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RESEARCH PAPER · Bulletin of the Chemical Society of Japan · 2021

Recent Progress on Mixed-Anion Materials for Energy Applications

Kazuhiko Maeda, Fumitaka Takeiri, Genki Kobayashi, Satoru Matsuishi, Hiraku Ogino, Shintaro Ida, Takao Mori, Yoshiharu Uchimoto, Setsuhisa Tanabe, Tetsuya Hasegawa, Nobuhito Imanaka, Hiroshi Kageyama

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Recent Progress on Mixed-Anion Materials for Energy ApplicationsOriginalA two-dimensional perovskite oxyfluoride Pb 3 Fe 2 O 5 F 2 as a catalyst for electrochemical oxidation of water to oxygen9Anionic ordering in Pb 2 Ti 4 O 9 F 2 revisited by nuclear magnetic resonance and density functional theory3Utility of NaMoO3F as a Precursor for Homogeneous Distribution of Cobalt Dopants in Molybdenum Oxynitrides2Pressure-induced structural phase transition in BaHCl3Orange Zn–Al–O–N Powder Active for Photocatalytic Water Reduction and Oxidation Synthesized from a Zn–Al Layered Double Hydroxide Using Urea as the Nitriding Agent4Strontium Nitridoborate Hydride Sr2BN2H Verified by Single-Crystal X-ray and Neutron Powder Diffraction7Computation-accelerated discovery of the K2NiF4-type oxyhydrides combing density functional theory and machine learning approach1Revealing Impacts of Anion Defect Species on Fluoride-Ion Conduction of Ruddlesden-Popper Oxyfluoride Ba2ScO3F10Experimental and Theoretical Correlation of Modulated Architectures of β-Ag2MoO4 Microcrystals: Effect of Different Synthesis Routes on the Morphology, Optical, Colorimetric, and Photocatalytic Properties23Molecular Machines and Microrobots: Nanoarchitectonics Developments and On-Water Performances18Biomass Nanoarchitectonics for Supercapacitor Applications22Highly sensitive UV photodetector based on solution-processed bismuth oxyiodide epitaxial thin films11Interlayer modification and single-layer exfoliation of the Ruddlesden–Popper perovskite oxynitride K 2 LaTa 2 O 6 N to improve photocatalytic H 2 evolution activity17Ultralow thermal conductivity in the mixed-anion solid solution Sn 2 SbS 2− x Se x I 319Z-scheme WOx/Cu-g-C3N4 heterojunction nanoarchitectonics with promoted charge separation and transfer towards efficient full solar-spectrum photocatalysis126Covalent nanoarchitectonics: Polymer synthesis with designer structures and sequences5Materials Nanoarchitectonics for Advanced Physics Research11In-situ Ni-oxidation-assisted coupling reduction of NiO and CO2 to synthesize core-shell Ni@octahedral carbon with energy storage properties12Interfacial nanoarchitectonics with porphyrins and related molecules: Langmuir-Blodgett method and layer-by-layer assembly7Rational Strategy for Tuning Electrocatalytic Oxygen Evolution Activity of Perovskite Oxides via Low-Temperature Fluorination13g‐C3N4 Nanosheet Nanoarchitectonics: H2 Generation and CO2 Reduction72Molecular nanoarchitectonics: unification of nanotechnology and molecular/materials science33Materials Nanoarchitectonics: Collaboration between Chem, Nano and Mat18A review on the synthesis, properties, and characterizations of graphitic carbon nitride (g-C3N4) for energy conversion and storage applications183Influence of the Hydride Content on the Local Structure of a Perovskite Oxyhydride BaTiO3–xHx7Evolutionary Algorithm Directed Synthesis of Mixed Anion Compounds LaF2X (X=Br, I) and LaFI28Evolutionary Algorithm Directed Synthesis of Mixed Anion Compounds LaF2X (X=Br, I) and LaFI22Structural Transformation in LnHS (Ln = La, Nd, Gd, and Er) with Coordination Change between an S-Centered Octahedron and a Trigonal Prism4Reduction of a Band Gap and Visible-Light Photocatalytic Activity Induced by the Interaction between 6s and 2p Orbitals known as Revised Lone Pair Model0Photocatalytic water splitting603La4Ga2S8O3: A Rare-Earth Gallium Oxysulfide with Disulfide Ions5Chemistry of Materials Nanoarchitectonics for Two-Dimensional Films: Langmuir–Blodgett, Layer-by-Layer Assembly, and Newcomers73Controlling the Luminescence of Rare-Earth Chalcogenide Iodides RE3(Ge1–xSix)2S8I (RE = La, Ce, and Pr) and Ce3Si2(S1–ySey)8I8Selective Synthesis of Perovskite Oxyhydrides Using a High-Pressure Flux