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RESEARCH PAPER · Angewandte Chemie International Edition · 2019

Freeing the Polarons to Facilitate Charge Transport in BiVO 4 from Oxygen Vacancies with an Oxidative 2D Precursor

Weitao Qiu, Shuang Xiao, Jingwen Ke, Zheng Wang, Songtao Tang, Kai Zhang, Wei Ping Qian, Yongchao Huang, Duan‐Ping Huang, Yexiang Tong, Shihe Yang

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Freeing the Polarons to Facilitate Charge Transport in BiVO 4 from Oxygen Vacancies with an Oxidative 2D PrecursorOriginalThe Role of Surface Oxygen Vacancies in BiVO 4168In Situ Formation of Oxygen Vacancies Achieving Near‐Complete Charge Separation in Planar BiVO4 Photoanodes375A cobalt silicate modified BiVO4 photoanode for efficient solar water oxidation96In situ growth of Fe2WO6 on WO3 nanosheets to fabricate heterojunction arrays for boosting solar water splitting27Improved hole extraction and durability of BiVO4 photoanode for solar water splitting under extreme pH condition34Activity and Stability Boosting of an Oxygen‐Vacancy‐Rich BiVO4 Photoanode by NiFe‐MOFs Thin Layer for Water Oxidation370Activity and Stability Boosting of an Oxygen‐Vacancy‐Rich BiVO4 Photoanode by NiFe‐MOFs Thin Layer for Water Oxidation40Anion exchange and successive ionic layer adsorption and reaction-assisted coating of BiVO4 with Bi2S3 to produce nanostructured photoanode for enhanced photoelectrochemical water splitting73First-Principle Insight Into the Effects of Oxygen Vacancies on the Electronic, Photocatalytic, and Optical Properties of Monoclinic BiVO4(001)31Vacancy defect engineering of BiVO 4 photoanodes for photoelectrochemical water splitting178Amorphous iron (III)-borate decorated electrochemically treated-BiVO4 photoanode for efficient photoelectrochemical water splitting58Controlling Charge Carrier Trapping and Recombination in BiVO 4 with the Oxygen Vacancy Oxidation State57Boosting the Photoelectrochemical Performance of BiVO4 Photoanodes by Modulating Bulk and Interfacial Charge Transfer26The gas sensor utilizing CeO2 nanorods for the low temperature detection of hydrogen36Recent progress of bismuth vanadate-based photoelectrocatalytic water splitting4A bridging coordination of urea tailoring metal hydroxides oxygen evolution catalysts promotes stable solar water splitting31Tungsten induced defects control on BiVO4 photoanodes for enhanced solar water splitting performance and photocorrosion resistance71BiVO4 Ceramic Photoanode with Enhanced Photoelectrochemical Stability6Influence of Oxygen Vacancies and Surface Facets on Water Oxidation Selectivity toward Oxygen or Hydrogen Peroxide with BiVO 457Boosting the Photoactivity of BiVO4 Photoanodes by a ZnCoFe‐LDH Thin Layer for Water Oxidation11Freeing the surface-bound excitons to facilitate water oxidation catalysis in BiVO4 photoanode9Boosting Charge Transport in BiVO4 Photoanode for Solar Water Oxidation260Charge-Compensated Doping Extends Carrier Lifetimes in SrTiO 3 by Passivating Oxygen Vacancy Defects42Enhancing the photocatalytic hydrogen production activity of BiVO 4 [110] facets using oxygen vacancies18Efficient NO removal and photocatalysis mechanism over Bi-metal@Bi2O2[BO2(OH)] with oxygen vacancies40Enhanced solar water splitting of BiVO 4 photoanodes by in situ surface band edge modulation52Harvesting of Infrared Part of Sunlight to Enhance Polaron Transport and Solar Water Splitting59Oxygen vacancy–based metal oxides photoanodes in photoelectrochemical water splitting214Built-in electron transport channels and interfacial ions doping in BiVO4 modified with