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RESEARCH PAPER · Nature Reviews Methods Primers · 2023

Photocatalytic water splitting

Shunta Nishioka, Frank E. Osterloh, Xinchen Wang, Thomas E. Mallouk, Kazuhiko Maeda

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Photocatalytic water splittingOriginalOrganic conjugation of graphitic carbon nitride nanocomposites for boosted photocatalytic water splitting16Low-Temperature Microwave-Assisted Hydrothermal Synthesis of Pb2Ti2O5.4F1.2 Photocatalyst for Improved H2 Evolution under Visible Light16Enhanced microwave absorption of g-C3N4/poly(vinylidene difluoride)/carbon black composites20ZnO/ZnS/CdS three-phase composite photocatalyst with a flower cluster structure: Research on its preparation and photocatalytic activity hydrogen production95Enhancing prediction accuracy of physical band gaps in semiconductor materials18Strategies to Enhance Interfacial Spatial Charge Separation for High‐Efficiency Photocatalytic Overall Water‐Splitting: A Review48Hybridization of covalent organic frameworks and photosensitive metal‐organic rings: A new strategy for constructing supramolecular Z‐scheme heterostructures for ultrahigh photocatalytic hydrogen evolution32Ultrasound-assisted piezoelectric photocatalysis: An effective strategy for enhancing hydrogen evolution from water splitting86Particulate metal chalcogenides for photocatalytic Z-scheme overall water splitting89Recent advances and mechanisms in magnetic field enhanced photocatalysis: A review35Urchin-like TiO2/CdS Nanoparticles Forming an S-scheme Heterojunction for Photocatalytic Hydrogen Production and CO2 Reduction35ZIF-67-derived hollow CoS and Mn0·2Cd0·8S to form a type-II heterojunction for boosting photocatalytic hydrogen evolution19Synthesis and characterization of erbium decorated V2CTx for water splitting properties43Cd(Eu)Se/CdS/CdZnS/ZnS quantum dots with hydrophilic alloy shell supported by flower-like ZnIn2S4: A S-scheme for efficient photocatalytic H2 evolution16Bimetallic nitride NiMoN loaded on graphitic carbon nitride for plasmon-enhanced visible light-driven photocatalytic hydrogen evolution from water splitting17Contact-electro-catalysis under natural and industrial conditions: mechanisms, strategies, and challenges31Effect of Phase Structure of Bi5o7i on the Photocatalytic Activity of S-Scheme Agbr/Ag/Bi5o7i23Extending 2D covalent organic frameworks by inserting anthracene for promoted white-light-mediated photocatalysis17Facets control charge separation during photoelectrochemical water oxidation with strontium titanate (SrTiO 3 ) single crystals36Future perspectives in green hydrogen production by catalyzed sono-photolysis of water20Impact of functional groups on cellulose nanofibers on the state of water molecules, photocatalytic water splitting, and photothermal water evaporation30Near-infrared photocatalysis with cyanines: synthesis, applications and perspectives44Photocatalytic applications of covalent organic frameworks: synthesis, characterization, and utility33Processing polymer photocatalysts for photocatalytic hydrogen evolution33Rational design of versatile 1D Ti–O-based core–shell nanostructures for efficient pollutant removal and solar fuel production15Recent progress in atomically precise metal nanoclusters for photocatalytic application51Recent progress on the photocatalytic hydrogen evolution reaction over a metal sulfide cocatalyst-mediated carbon nitride system26Single-molecule fluorescence imaging of photocatalytic nanomaterials19Solar fuel production through concentrating light irradiation24A Hybrid Photocatalytic System Splits Atmospheric Water to Produce Hydrogen55In-situ constructing ZnIn2S4@In(OH)3@CdS heterostructure for efficient photocatalytic H2 generation under visible light irradiation23Tailoring the catalytic sites by regulating photogenerated electron/hole pairs separation spatially for simultaneous selective oxidation of benzyl alcohol and hydrogen evolution42Molten salt synthesis of 1T/2H mixed phase MoS2 for boosting photocatalytic H2 evolution via Schottky junction under EY-sensitized system31TiO2-based S-scheme photocatalysts for solar energy conversion and environmental remediation154P‐N Bonds‐Mediated Atomic‐Level Charge‐Transfer Channel Fabricated between Violet Phosphorus and Carbon Nitride Favors Charge Separation and Water Splitting19Synchrotron