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RESEARCH PAPER · Chemical Communications · 2021

New nonlinear optical-active AAgGa 6 S 10 (A = K, Rb, Cs) featuring {[AgGa 6 S 10 ] − } ∞ framework and high laser damage threshold

Jia-Nuo Li, Xiaohui Li, Wen‐Dong Yao, Wenlong Liu, Sheng‐Ping Guo

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New nonlinear optical-active AAgGa 6 S 10 (A = K, Rb, Cs) featuring {[AgGa 6 S 10 ] − } ∞ framework and high laser damage thresholdOriginalSodium-Stuffed Open-Framework Quaternary Chalcogenide Built with (Cu2Ga6S18)16– Ribbons Cross-Linked by Unusual Linear Cu(I) Pillars2Transition-metal-based chalcogenides: A rich source of infrared nonlinear optical materials184Noncentrosymmetric Ba6In2Q10 (Q = S, Se): Structural Chemistry and Nonlinear-Optical Activity11Noncentrosymmetric chalcohalide K2Ba3Ge3S9Cl2: A new nonlinear optical material with remarkable laser-induced damage threshold17Phase Matchability Transformation in the Infrared Nonlinear Optical Materials with Diamond‐Like Frameworks63AAg 3 Ga 8 Se 14 (A = Rb, Cs): second-harmonic generation responses realized through the parallel arrangement of AgSe 4 and GaSe 4 tetrahedrons5First polar quaternary sulphide CsLiGa 6 S 10 with mixed ordered alkali cations displaying excellent infrared nonlinear optical properties16KAg3Ga8S14: An Mid- and Far-infrared Nonlinear Optical Material Exhibiting High Laser-induced Damage Threshold※3KEu 2 In 3 B 12 S 13 : a novel type of thioborate featuring B 12 S 12 cluster and unique In 6 S 6 12-membered ring10Pb 3 SBrI 3 : the first Pb-based chalcohalide with multiple halogens features a unique two-dimensional structure composed of diverse Pb-centered polyhedra12NaGa3Se5: An Infrared Nonlinear Optical Material with Balanced Performance Contributed by Complex {[Ga3Se5]−}∞ Anionic Network14First Investigation of Nonlinear Optical Oxychalcogenide with Three‐Dimensional Anionic Framework and Special Windmill‐Like Functional Motifs †28A comprehensive review on metal chalcogenides with three-dimensional frameworks for infrared nonlinear optical applications115(Na0.74Ag1.26)BaSnS4: A New AgGaS2‐Type Nonlinear Optical Sulfide with a Wide Band Gap and High Laser Induced Damage Threshold14Ba 3 HgGa 2 S 7 : A Zero-Dimensional Quaternary Sulfide Featuring a Unique [Hg 2 Ga 4 S 14 ] 12– String and Exhibiting a High Photocurrent Response27Ternary AGa5S8 (A = K, Rb, Cs): Promising infrared nonlinear optical materials rationally realized by “one-for-multiple substitution” strategy37Chalcohalides: A Rising Type of Second‐Order Nonlinear Optical Materials28Ag-based chalcogenides and derivatives as promising infrared nonlinear optical materials90Nonlinear Optical Sulfides LiMGa8S14 (M = Rb/Ba, Cs/Ba) Created by Li+ Driven 2D Centrosymmetric to 3D Noncentrosymmetric Transformation20Wide band gaps in nonlinear optical materials AMgAgGa6S11 (A = K, Rb) achieved by the incorporation of dual s-block elements in Ag-based sulfide11Excellent Nonlinear Optical M[M4Cl][Ga11S20] (M = A/Ba, A = K, Rb) Achieved by Unusual Cationic Substitution Strategy20Enlargement of Bandgap and Birefringence in Nonlinear Optical Alkali‐Metal Sulfate Crystals by the Substitution of Asymmetrical Non‐π‐Conjugated Cation8Ga-based IR nonlinear optical materials: Synthesis, structures, and properties65Excited state dependent fast switching NLO behavior investigation of sp hybridized donor crystal as D-π-A push–pull switches12Rational Design of Novel Promising Infrared Nonlinear Optical Materials: Structural Chemistry and Balanced Performances157Polysubstitution Induced Centrosymmetric-to-Noncentrosymmetric Structural Transformation and Nonlinear-Optical Behavior: The Case of Na0.45Ag0.55Ga3Se52Exploring the ON/OFF nonlinear optical (NLO) response in tetracene-based chromophores: A DFT study on solvent and frequency-dependent NLO properties for switching applications26ACuGa 6 S 10 (A = Rb, Cs): Design and Synthesis of Two New Cavity‐Chalcopyrite Chalcogenides Based on “Iterative Substitution” Strategy4Structural frustration effects by mixed alkali ions in ferroelectric Dion–Jacobson layered perovskites (Cs,Rb)NdNb 2 O 76Suppression of Ferroelectric Transitions by Symmetry Trapping in Dion–Jacobson-Layered Perovskites Cs(La,Nd)Nb2O74Emergent Mid‐Infrared Nonlinear Optical Candidates With Targeted Balance Performances18Rare‐Earth Substitution Induced Symmetry Breaking for The First Sc‐Based Nonlinear Optical Chalcogenide with High‐Performance31CsMgGa 5 S 9 : a diamond-like network made of mixed tetrahedral units for excellent nonlinear optical properties2Assembly between diverse polycations and diamond-like anionic frameworks in salt-inclusion phosphides enables excellent nonlinear optical properties4A Series of Pentanary Rare-Earth Oxysulfides Obtained by Heterovalent Cation and Anion Cosubstitution Exhibiting Nonlinear Optical Activity and Ultrawide Band Gaps1NaAg3Ga8S14: A new diamond-like framework infrared nonlinear optical material derived from AgGaS26高性能硫属化物红外非线性光学材料构效关系（特邀）0Rare-earth doping of AgGaGe3Se8: A pathway to multifunctional materials for tunable optoelectronics1Birefringence and Photocurrent Response of A Series of Rare-Earth Selenophosphates Cs4RE2(PSe4)2(P2Se6) (RE = La–Nd, Sm, Gd, Tb) Synthesized by the Metal Oxide–Boron–Chalcogen (MOBQ) Method0Eu5ZnGa6S15, Eu5Zn3Ga2Sn2S15, and Pb5HgGa6S15: Crystal Chemistry and Nonlinear Optical Properties0Variation of Tetrahedrons and Cations Regulates LIDTs in 3D‐DL Structure MIR‐NLO Crystals0Homologous lattice coupling drives the formation of tetrahedra-ordered phase exhibiting enhanced optical nonlinearity and band gap0

