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RESEARCH PAPER · Angewandte Chemie International Edition · 2024

Where do the Fluorine Atoms Go in Inorganic‐Oxide Fluorinations? A Fluorooxoborate Illustration under Terahertz Light

Chunjie Shen, Feng Zhang, Tetsuo Sasaki, Chaolu Eerdun, Michitoshi Hayashi, Houng‐Wei Wang, Keisuke Tominaga, Miriding Mutailipu, Shilie Pan

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42 direct citing works

Where do the Fluorine Atoms Go in Inorganic‐Oxide Fluorinations? A Fluorooxoborate Illustration under Terahertz LightOriginalDiscovery of a new bimetallic borate with strong optical anisotropy activated by π-conjugated [B 2 O 5 ] units3K, Rb-hydroxyborates series with deep-ultraviolet KRbB 5 O 8 (OH) possessing moderate second harmonic generation response0Pb 2 (SeO 3 )(SiF 6 ): the first selenite fluorosilicate with a wide bandgap and large birefringence achieved through perfluorinated group modification45Pb 6 Ba 3 Si 2 S 8 I 10 : a new thiohalide with a quasi-two-dimensional structure and wide band gap2Tunable Optical Anisotropy in Rare‐Earth Borates with Flexible [BO3] Clusters7[B3O3F4(OH)]2–: A Versatile Hydroxyfluorooxoborate Heteroanion Producing Compounds with Highly Tunable Optical Anisotropy19(C3N2H5)B3O3F2(OH)2: Realizing Large Birefringence via a Synergistic Effect between Anion F/OH‐Ratio Optimization and Cation Activation25Low-Frequency Vibrational Spectra of 4-Fluorophenol Studied by THz Spectroscopy and Solid-State Density Functional Theory8Constructing Ultraviolet Nonlinear Optical Crystals with Superior Thermal Stability Based on Organic π-Conjugated [HCOO] Groups6From B 3 O 3 (OH) 3 to B 3 O 3 F 3 : Uncovering Series of New Functional Units Based on [BO 2 F] Beneficial for Deep‐Ultraviolet Birefringence1Looking Back the Nonlinear Optical Crystals in a Functionalized Unit's Perspective109Emergent Mid‐Infrared Nonlinear Optical Candidates With Targeted Balance Performances17Cation tuning in anionic framework hydroborates: tailored deep-ultraviolet optical crystals with large birefringence1CN 4 H 7 B 3 O 3 F 2 (OH) 2 : short-wave UV hydroxyfluorooxyborate crystals with large birefringence2Expanding silver fluorooxoborate crystal chemistry: Ag 2 B 5 O 8 F with 3D double interpenetrating frameworks and Ag 3 B 5 O 8 F 2 with 2D layers5Exploring quaternary vanadates containing alkali metals, alkaline earth metals, and [VO 4 ] in the quest for nonlinear optical materials1Li 2 CeRbB 18 O 30 and Li 2 Cs 2 SrB 18 O 30 : promising low-birefringence materials for UV and deep UV zero-order waveplates4M 3 MoO 4 (HCO 3 ) (M = Rb and Cs): cation-tuned synthesis of two noncentrosymmetric molybdate-carbonates with isolated [MoO 4 ] and [HCO 3 ] groups0Pb 2 B 10 O 16 (OH) 2 ·B(OH) 3 ·H 2 O: significantly enhanced second harmonic generation via substituting metal cations in isostructural compounds with Pb 2+2Pb9Si8O22Cl6 and Pb3.07Ca1.93Si3O11: Two Ultraviolet Nonlinear Optical Materials Exhibit a Moderate Second Harmonic Generation Response1BaFS: Birefringence Enhanced by the Transformation from Optical Isotropy to Anisotropy via Interlayer Anion Substitution8Probing ultraviolet-induced dissociation of hydrogen bond networks in tyrosine by terahertz spectroscopy4K5NaZr4F22(H2O)2: A Hydrated Zirconium Fluoride with a Second-Harmonic Generation Effect and a Short Ultraviolet Cutoff Edge Induced by Cosubstitution with Heterovalent Cations6Borosilicates as deep-ultraviolet transparent nonlinear optical crystals: Structural motifs, performance limits and future directions9Probing the dehydration dynamics and structural transformation of oxalic acid dihydrate using terahertz spectroscopy0Probing Hydrogen Bond Network Evolution and Structural Relaxation during Solid-State Dehydration of Citric Acid Monohydrate by Terahertz Spectroscopy0Mechanism of Intermolecular Hydrogen Bonding Changes in the Blend Crystallization of Polylactic Acid Revealed by Terahertz Spectroscopy1[C 3 N 2 H 5 ]B 7 O 10 F 2 : Demonstrating a New Hydrogen‐Bond‐Induced Intralayer Charge‐Balanced Structure Model with Large Birefringence3Double-Atom Substitution for Suppressing the THz Absorption of LiNbO 30Breaking Inversion Symmetry via Vanadium Coordination Engineering in Bismuth Vanadium Selenites0Comparative analysis of terahertz responses of molecules in gas, liquid and solid phases: A review1Selective precious metal recovery and in-situ upcycling of E-waste into advanced electromagnetic wave absorber via halogen-assisted indirect Joule heating0From High Symmetry to High Symmetry: A Self‐Assembly Strategy for Synthesizing Large Birefringent Borates0

