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RESEARCH PAPER · Journal of the American Chemical Society · 2021

Structure Tuning, Strong Second Harmonic Generation Response, and High Optical Stability of the Polar Semiconductors Na1–xKxAsQ2

Abishek K. Iyer, Jeong Bin Cho, Hye Ryung Byun, Michael J. Waters, Shiqiang Hao, Benjamin M. Oxley, Venkat Gopalan, Christopher Wolverton, James M. Rondinelli, Joon Ik Jang, Mercouri G. Kanatzidis

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42 direct citing works

Structure Tuning, Strong Second Harmonic Generation Response, and High Optical Stability of the Polar Semiconductors Na1–xKxAsQ2OriginalPartial congener substitution induced centrosymmetric to noncentrosymmetric structural transformation and nonlinear optical properties of PbSnSiS413Li 3 [Al(PO 4 ) 2 (H 2 O) 1.5 ] and Na[AlP 2 O 7 ]: from 2D layered polar to 3D centrosymmetric framework structures8SrAgAsS4: A Noncentrosymmetric Sulfide with Good Infrared Nonlinear Optical Performance Induced by Aliovalent Substitution from Centrosymmetric SrGa2S412Additive‐Triggered Polar Polymorph Formation: β‐Sc(IO 3 ) 3 , a Promising Next‐Generation Mid‐Infrared Nonlinear Optical Material42Additive‐Triggered Polar Polymorph Formation: β‐Sc(IO3)3, a Promising Next‐Generation Mid‐Infrared Nonlinear Optical Material3Heteroanionic Control of Exemplary Second-Harmonic Generation and Phase Matchability in 1D LiAsS2–xSex43Solution-Grown Ternary Semiconductors: Nanostructuring and Stereoelectronic Lone Pair Distortions in I–V–VI 2 Materials27Isoreticular Design of KTiOPO 4 -Like Deep-Ultraviolet Transparent Materials Exhibiting Strong Second-Harmonic Generation68Ag[SC(NH2)2]2F: A Laser Damage-Tolerant Infrared Nonlinear Optical Material9AIB3IIC3IIIQ8VI: A New Family for the Design of Infrared Nonlinear Optical Materials by Coupling Octahedra and Tetrahedra Units152Stabilization of the Polar Structure and Giant Second‐Order Nonlinear Response of Single Crystal γ‐NaAs0.95Sb0.05Se219Na 2 Ba[Na 2 Sn 2 S 7 ]: Structural Tolerance Factor‐Guided NLO Performance Improvement50Na2Ba[Na2Sn2S7]: Structural Tolerance Factor‐Guided NLO Performance Improvement0Honeycomb layered topology construction for exceptional long-wave infrared nonlinear optical crystals29Toward Large Second-Harmonic Generation and Deep-UV Transparency in Strongly Electropositive Transition Metal Sulfates113Zn2BS3Br: An Infrared Nonlinear Optical Material with Significant Dual-Property Enhancements Designed through a Template Grafting Strategy20From Monofluorophosphates A2PO3F to Difluorophosphates APO2F2 (A = alkali metal): Design of a Potential Deep-Ultraviolet Nonlinear Optical Materials System with a Shortened Phase-Matching Wavelength41AgMAsS3 (M = Cd, Hg): Double d10 Cation-Containing Thioarsenites(III) Exhibiting High Photocurrent Response and Moderate Second Harmonic Generation11Structure, Second-, and Third-Harmonic Generation of Li4P2S6: A Wide Gap Material with a High Laser-Induced Damage Threshold15Functional Alkali Metal-Based Ternary Chalcogenides: Design, Properties, and Opportunities50Rb2Sn4Q9 (Q = S and Se): Low-Dimensional Noncentrosymmetric Chalcogenides with High Laser-Induced Damage Threshold10Design of a SnO2/Zeolite Gas Sensor to Enhance Formaldehyde Sensing Properties: From the Strategy of the Band Gap-Tunable Zeolite29Hg 3 AsS 4 X (X = Cl and Br): two Hg-based chalcogenides as long-wave infrared nonlinear optical crystals with superior comprehensive performances33Strongly Enhanced Polarization in a Ferroelectric Crystal by Conduction-Proton Flow19Record Second-Harmonic Generation and Birefringence in an Ultraviolet Antimonate by Bond Engineering157Vacancy‐Induced Extraordinary Second Harmonic Generation Response for Diamond‐Like Cu3PS49Homoatomic Polychalcogenide Nonlinear Optical Anionic Groups with Ultra-Large Optical Anisotropy31Pyro-phototronic Effect Enhanced Self-Powered Photoresponse in Lead-Free Hybrid Perovskite8Ca 2 La(MS 4 )(BS 3 ) (M = Ge/Si and Sn/Si): high-performance infrared nonlinear optical materials designed using an atomic site co-occupancy strategy9Symmetry over Chemistry: Harmonic Generation of Low-Dimensional Alkali Chalcopnictates RbMP2S6 (M = Sb, Bi)6Structure-property relationships in IR nonlinear optical chalcogenides with stereochemically active lone pairs29Entropy‐Driven Structural Modulation Enables High‐Efficiency Nonlinear Optical Performance in Defective Wurtzite Selenides3Dilute Soft-Cation Anchoring Stabilizes γ-NaAsSe2 against Moisture While Preserving Giant Mid-Infrared Nonlinearity0Mixed‐Valence Engineering in Ge 2+ Chalcogenides: Structural Modulation for Balanced Infrared Nonlinear Optics0

