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RESEARCH PAPER · ACS Applied Materials & Interfaces · 2022

Interstitial Li + Occupancy Enabling Radiative/Nonradiative Transition Control toward Highly Efficient Cr 3+ -Based Near-Infrared Luminescence

Fanquan He, Enhai Song, Hui Chang, Yayun Zhou, Zhiguo Xia, Qinyuan Zhang

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Interstitial Li + Occupancy Enabling Radiative/Nonradiative Transition Control toward Highly Efficient Cr 3+ -Based Near-Infrared LuminescenceOriginalRecent Advances in Chromium‐Doped Near‐Infrared Luminescent Materials: Fundamentals, Optimization Strategies, and Applications252Thermally stable and tunable broadband near-infrared emission from NIR-I to NIR-II in Bi-doped germanate glass for smart light sources19An Efficient Perovskite‐Like Phosphor with Peak Emission Wavelength at 850 nm for High‐Performance NIR LEDs43A Broadband Near-Infrared Sr3al9.8sio20:0.2cr Phosphor Realized by Crystallographic Site Engineering0Blue-light-excitable pure and efficient short-wave infrared luminescence via Cr 3+ → Yb 3+ energy transfer in a KYbP 2 O 7 :Cr 3+ phosphor24Highly efficient and thermally stable broadband near-infrared emitting garnet Ca 3 Sc 2 Ge 3 O 12 :Cr 3+ ,Ce 3+ phosphors for multiple pc-LED applications33K 2 LiScF 6 :Cr 3+ /Mn 4+ fluoride phosphor with enhanced broadband emission for NIR pc-LEDs29Optical enhancement of highly efficient organic–inorganic oxyfluoride red phosphors via the cation co-doping strategy8Theoretical calculations and photoluminescence properties of Sr 4 Al 14 O 25 :Mn 4+ red phosphors doped with Li +5Ion Substitution Strategy toward High-Efficiency Near-Infrared Photoluminescence of Cs2KIn1–yAlyF6:Cr3+ Solid Solutions54Versatile Ca 2 LnSbO 6 :Eu 3+ /Mn 4+ (Ln = La, Y, Gd, and Lu) phosphors for temperature sensing and plant growth LED19Screening of Broadband Near-Infrared Cr3+-Activated Phosphors Using Ce3+ as a Probe39Luminescence enhancement of Cr3+ doped garnet phosphor for high-performance LED towards smart NIR light source47Thermal Stability Improvement of Cr3+‐Activated Broadband Near‐Infrared Phosphors via State Population Optimization60Continuous Ultra‐Broadband Near‐Infrared Sc2O3‐Based Nanophosphor Realized by Spectral Bridge of Cr3+‐Yb3+‐Cr4+ for Multiple Optical Applications44The ultra-wideband near-infrared luminescence properties and applications of K2SrGe8O18:Cr3+ phosphor26Efficient CrIII Ion Governed Energy Migration for Broadband Near‐Infrared Emission in Ca3Sc2Ge3O12 Garnet Phosphor7Crystallization of Na2SrGe6O14:Cr3+,Yb3+ Glass Ceramics Enabling a Watt‐Level Output Power NIR‐I/NIR‐II Lighting Source56Subnano Te Cluster in Glass for Efficient Full‐Spectrum Conversion15Crystal structure, morphology and enhancement of luminescence properties of Cr3+-doped KZnF3 phosphor by using a HF-free hydrothermal method with different chromium sources3Cooperative cationic substitution strategy triggers high blue-light absorptance and near-infrared emission with high quantum efficiency in Cr3+-activated pyroxene-type assembly11Cr 3+ ↔Fe 3+ Energy Transfer Offset Enabling Anti‐Thermal Quenching Near‐Infrared Emission for Coded Wireless‐Communication Applications43High external quantum yield in near-infrared phosphor Bi2Ga4O9:Cr3+ excited by near-ultraviolet or blue light9Broadband Near-Infrared Sr3Al9.8SiO20:0.2Cr Phosphor Realized by Crystallographic Site Engineering5A broadband near-infrared emission Na 3 Al 2 (PO 4 ) 2 F 3 :Cr 3+ phosphor exhibiting zero photoluminescence quenching at 398 K17Abnormal spectral broadening of ordered-structure near-infrared phosphor La 2 CaHfO 6 :Cr 3+15Achieving spectrally tunable and thermally stable near-infrared emission in Fe 3+ -activated spinel phosphors via the cation site modulation strategy34Broadband short-wave infrared Mg 4 Nb 2 O 9 :Cr 3+ ,Li + phosphor for nondestructive safety detection and biomedical imaging17Remarkable near-infrared emission enhancement of Cr 3+ -activated BaGe 4 O 9 : the role of lithium ions12Site-selective occupancy of Cr 3+ enabling tunable emission from near infrared I to II in fluoride LiInF 4 :Cr 3+18Remote Control and Noninvasive Detection Enabled by a High-performance NIR pc-LED20Thermally stable fluoride phosphor Na3Sc2Li3F12:Cr3+ with broadband emission for NIR pc-LED applications23Te Cluster Engineering for Tunable Optical Response12Laser-driven broadband near-infrared light source with watt-level output280Broadband near infrared emission in Cr3+,Yb3+, Li+ tri-doped In2TeO614Li Substitution Strategy for Enhancing Quantum Efficiency and Improving Thermal Stability of Red‐Light Mn 4+ ‐Activated Fluoride for Wide‐Gamut Displays15Simultaneous NIR Emission and Thermal Stability Enhancement in Garnet‐Type NIR Phosphors through the Synergistic Effect of Lattice Distortion and Enhanced Rigidity60Intense NIR-II luminescence through stabilization of tetrahedral (Mn5+O4) lumophore in apatites with high external quantum efficiency36Hydrofluoric Acid-Free Broadband Near-Infrared Phosphors K2LiMF6:Cr3+ with Zero-Thermal Quenching: Structure, Luminescence, and Application29A Cr3+-Yb3+ co-doped high-efficiency near-infrared luminescent phosphor for NIR-II light source