-08-12

    Saravana Karthikeyan SKS, Shaik Gouse Peera, Chang Yi Kong

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  33. Domino‐Effect Amplification via Covalent‐Chain Engineering for Giant Birefringence in NaAsQ 2 (Q = S, Se) Crystals

    Laser & Photonics Review · 2026-09-24

    Bo Zhang, Weiqi Huang, Yang Chi, Xin‐Tao Wu, Hua Lin, Qi‐Long Zhu

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