Radiation Based X‐ray Absorption Spectroscopy: Fundamentals and Applications in Photocatalysis23Converting H2O and CO2 into chemical fuels by nickel via friction21Tunable Interfacial Electronic and Photoexcited Carrier Dynamics of an S-Scheme MoSi2N4/SnS2 Heterojunction2314.8% Quantum Efficient Gallium Phosphide Photocatalyst for Hydrogen Evolution37Spatially Separated Photoredox in a Covalent Organic Frameworks Heterostructure Boosting Overall Water Splitting37Mechanisms of noble metal-enhanced ferroelectric spontaneous polarized photocatalysis45Salt‐melt synthesis of poly(heptazine imide) in binary alkali metal bromides for enhanced visible‐light photocatalytic hydrogen production40Exploiting hot electrons from a plasmon nanohybrid system for the photoelectroreduction of CO217Hierarchical S-scheme heterojunctions of ZnIn2S4-decorated TiO2 for enhancing photocatalytic H2 evolution97Recent progresses in improving the photocatalytic potential of Bi4Ti3O12 as emerging material for environmental and energy applications19Recent advances in one-dimensional alkali-metal hexatitanate photocatalysts for environmental remediation and solar fuel production20Synergistic redox reactions toward co‐production of H2O2 and value‐added chemicals: Dual‐functional photocatalysis to achieving sustainability35A nanocage reactor with dense shareable hot spots for in-situ and dynamic SERS tracking photocatalytic reaction bonds variations20Efficient interfacial charge transfer in the MoSe2/SPtSe heterostructure improves the efficiency of hydrogen production from water splitting: A S-scheme photocatalyst29Laser fragmentation of a high-entropy oxide for enhanced photocatalytic carbon dioxide (CO2) conversion and hydrogen (H2) production22Self-assembled monolayer mediated fast charge transport of Sb2(S,Se)3 photocathode enabling high-performance unbiased water splitting20Unveiling the charge transfer dynamics regulated by bonding evolution in single-atom Pt/C3N5 for boosting hydrogen evolution25S-Scheme Heterojunction/Single-Atom Dual-Driven Charge Transport for Photocatalytic Hydrogen Production151Advances in Computational Methods for Modeling Photocatalytic Reactions: A Review of Recent Developments41S‐Scheme g‐C3N4/CdS Heterostructures Grafting Single Pd Atoms for Ultrafast Charge Transport and Efficient Visible‐Light‐Driven H2 Evolution84Cascade utilization of full spectrum solar energy for achieving simultaneous hydrogen production and all-day thermoelectric conversion24Hollow SrTiO3 photocatalyst with spatially separated OER and HER cocatalysts for photocatalytic overall water splitting22Solar‐Driven Biomass Reforming for Hydrogen Generation: Principles, Advances, and Challenges66Extended light absorption and accelerated charge migration in ultrathin twisted carbon nitride nanoplates for efficient solar hydrogen production67Synergy of oxygen doping and nitrogen vacancy for promoting photocatalytic hydrogen generation of g-C3N420Hydrogel composites based on chitosan and CuAuTiO2 photocatalysts for hydrogen production under simulated sunlight irradiation17The photocatalytic wastewater hydrogen production process with superior performance to the overall water splitting25Interface engineering of Z-scheme heterojunction for photocatalytic water splitting22A new family of septuple-layer 2D materials of MoSi2N4-like crystals76Water Structure in the First Layers on TiO2: A Key Factor for Boosting Solar-Driven Water-Splitting Performances64Molecular Engineering of Methylated Sulfone‐Based Covalent Organic Frameworks for Back‐Reaction Inhibited Photocatalytic Overall Water Splitting41Recent advances in zinc oxide-based photoanodes for photoelectrochemical water splitting51Carbon neutrality and hydrogen energy systems465Near-infrared light–driven biomass conversion61Piezoelectric, Thermoelectric, and Photocatalytic Water Splitting Properties of Janus Arsenic Chalcohalide Monolayers15Synergistic manipulation of sulfur vacancies and palladium doping of In2S3 for enhanced photocatalytic H2 production33Emerging breakthroughs in covalent triazine frameworks: From fundamentals towards photocatalytic water splitting and challenges75Construction of 4-Amino-1H-imidazole-5-carbonitrile Modified Carbon Nitride-based Donor-Acceptor Photocatalyst for Efficient Photocatalytic Hydrogen Evolution23Underlying Developments in Hydrogen Production Technologies: