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RESEARCH PAPER · Science China Materials · 2022

Ternary AGa5S8 (A = K, Rb, Cs): Promising infrared nonlinear optical materials rationally realized by “one-for-multiple substitution” strategy

Wen‐Fa Chen, Xiao‐Ming Jiang, Shao‐Min Pei, Ming‐Shu Zhang, Bin‐Wen Liu, Guo‐Cong Guo

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Ternary AGa5S8 (A = K, Rb, Cs): Promising infrared nonlinear optical materials rationally realized by “one-for-multiple substitution” strategyOriginalFirst polar quaternary sulphide CsLiGa 6 S 10 with mixed ordered alkali cations displaying excellent infrared nonlinear optical properties16Simple yet extraordinary: Super-polyhedra-built 3D chalcogenide framework of Cs5Ga9S16 with excellent infrared nonlinear optical performance29AeMg6Ga6S16 (Ae = Ca, Sr, Ba): The First Double Alkaline‐Earth Metal Chalcogenides with Excellent Performances29A new infrared nonlinear optical material BaZnGeS 4 with a wide band gap and large nonlinear optical response34Open honeycomb frameworks of sulphides AHg 4 Ga 5 S 12 (A = Rb, Cs) exhibiting infrared nonlinear optical properties12Recent progress on sulfide infrared nonlinear optical materials with large SHG response and wide band gap26[K2PbX][Ga7S12] (X = Cl, Br, I): The First Lead‐Containing Cationic Moieties with Ultrahigh Second‐Harmonic Generation and Band Gaps Exceeding the Criterion of 2.33 eV46Nonlinear Optical Sulfides LiMGa8S14 (M = Rb/Ba, Cs/Ba) Created by Li+ Driven 2D Centrosymmetric to 3D Noncentrosymmetric Transformation20Recent advances in IR nonlinear optical chalcogenides with well-balanced comprehensive performance56Cs4Zn5P6S18I2: the Largest Birefringence in Chalcohalide Achieved by Highly Polarizable Nonlinear Optical Functional Motifs21Wide band gaps in nonlinear optical materials AMgAgGa6S11 (A = K, Rb) achieved by the incorporation of dual s-block elements in Ag-based sulfide11A two-fold interpenetrated mixed-ligands acentric 3D coordination polymer Zn(OBA)(DIB)·0.5H2O: Topological analysis, fluorescent and second-order NLO properties7Mixed Anionic Tetrahedra Guided Design of New Infrared Nonlinear Optical Material Cs 3 Ga 8 S 13 Cl with High Laser‐Induced Damage Threshold26Excellent Nonlinear Optical M[M4Cl][Ga11S20] (M = A/Ba, A = K, Rb) Achieved by Unusual Cationic Substitution Strategy20Functional Alkali Metal-Based Ternary Chalcogenides: Design, Properties, and Opportunities50Double alkaline earth metals sulfide SrMgGeS4 with high laser-induced damage threshold and strong second-harmonic generation29Ga-based IR nonlinear optical materials: Synthesis, structures, and properties65Wide band gap selenide infrared nonlinear optical materials A II Mg 6 Ga 6 Se 16 with strong SHG responses and high laser-induced damage thresholds31LaMg6Ga6S16: a chemical stable divalent lanthanide chalcogenide70Phase Matching of Infrared Nonlinear Optical Salt-Inclusion Chalcogenides Achieved by the Modulation of the Fractal Dimension of Anionic Motifs18β-Pb3P2S8: A new optical crystal with exceptional birefringence effect11Emergent Mid‐Infrared Nonlinear Optical Candidates With Targeted Balance Performances17CsMgGa 5 S 9 : a diamond-like network made of mixed tetrahedral units for excellent nonlinear optical properties2From NaSc 3 Ga 2 Q 8 (Q = S, Se) to KGa 2 In 3 S 8 : substitution of Sc 3+ with In 3+ to achieve doubled birefringence17新型非线性光学晶体和双折射晶体的研究进展（特邀）4Assembly between diverse polycations and diamond-like anionic frameworks in salt-inclusion phosphides enables excellent nonlinear optical properties4Strong Second‐Harmonic Generation Responses in Salt‐Inclusion Oxychalcogenides Enabled by the Highly Distorted Polyhedra with Mixed‐Anions4Chalcophosphates: A plentiful source of infrared nonlinear optical materials42Achieving excellent nonlinear optical performance via “dimensionality elevation”-driven transformation from centrosymmetric to non-centrosymmetric structures1A balance in SHG response, band gap and birefringence in a series of rare-earth sulfate-iodate6Damage mechanisms of mid-infrared coating components induced by 2.1 μm nanosecond laser pulses3ABCQ4型硫属化物红外非线性光学材料的构效关系（特邀）0高性能硫属化物红外非线性光学材料构效关系（特邀）0KHg 4 Ga 5 S 12 : A Diamond-like Tetrahedral Chalcogenide Exhibiting Giant Phase-Matching Second Harmonic Generation6{[Ge 2 S 7 ] 6– } ∞ Chains-Mediated Framework Reorganization Triggers Dimensional Upgrade and Infrared Nonlinear Optical Response3Eu 2+ ‐Activated KGa 5 S 8 : A New Super‐Sensitive Green Emitting Phosphor for Pressure Sensing1AlGaS3: a wide band gap ternary diamond-like infrared nonlinear optical material with high laser-induced damage threshold1

