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RESEARCH PAPER · ACS Applied Materials & Interfaces · 2020

AMnAs3S6 (A = Cs, Rb): Phase-Matchable Infrared Nonlinear Optical Functional Motif [As3S6]3– Obtained via Surfactant–Thermal Method

Run Ye, Bin‐Wen Liu, Xiao‐Ming Jiang, Jian Lü, Hui‐Yi Zeng, Guo‐Cong Guo

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AMnAs3S6 (A = Cs, Rb): Phase-Matchable Infrared Nonlinear Optical Functional Motif [As3S6]3– Obtained via Surfactant–Thermal MethodOriginalA 3 Mn 2 Sb 3 S 8 (A = K and Rb): a new type of multifunctional infrared nonlinear optical material based on unique three-dimensional open frameworks53Na 4 SnS 4 and Na 4 SnSe 4 exhibiting multifunctional physicochemical performances as potential infrared nonlinear optical crystals and sodium ion conductors27Introduction of Li into Ag-Based Noncentrosymmetric Sulfides for High-Performance Infrared Nonlinear Optical Materials40Uncovering a Functional Motif of Nonlinear Optical Materials by In Situ Electron Density and Wavefunction Studies Under Laser Irradiation39Uncovering a Functional Motif of Nonlinear Optical Materials by In Situ Electron Density and Wavefunction Studies Under Laser Irradiation1ASb5S8 (A = K, Rb, and Cs): Thermal Switching of Infrared Nonlinear Optical Properties across the Crystal/Glass Transformation39AZn4Ga5Se12 (A = K, Rb, or Cs): Infrared Nonlinear Optical Materials with Simultaneous Large Second Harmonic Generation Responses and High Laser-Induced Damage Thresholds34Transition-metal-based chalcogenides: A rich source of infrared nonlinear optical materials184A Discrete Ligand-Free T3 Supertetrahedral Cluster of Gallium Sulfide3Cs 3 CuAs 4 Q 8 (Q = S, Se): unique two-dimensional layered inorganic thioarsenates with the lowest Cu-to-As ratio and remarkable photocurrent responses17AAg 3 Ga 8 Se 14 (A = Rb, Cs): second-harmonic generation responses realized through the parallel arrangement of AgSe 4 and GaSe 4 tetrahedrons5Crystalline chalcogenidometalate-based compounds from uncommon reaction media12Interesting dimensional transition through changing cations as the trigger in multinary thioarsenates displaying variable photocurrent response and optical anisotropy22Strong Photoelectric Properties of Mn-Based Seleniumstannates with Alkali Metals as Structure-Directing Agents5Infrared nonlinear optical performances of a new sulfide β-PbGa2S415Material research from the viewpoint of functional motifs103SrAgAsS4: A Noncentrosymmetric Sulfide with Good Infrared Nonlinear Optical Performance Induced by Aliovalent Substitution from Centrosymmetric SrGa2S412Eu 2 P 2 S 6 : The First Rare‐Earth Chalcogenophosphate Exhibiting Large Second‐Harmonic Generation Response and High Laser‐Induced Damage Threshold143Eu2P2S6: The First Rare‐Earth Chalcogenophosphate Exhibiting Large Second‐Harmonic Generation Response and High Laser‐Induced Damage Threshold7A comprehensive review on metal chalcogenides with three-dimensional frameworks for infrared nonlinear optical applications114Salt-inclusion chalcogenides: Double functional moieties design strategy toward excellent nonlinear optical materials12Recent progress in the design of IR nonlinear optical materials by partial chemical substitution: Structural evolution and performance optimization133Rational Design of a Rare‐Earth Oxychalcogenide Nd3[Ga3O3S3][Ge2O7] with Superior Infrared Nonlinear Optical Performance64AgMAsS3 (M = Cd, Hg): Double d10 Cation-Containing Thioarsenites(III) Exhibiting High Photocurrent Response and Moderate Second Harmonic Generation11ACu4AsS4 (A = K, Rb): Two infrared nonlinear optical crystals with strong second-harmonic generation responses originating from multiple chromophores12Homoatomic Polychalcogenide Nonlinear Optical Anionic Groups with Ultra-Large Optical Anisotropy31ACuGa 6 S 10 (A = Rb, Cs): Design and Synthesis of Two New Cavity‐Chalcopyrite Chalcogenides Based on “Iterative Substitution” Strategy4[TeSeS 2 ] 2− : The First Heterotriple‐Chalcogenide Motifs Decode Giant Mid‐Far Infrared Birefringence18[TeSeS 2 ] 2− : The First Heterotriple‐Chalcogenide Motifs Decode Giant Mid‐Far Infrared Birefringence4Structure-property relationships in IR nonlinear optical chalcogenides with stereochemically active lone pairs29A high-performance IR nonlinear optical material Sr 3 MnGe 2 S 8 achieved via partial cation substitution-induced structural transformation2Domino‐Effect Amplification via Covalent‐Chain Engineering for Giant Birefringence in NaAsQ 2 (Q = S, Se) Crystals0