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33 direct citing papers saved.

  1. Discovery of a new bimetallic borate with strong optical anisotropy activated by π-conjugated [B 2 O 5 ] units

    Dalton Transactions · 2024-01-01

    Meihui Chen, Wei Wei, Jiawei Zhao, Donghai An, Yanna Chen

    Read original paper ↗ ·

  2. K, Rb-hydroxyborates series with deep-ultraviolet KRbB 5 O 8 (OH) possessing moderate second harmonic generation response

    New Journal of Chemistry · 2024-01-01

    Aihaimaitijiang Ababaikeri, Xueting Pan, Xueling Hou, Jian Wei Han

    Read original paper ↗ ·

  3. Pb 2 (SeO 3 )(SiF 6 ): the first selenite fluorosilicate with a wide bandgap and large birefringence achieved through perfluorinated group modification

    Chemical Science · 2024-01-01

    Pengfei Li, Chun‐Li Hu, Jiang‐Gao Mao, Fang Kong

    Read original paper ↗ ·

  4. Pb 6 Ba 3 Si 2 S 8 I 10 : a new thiohalide with a quasi-two-dimensional structure and wide band gap

    Dalton Transactions · 2024-01-01

    Zhao Wang, Jiazheng Zhou, Linan Wang, Wenqi Jin, Yingying Kong, Yu Chu, Junjie Li

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  5. Tunable Optical Anisotropy in Rare‐Earth Borates with Flexible [BO3] Clusters

    Chemistry - A European Journal · 2024-05-02

    Xiangyu Long, Ran An, Yan An Lv, Xueyan Wu, Miriding Mutailipu

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  6. [B3O3F4(OH)]2–: A Versatile Hydroxyfluorooxoborate Heteroanion Producing Compounds with Highly Tunable Optical Anisotropy

    Chemistry of Materials · 2024-07-09

    Zeen Li, Congcong Jin, Changyou Liu, Juanjuan Lu, Zhihua Yang, Shilie Pan, Miriding Mutailipu

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  7. (C3N2H5)B3O3F2(OH)2: Realizing Large Birefringence via a Synergistic Effect between Anion F/OH‐Ratio Optimization and Cation Activation

    Small Structures · 2024-07-28

    Chenhui Hu, Chunjie Shen, Huan Zhou, Jian Wei Han, Zhihua Yang, Kenneth Reinhard Poeppelmeier, Feng Zhang, Shilie Pan

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  8. Low-Frequency Vibrational Spectra of 4-Fluorophenol Studied by THz Spectroscopy and Solid-State Density Functional Theory

    The Journal of Physical Chemistry Letters · 2024-08-30

    Feng Zhang, Houng‐Wei Wang, Tetsuo Sasaki, Michitoshi Hayashi, Keisuke Tominaga

    Read original paper ↗ ·

  9. Constructing Ultraviolet Nonlinear Optical Crystals with Superior Thermal Stability Based on Organic π-Conjugated [HCOO] Groups

    Inorganic Chemistry · 2024-09-25

    Zhiyuan Lei, Fangrong Liu, Xuan Pang, Yuanxue Yi, Chunmei Huang, Tao Yang

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  10. From B 3 O 3 (OH) 3 to B 3 O 3 F 3 : Uncovering Series of New Functional Units Based on [BO 2 F] Beneficial for Deep‐Ultraviolet Birefringence

