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RESEARCH PAPER · Angewandte Chemie · 2020

An Unprecedented Antimony(III) Borate with Strong Linear and Nonlinear Optical Responses

Youchao Liu, Xiaomeng Liu, Shuai Liu, Qingran Ding, Yanqiang Li, Lina Li, Sangen Zhao, Zheshuai Lin, Junhua Luo, Maochun Hong

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An Unprecedented Antimony(III) Borate with Strong Linear and Nonlinear Optical ResponsesOriginalTwo Pyrophosphates with Large Birefringences and Second‐Harmonic Responses as Ultraviolet Nonlinear Optical Materials137Two Pyrophosphates with Large Birefringences and Second‐Harmonic Responses as Ultraviolet Nonlinear Optical Materials29K 2 Sb(P 2 O 7 )F: Cairo Pentagonal Layer with Bifunctional Genes Reveal Optical Performance297K2Sb(P2O7)F: Cairo Pentagonal Layer with Bifunctional Genes Reveal Optical Performance38Giant Optical Anisotropy in the UV‐Transparent 2D Nonlinear Optical Material Sc(IO 3 ) 2 (NO 3 )212Giant Optical Anisotropy in the UV‐Transparent 2D Nonlinear Optical Material Sc(IO 3 ) 2 (NO 3 )57An Antimony(III) Fluoride Oxalate with Large Birefringence45Sb6O7(SO4)2: A Promising Ultraviolet Nonlinear Optical Material with an Enhanced Second‐Harmonic‐Generation Response Activated by SbIII Lone‐Pair Stereoactivity62Novel noncentrosymmetric polar coordination compounds derived from chiral histidine ligands36Pb 2 TiFO(SeO 3 ) 2 Br: a new polar compound with the strongest second harmonic generation in the selenite bromide family29Bi2[B2(SeO3)6]: A Metal Boroselenite with a Unique Zero-Dimensional [B2(SeO3)6]6– Anionic Group and Large Birefringence31Hydroxyfluorooxoborate Na[B3O3F2(OH)2]⋅[B(OH)3]: Optimizing the Optical Anisotropy with Heteroanionic Units for Deep Ultraviolet Birefringent Crystals146Hydroxyfluorooxoborate Na[B3O3F2(OH)2]⋅[B(OH)3]: Optimizing the Optical Anisotropy with Heteroanionic Units for Deep Ultraviolet Birefringent Crystals16Li 4 MgGe 2 S 7 : The First Alkali and Alkaline‐Earth Diamond‐Like Infrared Nonlinear Optical Material with Exceptional Large Band Gap213Li4MgGe2S7: The First Alkali and Alkaline‐Earth Diamond‐Like Infrared Nonlinear Optical Material with Exceptional Large Band Gap15High‐Temperature and Large‐Polarization Ferroelectric with Second Harmonic Generation Response in a Novel Crown Ether Clathrate16Li2MTeO6 (M=Ti, Sn): Mid‐Infrared Nonlinear Optical Crystal with Strong Second Harmonic Generation Response and Wide Transparency Range72Li2MTeO6 (M=Ti, Sn): Mid‐Infrared Nonlinear Optical Crystal with Strong Second Harmonic Generation Response and Wide Transparency Range4Preparation, structural, optical and thermal behavior of nonlinear Potassium DL-malato borate hydrate (C8H8BKO10H2O) single crystal5Sn2PO4I: An Excellent Birefringent Material with Giant Optical Anisotropy in Non π‐Conjugated Phosphate212Sn2PO4I: An Excellent Birefringent Material with Giant Optical Anisotropy in Non π‐Conjugated Phosphate22A New Nonlinear Optical Material with N(CN)2− Anion2Hierarchical Modulation of Optical Anisotropy Driven by Metal Cation Polyhedra in Fluorooxoborates MIIB4O6F2 (MII=Be, Mg, Pb, Zn, Cd)6Chiral coordination compounds with exceptional enantioselectivity10Introducing a New d0 Sc3+ Asymmetric Ion for Functional Materials: Large Birefringence Enhancement by ScO6 in Ba3Sc2(BO3)411A Hybrid Halide Perovskite Birefringent Crystal14A Hybrid Halide Perovskite Birefringent Crystal149Promising Deep‐Ultraviolet Birefringent Materials via Rational Design and Assembly of Planar π‐Conjugated [B(OH)3] and [B3O3(OH)3] Functional Species6Promising Deep‐Ultraviolet Birefringent Materials via Rational Design and Assembly of Planar π‐Conjugated [B(OH)3] and [B3O3(OH)3] Functional Species83Realization of Enlarged Birefringence from BaCdBe2(BO3)2F2 to NaMgBe2(BO3)2F via the Cation Size Effect as a Potential Deep-Ultraviolet Birefringent Material18An Optically Anisotropic Crystal with Large Birefringence Arising from Cooperative π Orbitals81An Optically Anisotropic Crystal with Large Birefringence Arising from Cooperative π Orbitals22A Hybrid Antiperovskite with Strong Linear and Second‐Order Nonlinear Optical Responses15A Hybrid Antiperovskite with Strong Linear and Second‐Order Nonlinear Optical Responses96Finding a Deep‐UV Borate BaZnB4O8 with Edge‐sharing [BO4] Tetrahedra and Strong Optical Anisotropy20Harnessing the dual role of DMSO in the synthesis of SbOCl·DMSO: an excellent nonlinear optical crystal with unique 1D spiral chain10Dual Chemical Scissors Strategy Enables 1D Antimony Selenates with Ultraviolet Nonlinear Optical Properties35Dual Chemical Scissors Strategy Enables 1D Antimony Selenates with Ultraviolet Nonlinear Optical Properties6pH‐Regulated Ring‐Opening/Closing Transformation in Polyoxometalates Enables High‐Performance Nonlinear Optical Crystals1Unit Symmetry‐Breaking and Layered Linear Ordering Enabling Superior Short‐Wave Ultraviolet Birefringent Crystal2Programmable Anisotropic in Diazapyrene Cocrystals With Birefringence Exceeding 1.21Lateral‐Site Unblocking Enables Bilateral π ‐Chromophore Organization for Giant Birefringence in One‐Dimensional Lead Hybrids0

