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RESEARCH PAPER · Angewandte Chemie International Edition · 2019

The Role of Polarization in Photocatalysis

Fang Chen, Hongwei Huang, Lin Guo, Yihe Zhang, Tianyi Ma

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The Role of Polarization in PhotocatalysisOriginalCu supported on polymeric carbon nitride for selective CO 2 reduction into CH 4 : a combined kinetics and thermodynamics investigation113Graphitic carbon nitride synthesized by simple pyrolysis: role of precursor in photocatalytic hydrogen production208Nanostructured materials for photocatalysis1082Quenching induced hierarchical 3D porous g-C 3 N 4 with enhanced photocatalytic CO 2 reduction activity108Rational nanostructure design of graphitic carbon nitride for photocatalytic applications230Reactive sites rich porous tubular yolk-shell g-C3N4 via precursor recrystallization mediated microstructure engineering for photoreduction112Enhanced Visible-Light-Induced Photoactivity of Type-II CeO 2 /g-C 3 N 4 Nanosheet toward Organic Pollutants Degradation213Effective steering of charge flow through synergistic inducing oxygen vacancy defects and p-n heterojunctions in 2D/2D surface-engineered Bi2WO6/BiOI cascade: Towards superior photocatalytic CO2 reduction activity274Electronic and nanostructure engineering of bifunctional MoS2 towards exceptional visible-light photocatalytic CO2 reduction and pollutant degradation129Nano‐Ferroelectric for High Efficiency Overall Water Splitting under Ultrasonic Vibration334Substantially enhanced photoelectrochemical performance of TiO2 nanorods/CdS nanocrystals heterojunction photoanode decorated with MoS2 nanosheets142Unraveling the mechanism of binary channel reactions in photocatalytic formaldehyde decomposition for promoted mineralization138Oxygen vacancy rich Bi2O4-Bi4O7-BiO2-x composites for UV–vis-NIR activated high efficient photocatalytic degradation of bisphenol A172Photocatalytic behavior of biochar-modified carbon nitride with enriched visible-light reactivity117Bi4NbO8Cl {001} nanosheets coupled with g-C3N4 as 2D/2D heterojunction for photocatalytic degradation and CO2 reduction164Few-layer transition metal dichalcogenides (MoS2, WS2, and WSe2) for water splitting and degradation of organic pollutants: Understanding the piezocatalytic effect320An Efficient Strategy for Boosting Photogenerated Charge Separation by Using Porphyrins as Interfacial Charge Mediators126One pot synthesis of CdS/BiOBr/Bi2O2CO3: A novel ternary double Z-scheme heterostructure photocatalyst for efficient degradation of atrazine272Novel Au/La-Bi5O7I Microspheres with Efficient Visible-Light Photocatalytic Activity for NO Removal: Synergistic Effect of Au Nanoparticles, La Doping, and Oxygen Vacancy100Photocatalytic water splitting by N-TiO2 on MgO (111) with exceptional quantum efficiencies at elevated temperatures267Inter-plane heterojunctions within 2D/2D FeSe2/g-C3N4 nanosheet semiconductors for photocatalytic hydrogen generation274Charge Coupling Enhanced Photocatalytic Activity of BaTiO3/MoO3 Heterostructures98Efficient BiVO4 Photoanodes by Postsynthetic Treatment: Remarkable Improvements in Photoelectrochemical Performance from Facile Borate Modification171Visible-light-driven WO3/BiOBr heterojunction photocatalysts for oxidative coupling of amines to imines: Energy band alignment and mechanistic insight95Surface‐Polarity‐Induced Spatial Charge Separation Boosts Photocatalytic Overall Water Splitting on GaN Nanorod Arrays140PW12/CN@Bi2WO6 composite photocatalyst