applications8Highly efficient Y 3-x Ba x Al 5-x Si x O 12 :Cr 3+ near-infrared phosphor for plant growth3Effect of Cr3+ doping concentration on the microstructure, mechanical properties and optical properties of Cr3+: SrF2 transparent ceramics3Tunable Broadband NIR-II Emission via Cr 4+ -Er 3+ Energy Transfer in CaMgGeO 4 :Cr 4+ ,Er 3+ Phosphors for Nondestructive Analysis16Photoluminescence properties of Li3Sc1-x(BO3)2:xCr3+ phosphors and enhanced near-infrared emission and thermal stability by Yb3+ codoping3Fluoride phosphors0Insight into Cr3+-activated NIR phosphor with extremely high thermal stability for NIR LEDs13Bi3+ ion enhanced self-activated blue phosphor Ba3Ga2O6 for temperature sensing7A novel AlF 3 :Cr 3+ NIR phosphor with high thermal quenching stability for advanced pc-LEDs8Lithium induced emission enhancement of Cr 3+ -activated fluoride with high thermal stability, toward night vision and information encryption applications3A cationic substitution strategy was employed to synthesize phosphor K2NaIn1-xAlxF6: Cr3+, Mn4+ with enhanced optical properties and thermal stability18High-efficiency and thermally stable Cr3+-doped BaSiF6 fluoride phosphors for broadband near-infrared LED applications5Direct Blue‐LED Pumped Broadband Long‐Wavelength Near‐Infrared Emitter Based on Ni 2+ Mono‐Doped Double Perovskite Materials for Versatile Optical Applications22Enhanced Short-Wave Infrared Luminescence in Yb 3+ -Doped Cr(PO 3 ) 3 Phosphor with over 60% External Quantum Efficiency9Controllable morphology and enhanced luminescence in hydrothermally Cr3+-Doped Na3GaF6 phosphors for NIR imaging7Eco-friendly synthesis and multifunctional applications of Ba2ZnGe2O7:Bi3+ phosphors for advanced radiation dosimetry and high-performance w-LEDs21Broadening and Enhancing the Emission of Phosphor Li2MgTi3O8:Cr3+ by Cation Substitution10Valence and Site Engineering Enable Efficient Broadband Near‐Infrared Emission at 960 nm in Cr 3+ ‐Activated Forsterite48Small Stokes Shift Induced Highly Efficient and Thermally Stable Broadband Near‐Infrared Antimonite Double Perovskite Emitters for Spectroscopy Applications8Li+ co-doping and hydrophobic surface modification enhance the luminescence and moisture resistance of Mn4+-doped fluoride phosphors4Near-Infrared Phosphors with Significantly Improved Luminescence Intensity and Zero-Thermal-Quenching for Light-Emitting Diodes3Enhanced Luminescence Performance of Cr-Doped CaMgSi2O6 Phosphor via Alkali Metal Ion Codoping5Interstitial‐Li Induced Oxygen Defect in Self‐Activated BaAl 2 B 2 O 7 for Enhancing Near‐Infrared Luminescence and Thermal Stability11Strategies to achieve Mn5 + -activated highly efficient phosphor for near infrared-II LED light source2Stabilizing Mn 5+ Valence States via Site Engineering and Oxidizing Sintering for High‐Efficiency Near‐Infrared II Light Sources0Lattice Site Competition Regulates the Luminescence Centers of Cr 3+ ‐Doped NIR Phosphor for Phonon Sidebands Ratiometric Thermometer and Night Vision2Breaking Concentration Quenching for Excellent Highly Efficient and Stable Narrowband Luminescence by Structural Ordering and Defect Regulation2Achieving High-Efficiency Near-Infrared Luminescence in LiScSi2O6:Cr3+ through In3+/Yb3+ Co-Doping and Its Application Exploration0Achieving High-Efficiency Near-Infrared Luminescence in LiScSi2O6:Cr3+ through In3+/Yb3+ Co-Doping and Its Application Exploration0High-performance multifunctional NIR phosphor K2NaAlF6:Mn4+,Cr3+ for pc-LED and X-ray imaging via efficient energy transfer3Li+ Charge compensation-induced enhancement of spectral, mechanical, and thermal properties in Cr3+-doped Ca3(VO4)2 single crystals0Cationic Engineering-Driven Al 3+ /Sc 3+ Codoping Achieves 60.9% EQE in Cr 3+ -Activated Mg 3 Ga 2 GeO 8 Near-Infrared Phosphors0Recent progress of fluoride phosphors doped with Mn4+ and Cr3+: A review3Tailoring Excited Bands and Impurity‐Host Interactions for Efficient NIR Emissions in Cr 3+ ‐Activated Perovskite Ca 2 Ga 1‐ x In x NbO 60Pixel‐Level X‐Ray to NIR Image Fusion Based on Lead‐Free Halide Perovskite for Biological Imaging15Efficient blue-light-excitable broadband NIR emission in Mo4+-doped double perovskite with robust thermal stability and efficient X-ray scintillation for pixel-level X-ray to NIR image fusion2The luminescence aging and mitigation strategies of Cr3+-Activated deep-red and near-infrared phosphors1Efficient Broadband Short‐Wave Infrared Luminescence at 1400 nm Enabled by Cr 3+ ‐Yb 3+ Energy Shuttle Design1Achieving high-efficiency near-infrared luminescence in LiScSi2O6:Cr3+ through In3+/Yb3+ Co-doping and its application exploration0A Multifunctional Fe 3+ ‐Activated Garnet Phosphor Enabling Near‐Infrared Imaging and Photochromic Information Encryption0Enhancing near‑infrared luminescence in Fe3+‑doped Na‑β‑Al2O3 phosphors via cation substitution for LED application0Study on the near-infrared luminescence properties of Cr3+-Yb3+ co-doped Sr2MgWO6 double-perovskite phosphors0Design and luminescence properties of novel Nb-based garnet phosphor LuCa2Ga4NbO12:Cr3+ for NIR pc-LEDs0Achieving High-Efficiency Broadband NIR Emission in Cr3+-Doped Double Perovskite via Rb+ Substitution Strategy for Versatile pc-LED Applications0