Method5Low-Temperature Microwave-Assisted Hydrothermal Synthesis of Pb2Ti2O5.4F1.2 Photocatalyst for Improved H2 Evolution under Visible Light16Liquid–Liquid Interfacial Nanoarchitectonics42Development of Electrochemical Anion Doping Technique for Expansion of Functional Material Exploration17Disease Diagnosis with Chemosensing, Artificial Intelligence, and Prospective Contributions of Nanoarchitectonics5Perovskite BaTaO 2 N: From Materials Synthesis to Solar Water Splitting44Photocatalytic Hydrogen Evolution Activity of Nitrogen/Fluorine-Codoped Rutile TiO22Nanoarchitectonics: the method for everything in materials science252Chiral and Polar Duality Design of Heteroanionic Compounds: Sr18Ge9O5S31 Based on [Sr3OGeS3]2+ and [Sr3SGeS3]2+ Groups20Fluorination strategy toward chemical and functional modification65A brief review of characteristic luminescence properties of Eu 3+ in mixed-anion compounds53Bio-gel nanoarchitectonics in tissue engineering28Chemical perspectives on heteroanionic compounds: a potential playground for multiferroics7Fluorosulfide La 2.7 Ba 6.3 F 8.7 S 6 with a double-layer honeycomb structure enabling fluoride-ion conduction3Internal strain-driven bond manipulation and band engineering in Bi 2− x Sb x YO 4 Cl photocatalysts with triple fluorite layers7Lateral nanoarchitectonics from nano to life: ongoing challenges in interfacial chemical science29Layer-by-layer designer nanoarchitectonics for physical and chemical communications in functional materials51Molecular machines working at interfaces: physics, chemistry, evolution and nanoarchitectonics25Potential application of bismuth oxyiodide (BiOI) when it meets light46Materials Nanoarchitectonics at Dynamic Interfaces: Structure Formation and Functional Manipulation18Novel synthetic approaches and morphological design of perovskite-type oxynitrides in powder and ceramic form5Mist Chemical Vapor Deposition of Bi 13 S 18 I 2 for Photoelectrochemical-type Photodetection132D Materials Nanoarchitectonics for 3D Structures/Functions8Confined Space Nanoarchitectonics for Dynamic Functions and Molecular Machines5Pinalites: Optical Properties and Quantum Magnetism of Heteroanionic A3MO5X2 Compounds6Modification of Visible‐Light‐Responsive Pb2Ti2O5.4F1.2 with Metal Oxide Cocatalysts to Improve Photocatalytic O2 Evolution toward Z‐Scheme Overall Water Splitting7Composite Nanoarchitectonics Towards Method for Everything in Materials Science12Influence of Composition and Structure on the Optoelectronic Properties of Photocatalytic Bi4NbO8Cl–Bi2GdO4Cl Intergrowths3Preparation of TaON thin films by nitridation of solution process-derived precursor films with urea4Liquid–Liquid and Liquid–Solid Interfacial Nanoarchitectonics11Interface‐Interactive Nanoarchitectonics: Solid and/or Liquid5Average Cubic BaTaO 2 N Crystal Structure Formed by 50 nm Size Domains with Polar Nanoregions Consisting of cis -TaO 4 N 2 Octahedral Chains6Ae3[TO3][SnOQ3] (Ae = Sr, Ba; T = Si, Ge; Q = S, Se) and Ba3[CO3][MQ4] (M = Ge, Sn; Q = S, Se): Design and Syntheses of a Series of Heteroanionic Antiperovskite-Type Oxychalcogenides29PVDF fluorination of La4Co3O10: Synthesis, structure and physical properties of La4Co3O10F25Characterization and Solid-State UV–Vis Investigations of Photoelectrocatalytically Active La5Cl7[TeO3]4, a Mixed Anion Compound with Alternating 2D Layers of Oxygen and Chlorine2La2O2MQ2 phases: Stability and synthetic challenges0In Situ Single-phase Formation of LaCl(CN2) Mixed-Anion Compound Via Controlled Pyrolysis of La3+ Modified Melamine Precursor1Supra-ceramics: a molecule-driven frontier of inorganic materials45Nanoarchitectonics for Biomedical Research: Post‐Nanotechnology Materials Approach for Bio‐Active Application6Layered nanoarchitectonics for condensed hard matter, soft matter, and living matter5Iron-Based Layered Perovskite Oxyfluoride Electrocatalyst for Oxygen Evolution: Insights from Crystal Facets with Heteroanionic Coordination15Effects of the anion exchange between I − and NCS − coordinated to Co 2+ -centered tetrahedra in the organic–inorganic hybrid halides0Excellent thermoelectric performance of Bi 2 MO 4 Cl (M = Y, La, and Bi) derived from ultra-low