    European Journal of Inorganic Chemistry · 2024-10-04

    Kewang Zhang, Dongdong Chu, Juanjuan Lu, Zhihua Yang, Shilie Pan

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  11. Looking Back the Nonlinear Optical Crystals in a Functionalized Unit's Perspective

    Advanced Functional Materials · 2024-12-15

    Miriding Mutailipu, Junjie Li, Shilie Pan

    Read original paper ↗ ·

  12. Emergent Mid‐Infrared Nonlinear Optical Candidates With Targeted Balance Performances

    Small · 2024-12-23

    Junben Huang, Ailijiang Abudurusuli, Zhihua Yang, Shilie Pan

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  13. Cation tuning in anionic framework hydroborates: tailored deep-ultraviolet optical crystals with large birefringence

    New Journal of Chemistry · 2025-01-01

    Yansheng Jiang, Hangwei Jia, Wenhu Wang, Muhammad Arif, Xiuling Yan, Xueling Hou

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  14. CN 4 H 7 B 3 O 3 F 2 (OH) 2 : short-wave UV hydroxyfluorooxyborate crystals with large birefringence

    Chemical Communications · 2025-01-01

    Chunjie Shen, Huan Zhou, Chenhui Hu, Zhihua Yang, Feng Zhang, Shilie Pan

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  15. Expanding silver fluorooxoborate crystal chemistry: Ag 2 B 5 O 8 F with 3D double interpenetrating frameworks and Ag 3 B 5 O 8 F 2 with 2D layers

    Dalton Transactions · 2025-01-01

    Sergey N. Volkov, Xia Yang, Vadim E. Kireev, A. M. Banaru, Shujuan Han, Alevtina N. Gosteva, M. Yu. Arsent’ev, Dmitri O. Charkin, Alexey V. Povolotskiy, Yevgeny E. Savchenko, Maria Georgievna Krzhizhanovskaya, Stepan A. Vorobiev, Yulia A. Vaitieva, Sergey M. Aksenov, Fangfang Zhang

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  16. Exploring quaternary vanadates containing alkali metals, alkaline earth metals, and [VO 4 ] in the quest for nonlinear optical materials

    CrystEngComm · 2025-01-01

    Xiaoming Wang, Qiuyuan Feng, Ketian Hou, Wei Wei, Juanjuan Lu, Lai Wei, Feng Zhang

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  17. Li 2 CeRbB 18 O 30 and Li 2 Cs 2 SrB 18 O 30 : promising low-birefringence materials for UV and deep UV zero-order waveplates

    Dalton Transactions · 2025-01-01

    Xiao-Ming Wang, Zhiyuan Zhang, Juanjuan Lu, Feng Zhang, Shilie Pan

    Read original paper ↗ ·

  18. M 3 MoO 4 (HCO 3 ) (M = Rb and Cs): cation-tuned synthesis of two noncentrosymmetric molybdate-carbonates with isolated [MoO 4 ] and [HCO 3 ] groups

    Journal of Materials Chemistry C · 2025-01-01

    Jianlong Huang, Wenhu Wang, JuanJuan Lu, Feng Yu

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  19. Pb 2 B 10 O 16 (OH) 2 ·B(OH) 3 ·H 2 O: significantly enhanced second harmonic generation via substituting metal cations in isostructural compounds with Pb 2+

    Journal of Materials Chemistry C · 2025-01-01

    Xintong Cai, Kaitong Liu, Yanhui Zhang

    Read original paper ↗ ·

  20. Pb9Si8O22Cl6 and Pb3.07Ca1.93Si3O11: Two Ultraviolet Nonlinear Optical Materials Exhibit a Moderate Second Harmonic Generation Response

    Inorganic Chemistry · 2025-01-04

    Meihui Chen, Wei Wei, Jiawei Zhao, Juanjuan Lu, Donghai An, Yanna Chen

    Read original paper ↗ ·

  21. BaFS: Birefringence Enhanced by the Transformation from Optical Isotropy to Anisotropy via Interlayer Anion Substitution

