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RESEARCH PAPER · Angewandte Chemie · 2017

Macroscopic Polarization Enhancement Promoting Photo‐ and Piezoelectric‐Induced Charge Separation and Molecular Oxygen Activation

Hongwei Huang, Shuchen Tu, Chao Liu Zeng, Tierui Zhang, A.H. Reshak, Yihe Zhang

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Macroscopic Polarization Enhancement Promoting Photo‐ and Piezoelectric‐Induced Charge Separation and Molecular Oxygen ActivationOriginalIn-depth insight into facet-dependent charge movement behaviors and photo-redox catalysis: A case of {0 0 1} and {0 1 0} facets BiOCl56Enhanced Visible Light Photocatalytic Hydrogenation of CO2 into Methane over a Pd/Ce-TiO2 Nanocomposition49Reactable polyelectrolyte-assisted preparation of flower-like Ag/AgCl/BiOCl composite with enhanced photocatalytic activity51Sulfide oxide XZnSO (X = Ca or Sr) as novel active photocatalytic water splitting solar-to-hydrogen energy conversion40Facile synthesis of Bi/BiVO 4 composite ellipsoids with high photocatalytic activity64Oxygen Reduction Reaction for Generating H 2 O 2 through a Piezo‐Catalytic Process over Bismuth Oxychloride125Mixing Halogens To Assemble an All‐Inorganic Layered Perovskite with Warm White‐Light Emission21Bi/BiVO4 Chainlike Hollow Microstructures: Synthesis, Characterization, and Application as Visible-Light-Active Photocatalysts70Compressible and Recyclable Monolithic g-C3N4/Melamine Sponge: A Facile Ultrasonic-Coating Approach and Enhanced Visible-Light Photocatalytic Activity27Magnetically Recyclable Fe3O4@Zn x Cd1– x S Core–Shell Microspheres for Visible Light-Mediated Photocatalysis29Constructing Mn3O4/Cu hybrid nanorods as superior photocatalyst14Enhanced photocatalytic H2 evolution and phenol degradation over sulfur doped meso/macroporous g-C3N4 spheres with continuous channels45Synthesis g-C3N4 of high specific surface area by precursor pretreatment strategy with SBA-15 as a template and their photocatalytic activity toward degradation of rhodamine B9Enabling PIEZOpotential in PIEZOelectric Semiconductors for Enhanced Catalytic Activities366Enabling PIEZOpotential in PIEZOelectric Semiconductors for Enhanced Catalytic Activities34Piezoelectric‐Effect‐Enhanced Full‐Spectrum Photoelectrocatalysis in p–n Heterojunction247Intramolecular Charge Transfer and Extended Conjugate Effects in Donor–π–Acceptor‐Type Mesoporous Carbon Nitride for Photocatalytic Hydrogen Evolution81The Role of Polarization in Photocatalysis930The Role of Polarization in Photocatalysis60Visible‐Light‐Driven Water Oxidation with a Polyoxometalate‐Complexed Hematite Core of 275 Iron Atoms64Visible‐Light‐Driven Water Oxidation with a Polyoxometalate‐Complexed Hematite Core of 275 Iron Atoms14Cs3Na(H2C3N3O3)4·3H2O: A Mixed Alkali‐Metal Hydroisocyanurate Nonlinear Optical Material Containing π‐Conjugated Six‐Membered‐Ring Units68Unprecedented Eighteen‐Faceted BiOCl with a Ternary Facet Junction Boosting Cascade Charge Flow and Photo‐redox314Unprecedented Eighteen‐Faceted BiOCl with a Ternary Facet Junction Boosting Cascade Charge Flow and Photo‐redox25Bismuth‐Based Photocatalysts for Solar Photocatalytic Carbon Dioxide Conversion190An Efficient Strategy for Boosting Photogenerated Charge Separation by Using Porphyrins as Interfacial Charge Mediators126An Efficient Strategy for Boosting Photogenerated Charge Separation by Using Porphyrins as Interfacial Charge Mediators12Graphitic carbon nitride tetragonal hollow prism with enhanced photocatalytic hydrogen evolution17Efficient BiVO4 Photoanodes by Postsynthetic Treatment: Remarkable Improvements in Photoelectrochemical Performance from Facile Borate Modification171Efficient BiVO4 Photoanodes by Postsynthetic Treatment: Remarkable Improvements in Photoelectrochemical Performance from Facile Borate Modification59Freeing the Polarons to Facilitate Charge Transport in BiVO 4 from Oxygen Vacancies with an Oxidative 2D Precursor90Freeing the Polarons to Facilitate Charge Transport in BiVO4 from Oxygen Vacancies with an Oxidative 2D Precursor33An Uncommon Hypervalent Fluorooxosilicophosphate5Harnessing the Photocatalytic Potential of Polypyrroles in Water through Nanointervension: Synthesis and Photophysical Evaluation of Biodegradable Polypyrrolic Nanoencapsulates22Unravelling the Synergy between Oxygen Vacancies and Oxygen Substitution in BiO 2− x for Efficient Molecular‐Oxygen Activation280Unravelling the Synergy between Oxygen Vacancies and Oxygen Substitution in BiO2−x for Efficient Molecular‐Oxygen Activation29Surface Engineering of g‐C3N4 by Stacked BiOBr Sheets Rich in Oxygen Vacancies for Boosting Photocatalytic Performance421Surface Engineering of g‐C3N4 by Stacked BiOBr Sheets Rich in Oxygen Vacancies for Boosting Photocatalytic Performance32A solvent-free strategy to realize the substitution of I − for IO 