prepared based on organic-inorganic hybrid system for removing pollutants in water220Internal electric field engineering for steering photogenerated charge separation and enhancing photoactivity260Coupling Piezocatalysis and Photocatalysis in Bi4NbO8X (X = Cl, Br) Polar Single Crystals367Surface Engineering of g‐C3N4 by Stacked BiOBr Sheets Rich in Oxygen Vacancies for Boosting Photocatalytic Performance421Insights into the enhanced adsorption/photocatalysis mechanism of a Bi4O5Br2/g-C3N4 nanosheet142Synergistic effect of photocatalysis and pyrocatalysis of pyroelectric ZnSnO3 nanoparticles for dye degradation113Defect engineering in photocatalysis: formation, chemistry, optoelectronics, and interface studies314Exclusive enhancement of catalytic activity in Bi 0.5 Na 0.5 TiO 3 nanostructures: new insights into the design of efficient piezocatalysts and piezo-photocatalysts159Ferroelectric polarization and thin-layered structure synergistically promoting CO 2 photoreduction of Bi 2 MoO 6164Implementation of ferroelectric materials in photocatalytic and photoelectrochemical water splitting122Surface engineered 2D materials for photocatalysis92Integrating 2D/2D CdS/α-Fe2O3 ultrathin bilayer Z-scheme heterojunction with metallic β-NiS nanosheet-based ohmic-junction for efficient photocatalytic H2 evolution265Structure-property relationship in nonlinear optical materials with π-conjugated CO3 triangles146Recent Advances of Ferro-, Piezo-, and Pyroelectric Nanomaterials for Catalytic Applications332NaOH-induced formation of 3D flower-sphere BiOBr/Bi4O5Br2 with proper-oxygen vacancies via in-situ self-template phase transformation method for antibiotic photodegradation96Construction of Hierarchical Hollow Co 9 S 8 /ZnIn 2 S 4 Tubular Heterostructures for Highly Efficient Solar Energy Conversion and Environmental Remediation345Enhanced photoreduction CO2 activity on g-C3N4: By synergistic effect of nitrogen defective-enriched and porous structure, and mechanism insights121Facet-charge-induced coupling dependent interfacial photocharge separation: A case of BiOI/g-C3N4 p-n junction291Preparation of Ag/β-cyclodextrin co-doped TiO2 floating photocatalytic membrane for dynamic adsorption and photoactivity under visible light110Macroscopic Spontaneous Polarization and Surface Oxygen Vacancies Collaboratively Boosting CO 2 Photoreduction on BiOIO 3 Single Crystals591Z-scheme g-C3N4/Bi2O2[BO2(OH)] heterojunction for enhanced photocatalytic CO2 reduction103Cooperation of oxygen vacancies and 2D ultrathin structure promoting CO2 photoreduction performance of Bi4Ti3O12224One-step preparation (3D/2D/2D) BiVO4/FeVO4@rGO heterojunction composite photocatalyst for the removal of tetracycline and hexavalent chromium ions in water417Recent progress and strategies for enhancing photocatalytic water splitting99Advances in Piezo‐Phototronic Effect Enhanced Photocatalysis and Photoelectrocatalysis619Fabrication of direct Z-scheme Co3O4/BiOI for ibuprofen and trimethoprim degradation under visible light irradiation149Preparation and characterization of Vanadium pentoxide (V2O5) for photocatalytic degradation of monoazo and diazo dyes176Designing a Deep-UV Nonlinear Optical Fluorooxosilicophosphate127Updates on the Roadmap for Photocatalysis470Oxygen vacancies engineering in TiO2 homojunction/ZnFe-LDH for enhanced photoelectrochemical water oxidation260MoS2‑Stratified CdS-Cu2– x S Core–Shell Nanorods for Highly Efficient Photocatalytic Hydrogen Production148Remarkable Piezophoto Coupling Catalysis Behavior of BiOX/BaTiO 3 (X = Cl, Br, Cl 