isolated Ni atoms anchored on carbon hollow matrix for boosting charge separation and transport efficiency23Recent Progress on Semiconductor Heterojunction‐Based Photoanodes for Photoelectrochemical Water Splitting188Improving PEC Performance of BiVO4 by Introducing Bulk Oxygen Vacancies by He+ Ion Irradiation22Electronic defects in metal oxide photocatalysts534In-situ preparation of S-scheme BiOI/BiVO4 heterojunctions with enhanced photocatalytic performance18Elucidating the Role of Hypophosphite Treatment in Enhancing the Performance of BiVO4 Photoanode for Photoelectrochemical Water Oxidation51Depleted Oxygen Defect State Enhancing Tungsten Trioxide Photocatalysis: A Quantum Dynamics Perspective31Roles of Cocatalysts on BiVO 4 Photoanodes for Photoelectrochemical Water Oxidation: A Minireview39Surface Modulation Inducing Bismuth-Rich Surface Composition in BiVO4 for Efficient Photoelectrochemical Water Splitting25Boosting the Performance of BiVO 4 Photoanodes by the Simultaneous Introduction of Oxygen Vacancies and Cocatalyst via Photoelectrodeposition30Conferring BiVO4 Nanorods with Oxygen Vacancies to Realize Enhanced Sonodynamic Cancer Therapy140Conferring BiVO4 Nanorods with Oxygen Vacancies to Realize Enhanced Sonodynamic Cancer Therapy7New Views on Carrier Diffusion and Recombination by Combining Small Perturbation Techniques: Application to BiVO4 Photoelectrodes13Low-bias photoelectrochemical water splitting via mediating trap states and small polaron hopping166Sulfur-Induced Vacancies in Ba2Bi1.4Nb0.6O6 Promoting Photocatalytic Tetracycline Hydrochloride Degradation4Halide perovskites and high-pressure technologies: a fruitful encounter12Sulfur tuning oxygen vacancy of Ba2Bi1.4Ta0.6O6 for boosted photocatalytic tetracycline hydrochloride degradation and hydrogen evolution19Critical parameters and essential strategies in designing photoanodes to overcome the sluggish water oxidation reaction37Photo‐Electrochemical Glycerol Conversion over a Mie Scattering Effect Enhanced Porous BiVO 4 Photoanode97Visible light and iodate/iodide mediated degradation of bisphenol A by self-assembly 3D hierarchical BiOIO3/Bi5O7I Z-scheme heterojunction: Intermediates identification, radical mechanism and DFT calculation73In Situ Monitoring of the Spatial Distribution of Oxygen Vacancies and Enhanced Photocatalytic Performance at the Single-Particle Level41Boosting charge separation and transfer at the boron-triggered BiVO4 interface for efficient and stable solar water splitting53Modulating Oxygen Vacancies in Lead Chromate for Photoelectrocatalytic Water Splitting61Polaron-Mediated Transport in BiVO 4 Photoanodes for Solar Water Oxidation77Engineering BiVO4 and Oxygen Evolution Cocatalyst Interfaces with Rapid Hole Extraction for Photoelectrochemical Water Splitting262Photothermal‐boosted polaron transport in Fe2O3 photoanodes for efficient photoelectrochemical water splitting111Enhancing photoelectrochemical water oxidation activity of BiVO4 photoanode through the Co-catalytic effect of Ni(OH)2 and carbon quantum dots20Key Strategies for Enhancing H 2 Production in Transition Metal Oxide Based Photocatalysts91Key Strategies for Enhancing H2 Production in Transition Metal Oxide Based Photocatalysts31The Positive Versus Negative Effects of Defect Engineering for Solar Water Splitting: A Review72Exploring the impact of surface oxygen vacancies on charge carrier dynamics in BiVO4 photoanodes through atmospheric pressure plasma jet post-treatment for efficiency improvement in photoelectrochemical water oxidation62Enhancing the Photocatalytic Performance of