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34 direct citing papers saved.

  1. Partial congener substitution induced centrosymmetric to noncentrosymmetric structural transformation and nonlinear optical properties of PbSnSiS4

    Journal of Alloys and Compounds · 2021-12-23

    Jiazheng Zhou, Ling Luo, Yu Chu, Peng Wang, Zhiyong Guo, Xin Su, Junjie Li

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  2. Li 3 [Al(PO 4 ) 2 (H 2 O) 1.5 ] and Na[AlP 2 O 7 ]: from 2D layered polar to 3D centrosymmetric framework structures

    CrystEngComm · 2022-01-01

    Xinlei Li, Yang Zhang, Yang Pan, Yucheng Hao, Yuan Hua Lin, Haijian Li, Minghua Li, Changzeng Fan, Evgeny V. Alekseev

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  3. SrAgAsS4: A Noncentrosymmetric Sulfide with Good Infrared Nonlinear Optical Performance Induced by Aliovalent Substitution from Centrosymmetric SrGa2S4

    Inorganic Chemistry · 2022-06-07

    Jian Tang, Fei Liang, Chunlan Tang, Wenhao Xing, Jieyun Wu, Wenlong Yin, Bin Kang, Jianguo Deng

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  4. Additive‐Triggered Polar Polymorph Formation: β‐Sc(IO 3 ) 3 , a Promising Next‐Generation Mid‐Infrared Nonlinear Optical Material

    Angewandte Chemie International Edition · 2022-07-12

    Chao Wu, Guangfeng Wei, Xingxing Jiang, Qinke Xu, Zheshuai Lin, Zhipeng Huang, Mark Graeme Humphrey, Chi Zhang

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  5. Additive‐Triggered Polar Polymorph Formation: β‐Sc(IO3)3, a Promising Next‐Generation Mid‐Infrared Nonlinear Optical Material

    Angewandte Chemie · 2022-07-12

    Chao Wu, Guangfeng Wei, Xingxing Jiang, Qinke Xu, Zheshuai Lin, Zhipeng Huang, Mark Graeme Humphrey, Chi Zhang

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  6. Heteroanionic Control of Exemplary Second-Harmonic Generation and Phase Matchability in 1D LiAsS2–xSex

    Journal of the American Chemical Society · 2022-07-22

    Benjamin M. Oxley, Jeong Bin Cho, Abishek K. Iyer, Michael J. Waters, Jingyang He, Nathan Smith, Chris M. Wolverton, Venkatraman Gopalan, James M. Rondinelli, Joon Ik Jang, Mercouri G. Kanatzidis

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  7. Solution-Grown Ternary Semiconductors: Nanostructuring and Stereoelectronic Lone Pair Distortions in I–V–VI 2 Materials

    Chemistry of Materials · 2022-08-10

    Alan M. Medina‐Gonzalez, Philip Yox, Yunhua Chen, Marquix A. S. Adamson, Bryan A. Rosales, Maranny Svay, Emily A. Smith, Richard D. Schaller, Kui Wu, Aaron J. Rossini, Kirill A. Kovnir, Javier Vela

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  8. Isoreticular Design of KTiOPO 4 -Like Deep-Ultraviolet Transparent Materials Exhibiting Strong Second-Harmonic Generation

    Journal of the American Chemical Society · 2022-10-19

    Chunbo Jiang, Xingxing Jiang, Chao Wu, Zhipeng Huang, Zheshuai Lin, Mark Graeme Humphrey, Chi Zhang

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  9. Ag[SC(NH2)2]2F: A Laser Damage-Tolerant Infrared Nonlinear Optical Material

    Chemistry of Materials · 2022-10-21

    Mengya Ji, Chun‐Li Hu, Yilin Li, Bingxuan Li, Jiang‐Gao Mao

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  10. AIB3IIC3IIIQ8VI: A New Family for the Design of Infrared Nonlinear Optical Materials by Coupling Octahedra and Tetrahedra Units