0.166 Br 0.834 ) Piezoelectric Composites209Effective promoting piezocatalytic property of zinc oxide for degradation of organic pollutants and insight into piezocatalytic mechanism193Piezopotential-driven simulated electrocatalytic nanosystem of ultrasmall MoC quantum dots encapsulated in ultrathin N-doped graphene vesicles for superhigh H2 production from pure water178Piezocatalytic Tumor Therapy by Ultrasound‐Triggered and BaTiO 3 ‐Mediated Piezoelectricity642Ferroelectric-field accelerated charge transfer in 2D CuInP2S6 heterostructure for enhanced photocatalytic H2 evolution140Tuning piezoelectric field for optimizing the coupling effect of piezo-photocatalysis186Recent progress on piezoelectric materials for renewable energy conversion108Photocatalysis Enhanced by External Fields460Facile assembled N, S-codoped corn straw biochar loaded Bi2WO6 with the enhanced electron-rich feature for the efficient photocatalytic removal of ciprofloxacin and Cr(VI)102Precise fabrication of single-atom alloy co-catalyst with optimal charge state for enhanced photocatalysis183Piezocatalysis and Piezo‐Photocatalysis: Catalysts Classification and Modification Strategy, Reaction Mechanism, and Practical Application986Coupling Effect of Piezo–Flexocatalytic Hydrogen Evolution with Hybrid 1T‐ and 2H‐Phase Few‐Layered MoSe2 Nanosheets105Insight into the piezo-photo coupling effect of PbTiO3/CdS composites for piezo-photocatalytic hydrogen production345Inside‐and‐Out Semiconductor Engineering for CO 2 Photoreduction: From Recent Advances to New Trends411Photocatalysis‐Assisted Co3O4/g‐C3N4 p–n Junction All‐Solid‐State Supercapacitors: A Bridge between Energy Storage and Photocatalysis153High visible light photocatalytic activities obtained by integrating g-C3N4 with ferroelectric PbTiO395Ultrathin Porous Carbon Nitride Bundles with an Adjustable Energy Band Structure toward Simultaneous Solar Photocatalytic Water Splitting and Selective Phenylcarbinol Oxidation379A review: Synthesis, modification and photocatalytic applications of ZnIn2S4360Coupling ferroelectric polarization and anisotropic charge migration for enhanced CO2 photoreduction1191 + 1 > 2: A critical review of MOF/bismuth-based semiconductor composites for boosted photocatalysis139Single Pd Atoms Synergistically Manipulating Charge Polarization and Active Sites for Simultaneously Photocatalytic Hydrogen Production and Oxidation of Benzylamine148Atomic‐Level Charge Separation Strategies in Semiconductor‐Based Photocatalysts505Bi4O5Br2 nanosheets with vertical aligned facets for efficient visible-light-driven photodegradation of BPA125Insights into the tribo-/pyro-catalysis using Sr-doped BaTiO3 ferroelectric nanocrystals for efficient water remediation118Enhanced charges separation to improve hydrogen production efficiency by organic piezoelectric film polarization113Recent advances on water disinfection using bismuth based modified photocatalysts: Strategies and challenges220Recent Advances in Noncontact External-Field-Assisted Photocatalysis: From Fundamentals to Applications357A critical review on strategies for improving efficiency of BaTiO3-based photocatalysts for wastewater treatment171Role of transition metal oxides in g-C3N4-based heterojunctions for photocatalysis and supercapacitors230Synergistic Polarization Engineering on Bulk and Surface for Boosting CO 2 Photoreduction3062D Graphitic Carbon Nitride for Energy Conversion and Storage448Flexoelectricity-induced enhancement in carrier separation and photocatalytic activity of a