3 − in a BiOIO 3 photocatalyst with an opposite charge transfer path37Next Generation of Applications of Metal-Organic Frameworks for Energy and Environmental Sustainability0An Unprecedented Antimony(III) Borate with Strong Linear and Nonlinear Optical Responses224An Unprecedented Antimony(III) Borate with Strong Linear and Nonlinear Optical Responses42Two Covalent Ultraviolet Nonlinear Optical Crystals3Efficient Separation of Photogenerated Charges in Sandwiched Bi2S3−BiOCl Nanoarrays/BiVO4 Nanosheets Composites for Enhanced Photocatalytic Activity9Role of thermal decomposition process in the photocatalytic or photoluminescence properties of BiPO4 polymorphs36Designing 3D‐MoS2Sponge as Excellent Cocatalysts in Advanced Oxidation Processes for Pollutant Control496Designing 3D‐MoS2Sponge as Excellent Cocatalysts in Advanced Oxidation Processes for Pollutant Control87Enhanced Performance of a Novel Quaternary Nanocomposite CuO/ZnO/ZnS/CuS towards Removal of Dye Pollutant under Simulated Sunlight Irradiation5Photocatalysis Enhanced by External Fields460Photocatalysis Enhanced by External Fields46Plasmonic Hot Electrons from Oxygen Vacancies for Infrared Light‐Driven Catalytic CO 2 Reduction on Bi 2 O 3− x284Plasmonic Hot Electrons from Oxygen Vacancies for Infrared Light‐Driven Catalytic CO2 Reduction on Bi2O3−x71Structural and spectroscopic characterizations of boron doped TiO2–CeO2 nanocomposite synthesized by solution combustion technique for photocatalytic applications6Construction of K+ ions gradient in crystalline carbon nitride to accelerate charge separation for efficient visible light H2 production0Effect of ferroelectric Ba0.8Sr0.2TiO3 on the charge carrier separation of BiOBr at different temperature21Review on Bismuth‐Based Photocatalyst for CO2 Conversion50Efficient piezocatalytic removal of BPA and Cr(VI) with SnS2/CNFs membrane by harvesting vibration energy169Synergistic Polarization Engineering on Bulk and Surface for Boosting CO 2 Photoreduction306Synergistic Polarization Engineering on Bulk and Surface for Boosting CO2 Photoreduction21Ultrasound and water flow driven piezophototronic effect in self-polarized flexible α-Fe2O3 containing PVDF nanofibers film for enhanced catalytic oxidation113The Mechanism of Piezocatalysis: Energy Band Theory or Screening Charge Effect?321The Mechanism of Piezocatalysis: Energy Band Theory or Screening Charge Effect?206Spontaneous polarisation of ferroelectric BaTiO3/ZnO heterostructures with enhanced performance in a Fenton-like catalytic reaction24Self-Powered Water Flow-Triggered Piezocatalytic Generation of Reactive Oxygen Species for Water Purification in Simulated Water Drainage92Oxygen Vacancies Promoted Piezoelectricity toward Piezo-Photocatalytic Decomposition of Tetracycline over SrBi 4 Ti 4 O 15104Chemically Bonded α‐Fe2O3/Bi4MO8Cl Dot‐on‐Plate Z‐Scheme Junction with Strong Internal Electric Field for Selective Photo‐oxidation of Aromatic Alcohols13Chemically Bonded α‐Fe2O3/Bi4MO8Cl Dot‐on‐Plate Z‐Scheme Junction with Strong Internal Electric Field for Selective Photo‐oxidation of Aromatic Alcohols156Improved Polarization in the Sr6Cd2Sb6O7Se10 Oxyselenide through Design of Lateral Sublattices for Efficient Photoelectric Conversion4Improved Polarization in the Sr6Cd2Sb6O7Se10 Oxyselenide through Design of Lateral Sublattices for Efficient Photoelectric Conversion16Unsaturated Nd-Bi dual-metal sites enable efficient NIR light-driven O2 activation for water purification41Piezocatalytic Techniques in Environmental Remediation58Piezocatalytic Techniques in Environmental Remediation227Recent Advances in Tetra- (Ti, Sn, Zr, Hf) and Pentavalent (Nb, V, Ta) Metal-Substituted Molecular Sieve Catalysis123Dual‐Atomic‐Site Catalysts for Molecular Oxygen Activation in Heterogeneous Thermo‐/Electro‐catalysis82Dual‐Atomic‐Site Catalysts for Molecular Oxygen Activation in Heterogeneous Thermo‐/Electro‐catalysis14Emergence of Non‐photoresponsive Catalytic Techniques for Environmental Remediation and Energy Generation32One-pot synthesis of CdS nanoparticles with surface-phase junctions to catalyze the photo-reduction of CO2 into CO and CH4 selectively1A novel lateral epitaxial Bi2O3@BiOCl heterostructure for photocatalytic antibiotic degradation in an internal circulation fluidized bed reactor26Inducing piezoelectricity in distorted rutile TiO 2 for enhanced tetracycline hydrochloride degradation through photopiezocatalysis24New insight for enhanced photocatalytic activity of Bi4-xLaxTi3O12 (0 ≤ x ≤ 1) solid solution: A case study on degradation of Rhodamine B under UV light irradiation21Boosting PMS Activation Efficiency through Constructed Built-In Electric Field in ZnO/CuO Heterojunctions for Effective Sulfamethoxazole Degradation2Minimizing H 2 O 2 Loss in Industrial Electrosynthesis via Asymmetric Main‐Group Sn Single‐Atom Catalysts4