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  1. A 3 Mn 2 Sb 3 S 8 (A = K and Rb): a new type of multifunctional infrared nonlinear optical material based on unique three-dimensional open frameworks

    Inorganic Chemistry Frontiers · 2021-01-01

    Yu Xiao, Man-Man Chen, Yaying Shen, Pengfei Liu, Hua Lin, Yi Liu

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  2. Na 4 SnS 4 and Na 4 SnSe 4 exhibiting multifunctional physicochemical performances as potential infrared nonlinear optical crystals and sodium ion conductors

    New Journal of Chemistry · 2021-01-01

    Lihua Gao, Gang Bian, Ya Feng Yang, Bingbing Zhang, Xiaowen Wu, Kui Wu

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  3. Introduction of Li into Ag-Based Noncentrosymmetric Sulfides for High-Performance Infrared Nonlinear Optical Materials

    Inorganic Chemistry · 2021-03-16

    Wenfeng Zhou, Wen‐Dong Yao, Qing Zhang, Huaiguo Xue, Sheng‐Ping Guo

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  4. Uncovering a Functional Motif of Nonlinear Optical Materials by In Situ Electron Density and Wavefunction Studies Under Laser Irradiation

    Angewandte Chemie International Edition · 2021-03-22

    Xiao‐Ming Jiang, Shujuan Lin, Chao He, Bin‐Wen Liu, Guo‐Cong Guo

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  5. Uncovering a Functional Motif of Nonlinear Optical Materials by In Situ Electron Density and Wavefunction Studies Under Laser Irradiation

    Angewandte Chemie · 2021-03-22

    Xiao‐Ming Jiang, Shujuan Lin, Chao He, Bin‐Wen Liu, Guo‐Cong Guo

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  6. ASb5S8 (A = K, Rb, and Cs): Thermal Switching of Infrared Nonlinear Optical Properties across the Crystal/Glass Transformation

    Chemistry of Materials · 2021-05-11

    Wen‐Fa Chen, Bin‐Wen Liu, Shao‐Min Pei, Qiu-Nan Yan, Xiao‐Ming Jiang, Guo‐Cong Guo

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  7. AZn4Ga5Se12 (A = K, Rb, or Cs): Infrared Nonlinear Optical Materials with Simultaneous Large Second Harmonic Generation Responses and High Laser-Induced Damage Thresholds

    Inorganic Chemistry · 2021-06-17

    Man-Man Chen, Shenghua Zhou, Wenbo Wei, Xintao Wu, Hua Lin, Qi‐Long Zhu

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  8. Transition-metal-based chalcogenides: A rich source of infrared nonlinear optical materials

    Coordination Chemistry Reviews · 2021-08-26

    Hong Chen, Wenbo Wei, Hua Lin, Xintao Wu

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  9. A Discrete Ligand-Free T3 Supertetrahedral Cluster of Gallium Sulfide

    Molecules · 2021-09-06

    Sarah Makin, Paz Vaqueiro

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  10. Cs 3 CuAs 4 Q 8 (Q = S, Se): unique two-dimensional layered inorganic thioarsenates with the lowest Cu-to-As ratio and remarkable photocurrent responses

    Dalton Transactions · 2021-12-07

    Chang Liu, Hedi Yang, Pei-Pei Hou, Yu Xiao, Yi Liu, Hua Lin

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  11. AAg 3 Ga 8 Se 14 (A = Rb, Cs): second-harmonic generation responses realized through the parallel arrangement of AgSe 4 and GaSe 4 tetrahedrons

    Dalton Transactions · 2022-01-01

    Zhi-Xin Qiu, Shao‐Min Pei, Wen‐Fa Chen, Xiao‐Ming Jiang, Bin‐Wen Liu, Guo‐Cong Guo

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  12. Crystalline chalcogenidometalate-based compounds from uncommon reaction media

    Chemical Communications · 2022-01-01

    Zhou Wu, Gina Stuhrmann, Stefanie Dehnen

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  13. Interesting dimensional transition through changing cations as the trigger in multinary thioarsenates displaying variable photocurrent response and optical anisotropy

    Inorganic Chemistry Frontiers · 2022-01-01

    Chao Zhang, Shenghua Zhou, Yu Xiao, Hua Lin, Yi Liu

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  14. Strong Photoelectric Properties of Mn-Based Seleniumstannates with Alkali Metals as Structure-Directing Agents

    European Journal of Inorganic Chemistry · 2022-01-01

    Gele Teri, Xin Liu, Na Li, Muge Shele, E. Namila, Liming Qi, Sagala Bai, Menghe Baiyin

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  15. Infrared nonlinear optical performances of a new sulfide β-PbGa2S4