photocatalyst137Polarization-enhanced photocatalytic activity in non-centrosymmetric materials based photocatalysis: A review132Anion-exchange-mediated internal electric field for boosting photogenerated carrier separation and utilization136Defect engineering in metal sulfides for energy conversion and storage215Strain-Induced Ferroelectric Heterostructure Catalysts of Hydrogen Production through Piezophototronic and Piezoelectrocatalytic System110Facet Junction Engineering for Photocatalysis: A Comprehensive Review on Elementary Knowledge, Facet‐Synergistic Mechanisms, Functional Modifications, and Future Perspectives141Construction double electric field of sulphur vacancies as medium ZnS/Bi2S3-PVDF self-supported recoverable piezoelectric film photocatalyst for enhanced photocatalytic performance134Van Der Waals gap-rich BiOCl atomic layers realizing efficient, pure-water CO2-to-CO photocatalysis326Piezo‐Photocatalysis over Metal–Organic Frameworks: Promoting Photocatalytic Activity by Piezoelectric Effect418Enhancing the macroscopic polarization of CdS for piezo-photocatalytic water splitting154Facet junction of BiOBr nanosheets boosting spatial charge separation for CO2 photoreduction135Black phosphorus-based heterostructures for photocatalysis and photoelectrochemical water splitting107Recent advances in degradation of organic pollutant in aqueous solutions using bismuth based photocatalysts: A review143Local Spatial Polarization Induced Efficient Charge Separation of Squaraine‐Linked COF for Enhanced Photocatalytic Performance173Modulation of electric dipoles inside electrospun BaTiO3@TiO2 core-shell nanofibers for enhanced piezo-photocatalytic degradation of organic pollutants112Water treatment technologies in removing heavy metal ions from wastewater: A review491Enhanced Piezocatalytic Activity in Ion-Doped Sns2 Via Lattice Distortion Engineering for Bpa Degradation and Hydrogen Production131Recent advances and perspectives for solar-driven water splitting using particulate photocatalysts871High Photocatalytic Oxygen Evolution via Strong Built‐In Electric Field Induced by High Crystallinity of Perylene Imide Supramolecule207Utilizing electrostatic effect in fibrous filters for efficient airborne particles removal: Principles, fabrication, and material properties138Unraveling Charge‐Separation Mechanisms in Photocatalyst Particles by Spatially Resolved Surface Photovoltage Techniques1662D materials and heterostructures for photocatalytic water-splitting: a theoretical perspective251Engineering the Defects and Microstructures in Ferroelectrics for Enhanced/Novel Properties: An Emerging Way to Cope with Energy Crisis and Environmental Pollution144Photoelectrocatalytic degradation of refractory pollutants over WO3/W network photoelectrode with heterophase junction for enhancing mass transportation and charge separation93Oxygen Vacancies Promoted Piezoelectricity toward Piezo-Photocatalytic Decomposition of Tetracycline over SrBi 4 Ti 4 O 15104Steering Unit Cell Dipole and Internal Electric Field by Highly Dispersed Er atoms Embedded into NiO for Efficient CO2 Photoreduction111Chemically Bonded α‐Fe2O3/Bi4MO8Cl Dot‐on‐Plate Z‐Scheme Junction with Strong Internal Electric Field for Selective Photo‐oxidation of Aromatic Alcohols156Excellent piezo-photocatalytic performance of Bi4Ti3O12 nanoplates synthesized by molten-salt method172Layered bismuth-based photocatalysts300Piezocatalytic and Photocatalytic Hydrogen Peroxide Evolution of Sulfide Solid Solution Nano‐Branches from Pure Water and Air112Solar Energy Catalysis241A