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  1. Sodium-Stuffed Open-Framework Quaternary Chalcogenide Built with (Cu2Ga6S18)16– Ribbons Cross-Linked by Unusual Linear Cu(I) Pillars

    Inorganic Chemistry · 2021-07-26

    Srikanth Balijapelly, Amit Adhikary, Sudip Mohapatra, Aleksandr Chernatynskiy, Amitava Choudhury

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  2. Transition-metal-based chalcogenides: A rich source of infrared nonlinear optical materials

    Coordination Chemistry Reviews · 2021-08-26

    Hong Chen, Wenbo Wei, Hua Lin, Xintao Wu

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  3. Noncentrosymmetric Ba6In2Q10 (Q = S, Se): Structural Chemistry and Nonlinear-Optical Activity

    Inorganic Chemistry · 2021-11-05

    Xiao Fen Huang, Sihan Yang, Wenlong Liu, Sheng‐Ping Guo

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  4. Noncentrosymmetric chalcohalide K2Ba3Ge3S9Cl2: A new nonlinear optical material with remarkable laser-induced damage threshold

    Journal of Alloys and Compounds · 2021-11-13

    Wenfeng Zhou, Zhi‐Hui Shi, Wenlong Liu, Sheng‐Ping Guo

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  5. Phase Matchability Transformation in the Infrared Nonlinear Optical Materials with Diamond‐Like Frameworks

    Advanced Optical Materials · 2021-12-30

    Man‐Man Chen, Shenghua Zhou, Wenbo Wei, Xintao Wu, Hua Lin, Qi‐Long Zhu

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  6. AAg 3 Ga 8 Se 14 (A = Rb, Cs): second-harmonic generation responses realized through the parallel arrangement of AgSe 4 and GaSe 4 tetrahedrons

    Dalton Transactions · 2022-01-01

    Zhi-Xin Qiu, Shao‐Min Pei, Wen‐Fa Chen, Xiao‐Ming Jiang, Bin‐Wen Liu, Guo‐Cong Guo

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  7. First polar quaternary sulphide CsLiGa 6 S 10 with mixed ordered alkali cations displaying excellent infrared nonlinear optical properties

    Inorganic Chemistry Frontiers · 2022-01-01

    Zi Wang, Bin‐Wen Liu, Guo‐Cong Guo

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  8. KAg3Ga8S14: An Mid- and Far-infrared Nonlinear Optical Material Exhibiting High Laser-induced Damage Threshold※

    化学学报 · 2022-01-01

    Jin-Xu Zhao, Mingshu Zhang, Wen‐Fa Chen, Xiao‐Ming Jiang, Binwen Liu, Guo‐Cong Guo