    Journal of Alloys and Compounds · 2022-02-02

    Wen‐Fa Chen, Bin‐Wen Liu, Xiao‐Ming Jiang, Guo‐Cong Guo

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  16. Material research from the viewpoint of functional motifs

    National Science Review · 2022-02-10

    Xiao‐Ming Jiang, Shuiquan Deng, Myung‐Hwan Whangbo, Guo‐Cong Guo

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  17. SrAgAsS4: A Noncentrosymmetric Sulfide with Good Infrared Nonlinear Optical Performance Induced by Aliovalent Substitution from Centrosymmetric SrGa2S4

    Inorganic Chemistry · 2022-06-07

    Jian Tang, Fei Liang, Chunlan Tang, Wenhao Xing, Jieyun Wu, Wenlong Yin, Bin Kang, Jianguo Deng

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  18. Eu 2 P 2 S 6 : The First Rare‐Earth Chalcogenophosphate Exhibiting Large Second‐Harmonic Generation Response and High Laser‐Induced Damage Threshold

    Angewandte Chemie International Edition · 2022-06-08

    Xiao Fen Huang, Sihan Yang, Xiaohui Li, Wenlong Liu, Sheng‐Ping Guo

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  19. Eu2P2S6: The First Rare‐Earth Chalcogenophosphate Exhibiting Large Second‐Harmonic Generation Response and High Laser‐Induced Damage Threshold

    Angewandte Chemie · 2022-06-08

    Xiao Fen Huang, Sihan Yang, Xiaohui Li, Wenlong Liu, Sheng‐Ping Guo

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  20. A comprehensive review on metal chalcogenides with three-dimensional frameworks for infrared nonlinear optical applications

    Coordination Chemistry Reviews · 2022-07-19

    Hong Chen, Mao‐Yin Ran, Wenbo Wei, Xintao Wu, Hua Lin, Qi‐Long Zhu

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  21. Salt-inclusion chalcogenides: Double functional moieties design strategy toward excellent nonlinear optical materials

    Chinese Journal of Structural Chemistry · 2023-02-07

    Chao-Hong Xie, Bin‐Wen Liu, Guo‐Cong Guo

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  22. Recent progress in the design of IR nonlinear optical materials by partial chemical substitution: Structural evolution and performance optimization

    Coordination Chemistry Reviews · 2023-02-08

    Mao‐Yin Ran, A-Yang Wang, Wenbo Wei, Xintao Wu, Hua Lin, Qi‐Long Zhu

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  23. Rational Design of a Rare‐Earth Oxychalcogenide Nd3[Ga3O3S3][Ge2O7] with Superior Infrared Nonlinear Optical Performance

    Small · 2023-02-12

    Mao‐Yin Ran, Shenghua Zhou, Wenbo Wei, Bingxuan Li, Xin‐Tao Wu, Hua Lin, Qi‐Long Zhu

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  24. AgMAsS3 (M = Cd, Hg): Double d10 Cation-Containing Thioarsenites(III) Exhibiting High Photocurrent Response and Moderate Second Harmonic Generation

    Inorganic Chemistry · 2023-08-30

    Jian Tang, Fei Liang, Wenhao Xing, Chunlan Tang, Wenlong Yin, Bin Kang, Jianguo Deng

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  25. ACu4AsS4 (A = K, Rb): Two infrared nonlinear optical crystals with strong second-harmonic generation responses originating from multiple chromophores

    Scripta Materialia · 2023-12-20

    Xin Lei Zhao, Chensheng Lin, Chao Wang, Haotian Tian, Pengxiang Dong, Tao Yan, Bingxuan Li, Ning Ye, Min Luo

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  26. Homoatomic Polychalcogenide Nonlinear Optical Anionic Groups with Ultra-Large Optical Anisotropy

    Journal of the American Chemical Society · 2024-05-31

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  27. ACuGa 6 S 10 (A = Rb, Cs): Design and Synthesis of Two New Cavity‐Chalcopyrite Chalcogenides Based on “Iterative Substitution” Strategy

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  28. [TeSeS 2 ] 2− : The First Heterotriple‐Chalcogenide Motifs Decode Giant Mid‐Far Infrared Birefringence

    Angewandte Chemie International Edition · 2025-06-17

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  29. [TeSeS 2 ] 2− : The First Heterotriple‐Chalcogenide Motifs Decode Giant Mid‐Far Infrared Birefringence

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  30. Structure-property relationships in IR nonlinear optical chalcogenides with stereochemically active lone pairs

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  31. A high-performance IR nonlinear optical material Sr 3 MnGe 2 S 8 achieved via partial cation substitution-induced structural transformation

    Inorganic Chemistry Frontiers · 2025-11-14

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  32. Domino‐Effect Amplification via Covalent‐Chain Engineering for Giant Birefringence in NaAsQ 2 (Q = S, Se) Crystals

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