redox-active perylene-anthraquinone donor-acceptor conjugated microporous polymer with an unusual electron delocalization channel for photocatalytic reduction of uranium (VI) in strongly acidic solution162Challenges of photocatalysis and their coping strategies379Directing Charge Transfer in a Chemical‐Bonded BaTiO3@ReS2 Schottky Heterojunction for Piezoelectric Enhanced Photocatalysis294Dual vacancies induced local polarization electric field for high-performance photocatalytic H2 production112Polarization and external-field enhanced photocatalysis158Electric-/magnetic-field-assisted photocatalysis: Mechanisms and design strategies155Piezo-enhanced photocatalytic performance of ZnO nanorod array for pollutants degradation in dynamic water: Insight into the effect of velocity and inner flow field111Work function mediated interface charge kinetics for boosting photocatalytic water sterilization98Construction of a novel S-scheme heterojunction piezoelectric photocatalyst V-BiOIO3/FTCN and immobilization with floatability for tetracycline degradation165Piezocatalytic Techniques in Environmental Remediation227Precisely Constructed Metal Sulfides with Localized Single‐Atom Rhodium for Photocatalytic C−H Activation and Direct Methanol Coupling to Ethylene Glycol92Intrinsic Charge Polarization in Bi 19 S 27 Cl 3 Nanorods Promotes Selective CC Coupling Reaction during Photoreduction of CO 2 to Ethanol127Ultrasound-triggered piezocatalytic composite hydrogels for promoting bacterial-infected wound healing144Piezoelectric materials and techniques for environmental pollution remediation160Enabling Internal Electric Fields to Enhance Energy and Environmental Catalysis235Water flow induced piezoelectric polarization and sulfur vacancy boosting photocatalytic hydrogen peroxide evolution of cadmium sulfide nanorods105g-C3N4/TiO2/ZnIn2S4 graphene aerogel photocatalysts with double S-scheme heterostructure for improving photocatalytic multifunctional performances96Piezo-photocatalysts in the field of energy and environment: Designs, applications, and prospects186Nearly 100% selective and visible-light-driven methane conversion to formaldehyde via. single-atom Cu and Wδ+154Improving Interface Matching in MOF-on-MOF S-Scheme Heterojunction through π–π Conjugation for Boosting Photoelectric Response103Dipole field in nitrogen-enriched carbon nitride with external forces to boost the artificial photosynthesis of hydrogen peroxide263Piezoelectricity, Pyroelectricity, and Ferroelectricity in Biomaterials and Biomedical Applications198Hydrogel-based dressings designed to facilitate wound healing210Recent developments, advances and strategies in heterogeneous photocatalysts for water splitting221One-dimensional single atom arrays on ferroelectric nanosheets for enhanced CO2 photoreduction122Advances in Defect Engineering of Metal Oxides for Photocatalytic CO 2 Reduction138Harnessing the potential of hydrogels for advanced therapeutic applications: current achievements and future directions667Manipulating Ferroelectric Polarization and Spin Polarization of 2D CuInP 2 S 6 Crystals for Photocatalytic CO 2 Reduction95The photocatalytic H2O2 production: Design strategies, Photocatalyst advancements, environmental applications and future prospects212Enhancing photocatalytic performance of covalent organic frameworks via ionic polarization126Unraveling the dipole field in ultrathin, porous, and defective carbon nitride nanosheets for record-high piezo-photocatalytic H2O2 production95COF‐Based S‐Scheme Heterojunction Photocatalyst120