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  2. Enhanced Visible Light Photocatalytic Hydrogenation of CO2 into Methane over a Pd/Ce-TiO2 Nanocomposition

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  3. Reactable polyelectrolyte-assisted preparation of flower-like Ag/AgCl/BiOCl composite with enhanced photocatalytic activity

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  4. Sulfide oxide XZnSO (X = Ca or Sr) as novel active photocatalytic water splitting solar-to-hydrogen energy conversion

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  5. Facile synthesis of Bi/BiVO 4 composite ellipsoids with high photocatalytic activity

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  6. Oxygen Reduction Reaction for Generating H 2 O 2 through a Piezo‐Catalytic Process over Bismuth Oxychloride

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  7. Mixing Halogens To Assemble an All‐Inorganic Layered Perovskite with Warm White‐Light Emission

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  14. Enabling PIEZOpotential in PIEZOelectric Semiconductors for Enhanced Catalytic Activities

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  16. Piezoelectric‐Effect‐Enhanced Full‐Spectrum Photoelectrocatalysis in p–n Heterojunction

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  17. Intramolecular Charge Transfer and Extended Conjugate Effects in Donor–π–Acceptor‐Type Mesoporous Carbon Nitride for Photocatalytic Hydrogen Evolution

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  18. The Role of Polarization in Photocatalysis

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  19. The Role of Polarization in Photocatalysis

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  20. Visible‐Light‐Driven Water Oxidation with a Polyoxometalate‐Complexed Hematite Core of 275 Iron Atoms

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  22. Cs3Na(H2C3N3O3)4·3H2O: A Mixed Alkali‐Metal Hydroisocyanurate Nonlinear Optical Material Containing π‐Conjugated Six‐Membered‐Ring Units

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  50. Photocatalysis Enhanced by External Fields

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