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  1. Two Pyrophosphates with Large Birefringences and Second‐Harmonic Responses as Ultraviolet Nonlinear Optical Materials

    Angewandte Chemie International Edition · 2020-06-19

    Xuefang Lu, Zhaohui Chen, Xuerui Shi, Qun Jing, Ming‐Hsien Lee

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  2. Two Pyrophosphates with Large Birefringences and Second‐Harmonic Responses as Ultraviolet Nonlinear Optical Materials

    Angewandte Chemie · 2020-06-19

    Xuefang Lu, Zhaohui Chen, Xuerui Shi, Qun Jing, Ming‐Hsien Lee

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  3. K 2 Sb(P 2 O 7 )F: Cairo Pentagonal Layer with Bifunctional Genes Reveal Optical Performance

    Angewandte Chemie International Edition · 2020-08-03

    Yalan Deng, Ling Huang, Xuehua Dong, Lei Wang, Kang Min Ok, Hongmei Zeng, Zhien Lin, Guohong Zou

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  4. K2Sb(P2O7)F: Cairo Pentagonal Layer with Bifunctional Genes Reveal Optical Performance

    Angewandte Chemie · 2020-08-03

    Yalan Deng, Ling Huang, Xuehua Dong, Lei Wang, Kang Min Ok, Hongmei Zeng, Zhien Lin, Guohong Zou

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  5. Giant Optical Anisotropy in the UV‐Transparent 2D Nonlinear Optical Material Sc(IO 3 ) 2 (NO 3 )

    Angewandte Chemie International Edition · 2020-11-04

    Chao Wu, Xingxing Jiang, Zujian Wang, Lin Lin, Zheshuai Lin, Zhipeng Huang, Xifa Long, Mark Graeme Humphrey, Chi Zhang

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  6. Giant Optical Anisotropy in the UV‐Transparent 2D Nonlinear Optical Material Sc(IO 3 ) 2 (NO 3 )

    Angewandte Chemie · 2020-11-04

    Chao Wu, Xingxing Jiang, Zujian Wang, Lin Lin, Zheshuai Lin, Zhipeng Huang, Xifa Long, Mark Graeme Humphrey, Chi Zhang

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  7. An Antimony(III) Fluoride Oxalate with Large Birefringence