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  10. Ion Substitution Strategy toward High-Efficiency Near-Infrared Photoluminescence of Cs2KIn1–yAlyF6:Cr3+ Solid Solutions

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  45. Fluoride phosphors

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  47. Bi3+ ion enhanced self-activated blue phosphor Ba3Ga2O6 for temperature sensing

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  48. A novel AlF 3 :Cr 3+ NIR phosphor with high thermal quenching stability for advanced pc-LEDs

    Journal of Materials Chemistry C · 2025-01-01

    Wenqiang Li, Qihao Li, Yuehua Chen, Cailing Liu, Wenjing Zhong, Xiang Zhang, Yayun Zhou, Tingting Deng, Jian-tao Lü, Ting Fan

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  49. Lithium induced emission enhancement of Cr 3+ -activated fluoride with high thermal stability, toward night vision and information encryption applications

    Journal of Materials Chemistry C · 2025-01-01

    Shuang Wu, Yongqi Zhu, Yongqi Zhu, Nanfeng Zheng, Hui Liu, Yiwen Zhu, Yiwen Zhu, Xinyue Li, Yifan Chen, Daqin Chen

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  50. A cationic substitution strategy was employed to synthesize phosphor K2NaIn1-xAlxF6: Cr3+, Mn4+ with enhanced optical properties and thermal stability

    Ceramics International · 2025-01-04

    Wenxia Li, Ruihan Liang, Jipeng Rao, Xiaoyun Mi, Xiuling Liu

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