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  1. First polar quaternary sulphide CsLiGa 6 S 10 with mixed ordered alkali cations displaying excellent infrared nonlinear optical properties

    Inorganic Chemistry Frontiers · 2022-01-01

    Zi Wang, Bin‐Wen Liu, Guo‐Cong Guo

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  2. Simple yet extraordinary: Super-polyhedra-built 3D chalcogenide framework of Cs5Ga9S16 with excellent infrared nonlinear optical performance

    Chinese Chemical Letters · 2022-09-23

    Hong Chen, Mao‐Yin Ran, Shenghua Zhou, Xintao Wu, Hua Lin, Qi‐Long Zhu

    Read original paper ↗ ·

  3. AeMg6Ga6S16 (Ae = Ca, Sr, Ba): The First Double Alkaline‐Earth Metal Chalcogenides with Excellent Performances

    Advanced Optical Materials · 2022-11-24

    Jiale Chen, Yu-Jie Zhang, Hongping Wu, Zhanggui Hu, Jiyang Wang, Yicheng Wu, Hongwei Yu

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  4. A new infrared nonlinear optical material BaZnGeS 4 with a wide band gap and large nonlinear optical response

    Inorganic Chemistry Frontiers · 2023-01-01

    Hongshan Wang, Xueting Pan, Wang Zhao, Yu Chu, Junjie Li

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  5. Open honeycomb frameworks of sulphides AHg 4 Ga 5 S 12 (A = Rb, Cs) exhibiting infrared nonlinear optical properties

    Dalton Transactions · 2023-01-01

    Xiao-Yu Lou, Yu Zhou, Wen‐Fa Chen, Xiao‐Ming Jiang, Bin‐Wen Liu, Guo‐Cong Guo

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  6. Recent progress on sulfide infrared nonlinear optical materials with large SHG response and wide band gap

    Chinese Journal of Structural Chemistry · 2023-01-01

    Linan Wang, Qi Sun, Junjie Li

    Read original paper ↗ ·

  7. [K2PbX][Ga7S12] (X = Cl, Br, I): The First Lead‐Containing Cationic Moieties with Ultrahigh Second‐Harmonic Generation and Band Gaps Exceeding the Criterion of 2.33 eV

    Advanced Science · 2023-02-27

    Wen‐Fa Chen, Bin‐Wen Liu, Shao‐Min Pei, Xiao‐Ming Jiang, Guo‐Cong Guo

    Read original paper ↗ ·

  8. Nonlinear Optical Sulfides LiMGa8S14 (M = Rb/Ba, Cs/Ba) Created by Li+ Driven 2D Centrosymmetric to 3D Noncentrosymmetric Transformation

    Small · 2023-05-05

    Ming‐Shu Zhang, Bin‐Wen Liu, Xiao‐Ming Jiang, Guo‐Cong Guo

    Read original paper ↗ ·

  9. Recent advances in IR nonlinear optical chalcogenides with well-balanced comprehensive performance

    Materials Today Physics · 2023-05-26

    Hedi Yang, Mao‐Yin Ran, Wenbo Wei, Xin‐Tao Wu, Hua Lin, Qi‐Long Zhu

    Read original paper ↗ ·

  10. Cs4Zn5P6S18I2: the Largest Birefringence in Chalcohalide Achieved by Highly Polarizable Nonlinear Optical Functional Motifs

    Small · 2023-07-18

    Xian‐Dan Chai, Mingze Li, Shujuan Lin, Wen‐Fa Chen, Xiao‐Ming Jiang, Bin‐Wen Liu, Guo‐Cong Guo

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  11. Wide band gaps in nonlinear optical materials AMgAgGa6S11 (A = K, Rb) achieved by the incorporation of dual s-block elements in Ag-based sulfide