    Chemistry - A European Journal · 2020-12-10

    Yangxin Chen, Zhangxian Chen, Zhou Yang, Yanqiang Li, Youchao Liu, Qingran Ding, Xin Chen, Sangen Zhao, Junhua Luo

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  8. Sb6O7(SO4)2: A Promising Ultraviolet Nonlinear Optical Material with an Enhanced Second‐Harmonic‐Generation Response Activated by SbIII Lone‐Pair Stereoactivity

    Chemistry - A European Journal · 2020-12-23

    Qi Wei, Chao He, Kui Wang, Xiao‐Fang Duan, Xing‐Tao An, Jinhua Li, Guo‐Ming Wang

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  9. Novel noncentrosymmetric polar coordination compounds derived from chiral histidine ligands

    Inorganic Chemistry Frontiers · 2021-01-01

    Wooyoung Seo, Kang Min Ok

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  10. Pb 2 TiFO(SeO 3 ) 2 Br: a new polar compound with the strongest second harmonic generation in the selenite bromide family

    Journal of Materials Chemistry C · 2021-01-01

    Lili Liu, Bingbing Zhang, P. Shiv Halasyamani, Weiguo Zhang

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  11. Bi2[B2(SeO3)6]: A Metal Boroselenite with a Unique Zero-Dimensional [B2(SeO3)6]6– Anionic Group and Large Birefringence

    Inorganic Chemistry · 2021-03-02

    Ru‐Ling Tang, Chun‐Li Hu, Weijie Xie, Q. Huang, Jiang‐Gao Mao

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  12. Hydroxyfluorooxoborate Na[B3O3F2(OH)2]⋅[B(OH)3]: Optimizing the Optical Anisotropy with Heteroanionic Units for Deep Ultraviolet Birefringent Crystals

    Angewandte Chemie International Edition · 2021-06-21

    Congcong Jin, Xuping Shi, Hao Zeng, Shujuan Han, Zhen Chen, Zhihua Yang, Miriding Mutailipu, Shilie Pan

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  13. Hydroxyfluorooxoborate Na[B3O3F2(OH)2]⋅[B(OH)3]: Optimizing the Optical Anisotropy with Heteroanionic Units for Deep Ultraviolet Birefringent Crystals

    Angewandte Chemie · 2021-06-21

    Congcong Jin, Xuping Shi, Hao Zeng, Shujuan Han, Zhen Chen, Zhihua Yang, Miriding Mutailipu, Shilie Pan

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  14. Li 4 MgGe 2 S 7 : The First Alkali and Alkaline‐Earth Diamond‐Like Infrared Nonlinear Optical Material with Exceptional Large Band Gap

    Angewandte Chemie International Edition · 2021-07-24

    Ailijiang Abudurusuli, Junben Huang, Peng Wang, Zhihua Yang, Shilie Pan, Junjie Li

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  15. Li4MgGe2S7: The First Alkali and Alkaline‐Earth Diamond‐Like Infrared Nonlinear Optical Material with Exceptional Large Band Gap

    Angewandte Chemie · 2021-07-24

    Ailijiang Abudurusuli, Junben Huang, Peng Wang, Zhihua Yang, Shilie Pan, Junjie Li

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  16. High‐Temperature and Large‐Polarization Ferroelectric with Second Harmonic Generation Response in a Novel Crown Ether Clathrate

    Chemistry - A European Journal · 2021-07-28

    Ding Chong Han, Yu Tan, Yu Kong Li, Jia Hui Wen, Yun‐Zhi Tang, Wen Juan Wei, Peng-kang Du, Hao Zhang

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  17. Li2MTeO6 (M=Ti, Sn): Mid‐Infrared Nonlinear Optical Crystal with Strong Second Harmonic Generation Response and Wide Transparency Range

    Angewandte Chemie International Edition · 2021-08-30

    Xiaoli Du, Xiaojie Guo, Zeliang Gao, Fuan Liu, Feifei Guo, Siyuan Wang, Haoyuan Wang, Youxuan Sun, Xutang Tao

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  18. Li2MTeO6 (M=Ti, Sn): Mid‐Infrared Nonlinear Optical Crystal with Strong Second Harmonic Generation Response and Wide Transparency Range