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  9. KEu 2 In 3 B 12 S 13 : a novel type of thioborate featuring B 12 S 12 cluster and unique In 6 S 6 12-membered ring

    Dalton Transactions · 2022-01-01

    Shanshan Han, Qian-Ting Xu, Wenlong Liu, Sheng‐Ping Guo

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  10. Pb 3 SBrI 3 : the first Pb-based chalcohalide with multiple halogens features a unique two-dimensional structure composed of diverse Pb-centered polyhedra

    Dalton Transactions · 2022-01-01

    Mei Yan, Ru‐Ling Tang, Wenfeng Zhou, Wenlong Liu, Sheng‐Ping Guo

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  11. NaGa3Se5: An Infrared Nonlinear Optical Material with Balanced Performance Contributed by Complex {[Ga3Se5]−}∞ Anionic Network

    Inorganic Chemistry · 2022-03-28

    Qian-Ting Xu, Shanshan Han, Jia-Nuo Li, Sheng‐Ping Guo

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  12. First Investigation of Nonlinear Optical Oxychalcogenide with Three‐Dimensional Anionic Framework and Special Windmill‐Like Functional Motifs †

    Chinese Journal of Chemistry · 2022-07-14

    Jia-Nuo Li, Xiaohui Li, Ying‐Xuan Xu, Wenlong Liu, Sheng‐Ping Guo

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  13. A comprehensive review on metal chalcogenides with three-dimensional frameworks for infrared nonlinear optical applications

    Coordination Chemistry Reviews · 2022-07-19

    Hong Chen, Mao‐Yin Ran, Wenbo Wei, Xintao Wu, Hua Lin, Qi‐Long Zhu

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  14. (Na0.74Ag1.26)BaSnS4: A New AgGaS2‐Type Nonlinear Optical Sulfide with a Wide Band Gap and High Laser Induced Damage Threshold

    Chemistry - A European Journal · 2022-08-10

    Wenfeng Zhou, Wenlong Liu, Sheng‐Ping Guo

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  15. Ba 3 HgGa 2 S 7 : A Zero-Dimensional Quaternary Sulfide Featuring a Unique [Hg 2 Ga 4 S 14 ] 12– String and Exhibiting a High Photocurrent Response

    Inorganic Chemistry · 2022-08-10

    Xiao Fen Huang, Sihan Yang, Wenlong Liu, Sheng‐Ping Guo

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  16. Ternary AGa5S8 (A = K, Rb, Cs): Promising infrared nonlinear optical materials rationally realized by “one-for-multiple substitution” strategy

    Science China Materials · 2022-09-23

    Wen‐Fa Chen, Xiao‐Ming Jiang, Shao‐Min Pei, Ming‐Shu Zhang, Bin‐Wen Liu, Guo‐Cong Guo

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  17. Chalcohalides: A Rising Type of Second‐Order Nonlinear Optical Materials

    European Journal of Inorganic Chemistry · 2022-10-05

    Jun Li, Shanshan Han, Sheng‐Ping Guo

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  18. Ag-based chalcogenides and derivatives as promising infrared nonlinear optical materials

    Coordination Chemistry Reviews · 2022-11-26

    Wenfeng Zhou, Jiajing Wu, Wenlong Liu, Sheng‐Ping Guo

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  19. Nonlinear Optical Sulfides LiMGa8S14 (M = Rb/Ba, Cs/Ba) Created by Li+ Driven 2D Centrosymmetric to 3D Noncentrosymmetric Transformation

    Small · 2023-05-05

    Ming‐Shu Zhang, Bin‐Wen Liu, Xiao‐Ming Jiang, Guo‐Cong Guo

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  20. Wide band gaps in nonlinear optical materials AMgAgGa6S11 (A = K, Rb) achieved by the incorporation of dual s-block elements in Ag-based sulfide

    Materials Today Physics · 2023-08-09

    Wen‐Fa Chen, Xiao‐Ming Jiang, Bin‐Wen Liu, Guo‐Cong Guo

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  21. Excellent Nonlinear Optical M[M4Cl][Ga11S20] (M = A/Ba, A = K, Rb) Achieved by Unusual Cationic Substitution Strategy

    Small · 2023-09-11

    Xiao‐Yu Lou, Xiao‐Ming Jiang, Bin‐Wen Liu, Guo‐Cong Guo

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  22. Enlargement of Bandgap and Birefringence in Nonlinear Optical Alkali‐Metal Sulfate Crystals by the Substitution of Asymmetrical Non‐π‐Conjugated Cation

    Advanced Optical Materials · 2023-10-02

    Pengfei Zhu, Pifu Gong, Zhenyan Wang, Huatong Jiang, Jianfu Zhao, Chao Li, Zheshuai Lin, Xiulan Duan, Fapeng Yu