lattice thermal conductivity10Fluoride-target-assisted growth of Pb 2 OF 2 oxyfluoride films with anion ordering and high dielectric constant0Influence of anion ordering on defect diffusion anisotropy in layered perovskite Sr 2 TaO 3 N: implications for oxynitride stability2La 2 ZnGa 2 S 6 O: a melilite-type transition metal oxysulfide achieving a well-balanced nonlinear optical behavior5Mechanochemical preparation of perovskite-type oxyhydrides BaLnO 2 H (Ln = Tb–Lu) and their catalytic activity for ammonia synthesis3Mixed-anion chalcogenide-halide semiconductors A 2 BaTaS 4 Cl (A = K, Rb, Cs) and K 2 BaNbS 4 Cl1Preparation of multi-element soluted metal oxynitrides with a perovskite structure using precursors synthesized through a liquid-phase process1Synthesis and large crystal growth of a family of mixed-anionic methanesulfonate salts by anionic site-substitution: Na 5 (SO 3 CH 3 ) 4 (X) (X = BF 4 − , ClO 4 − , PF 6 − , I − )9Synthesis of a series of rare-earth-based multi-anion chalcogenide iodides RE 3 Si 2 Se x S 8− x I (RE = La, Ce, Pr, and Nd) using the flux-assisted boron–chalcogen mixture method14Synthesis, structure, and ionic transport properties of lithium monothiophosphate pentahydrate Li 3 PO 3 S·5H 2 O and its anhydrous form Li 3 PO 3 S0Tunable optical properties in the (110) p -oriented layered halide perovskite FA 4 Pb 2 I 7.5 (SCN) 0.5 by Br substitution0Layered Anion‐Mixed Oxycompounds: Synthesis, Properties, and Applications29Solid-State Synthesis Enables Enhanced Crystallinity and Tunable Optical Properties in Lanthanum Oxytelluride2Photocatalytic and photoelectrochemical H2 generation for sustainable future: Performance improvement, techno-economic analysis, and life cycle assessment for shaping the reality24Investigation of atmospheric moisture interaction on modified copper surfaces using thermoelectric cooling1Oxyfluorides for electrochemical and photoelectrochemical water oxidation: a review and basic tutorial0Enhancing fluoride-ion conduction via doping-induced anionic ordering in an n = 1 Ba-based Ruddlesden-Popper oxyfluoride structure0Anion-Controlled Inorganic Materials as Catalysts for Small-Molecule Conversion Reactions8Hidden Complexity in the TiO 2 to TiN Transformation Unveiled through Compositional Analysis4Unveiling anionic migration mechanisms governed by mixed-anion chemistry in melilite oxyfluorides2Mixed-anion thermoelectrics: Advanced tuning of electron and phonon transport10Tracing nitridation reaction toward efficient production of oxynitride glasses as hosts for bright luminescence centers0A new non-stoichiometric orthopyrophosphate Na2.48Cd4.15(P2O7)2(PO4): Crystal structure, defect chemistry and Eu3+-activated luminescence0Anion-gradient engineering of superconductivity in mixed-anion Nb(O,N) epitaxial thin films0Experimental and machine learning-assisted prediction of nitridation of Ta2O5 to TaON1Te–Se replacement induced structural transition and enhanced band gaps in Cd 5 Se 4 O 12 Cl 2 and Cd 5 Se 4 O 12 Br 21Unveiling the impact of bonding asymmetry on the lattice thermal conductivity of MnXS2Cl (X=Sb, Bi) for promising thermoelectric applications1The Mixed Halogen-Ion Effect in Lead Silicate Glasses: A Correlative Study of Ionic Transport and Optical Spectroscopy in the 45PbO–xPbF2–(20−x)PbCl2–35SiO2 System1A Lead(II)-Based Coordination Polymer Exhibiting Photocatalytic and Electrochemical CO 2 Reduction Activities0Pseudocapacitive MOXEN-based asymmetric supercapacitors: A comprehensive review on design strategies, electrochemical insights, and commercial prospects1Cu 7.62 Bi 6 Se 12 Cl 6 I: Discovery of a Low Band Gap, Low Thermal Conductivity Mixed-Anion Material0Changing Polyhedral Connectivity through Sulfide Introduction in an Ionically Conducting Na–Ta–Cl–S Mixed Anion System3Strain effects on the photocatalytic properties of perovskite Mg3PBr3: A first-principles study0First-principles investigation of structural, electronic, thermal, and optical properties of three dimensional mixed-anion LuSeF1Mixed-Anion-Induced Asymmetric Orbital Hybridization Governs Carrier Transport and Photoresponse in Monolayer TiOS0

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