    Angewandte Chemie · 2021-08-30

    Xiaoli Du, Xiaojie Guo, Zeliang Gao, Fuan Liu, Feifei Guo, Siyuan Wang, Haoyuan Wang, Youxuan Sun, Xutang Tao

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  19. Preparation, structural, optical and thermal behavior of nonlinear Potassium DL-malato borate hydrate (C8H8BKO10H2O) single crystal

    Journal of Molecular Structure · 2021-09-02

    D.S. Ajisha, R. Ezhil Vizhi

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  20. Sn2PO4I: An Excellent Birefringent Material with Giant Optical Anisotropy in Non π‐Conjugated Phosphate

    Angewandte Chemie International Edition · 2021-09-15

    Jingyu Guo, Abudukadi Tudi, Shujuan Han, Zhihua Yang, Shilie Pan

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  21. Sn2PO4I: An Excellent Birefringent Material with Giant Optical Anisotropy in Non π‐Conjugated Phosphate

    Angewandte Chemie · 2021-09-15

    Jingyu Guo, Abudukadi Tudi, Shujuan Han, Zhihua Yang, Shilie Pan

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  22. A New Nonlinear Optical Material with N(CN)2− Anion

    Chemistry - A European Journal · 2021-10-20

    Xin Chen, Han Wang, Youchao Liu, Zhou Yang, Weiqi Huang, Minjuan Li, Yanqiang Li, Yangxin Chen, Sangen Zhao, Junhua Luo

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  23. Hierarchical Modulation of Optical Anisotropy Driven by Metal Cation Polyhedra in Fluorooxoborates MIIB4O6F2 (MII=Be, Mg, Pb, Zn, Cd)

    Chemistry - A European Journal · 2021-12-27

    Shan Shu, Junben Huang, Chenhui Hu, Shilie Pan, Zhihua Yang

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  24. Chiral coordination compounds with exceptional enantioselectivity

    Journal of Materials Chemistry C · 2022-01-01

    Minju Lee, Kang Min Ok

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  25. Introducing a New d0 Sc3+ Asymmetric Ion for Functional Materials: Large Birefringence Enhancement by ScO6 in Ba3Sc2(BO3)4

    ChemPhysChem · 2022-02-11

    Jingfang Zhou, Rukang K. Li

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  26. A Hybrid Halide Perovskite Birefringent Crystal

    Angewandte Chemie · 2022-03-15

    Weiqi Huang, Xu Zhang, Yanqiang Li, Yang Zhou, Xin Chen, Xiaoqi Li, Fafa Wu, Maochun Hong, Junhua Luo, Sangen Zhao

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  27. A Hybrid Halide Perovskite Birefringent Crystal

    Angewandte Chemie International Edition · 2022-03-15

    Weiqi Huang, Xu Zhang, Yanqiang Li, Yang Zhou, Xin Chen, Xiaoqi Li, Fafa Wu, Maochun Hong, Junhua Luo, Sangen Zhao

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  28. Promising Deep‐Ultraviolet Birefringent Materials via Rational Design and Assembly of Planar π‐Conjugated [B(OH)3] and [B3O3(OH)3] Functional Species

    Angewandte Chemie · 2022-04-29

    Jiahao Jiao, Meng Cheng, Rong Yang, Yuchen Yan, Min Zhang, Fangfang Zhang, Zhihua Yang, Shilie Pan

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  29. Promising Deep‐Ultraviolet Birefringent Materials via Rational Design and Assembly of Planar π‐Conjugated [B(OH)3] and [B3O3(OH)3] Functional Species

    Angewandte Chemie International Edition · 2022-04-29

    Jiahao Jiao, Meng Cheng, Rong Yang, Yuchen Yan, Min Zhang, Fangfang Zhang, Zhihua Yang, Shilie Pan

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  30. Realization of Enlarged Birefringence from BaCdBe2(BO3)2F2 to NaMgBe2(BO3)2F via the Cation Size Effect as a Potential Deep-Ultraviolet Birefringent Material

    Inorganic Chemistry · 2022-05-02

    Ruixin Guo, Xingxing Jiang, Shu Hai Guo, Mingjun Xia, Lijuan Liu, Zheshuai Lin, Xiaoyang Wang

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  31. An Optically Anisotropic Crystal with Large Birefringence Arising from Cooperative π Orbitals