    Journal of the American Chemical Society · 2022-11-18

    Ling Luo, Linan Wang, Jianbang Chen, Jiazheng Zhou, Zhihua Yang, Shilie Pan, Junjie Li

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  11. Stabilization of the Polar Structure and Giant Second‐Order Nonlinear Response of Single Crystal γ‐NaAs0.95Sb0.05Se2

    Advanced Functional Materials · 2022-12-19

    Abishek K. Iyer, Jingyang He, Hongyao Xie, Devin Goodling, Duck Young Chung, Venkatraman Gopalan, Mercouri G. Kanatzidis

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  12. Na 2 Ba[Na 2 Sn 2 S 7 ]: Structural Tolerance Factor‐Guided NLO Performance Improvement

    Angewandte Chemie International Edition · 2022-12-21

    Rui‐An Li, Qianqian Liu, Xin Liu, Youquan Liu, Xingxing Jiang, Zheshuai Lin, Fei Jia, Lin Xiong, Ling Chen, Li‐Ming Wu

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  13. Na2Ba[Na2Sn2S7]: Structural Tolerance Factor‐Guided NLO Performance Improvement

    Angewandte Chemie · 2022-12-21

    Rui‐An Li, Qianqian Liu, Xin Liu, Youquan Liu, Xingxing Jiang, Zheshuai Lin, Fei Jia, Lin Xiong, Ling Chen, Li‐Ming Wu

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  14. Honeycomb layered topology construction for exceptional long-wave infrared nonlinear optical crystals

    Materials Horizons · 2023-01-01

    Jindong Chen, Chensheng Lin, Xiaotian Jiang, Guangsai Yang, Min Luo, Xin Zhao, Bingxuan Li, Guang Peng, Ning Ye, Zhanggui Hu, Jiyang Wang, Yicheng Wu

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  15. Toward Large Second-Harmonic Generation and Deep-UV Transparency in Strongly Electropositive Transition Metal Sulfates

    Journal of the American Chemical Society · 2023-01-12

    Chao Wu, Chunbo Jiang, Guangfeng Wei, Xingxing Jiang, Zujian Wang, Zheshuai Lin, Zhipeng Huang, Mark Graeme Humphrey, Chi Zhang

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  16. Zn2BS3Br: An Infrared Nonlinear Optical Material with Significant Dual-Property Enhancements Designed through a Template Grafting Strategy

    Chemistry of Materials · 2023-03-15

    Chun‐Li Hu, Ya‐Xiang Han, Zhi Gang Fang, Jiang‐Gao Mao

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  17. From Monofluorophosphates A2PO3F to Difluorophosphates APO2F2 (A = alkali metal): Design of a Potential Deep-Ultraviolet Nonlinear Optical Materials System with a Shortened Phase-Matching Wavelength

    Chemistry of Materials · 2023-07-06

    Wenqi Jin, Congwei Xie, Xueling Hou, Meng Cheng, Evgenii Tikhonov, Mengfan Wu, Shilie Pan, Zhihua Yang

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  18. AgMAsS3 (M = Cd, Hg): Double d10 Cation-Containing Thioarsenites(III) Exhibiting High Photocurrent Response and Moderate Second Harmonic Generation

    Inorganic Chemistry · 2023-08-30

    Jian Tang, Fei Liang, Wenhao Xing, Chunlan Tang, Wenlong Yin, Bin Kang, Jianguo Deng

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  19. Structure, Second-, and Third-Harmonic Generation of Li4P2S6: A Wide Gap Material with a High Laser-Induced Damage Threshold

    Chemistry of Materials · 2023-08-31

    Benjamin M. Oxley, Kyeong‐Hyeon Lee, Thomas S. Ie, Jae Mo Lee, Michael J. Waters, James M. Rondinelli, Joon Ik Jang, Mercouri G. Kanatzidis

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  20. Functional Alkali Metal-Based Ternary Chalcogenides: Design, Properties, and Opportunities

    Chemistry of Materials · 2023-09-22

    Hannah McKeever, Niraj Nitish Patil, Manoj Palabathuni, Shalini Singh

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  21. Rb2Sn4Q9 (Q = S and Se): Low-Dimensional Noncentrosymmetric Chalcogenides with High Laser-Induced Damage Threshold

    Chemistry of Materials · 2023-10-06

    Abishek K. Iyer, Seung Heon Ha, Michael J. Waters, Thomas S. Ie, Seung Han Shin, James M. Rondinelli, Joon Ik Jang, Mercouri G. Kanatzidis

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  22. Design of a SnO2/Zeolite Gas Sensor to Enhance Formaldehyde Sensing Properties: From the Strategy of the Band Gap-Tunable Zeolite