Economic Aspects and Existent Challenges41Manipulating Photoconduction in Supramolecular Networks for Solar-Driven Nitrate Conversion to Ammonia and Oxygen24The future of alkaline water splitting from the perspective of electrocatalysts-seizing today's opportunities140Unraveling the Microstructure‐Property Relationship of Fe Single‐Atoms via Introducing Asymmetric P‐Coordination for Photocatalytic Hydrogen Evolution32Coupling Photocatalytic Hydrogen Production with Key Oxidation Reactions161In situ decoration of 2D-MoS2/ZIF-67 type II heterojunction for enhanced hydrogen production under simulated sunlight18Photo Electrocatalytic Water Splitting Using Sn Doped In 2 S 3 Homologous Series Synthesized in Oxygen Deficient Flame24Tightly Interfaced Cu2O with In2O3 to Promote Hydrogen Evolution in Presence of Biomass‐Derived Alcohols19Modulating d-p-band electron coupling by N-doping for promoting CuSAs-N/TiO2 photocatalytic hydrogen evolution16Synergizing black gold and light: A comprehensive analysis of biochar-photocatalysis integration for green remediation23Insight into the Rate-Determining Step in Photocatalytic Z-Scheme Overall Water Splitting by Employing A Series of Perovskite RTaON2 (R = Pr, Nd, Sm, and Gd) as Model Photocatalysts43Advancements in MXene-based frameworks towards photocatalytic hydrogen production, carbon dioxide reduction and pollutant degradation: Current challenges and future prospects106Advances in hybrid strategies for enhanced photocatalytic water splitting: Bridging conventional and emerging methods24Dual electron transfer path and Ti3C2Tx LSPR photothermal enhancement in 2D/2D/2D Ti3C2Tx MXene@TiO2/CdIn2S4 ternary heterojunction for enhanced photocatalytic H2 production: Construction, kinetics, and mechanistic insights63Recent Progress in External‐Field Enhanced Photo‐Electrochemistry20Robust photocatalytic hydrogen evolution performance of 0D/1D NiO/CdS S-scheme heterojunction27Visualizing Ultrafast Photogenerated Electron and Hole Separation in Facet-Engineered Bismuth Vanadate Crystals44Conjugated carbon network mediated – Graphdiyne based Cu2MoS4 homojunction for enhanced charge transfer dynamics17Recent advances in hybrid photocatalysts for efficient solar photocatalytic hydrogen production41Atomically dispersed metal site materials for hydrogen energy utilization: Theoretical and experimental study in fuel cells and water electrolysis16Defect-Induced Atomical Zn–O/N–C Bonding Promotes Efficient Charge Transfer in S-Scheme Interface for Bubble Level Solar Hydrogen Production27Recent Advances of Photocatalytic CO2 Reduction Based on Hybrid Molecular Catalyst/Semiconductor Photocatalysts: A Review21Recent advances in inorganic oxide semiconductor-based S-scheme heterojunctions for photocatalytic hydrogen evolution44Oxygen vacancy-rich 2D/2D S-scheme photocatalyst CN/BiOBr-OV for efficient azo dye degradation26Insights into Bubble Dynamics in Water Splitting79Photocatalytic production of H2O2 over rutile TiO2 supported with Pd nanoparticles25Manipulating p ‐π Resonance through Methoxy Group Engineering in Covalent Organic Frameworks for an Efficient Photocatalytic Hydrogen Evolution58N, O-Doped surface modulation of ZnIn2S4 with high hydrophilicity for enhanced photocatalytic hydrogen evolution28Cryo‐Electrochemical Deposition of Gold Single Atoms on G ‐C 3 N 4 for Photoelectrochemical Water Reduction16Pd single atoms on g-C 3 N 4 photocatalysts: minimum loading for maximum activity39Recent advances in MOF composites for photocatalysis122Semiconductor photocatalysts for hydrogen evolution: critical role of cocatalysts in enhancing performance38Precise Manipulation on the Structural Defects of Poly (Triazine Imide) Single Crystals for Efficient Photocatalytic Overall Water Splitting75A novel breakthrough in the invention, properties, synthesis of covalent heptazine framework for its sustainable applications24Rapid Charge Transfer Endowed by Heteroatom Doped Z‐Scheme Van Der Waals Heterojunction for Boosting Photocatalytic Hydrogen Evolution29Harnessing Hydrogen Spillover by Lattice Strain for Enhanced Photocatalytic Hydrogen Evolution of ZnIn 2 S 485Exceptional anti-fouling, self-cleaning and high-flux ZIF-8@polyacrylonitrile based nanofiber composite membrane via in situ growth of seaweed-like ZnIn2S4 for efficient separation of emulsified oily wastewater41Efficient Hole Extraction and *OH Alleviation by Pd Nanoparticles on GaN Nanowires in Seawater for Solar‐Driven H 2 and H 2 O 2 Generation38Engineering electron delocalization of ultrathin covalent organic framework nanosheets to elevate photocatalytic hydrogen evolution in seawater27Versatile BiFeO 3 shining in piezocatalysis: From materials engineering to diverse applications31Photocatalytic Hydrogenation of Levulinic Acid and Furfural to Fuel Additives over Ru-Decorated Carbon-Channelized Catalyst19Molecular Photoelectrodes with Enhanced Photogenerated Charge Transport for Efficient Solar Hydrogen Evolution32Recent advances of covalent organic frameworks-based photocatalysts: Principles, designs, and applications99ZnIn2S4/Cs3PMo12O40 heterojunction with enhanced photocatalytic performance for formaldehyde degradation and tetracycline removal43Advances in Atomically Dispersed Catalysts for Water Splitting36Inorganic–Organic Bi 4 Nb 1– x Ta x O 8 Cl/rGO/SA-PTA Z-Scheme Heterojunction with a Third-Order Polarized Electric Field and a Fast Electron Transfer Channel for Photocatalytic Overall Water Splitting37Single‐atom catalysts in photocatalysis: unveiling the essential roles of water17Charge-transfer dynamics in S-scheme photocatalyst579Development in Photoelectrochemical Water Splitting Using Carbon-Based Materials: A Path to Sustainable Hydrogen Production21A superlattice interface and S-scheme heterojunction of Mn0.5Cd0.5S/MnWO4 for enhancing photocatalytic H2 production34Defect‐Rich UiO‐66‐NH 2 /LDHs for Photocatalytic Hydrogen Generation from Seawater21Simultaneously Tailoring Hydrostability and Photoelectroactivity in Heterocluster Metal–Organic Frameworks for Efficient Photocatalytic Hydrogen Production39A current review of TiO2 thin films: synthesis and modification effect to the mechanism and photocatalytic activity40Tunable multi-electron redox polyoxometalates for decoupled water splitting driven by sunlight40Etched BiVO4 photocatalyst with charge separation efficiency exceeding 90%83Photocatalytic Hydrogen Production Using Semiconductor (CdSe) 13 Clusters18Nanomaterial ZnO Synthesis and Its Photocatalytic Applications: A Review124Production of H 2 O 2 via Energy Transfer Photocatalysis by Coupling with Furfuryl Alcohol Conversion over an Amide‐Functionalized Heptazine Framework16Review and Outlook of Graphene-Based Catalysis: Revolutionizing Water Splitting for Sustainable Hydrogen Production43Scalable and Integrated Photocatalytic Reactor Systems for Solar‐to‐Fuel Production: Photoredox and Photoreforming Processes38Halide Perovskite Photocatalysts for Clean Fuel Production and Organic Synthesis: Opportunities and Challenges68The advances on scaling-up of photocatalytic and photoelectrochemical hydrogen production and field demonstration35Immobilization of Covalent Triazine Framework into Hydrogels for Photothermal‐Promoted Gas‐Solid Photocatalytic Hydrogen Production42Breaking Barriers: Synergistic Interactions Between Pt Single Atoms and Nitrogen‐Rich g‐C3N4 for Maximized Photocatalytic Hydrogen Production21Classification and Characterization Methods for Heterojunctions68Green and sustainable metal-organic frameworks (MOFs) in wastewater treatment: A review63Green and blue hydrogen production and purification technologies28Toward Doping in Graphitic Carbon Nitride: Progress and Perspectives on Catalytic Hydrogen Production19Materials and systems for large-scale photocatalytic water splitting202Gas-involved photo- and electro-catalysis roadmap towards 203025Insights into the physical properties of NaGeH3 perovskite hydride for hydrogen storage applications: A first-principles study22Synergistic Integration of Atmospheric Water Harvesting and Solar‐Driven Hydrogen Production via Multifunctional Hygroscopic‐Photocatalytic Hydrogel Nanocomposite43Design Strategies and Roles of Hydrogels for Sustainable Energy Conversion and Harvesting from Natural and Biological Environments28High-entropy perovskites as new photocatalysts for cocatalyst-free water splitting25Ni–N bonds boost S-scheme charge transfer in NiSe/Cv-C3N5 for efficient water splitting26Recent advances in graded nanomaterial-based photocatalysts: Principles, designs, and applications30Ligand Conjugation‐Induced Microenvironment Modulation in Defective Metal‐Organic Framework Promotes Photocatalytic Hydrogen Evolution28

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