    Small · 2025-01-14

    Chao‐Hong Xie, Xiao‐Ming Jiang, Bin‐Wen Liu, Guo‐Cong Guo

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  22. Probing ultraviolet-induced dissociation of hydrogen bond networks in tyrosine by terahertz spectroscopy

    Spectrochimica Acta Part A Molecular and Biomolecular Spectroscopy · 2025-03-07

    Zhenqi Zhu, Hui Fang Xu, Ting Zhang, Jiafeng Meng, Yanwei Tong, Kun Wang, Bing Zhang, Bin Yang

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  23. K5NaZr4F22(H2O)2: A Hydrated Zirconium Fluoride with a Second-Harmonic Generation Effect and a Short Ultraviolet Cutoff Edge Induced by Cosubstitution with Heterovalent Cations

    Inorganic Chemistry · 2025-08-27

    Bing-Wei Miao, Guo-Ren Zhu, Ling Wang, Wenfeng Zhou, Wenlong Liu, Ru‐Ling Tang

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  24. Borosilicates as deep-ultraviolet transparent nonlinear optical crystals: Structural motifs, performance limits and future directions

    Chinese Journal of Structural Chemistry · 2025-09-01

    Yangfeifei Ou, Xiaoliang Zhou, You‐Zhao Lan, Jian‐Wen Cheng

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  25. Probing the dehydration dynamics and structural transformation of oxalic acid dihydrate using terahertz spectroscopy

    Spectrochimica Acta Part A Molecular and Biomolecular Spectroscopy · 2025-11-06

    Zhenqi Zhu, Hui Fang Xu, Bin Yang

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  26. Probing Hydrogen Bond Network Evolution and Structural Relaxation during Solid-State Dehydration of Citric Acid Monohydrate by Terahertz Spectroscopy

    SSRN Electronic Journal · 2026-01-01

    Zhenqi Zhu, Xun Zhang, Hui Xu, Xingfeng Yang, Hanhengye Zou, Chaoxi Liu, Yutong Wu, Bin Yang, XianChang Li

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  27. Mechanism of Intermolecular Hydrogen Bonding Changes in the Blend Crystallization of Polylactic Acid Revealed by Terahertz Spectroscopy

    Analytical Chemistry · 2026-01-27

    Zhenqi Zhu, Hui Xu, Lien Zhu, Sha Yin, Bin Yang

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  28. [C 3 N 2 H 5 ]B 7 O 10 F 2 : Demonstrating a New Hydrogen‐Bond‐Induced Intralayer Charge‐Balanced Structure Model with Large Birefringence

    Small · 2026-02-20

    Chunjie Shen, Huan Zhou, Zhihua Yang, Xueling Hou, Feng Zhang, Shilie Pan

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  29. Double-Atom Substitution for Suppressing the THz Absorption of LiNbO 3

    The Journal of Physical Chemistry C · 2026-03-28

    Jiale Shan, Jinlei Cheng, Jinfeng YANG, Chencheng ZHAO, Xiaoming Yang, Shilie Pan, Feng Zhang

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  30. Breaking Inversion Symmetry via Vanadium Coordination Engineering in Bismuth Vanadium Selenites

    Small · 2026-05-07

    Chanhee Ko, Congcong Jin, Taek Rim Kim, Seung Han Shin, Yunseung Kuk, Jiachen Lu, Chong‐An Chen, Wei Zeng, Joon Ik Jang, Kang Min Ok

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  31. Comparative analysis of terahertz responses of molecules in gas, liquid and solid phases: A review

    TrAC Trends in Analytical Chemistry · 2026-07-13

    Yuxin Huang, Yipeng Zhang, Mingyu Ye, Rui Xu, Yang Pan, Yong Tang

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  32. Selective precious metal recovery and in-situ upcycling of E-waste into advanced electromagnetic wave absorber via halogen-assisted indirect Joule heating

    Chemical Engineering Journal · 2026-07-24

    Bingfu Chen, MuFei Li, T H Chen, Hanyang Sun, Binbin Yu, Yijing Xia, Qunxing Huang, Chen Sun

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  33. From High Symmetry to High Symmetry: A Self‐Assembly Strategy for Synthesizing Large Birefringent Borates

    Small · 2026-08-03

    Chunjie Shen, Junwei Feng, Zhihua Yang, Shilie Pan, Feng Zhang

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