    ACS Applied Materials & Interfaces · 2023-11-07

    Yanhui Sun, Shouhang Fu, Shupeng Sun, Jiawen Cui, Zhixin Luo, Zefeng Lei, Yue Hou

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  23. Hg 3 AsS 4 X (X = Cl and Br): two Hg-based chalcogenides as long-wave infrared nonlinear optical crystals with superior comprehensive performances

    Inorganic Chemistry Frontiers · 2024-01-01

    Feng Xu, Xiang Xu, Bingxuan Li, Ge Zhang, Chan Zheng, Jindong Chen, Ning Ye

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  24. Strongly Enhanced Polarization in a Ferroelectric Crystal by Conduction-Proton Flow

    Journal of the American Chemical Society · 2024-01-02

    Junichi Yanagisawa, Takuya Aoyama, Kotaro Fujii, Masatomo Yashima, Yoshiyuki Inaguma, Akihide Kuwabara, Kazuki Shitara, Benjamin Le Ouay, Shinya Hayami, Masaaki Ohba, Ryo Ohtani

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  25. Record Second-Harmonic Generation and Birefringence in an Ultraviolet Antimonate by Bond Engineering

    Journal of the American Chemical Society · 2024-03-11

    Qi Lu, Xingxing Jiang, Kaining Duanmu, Chao Wu, Zheshuai Lin, Zhipeng Huang, Mark Graeme Humphrey, Chi Zhang

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  26. Vacancy‐Induced Extraordinary Second Harmonic Generation Response for Diamond‐Like Cu3PS4

    Advanced Optical Materials · 2024-04-10

    Weiping Guo, Yudi Fu, Hong‐Hua Cui, Lingyun Li, Yan Yu, Zhong‐Zhen Luo, Zhigang Zou

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  27. Homoatomic Polychalcogenide Nonlinear Optical Anionic Groups with Ultra-Large Optical Anisotropy

    Journal of the American Chemical Society · 2024-05-31

    Aoge Yao, Fan Liu, Bohui Xu, Hao Huo, Zheshuai Lin, Lei Kang

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  28. Pyro-phototronic Effect Enhanced Self-Powered Photoresponse in Lead-Free Hybrid Perovskite

    ACS Applied Materials & Interfaces · 2024-10-25

    Dongying Fu, Yanli Ma, Shufang Wu, Qi Wang, Ruifang Zhao, Lin Pan, Junhua Luo

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  29. Ca 2 La(MS 4 )(BS 3 ) (M = Ge/Si and Sn/Si): high-performance infrared nonlinear optical materials designed using an atomic site co-occupancy strategy

    Inorganic Chemistry Frontiers · 2025-01-01

    Ya‐Xiang Han, Chun‐Li Hu, Jiang‐Gao Mao

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  30. Symmetry over Chemistry: Harmonic Generation of Low-Dimensional Alkali Chalcopnictates RbMP2S6 (M = Sb, Bi)

    Chemistry of Materials · 2025-03-21

    Benjamin M. Oxley, Joshua Lim, Kyeong‐Hyeon Lee, Jeong-Bin Cho, Saugata Sarker, Jadupati Nag, Michael J. Waters, James M. Rondinelli, Venkatraman Gopalan, Joon Ik Jang, Mercouri G. Kanatzidis

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  31. Structure-property relationships in IR nonlinear optical chalcogenides with stereochemically active lone pairs

    Coordination Chemistry Reviews · 2025-09-03

    Hong Chen, Xin‐Tao Wu, Hua Lin

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  32. Entropy‐Driven Structural Modulation Enables High‐Efficiency Nonlinear Optical Performance in Defective Wurtzite Selenides

    Laser & Photonics Review · 2026-05-07

    Jian Cheng, Mao‐Yin Ran, Zi-Nan Chen, Sheng‐Ping Guo

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  33. Dilute Soft-Cation Anchoring Stabilizes γ-NaAsSe2 against Moisture While Preserving Giant Mid-Infrared Nonlinearity

    Journal of the American Chemical Society · 2026-08-03

    Paribesh Acharyya, Himirkanti Sarkar, Michael J. Waters, Thomas S. Ie, Saugata Sarker, Jadupati Nag, Safdar Imam, Pronoy Nandi, James M. Rondinelli, Venkatraman Gopalan, Mercouri G. Kanatzidis

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  34. Mixed‐Valence Engineering in Ge 2+ Chalcogenides: Structural Modulation for Balanced Infrared Nonlinear Optics

    Advanced Optical Materials · 2026-09-23

    Chunlan Tang, Aoge Yao, Wenhao Xing, Cihai Hong, Jian Tang, Lei Kang, Jiang Huang, Jieyun Wu, Wenlong Yin, Bin Kang

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