BiVO4 for Micropollutant Degradation by Fe and Ag Photomodification5De‐Pinning Fermi Level and Accelerating Surface Kinetics with an ALD Finish Boost the Fill Factor of BiVO 4 Photoanodes to 44%21Synergistic integration of MoOx co-catalyst with oxygen vacancies-engineered on BiVO4 for enhancing the sensitivity of photoelectrochemical DNA biosensing19Novel Two-Dimensional MoC/MnSe Composites for Supercapacitors and Hydrogen Evolution Reaction7Correlation between Dynamics of Polaronic Photocarriers and Photoelectrochemical Performance in Mo-Doped Bismuth Vanadate3Simultaneous enhancement of charge transfer and surface catalysis through a polymetallic oxide cocatalyst on BiVO4 photoanodes for highly efficient and stable water oxidation8Tailoring of bulk oxygen vacancies in BiVO4 photoanodes via crystallization dynamics engineering for boosted photoelectrochemical water oxidation12Oxygen-Vacancy-Induced Enhancement of BiVO4 Bifunctional Photoelectrochemical Activity for Overall Water Splitting11Imaging charge carrier transfer in facet-dependent semiconductor photocatalysts by single-particle fluorescence spectroscopy4BiVO4 Polaron-Hopping State-Induced Low-Bias Spintronic Water Splitting Device4BiVO 4 ‐Based Photoelectrochemical Water Splitting37Activation of lattice oxygen in a medium-entropy oxide to facilitate an enhanced oxygen evolution reaction4The NaBH4 Reduction and pH Effects on the Optical Property of Bismuth Vanadate1Tailoring the special hole transfer layer between BiVO4 and oxygen evolution co-catalysts interfaces for boosting photoelectrochemical water splitting19Oxygen network formation for efficient charge transport and durable BiVO4 photoanodes with ultra-thin TiO2 layer in solar water splitting4Etched BiVO4 photocatalyst with charge separation efficiency exceeding 90%83Exposed Cocatalyst Interface with Cr–In Bonding for Efficient Solar‐Driven Fuel Production6Revealing the activity and stability origin of a B-modified BiVO4 photoanode with a NiFeCoBi cocatalyst for photoelectrochemical water oxidation and glycerol oxidation4Defect-engineered cocatalysts for photoelectrochemical water splitting: Recent advances in synthesis, characterization, and performance optimization5Coupling Facet‐Selective Photodeposition with Oxygen Vacancy‐Mediated Size Control of Pd Cocatalyst Over BiVO 4 for Solar‐Driven H 2 O 2 Production1Surface phosphate functionalization regulates electron-phonon coupling and glycerol oxidation pathway for dihydroxyacetone production over BiVO4 photoanodes0Thermally-enhanced charge collection boosts photoelectrochemical performance of hematite0Ion implantation-driven defect engineering in BiVO4 thin films for catalytic applications4Surface hole polaron site tuning governs charge carrier separation in BiVO4 photoanodes13Thermal Field–Enhanced Electro‐, Photo‐, and Photoelectrocatalytic Processes: Fundamentals, Material Design, and Applications3Harnessing the photothermal effect of PDA-mediated plasmon Ag NPs to activate fluorinated BiVO4 for enhanced solar water oxidation2Unlocking a High Photovoltage in BiVO 4 Photoanodes via Repairing Oxygen‐Defect‐Induced Surface Traps Boosting Photoelectrochemical Performance4Cationic vacancy in BiVO4 photoanode boosted microplastic degradation in aquatic environments1Surface phosphate functionalization regulates electron polaron and glycerol oxidation pathway for dihydroxyacetone production over BiVO4 photoanodes8Lattice engineering in NiO via Ti-incorporation for ultralong life hybrid aqueous zinc-ion capacitors0Single-Particle View of Doping-Controlled Charge Recombination in BiVO40