    Materials Today Physics · 2023-08-09

    Wen‐Fa Chen, Xiao‐Ming Jiang, Bin‐Wen Liu, Guo‐Cong Guo

    Read original paper ↗ ·

  12. A two-fold interpenetrated mixed-ligands acentric 3D coordination polymer Zn(OBA)(DIB)·0.5H2O: Topological analysis, fluorescent and second-order NLO properties

    Journal of Molecular Structure · 2023-09-05

    Jian‐Di Lin, Zhenfei Li, Zu‐Jin Lin, Fa‐Kun Zheng

    Read original paper ↗ ·

  13. Mixed Anionic Tetrahedra Guided Design of New Infrared Nonlinear Optical Material Cs 3 Ga 8 S 13 Cl with High Laser‐Induced Damage Threshold

    Advanced Optical Materials · 2023-09-10

    Linan Wang, Chenchen Tu, Jiazheng Zhou, Yu Chu, Zhihua Yang, Shilie Pan, Junjie Li

    Read original paper ↗ ·

  14. Excellent Nonlinear Optical M[M4Cl][Ga11S20] (M = A/Ba, A = K, Rb) Achieved by Unusual Cationic Substitution Strategy

    Small · 2023-09-11

    Xiao‐Yu Lou, Xiao‐Ming Jiang, Bin‐Wen Liu, Guo‐Cong Guo

    Read original paper ↗ ·

  15. Functional Alkali Metal-Based Ternary Chalcogenides: Design, Properties, and Opportunities

    Chemistry of Materials · 2023-09-22

    Hannah McKeever, Niraj Nitish Patil, Manoj Palabathuni, Shalini Singh

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  16. Double alkaline earth metals sulfide SrMgGeS4 with high laser-induced damage threshold and strong second-harmonic generation

    Materials Today Physics · 2023-09-29

    Hongshan Wang, Yu Chu, Xueting Pan, Zhihua Yang, Shilie Pan, Junjie Li

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  17. Ga-based IR nonlinear optical materials: Synthesis, structures, and properties

    Coordination Chemistry Reviews · 2023-12-21

    Jiaxiang Zhang, Ping Feng, Mao‐Yin Ran, Xintao Wu, Hua Lin, Qi‐Long Zhu

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  18. Wide band gap selenide infrared nonlinear optical materials A II Mg 6 Ga 6 Se 16 with strong SHG responses and high laser-induced damage thresholds

    Chemical Science · 2024-01-01

    Linan Wang, Dongdong Chu, Zhihua Yang, Junjie Li, Shilie Pan

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  19. LaMg6Ga6S16: a chemical stable divalent lanthanide chalcogenide

    Nature Communications · 2024-04-05

    Yu-Jie Zhang, Jiale Chen, Kaixuan Li, Hongping Wu, Zhanggui Hu, Jiyang Wang, Yicheng Wu, Hongwei Yu

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  20. Phase Matching of Infrared Nonlinear Optical Salt-Inclusion Chalcogenides Achieved by the Modulation of the Fractal Dimension of Anionic Motifs

    Chemistry of Materials · 2024-04-24

    Yan Guo, Wen‐Fa Chen, Mingxin Li, Fan Wu, Qiu-Pei Qin, Bin‐Wen Liu, Xiao‐Ming Jiang, Guo‐Cong Guo

    Read original paper ↗ ·

  21. β-Pb3P2S8: A new optical crystal with exceptional birefringence effect

    Chinese Chemical Letters · 2024-07-15

    Weiping Guo, Ying Zhu, Hong‐Hua Cui, Lingyun Li, Yan Yu, Zhong‐Zhen Luo, Zhigang Zou

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  22. Emergent Mid‐Infrared Nonlinear Optical Candidates With Targeted Balance Performances

    Small · 2024-12-23

    Junben Huang, Ailijiang Abudurusuli, Zhihua Yang, Shilie Pan

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  23. CsMgGa 5 S 9 : a diamond-like network made of mixed tetrahedral units for excellent nonlinear optical properties

    Chemical Communications · 2025-01-01

    Yi-Bing Huang, Bin‐Wen Liu, Guo‐Cong Guo

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  24. From NaSc 3 Ga 2 Q 8 (Q = S, Se) to KGa 2 In 3 S 8 : substitution of Sc 3+ with In 3+ to achieve doubled birefringence

    Chemical Science · 2025-01-01

    Yun Xie, Wen‐Dong Yao, Qiu-Yang Du, Wenfeng Zhou, Nian‐Tzu Suen, Wenlong Liu, Sheng‐Ping Guo

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  25. 新型非线性光学晶体和双折射晶体的研究进展（特邀）