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  23. Ga-based IR nonlinear optical materials: Synthesis, structures, and properties

    Coordination Chemistry Reviews · 2023-12-21

    Jiaxiang Zhang, Ping Feng, Mao‐Yin Ran, Xintao Wu, Hua Lin, Qi‐Long Zhu

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  24. Excited state dependent fast switching NLO behavior investigation of sp hybridized donor crystal as D-π-A push–pull switches

    Results in Chemistry · 2024-01-01

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  25. Rational Design of Novel Promising Infrared Nonlinear Optical Materials: Structural Chemistry and Balanced Performances

    Accounts of Chemical Research · 2024-02-01

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  26. Polysubstitution Induced Centrosymmetric-to-Noncentrosymmetric Structural Transformation and Nonlinear-Optical Behavior: The Case of Na0.45Ag0.55Ga3Se5

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  27. Exploring the ON/OFF nonlinear optical (NLO) response in tetracene-based chromophores: A DFT study on solvent and frequency-dependent NLO properties for switching applications

    Journal of Molecular Liquids · 2024-08-08

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  28. ACuGa 6 S 10 (A = Rb, Cs): Design and Synthesis of Two New Cavity‐Chalcopyrite Chalcogenides Based on “Iterative Substitution” Strategy

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  29. Structural frustration effects by mixed alkali ions in ferroelectric Dion–Jacobson layered perovskites (Cs,Rb)NdNb 2 O 7

    Journal of Materials Chemistry C · 2024-11-25

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  30. Suppression of Ferroelectric Transitions by Symmetry Trapping in Dion–Jacobson-Layered Perovskites Cs(La,Nd)Nb2O7

    Inorganic Chemistry · 2024-11-27

    Zhen‐Tao Lu, Kai Nishioka, Yang Zhang, Koji Fujita, Katsuro Hayashi, Hirofumi Akamatsu

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  31. Emergent Mid‐Infrared Nonlinear Optical Candidates With Targeted Balance Performances

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  32. Rare‐Earth Substitution Induced Symmetry Breaking for The First Sc‐Based Nonlinear Optical Chalcogenide with High‐Performance

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    Chen‐Yi Zhao, Chun‐Li Hu, Nian‐Tzu Suen, Xiaohui Li, Haiping Xu, Wenfeng Zhou, Sheng‐Ping Guo

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  33. CsMgGa 5 S 9 : a diamond-like network made of mixed tetrahedral units for excellent nonlinear optical properties

    Chemical Communications · 2025-01-01

    Yi-Bing Huang, Bin‐Wen Liu, Guo‐Cong Guo

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  34. Assembly between diverse polycations and diamond-like anionic frameworks in salt-inclusion phosphides enables excellent nonlinear optical properties

    Science China Chemistry · 2025-02-11

    Ming‐Shu Zhang, Shao‐Min Pei, Bin‐Wen Liu, Xiao‐Ming Jiang, Guo‐Cong Guo

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  35. A Series of Pentanary Rare-Earth Oxysulfides Obtained by Heterovalent Cation and Anion Cosubstitution Exhibiting Nonlinear Optical Activity and Ultrawide Band Gaps

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    Zhi Bing Deng, Qiu-Yang Du, Fang-Xu Tian, Zong-Ze Li, Mingyang Li, Mao‐Yin Ran, Wenlong Liu, Sheng‐Ping Guo

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  36. NaAg3Ga8S14: A new diamond-like framework infrared nonlinear optical material derived from AgGaS2

    Chinese Journal of Structural Chemistry · 2025-10-15

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  37. 高性能硫属化物红外非线性光学材料构效关系（特邀）

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  38. Rare-earth doping of AgGaGe3Se8: A pathway to multifunctional materials for tunable optoelectronics

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  39. Birefringence and Photocurrent Response of A Series of Rare-Earth Selenophosphates Cs4RE2(PSe4)2(P2Se6) (RE = La–Nd, Sm, Gd, Tb) Synthesized by the Metal Oxide–Boron–Chalcogen (MOBQ) Method

    Inorganic Chemistry · 2026-08-10

    Si Yang, Zong-Ze Li, Ning Wang, Xin Lei Zhao, Sheng‐Ping Guo

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  40. Eu5ZnGa6S15, Eu5Zn3Ga2Sn2S15, and Pb5HgGa6S15: Crystal Chemistry and Nonlinear Optical Properties

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  41. Variation of Tetrahedrons and Cations Regulates LIDTs in 3D‐DL Structure MIR‐NLO Crystals

    ChemistrySelect · 2026-09-01

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  42. Homologous lattice coupling drives the formation of tetrahedra-ordered phase exhibiting enhanced optical nonlinearity and band gap

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