    Angewandte Chemie International Edition · 2022-07-29

    Yanqiang Li, Xu Zhang, Zhou Yang, Weiqi Huang, Yipeng Song, Han Wang, Minjuan Li, Maochun Hong, Junhua Luo, Sangen Zhao

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  32. An Optically Anisotropic Crystal with Large Birefringence Arising from Cooperative π Orbitals

    Angewandte Chemie · 2022-07-29

    Yanqiang Li, Xu Zhang, Zhou Yang, Weiqi Huang, Yipeng Song, Han Wang, Minjuan Li, Maochun Hong, Junhua Luo, Sangen Zhao

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  33. A Hybrid Antiperovskite with Strong Linear and Second‐Order Nonlinear Optical Responses

    Angewandte Chemie · 2022-08-26

    Minjuan Li, Xu Zhang, Zheyao Xiong, Yanqiang Li, Zhou Yang, Xin Chen, Yipeng Song, Maochun Hong, Junhua Luo, Sangen Zhao

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  34. A Hybrid Antiperovskite with Strong Linear and Second‐Order Nonlinear Optical Responses

    Angewandte Chemie International Edition · 2022-08-26

    Minjuan Li, Xu Zhang, Zheyao Xiong, Yanqiang Li, Zhou Yang, Xin Chen, Yipeng Song, Maochun Hong, Junhua Luo, Sangen Zhao

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  35. Finding a Deep‐UV Borate BaZnB4O8 with Edge‐sharing [BO4] Tetrahedra and Strong Optical Anisotropy

    Chemistry - A European Journal · 2022-10-25

    Jian Wei Han, Kaitong Liu, Long Chen, Fuming Li, Zhihua Yang, Fangfang Zhang, Shilie Pan, Miriding Mutailipu

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  36. Harnessing the dual role of DMSO in the synthesis of SbOCl·DMSO: an excellent nonlinear optical crystal with unique 1D spiral chain

    Inorganic Chemistry Frontiers · 2025-01-01

    Xiande Peng, Xiangyuan Li, Yingzi Zhang, Xuehua Dong, Ling Huang, Liling Cao, Daojiang Gao, Guohong Zou

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  37. Dual Chemical Scissors Strategy Enables 1D Antimony Selenates with Ultraviolet Nonlinear Optical Properties

    Angewandte Chemie International Edition · 2025-06-20

    Xuehua Dong, Ling Huang, Hongmei Zeng, Zhien Lin, Kang Min Ok, Guohong Zou

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  38. Dual Chemical Scissors Strategy Enables 1D Antimony Selenates with Ultraviolet Nonlinear Optical Properties

    Angewandte Chemie · 2025-06-20

    Xuehua Dong, Ling Huang, Hongmei Zeng, Zhien Lin, Kang Min Ok, Guohong Zou

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  39. pH‐Regulated Ring‐Opening/Closing Transformation in Polyoxometalates Enables High‐Performance Nonlinear Optical Crystals

    Angewandte Chemie · 2025-11-06

    Wei Zeng, Jing Zhang, Yao Tian, Hongmei Zeng, Zhien Lin, Liujiang Zhou, Kang Min Ok, Guohong Zou

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  40. Unit Symmetry‐Breaking and Layered Linear Ordering Enabling Superior Short‐Wave Ultraviolet Birefringent Crystal

    Angewandte Chemie · 2026-01-14

    Xin Wen, Dequan Kong, Jingyao Lu, Jindong Chen, Haohai Yu, Huaijin Zhang, Zhanggui Hu, Jiyang Wang, Ning Ye, Guang Peng

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  41. Programmable Anisotropic in Diazapyrene Cocrystals With Birefringence Exceeding 1.2

    Angewandte Chemie · 2026-01-28

    Lingyan Sun, Gangji Yi, Guohong Zou, Cheng Jiang Zhang

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  42. Lateral‐Site Unblocking Enables Bilateral π ‐Chromophore Organization for Giant Birefringence in One‐Dimensional Lead Hybrids

    Angewandte Chemie · 2026-08-07

    Yu Yan, Yingzi Zhang, Liyi Zhang, Ling Huang, Yuqiao Zhou, Xuehua Dong, Guohong Zou

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