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  1. The Role of Surface Oxygen Vacancies in BiVO 4

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  2. In Situ Formation of Oxygen Vacancies Achieving Near‐Complete Charge Separation in Planar BiVO4 Photoanodes

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  3. A cobalt silicate modified BiVO4 photoanode for efficient solar water oxidation

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  4. In situ growth of Fe2WO6 on WO3 nanosheets to fabricate heterojunction arrays for boosting solar water splitting

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  5. Improved hole extraction and durability of BiVO4 photoanode for solar water splitting under extreme pH condition

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  6. Activity and Stability Boosting of an Oxygen‐Vacancy‐Rich BiVO4 Photoanode by NiFe‐MOFs Thin Layer for Water Oxidation

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  7. Activity and Stability Boosting of an Oxygen‐Vacancy‐Rich BiVO4 Photoanode by NiFe‐MOFs Thin Layer for Water Oxidation

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  8. Anion exchange and successive ionic layer adsorption and reaction-assisted coating of BiVO4 with Bi2S3 to produce nanostructured photoanode for enhanced photoelectrochemical water splitting

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  9. First-Principle Insight Into the Effects of Oxygen Vacancies on the Electronic, Photocatalytic, and Optical Properties of Monoclinic BiVO4(001)

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  10. Vacancy defect engineering of BiVO 4 photoanodes for photoelectrochemical water splitting

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  11. Amorphous iron (III)-borate decorated electrochemically treated-BiVO4 photoanode for efficient photoelectrochemical water splitting

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  12. Controlling Charge Carrier Trapping and Recombination in BiVO 4 with the Oxygen Vacancy Oxidation State

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  13. Boosting the Photoelectrochemical Performance of BiVO4 Photoanodes by Modulating Bulk and Interfacial Charge Transfer

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  14. The gas sensor utilizing CeO2 nanorods for the low temperature detection of hydrogen

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  15. Recent progress of bismuth vanadate-based photoelectrocatalytic water splitting

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  16. A bridging coordination of urea tailoring metal hydroxides oxygen evolution catalysts promotes stable solar water splitting

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  17. Tungsten induced defects control on BiVO4 photoanodes for enhanced solar water splitting performance and photocorrosion resistance

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  18. BiVO4 Ceramic Photoanode with Enhanced Photoelectrochemical Stability

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  19. Influence of Oxygen Vacancies and Surface Facets on Water Oxidation Selectivity toward Oxygen or Hydrogen Peroxide with BiVO 4

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  20. Boosting the Photoactivity of BiVO4 Photoanodes by a ZnCoFe‐LDH Thin Layer for Water Oxidation

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  21. Freeing the surface-bound excitons to facilitate water oxidation catalysis in BiVO4 photoanode

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  22. Boosting Charge Transport in BiVO4 Photoanode for Solar Water Oxidation

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  24. Enhancing the photocatalytic hydrogen production activity of BiVO 4 [110] facets using oxygen vacancies

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  25. Efficient NO removal and photocatalysis mechanism over Bi-metal@Bi2O2[BO2(OH)] with oxygen vacancies

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  26. Enhanced solar water splitting of BiVO 4 photoanodes by in situ surface band edge modulation

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  34. Elucidating the Role of Hypophosphite Treatment in Enhancing the Performance of BiVO4 Photoanode for Photoelectrochemical Water Oxidation

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  36. Roles of Cocatalysts on BiVO 4 Photoanodes for Photoelectrochemical Water Oxidation: A Minireview

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  37. Surface Modulation Inducing Bismuth-Rich Surface Composition in BiVO4 for Efficient Photoelectrochemical Water Splitting

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  38. Boosting the Performance of BiVO 4 Photoanodes by the Simultaneous Introduction of Oxygen Vacancies and Cocatalyst via Photoelectrodeposition

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  39. Conferring BiVO4 Nanorods with Oxygen Vacancies to Realize Enhanced Sonodynamic Cancer Therapy

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  40. Conferring BiVO4 Nanorods with Oxygen Vacancies to Realize Enhanced Sonodynamic Cancer Therapy

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  41. New Views on Carrier Diffusion and Recombination by Combining Small Perturbation Techniques: Application to BiVO4 Photoelectrodes

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  42. Low-bias photoelectrochemical water splitting via mediating trap states and small polaron hopping

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  43. Sulfur-Induced Vacancies in Ba2Bi1.4Nb0.6O6 Promoting Photocatalytic Tetracycline Hydrochloride Degradation

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  44. Halide perovskites and high-pressure technologies: a fruitful encounter

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  45. Sulfur tuning oxygen vacancy of Ba2Bi1.4Ta0.6O6 for boosted photocatalytic tetracycline hydrochloride degradation and hydrogen evolution

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  46. Critical parameters and essential strategies in designing photoanodes to overcome the sluggish water oxidation reaction

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  47. Photo‐Electrochemical Glycerol Conversion over a Mie Scattering Effect Enhanced Porous BiVO 4 Photoanode

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  48. Visible light and iodate/iodide mediated degradation of bisphenol A by self-assembly 3D hierarchical BiOIO3/Bi5O7I Z-scheme heterojunction: Intermediates identification, radical mechanism and DFT calculation

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  49. In Situ Monitoring of the Spatial Distribution of Oxygen Vacancies and Enhanced Photocatalytic Performance at the Single-Particle Level

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  50. Boosting charge separation and transfer at the boron-triggered BiVO4 interface for efficient and stable solar water splitting

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