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  40. Electronic and nanostructure engineering of bifunctional MoS2 towards exceptional visible-light photocatalytic CO2 reduction and pollutant degradation

    Journal of Hazardous Materials · 2019-08-07

    Bilawal Khan, Fazal Raziq, M. Bilal Faheem, Muhammad Umar Farooq, Sadam Hussain, Farman Ali, Abid Ullah, Abdurashid Mavlonov, Yang Zhao, Zhongran Liu, He Tian, Huahai Shen, Xiaotao Zu, Sean Li, Haiyan Xiao, Xia Xiang, Liang Qiao

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  41. The Influence of pH on Phase and Morphology of BiOIO3 Nanoplates Synthesized by Microwave-Assisted Method and Their Photocatalytic Activities

    Journal of Inorganic and Organometallic Polymers and Materials · 2019-08-09

    Panudda Patiphatpanya, Anukorn Phuruangrat, Somchai Thongtem, Phattranit Dumrongrojthanath, Titipun Thongtem A

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  42. Nano‐Ferroelectric for High Efficiency Overall Water Splitting under Ultrasonic Vibration

    Angewandte Chemie International Edition · 2019-08-12

    Ran Su, H. Alex Hsain, Ming Wu, Dawei Zhang, Xinghao Hu, Zhipeng Wang, Xiaojing Wang, Fa‐tang Li, Xuemin Chen, Li‐Na Zhu, Yong Yang, Yaodong Yang, Xiaojie Lou, Stephen John Pennycook

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  43. Nano‐Ferroelectric for High Efficiency Overall Water Splitting under Ultrasonic Vibration

    Angewandte Chemie · 2019-08-12

    Ran Su, H. Alex Hsain, Ming Wu, Dawei Zhang, Xinghao Hu, Zhipeng Wang, Xiaojing Wang, Fa‐tang Li, Xuemin Chen, Li‐Na Zhu, Yong Yang, Yaodong Yang, Xiaojie Lou, Stephen John Pennycook

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  44. Silver-loaded In2S3-CdIn2S4@X(X=Ag, Ag3PO4, AgI) ternary heterostructure nanotubes treated by electron beam irradiation with enhanced photocatalytic activity

    The Science of The Total Environment · 2019-08-12

    Jing Wang, Tianli Yang, Ren He, Kehui Xue, Renrui Sun, Wenlei Wang, Juntao Wang, Ting Yang, Yuanlan Wang

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  45. Remarkably efficient charge transfer through a double heterojunction mechanism by a CdS-SnS-SnS2/rGO composite with excellent photocatalytic performance under visible light

    Journal of Hazardous Materials · 2019-08-14

    Mingxing Liang, Yajing Yu, Ying Wang, Yan Yu

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  46. Ultrathin graphitic carbon nitride modified PbBiO2Cl microspheres with accelerating interfacial charge transfer for the photodegradation of organic contaminants

    Colloids and Surfaces A Physicochemical and Engineering Aspects · 2019-08-15

    Qingsong Hu, Sheng Yin, Yi Ding, Ting Wu, Ming Li, Bin Wang, Yong Chen, Jun Di, Jiexiang Xia, Huaming Li

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  47. Substantially enhanced photoelectrochemical performance of TiO2 nanorods/CdS nanocrystals heterojunction photoanode decorated with MoS2 nanosheets

    Applied Catalysis B: Environmental · 2019-08-18

    Swetha S. M. Bhat, Sachin A. Pawar, Darshna D. Potphode, Chang‐Ki Moon, Jun Min Suh, Changyeon Kim, Seokhoon Choi, Dipali S. Patil, Jang‐Joo Kim, Jae Cheol Shin, Ho Won Jang

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  48. Competition of luminescence and photocatalysis in melilite: Recombination and transportation of electrons

    Physica B Condensed Matter · 2019-08-19

    Liwen Zhang, Haoyi Wu, Yahong Jin, Huangcheng Sun, Dong Liu, Yang Lv, Guifang Ju, Li Chen, Yihua Hu

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  49. Improving the Water Oxidation Efficiency with a Light-Induced Electric Field in Nanograting Photoanodes

    Nano Letters · 2019-08-20

    Wenrong Wang, Beidou Guo, Haitao Dai, Chang Ming Zhao, Guancai Xie, Renping Ma, Muhammad Zain Akram, Hangyong Shan, Congzhong Cai, Zheyu Fang, Jian Ru Gong

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  50. Ag-doped graphitic carbon nitride photocatalyst with remarkably enhanced photocatalytic activity towards antibiotic in hospital wastewater under solar light

    Journal of Industrial and Engineering Chemistry · 2019-08-22

    Nguyen Le Minh Tri, Ji-Tae Kim, Bạch Long Giang, Talal Mohammed Al tahtamouni, Phạm Thị Mai Hương, Changha Lee, Nguyen Minh Viet, Do Quang Trung

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