    Chinese Journal of Lasers · 2025-01-01

    韩树娟 Han Shujuan, 杨志华 Yang Zhihua, 张方方 Zhang Fangfang, 李广卯 Li Guangmao, 李俊杰 Li Junjie, 吴雅博 Wu Yabo, 储冬冬 Chu Dongdong, 程孟 Cheng Meng, 张文彬 Zhang Wenbin, 丁文 Ding Wen, 潘世烈 Pan Shilie

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  26. Assembly between diverse polycations and diamond-like anionic frameworks in salt-inclusion phosphides enables excellent nonlinear optical properties

    Science China Chemistry · 2025-02-11

    Ming‐Shu Zhang, Shao‐Min Pei, Bin‐Wen Liu, Xiao‐Ming Jiang, Guo‐Cong Guo

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  27. Strong Second‐Harmonic Generation Responses in Salt‐Inclusion Oxychalcogenides Enabled by the Highly Distorted Polyhedra with Mixed‐Anions

    Advanced Optical Materials · 2025-02-18

    Meng‐Na Jing, Si‐Fan Lu, Ming‐Xin Li, Xiao‐Ming Jiang, Bin‐Wen Liu, Guo‐Cong Guo

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  28. Chalcophosphates: A plentiful source of infrared nonlinear optical materials

    Coordination Chemistry Reviews · 2025-02-26

    Yingying Kong, Guansong Zheng, Yi Du, Junjie Li, Shilie Pan

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  29. Achieving excellent nonlinear optical performance via “dimensionality elevation”-driven transformation from centrosymmetric to non-centrosymmetric structures

    Science China Chemistry · 2025-06-28

    Lin‐Tao Jiang, Jun-Long Chen, Ming‐Shu Zhang, Xiao‐Ming Jiang, Bin‐Wen Liu, Guo‐Cong Guo

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  30. A balance in SHG response, band gap and birefringence in a series of rare-earth sulfate-iodate

    Journal of Molecular Structure · 2025-07-01

    Chunxiang Wu, Y. X. Li, Zhengli Liang, Xiao Mei Jiang, Xiao Jiang, Hui Fang, Lixiang Qin, Xingyuan Bai, Lehui Liu, Lehui Liu, Xingxing Jiang, Xingxing Jiang, Hongming Liu, Hongming Liu

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  31. Damage mechanisms of mid-infrared coating components induced by 2.1 μm nanosecond laser pulses

    Optics & Laser Technology · 2025-07-29

    Jiansheng He, H. C. Wang, Mengxia Wang, Mengxia Wang, Meng Guo, Yuchun Liu, Chuanpeng Qian, Xisheng Ye, Yujie Peng, Jianke Yao, Yuxin Leng, Jianda Shao, Jianda Shao

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  32. ABCQ4型硫属化物红外非线性光学材料的构效关系（特邀）

    Chinese Journal of Lasers · 2026-01-01

    王硕 Wang Shuo, 张成龙 Zhang Chenglong, 黄君本 Huang Junben, Ailijiang Abudurusuli, 吐沙姑·阿不都吾甫 Abudouwufu Tushagu

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  33. 高性能硫属化物红外非线性光学材料构效关系（特邀）

    Chinese Journal of Lasers · 2026-01-01

    张成龙 Zhang Chenglong, 王硕 Wang Shuo, Ailijiang Abudurusuli, 黄君本 Huang Junben

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  34. KHg 4 Ga 5 S 12 : A Diamond-like Tetrahedral Chalcogenide Exhibiting Giant Phase-Matching Second Harmonic Generation

    Chemistry of Materials · 2026-02-03

    Weiping Guo, Chao Yang, Bingxuan Li, Hong‐Hua Cui, Lingyun Li, Yan Yu, Zhong‐Zhen Luo, Zhigang Zou

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  35. {[Ge 2 S 7 ] 6– } ∞ Chains-Mediated Framework Reorganization Triggers Dimensional Upgrade and Infrared Nonlinear Optical Response

    Chemistry of Materials · 2026-03-19

    Wen-Rui Zhou, Zhen-Cheng Wu, Yong-han WU Xue-jiao LIU, Mao‐Yin Ran, Sheng‐Ping Guo

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  36. Eu 2+ ‐Activated KGa 5 S 8 : A New Super‐Sensitive Green Emitting Phosphor for Pressure Sensing

    Small · 2026-06-03

    Chen Bai, Jiarui Duan, Deyin Wang, Yuhua Wang

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  37. AlGaS3: a wide band gap ternary diamond-like infrared nonlinear optical material with high laser-induced damage threshold

    Science China Materials · 2026-09-04

    Yunfei Shi, Hongshan Wang, Yu Chu, Xin Su, Zhenglong Li, Juanjuan Lu, Ailijiang Abudurusuli, Junjie Li, Shilie Pan

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